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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Progress on Associated-Particle Imaging Algorithms, 2022

The present work describes progress on developing imaging algorithms that use fast neutron signatures acquired using the associated-particle imaging (API) method. The present work complements ongoing work to develop neutron source and detector hardware to enable field inspection by investigating algorithms that are capable of discriminating among critical materials or extracting three-dimensional (3D) geometrical information from single-sided or transmission measurements. The present work is divided into three approaches: 1.Iterative reconstruction of inelastic gamma-ray emissions to perform 3D time-of-flight (TOF) imaging in a single view in either transmission or backscatter configurations. Iterative reconstruction enables image resolution better than the inherent TOF resolution. 2.Decomposition of registered neutron and x-ray radiographs into an assumed material list for each pixel in the image. 3.Material identification using full spectral analysis that includes the emergent neutron and gamma ray energies, times, and angles. Progress for each approach is summarized for fiscal year (FY) 2022.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Fast timing with µRWELL-PICOSEC detector technology

The µWELL-PICOSEC detector, which is based on Resistive Micro-Well (µRWELL) technology, is a novel concept for fast timing gaseous detectors that can provide timing resolution in the tens of picosecond range, making it ideal candidate for time-of-flight (TOF) technology for particle identification (PID) in particle physics experiments as well as for future medical instrumentation. The µRWELL-PICOSEC concept is based on a Cerenkov radiator that produces Cerenkov photons from high energetic charged particles, a photocathode layer that converts the Cerenkov photons into primary electrons, a µRWELL amplification layer that multiply the electrons through amplification in a CF4-based gas mixture and a pad-segmentation anode readout coupled with fast timing electronics to provide fast signal. Beam tests were carried out at the CERN SPS H4 beamline in summer 2023 and 2024. Preliminary results show timing performance of the order of 23 ps achievable with µRWELL-PICOSEC prototype. and position scan of the 100-pads of a multi-channel prototype was also performed to study time response uniformity of large area detector. In this talk, after a brief overview of the PICOSEC technology, we will present recent results with different single channel µRWELL-PICOSEC prototype designs and also the position scan results of the 100-pads large prototype to study timing response uniformity for large area µRWELL-PICOSEC detector. Finally, we will discuss the ongoing R&D effort to further improve the timing resolution and allow good position capabilities through charge sharing for large area.

Gnanvo, Kondo↗
DOE OSTI2020

Angular scattering of protons through ultrathin graphene foils: Application for time-of-flight instrumentation

Space plasma instruments often rely on ultrathin carbon foils for incident ion detection, time-of-flight (TOF) mass spectrometry, and ionization of energetic neutral atoms. Angular scattering and energy loss of ions or neutral atoms in the foil can degrade instrument performance, including sensitivity and mass resolution; thus, there is an ongoing effort to manufacture thinner foils. Using new 3-layer graphene foils manufactured at the Los Alamos National Laboratory, we demonstrate that these are the thinnest foils reported to date and discuss future testing required for application in space instrumentation. We characterize the angular scattering distribution for 3–30 keV protons through the foils, which is used as a proxy for the foil thickness. We show that these foils are ~2.5–4.5 times thinner than the state-of-the-art carbon foils and ~1.6 times thinner than other graphene foils described in the literature. We find that the inverse relationship between angular scattering and energy no longer holds, reaffirming that this may indicate a new domain of beam–foil interactions for ultrathin (few-layer) graphene foils.

47 OTHER INSTRUMENTATION↗
NASA NTRS2001

Evaluating Mass Analyzers as Candidates for Small, Portable, Rugged Single Point Mass Spectrometers for Analysis of Permanent Gases

For Space Shuttle launch safety, there is a need to monitor the concentration of H2, He, O2 and Ar around the launch vehicle. Currently a large mass spectrometry system performs this task, using long transport lines to draw in samples. There is great interest in replacing this stationary system with several miniature, portable, rugged mass spectrometers which act as point sensors which can be placed at the sampling point. Five commercial and two non-commercial analyzers are evaluated. The five commercial systems include the Leybold Inficon XPR-2 linear quadrupole, the Stanford Research (SRS-100) linear quadrupole, the Ferran linear quadrupole array, the ThermoQuest Polaris-Q quadrupole ion trap, and the IonWerks Time-of-Flight (TOF). The non-commercial systems include a compact double focusing sector (CDFMS) developed at the University of Minnesota, and a quadrupole ion trap (UF-IT) developed at the University of Florida. The System Volume is determined by measuring the entire system volume including the mass analyzer, its associated electronics, the associated vacuum system, the high vacuum pump and rough pump. Also measured are any ion gauge controllers or other required equipment. Computers are not included. Scan Time is the time required for one scan to be acquired and the data to be transferred. It is determined by measuring the time required acquiring a known number of scans and dividing by said number of scans. Limit of Detection is determined first by performing a zero-span calibration (using a 10-point data set). Then the limit of detection (LOD) is defined as 3 times the standard deviation of the zero data set. (An LOD of 10 ppm or less is considered acceptable.)

Arkin, C. Richard↗
DOE OSTI2023

µRWELL-PICOSEC: The Development of Fast Timing Resistive Micro-WELL Detector Technology.

We present the development of a new concept of fast timing gaseous detector, the ?RWELL-PICOSEC detector based on Resistive Micro-Well (?RWELL) technology to provide timing resolution in the tens of picosecond range for application as time-of-flight (TOF) technology in the particle physics and medical instrumentation fields. The ?RWELL-PICOSEC technology combined a Cerenkov radiator for the generation of Cerenkov photons from high energy charged particles, a photocathode for the conversion of the produced photons into primary electrons and the ?RWELL foil for the multiplication of the electron to produce large signal on pad segmentation readout. The proof of concept of ?RWELL-PICOSEC is demonstrated with a small single-channel prototype and preliminary timing performance of 90 ps has been measured. Optimization study the amplification structure of ?RWELL-PICOSEC for the improvement of timing resolution is discussed and results on timing performance studies in beam at CERN are presented. The development of large area (100 mm × 100 mm) ?RWELL-PICOSEC and associated multichannel fast readout electronics and data acquisition system are also reported

Weisenberger, Andrew↗
DOE OSTI2024

On the instrument-dependent appearance of ion dissociation events in atom probe tomography mass spectra

The successful application of atom probe tomography (APT) relies on the accurate interpretation of the mass spectrum (i.e. m/z histogram) from a sample. Some materials yield mass spectra that are amenable to a straightforward peak assignment/ranging, however, there are many materials that produce mass spectra with features that defy simple interpretation. One such example is Ga 2 O 3 which yields mass spectra containing several broad and difficult to interpret features. Herein, we study the GaO 2+ → O 1+ + Ga 1+ dissociation and we explain how this dissociation process gives rise to broad and previously unassigned features in the mass spectrum. Trajectory simulations are performed for the dissociation reaction utilizing realistic electrostatic models and compared to experiments using commercially available straight flight and reflectron based local electrode (LE) APT instruments. It is shown that the appearance of these features is strongly dependent on the specific design of the time-of-flight (ToF) mass analyzer. Additionally, we explore how various experimental parameters can affect the appearance of the dissociation process in the one-dimensional (1D) mass spectrum and in the two-dimensional (2D) correlation histogram. While the focus of this work is on a particular dissociation process related to Ga 2 O 3 , the understanding gained in the course of these simulations and experiments should be applicable to the interpretation of dissociation processes in other materials.

47 OTHER INSTRUMENTATION↗
DOE OSTI2023

POWTEX visits POWGEN

The high-intensity time-of-flight (TOF) neutron diffractometer POWTEX for powder and texture analysis is currently being built prior to operation in the eastern guide hall of the research reactor FRM II at Garching close to Munich, Germany. Because of the world-wide 3 He crisis in 2009, the authors promptly initiated the development of 3 He-free detector alternatives that are tailor-made for the requirements of large-area diffractometers. Herein is reported the 2017 enterprise to operate one mounting unit of the final POWTEX detector on the neutron powder diffractometer POWGEN at the Spallation Neutron Source located at Oak Ridge National Laboratory, USA. As a result, presented here are the first angular- and wavelength-dependent data from the POWTEX detector, unfortunately damaged by a 50 g shock but still operating, as well as the efforts made both to characterize the transport damage and to successfully recalibrate the voxel positions in order to yield nonetheless reliable measurements. Also described is the current data reduction process using the PowderReduceP2D algorithm implemented in Mantid [Arnold et al. (2014). Nucl. Instrum. Methods Phys. Res. A , 764 , 156–166]. The final part of the data treatment chain, namely a novel multi-dimensional refinement using a modified version of the GSAS-II software suite [Toby & Von Dreele (2013). J. Appl. Cryst. 46 , 544–549], is compared with a standard data treatment of the same event data conventionally reduced as TOF diffraction patterns and refined with the unmodified version of GSAS-II . This involves both determining the instrumental resolution parameters using POWGEN's powdered diamond standard sample and the refinement of a friendly-user sample, BaZn(NCN) 2 . Although each structural parameter on its own looks similar upon comparing the conventional (1D) and multi-dimensional (2D) treatments, also in terms of precision, a closer view shows small but possibly significant differences. For example, the somewhat suspicious proximity of the a and b lattice parameters of BaZn(NCN) 2 crystallizing in Pbca as resulting from the 1D refinement (0.008 Å) is five times less pronounced in the 2D refinement (0.038 Å). Similar features are found when comparing bond lengths and bond angles, e.g. the two N—C—N units are less differently bent in the 1D results (173 and 175°) than in the 2D results (167 and 173°). The results are of importance not only for POWTEX but also for other neutron TOF diffractometers with large-area detectors, like POWGEN at the SNS or the future DREAM beamline at the European Spallation Source.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Imaging Bragg Edge Analysis TooLs for Engineering Structures (iBeatles)

The Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL) provides pulsed neutrons with energies varying from epithermal to cold. In preparation for VENUS, the neutron imaging beamline to be located at beam port 10, we have performed a series of experiments focused on wavelength-dependent radiography and computed tomography for a broad range of applications, from materials science to biological tissues.One of the time-of-flight (TOF) techniques that is of interest to the scientific community is the 2-dimensional mapping of phases and average crystalline plane orientation in samples both ex-situ and during applied stresses such as tensile loading and heating. This technique is known as Bragg edgeimaging and relies on the identification of changes of transmission values, fitting of the edge to measure its displacement, and thus identify the shift in lattice parameter due to stresses. One of the challenges of TOF imaging measurements is the amount of data and the inability to observe Bragg edge shifts in real time during an experiment. Thus, we have been focusing on creating a Python-based interface that allows fast data processing and instantaneous mapping and fitting of the Bragg edges, and their evolution through time. Python libraries and Jupyter notebooks have been implemented to facilitate decision making during an experiment. The advantage of the notebooks is the possibility to guide an experiment as they can quickly process and display Bragg edge data. These notebooks can be used independently, or can be combined in a Python Graphical User Interface (GUI) tool called iBeatles. This interface permits visualization and fitting of the Bragg edges, and ultimately back-projects the fitting results onto the radiographs to display a strain map. Assuming data collection has sufficient statistics, the strain mapping analysis can be performed on a pixel-by-pixel basis. This development is a step forward toward a better user experience at the future VENUS beamline in terms of live feedback and productivity. Analysis that used to take days of switching between different applications can now be done in minutes within the

Bilheux, JeanChristophe [Oak Ridge National Labora↗
DOE OSTI2022

Nonlocal subpicosecond delay metrology using spectral quantum interference

Precise knowledge of position and timing information is critical to support elementary protocols such as entanglement swapping on quantum networks. While approaches have been devised to use quantum light for such metrology, they largely rely on time-of-flight (ToF) measurements with single-photon detectors and, therefore, are limited to picosecond-scale resolution owing to detector jitter. In this work, we demonstrate an approach to distributed sensing that leverages phase modulation to map changes in the spectral phase to coincidence probability, thereby overcoming the limits imposed by single-photon detection. By extracting information about the joint biphoton phase, we measure a generalized delay—the difference in signal–idler arrival, relative to local radio frequency (RF) phase modulation. For nonlocal ranging measurements, we achieve (2$σ$) precision of ±0.04 ps and for measurements of the relative RF phase, (2$σ$) precision of ±0.7°. We complement this fine timing information with ToF data from single-photon time-tagging to demonstrate absolute measurement of time delay. By relying on off-the-shelf telecommunications equipment and standard quantum resources, this approach has the potential to reduce overhead in practical quantum networks.

42 ENGINEERING↗
DOE OSTI2024

Proton discrimination in CLYC for fast neutron spectroscopy

The Cs 2 LiYCl 6 :Ce (CLYC) elpasolite scintillator is known for its response to fast and thermal neutrons along with good γ-ray energy resolution. While the 35 Cl(n,p) reaction has been identified as a potential means for CLYC-based fast neutron spectroscopy in the absence of time-of-flight (TOF), previous efforts to functionalize CLYC as a fast neutron spectrometer have been thwarted by the inability to isolate proton interactions from 6 Li(n,α) and 35 Cl(n,α) signals. This work introduces a new approach to particle discrimination in CLYC for fission spectrum neutrons using a multi-gate charge integration algorithm that provides excellent separation between protons and heavier charged particles. Neutron TOF data were collected using a 252 Cf source, an array of EJ-309 organic liquid scintillators, and a 6 Li-enriched CLYC scintillator outfitted with fast electronics. Modal waveforms were constructed corresponding to the different reaction channels, revealing significant differences in the pulse characteristics of protons and heavier charged particles at ultrafast, fast, and intermediate time scales. These findings informed the design of a pulse shape discrimination algorithm, which was validated using the TOF data. This study also proposes an iterative subtraction method to mitigate contributions from confounding reaction channels in proton and heavier charged particle pulse height spectra, opening the door for CLYC-based fast neutron and γ-ray spectroscopy while preserving sensitivity to thermal neutron capture signals.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Optimizing Transmission of Acoustic Signals to Monitor Internal Conditions of Canisters for Dry Storage of Commercial Spent Nuclear Fuel

Safe storage of spent nuclear fuel (SNF) is critical to the nuclear fuel cycle and the future of nuclear energy. In the United States, SNF is stored primarily via two methods regulated by the U.S. Nuclear Regulatory Commission: wet storage in SNF pools and dry storage in dry cask storage systems (DCSSs). After about five years of cooling in spent fuel pools, the fuel assemblies are transferred into DCSSs, and the systems are filled with helium and sealed by welding. Deterioration of conditions inside of a DCSS is reflected in changes in the internal gas properties; this motivates the development of acoustic techniques to monitor internal gas properties, over extended storage periods, using sensors mounted on the exterior of the storage packages. However, a major challenge in collecting acoustic signals is the impedance mismatch between the steel canister shell and the gas. Only a small fraction of the ultrasonic signal can be transmitted through the gas medium. This paper documents experimental studies conducted on a full-scale canister mock-up to capture the gas-borne signals. Damping materials were pasted on the outside, and blocking and unblocking tests were conducted to identify the gas-borne signal. The results show that the excitation frequency plays an important role in maximizing the gas-borne signals. The gas-borne signal was successfully detected at around the theoretical time-of-flight. A high signal-to-noise ratio was achieved in the measurements. Next, the acoustic impedance matching layers were introduced, and the gas signal was drastically improved compared with that using no AIM layers.

Spent nuclear fuel (SNF), Canisters, Internal cond↗
DOE OSTI2024

Performance of the ATLAS forward proton Time-of-Flight detector in Run 2

We present performance studies of the Time-of-Flight (ToF) subdetector of the ATLAS Forward Proton (AFP) detector at the LHC. Efficiencies and resolutions are measured using high-statistics data samples collected at low and moderate pile-up in 2017, the first year when the detectors were installed on both sides of the interaction region. While low efficiencies are observed, of the order of a few percent, the resolutions of the two ToF detectors measured individually are 21 ps and 28 ps, yielding an expected resolution of the longitudinal position of the interaction, z vtx , in the central ATLAS detector of 5.3 ± 0.6 mm. This is in agreement with the observed width of the distribution of the difference between z vtx , measured independently by the central ATLAS tracker and by the ToF detector, of 6.0 ± 2.0 mm.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2025

Influence of Photoemission Geometry on Timing and Efficiency in 4D Ultrafast Electron Microscopy

Broader adoption of 4D ultrafast electron microscopy (UEM) for the study of chemical, materials, and quantum systems is being driven by development of new instruments as well as continuous improvement and characterization of existing technologies. Perhaps owing to the still-high barrier to entry, the full range of capabilities of laser-driven 4D UEM instruments has yet to be established, particularly when operated at extremely low beam currents (~fA). Accordingly, with an eye on beam stability, we have conducted particle tracing simulations of unconventional off-axis photoemission geometries in a UEM equipped with a thermionic-emission gun. Specifically, we have explored the impact of experimentally adjustable parameters on the time-of-flight (TOF), the collection efficiency (CE), and the temporal width of ultrashort photoelectron packets. The adjustable parameters include the Wehnelt aperture diameter (DW), the cathode set-back position (Ztip), and the position of the femtosecond laser on the Wehnelt aperture surface relative to the optic axis (Rphoto). Notable findings include significant sensitivity of TOF to DW and Ztip, as well as non-intuitive responses of CE and temporal width to varying Rphoto. As a means to improve accessibility, practical implications and recommendations are emphasized wherever possible.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2024

Properties of the QCD matter: review of selected results from the relativistic heavy ion collider beam energy scan (RHIC BES) program

In the paper, we discuss the development of the multigap resistive plate chamber time-of-flight (TOF) technology and the production of the solenoidal tracker at RHIC (STAR) TOF detector in China at the beginning of the twenty-first century. Subsequently, recent experimental results from the first beam energy scan program (BES-I) at the Relativistic Heavy Ion Collider (RHIC) pertaining to measurements of collectivity, chirality, criticality, global polarization, strangeness, heavy flavor, dilepton and light nuclei productions are reviewed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Antihelium-3 sensitivity for the GRAMS experiment

The Gamma-Ray and AntiMatter Survey (GRAMS) is a next-generation balloon/satellite mission utilizing a Liquid Argon Time Projection Chamber (LArTPC) detector to measure both MeV gamma rays and antinuclei produced by dark matter annihilation or decay. The GRAMS can identify antihelium-3 events based on the measurements of X-rays and charged pions from the decay of the exotic atoms, Time of Flight (TOF), energy deposition, and stopping range. This paper shows the antihelium-3 sensitivity estimation using a GEANT4 Monte Carlo simulation. For the proposed long-duration balloon (LDB) flight program (35 days x 3 flights) and future satellite mission (2-year observation/10-year observation), the sensitivities become 1.47 × 10 −7 [m 2 s sr GeV/n] −1 and 1.55 × 10 −9 [m 2 s sr GeV/n] −1 /3.10 x 10 -10 [m 2 s sr GeV/n] −1 , respectively. The results indicate that GRAMS can extensively investigate various dark matter models through the antihelium-3 measurements.

Antihelium-3↗
DOE OSTI2022

Vertical gradient freeze growth of detector grade CdZnTeSe single crystals

Here, we report the growth of detector grade Cd 0.9 Zn 0.1 Te 0.97 Se 0.03 (CZTS) single crystals, a recently discovered quaternary semiconductor for room temperature radiation detection, by a vertical gradient freeze (VGF) method. VGF is a comparatively low-temperature growth method and avoids relative motion between the heater and the ampoule containing the precursor materials which minimizes any thermal drift or temperature fluctuations. As a result, CZTS single crystals with superior charge transport properties has been obtained. Growth of detector-grade CZTS single crystals using VGF method has not been reported yet. X-ray spectroscopy based elemental analysis showed that the grown crystals demonstrated the desired stoichiometry required for high resolution radiation detection. Planar detectors fabricated by deposition of gold contacts (~0.07 cm 2 ) demonstrated high bulk resistivity ~10 10 Ω-cm and a very low leakage current density of 2.8 × 10 –8 A/cm 2 at a bias of 100 V when measured at room temperature. The detectors showed excellent radiation response with 100 % charge collection efficiency when exposed to 5486 keV alpha particles. The electron mobility-lifetime (μτ) product was measured to be 3 × 10 –3 cm 2 /V using a single polarity Hecht analysis which is at par with the recently reported values measured in CZTS grown using conventional Bridgman or travelling heater method. The electron mobility has been calculated to be 964 cm 2 V –1 s –1 using a time-of-flight (TOF) method, a substantial improvement over that obtained from conventionally grown CZTS single crystals.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Impurity gas monitoring using ultrasonic sensing and neural networks: forward and inverse problems

Ultrasonic sensing is a non-invasive technique for monitoring impurity gas composition in various industrial applications where safety and regulatory compliance are crucial. In this study, ultrasonic sensing and neural networks were used to analyze impurity gases (i.e., air and argon) in helium. An experimental platform was established to acquire ultrasonic data. In the forward problem, an artificial neural network (ANN) model was used to forecast the response and time-of-flight (TOF) based on the excitation, and argon and air concentrations. The inverse problem was solved using a convolutional neural network (CNN) to predict the argon and air concentrations given the ultrasonic response and excitation. The results showed that the ANN accurately predicted the ultrasonic response and the change in TOF with concentration. As the air concentration was increased from 0 to 9.8%, the TOF sensitivity to detect argon decreased by 39.8% and 16.1% from ANN and sound speed theory, respectively. The CNN demonstrated high accuracy in predicting concentrations for inputs in the testing dataset. The application of the trained CNN indicated that it over-predicts air concentration while under-predicting the argon concentration. To improve accuracy, the predicted air and argon concentrations should be corrected by -0.992% and 1.027% bias, respectively.

47 OTHER INSTRUMENTATION↗
DOE OSTI2022

Characterization and description of a spectrum unfolding method for the $\mathrm{CATRiNA}$ neutron detector array

We report the CATRiNA deuterated neutron detector array at Florida State University consists of 16 2" x 2" and 16 $" x 2" EJ-315 detectors with characteristic light output and pulse-shape discrimination capabilities. The unique properties of the detectors, in part due to the anisotropic nature of (d,n) scattering, are used to extract the energy of neutrons via pulse-height spectrum unfolding. The unfolding method uses the light output and response matrix of the detectors to extract neutron energies, independent of the traditional time-of-flight (ToF) technique. Detailed response matrices of the CATRiNA detectors were measured at the Edwards Accelerator Laboratory at Ohio University via the 9 Be(d,n) and 27 Al(d,n) reactions. Full characterization of the detectors using digital electronics, as well as a description of the unfolding method are reported.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗