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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
NASA NTRS1981

Possible detection of far-ultraviolet line emission from a hot galactic corona

The presence of an emission-line component to the radiation field is suggested by rocket observations, at low resolution, of the spectrum of the diffuse, far-ultraviolet background near the north galactic pole. Removal of the line emission leaves a residual uniform cosmic ultraviolet background radiation of only 150 + or - 50 photons/sq cm s sr A, or about half that previously reported. The lines, which are at the wavelengths of the collisionally-excited atom emissions that have been predicted to arise from a hot galactic corona, suggest that there is no need to explain observed high-ionization states at high galactic latitudes as being due to photoionization caused by neutrino decay.

Feldman, P. D.↗
NASA NTRS2004

The Cloud Detection and UV Monitoring Experiment (CLUE)

We propose a large-area, low-power instrument to perform CLoud detection and Ultraviolet monitoring, CLUE. CLUE will combine the W detection capabilities of the NIGHTGLOW payload, with an array of infrared sensors to perform cloud slicing measurements. Missions such as EUSO and OWL which seek to measure UHE cosmic-rays at 1W20 eV use the atmosphere as a fluorescence detector. CLUE will provide several important correlated measurements for these missions, including: monitoring the atmospheric W emissions &om 330 - 400 nm, determining the ambient cloud cover during those W measurements (with active LIDAR), measuring the optical depth of the clouds (with an array of narrow band-pass IR sensors), and correlating LIDAR and IR cloud cover measurements. This talk will describe the instrument as we envision it.

Barbier, L.↗
NASA NTRS1994

The Galactic far-ultraviolet sky as seen by Faust: Modeling and observations

We test the model of the Galactic point source sky recently extended to the far-ultraviolet by Cohen (1994) against the set of Galactic far-ultraviolet point sources detected by the Far Ultraviolet Space Telescope (FAUST) experiment. We find excellent agreement between the predicted (log N, log S) and the observed source counts for a range of Galactic directions observed by Faust. At low galactic latitudes, we can directly infer the amount of interstellar extinction in a given direction associated with local molecular complexes, based on comparison of model calculations and FAUST star counts. The model can also be used to predict the statistical stellar content of any field. We compare the model predcitions with the observations of Brosch et al. (1994), who have spectroscopically studied an optically identified complete sample of FAUST objects in a region near the north Galactic pole. We have used the model to determine that the contribution of far-ultraviolet stars fainter than 6 x 10(exp -14) ergs/s/sq cm/A (the FAUST detection limit) is less than 1% of the diffuse sky brightness, and less than about 4% of the total point source flux.

Cohen, Martin↗
DOE OSTI2024

Infrared signature of the hydroperoxyalkyl intermediate (·QOOH) in cyclohexane oxidation: An isomer-resolved spectroscopic study

Infrared (IR) action spectroscopy is utilized to characterize carbon-centered hydroperoxy-cyclohexyl radicals (·QOOH) transiently formed in cyclohexane oxidation. The oxidation pathway leads to three nearly degenerate ·QOOH isomers, β-, γ-, and δ-QOOH, which are generated in the laboratory by H-atom abstraction from the corresponding ring sites of the cyclohexyl hydroperoxide (CHHP) precursor. The IR spectral features of jet-cooled and stabilized ·QOOH radicals are observed from 3590 to 7010 cm −1 (∼10–20 kcal mol −1 ) at energies in the vicinity of the transition state (TS) barrier leading to OH radicals that are detected by ultraviolet laser-induced fluorescence. The experimental approach affords selective detection of β-QOOH, arising from its significantly lower TS barrier to OH products compared to γ and δ isomers, which results in rapid unimolecular decay and near unity branching to OH products. The observed IR spectrum of β-QOOH includes fundamental and overtone OH stretch transitions, overtone CH stretch transitions, and combination bands involving OH or CH stretch with lower frequency modes. The assignment of β-QOOH spectral features is guided by anharmonic frequencies and intensities computed using second-order vibrational perturbation theory. The overtone OH stretch (2ν OH ) of β-QOOH is shifted only a few wavenumbers from that observed for the CHHP precursor, yet they are readily distinguished by their prompt vs slow dissociation rates to OH products.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1993

The ultraviolet photochemistry of diacetylene - Direct detection of primary products of the metastable C4H2* + C4H2 reaction

The products of diacetylene's ultraviolet photochemistry over the 245-220 nm region were directly determined in experiments where C4H2 was excited within a small reaction tube attached to a pulsed nozzle. The products formed in the collisions of C4H2* with C4H2 were subsequently ionized by vacuum UV radiation (at 118 nm) in the ion source of a time-of-flight mass spectrometer. It was found that the reaction of C4H2* with C4H2 produces C6H2 (+C2H2), C8H2 (+2H,H2), and C8H3 (+H), confirming the results of Glicker and Okabe (1987). Under certain conditions, secondary products were observed. Mechanisms for the observed reactions are proposed.

Bandy, Ralph E.↗
DOE OSTI2021

Dynamics of Product Branching from Radical Intermediates in Elementary Combustion Reactions (Final Technical Report)

While the total rate constant for many elementary reactions is well-characterized, understanding the product branching in complex reactions presents a formidable challenge. To gain an incisive probe of such reactions, our experiments investigate the dynamics of the product channels that arise from transient radical intermediates along the bimolecular reaction coordinates. Our recent published work uses the methodology developed in my group in the last fifteen years, using both imaging and scattering apparatuses. The experiments generate a particular isomeric form of an unstable radical intermediate along a bimolecular reaction coordinate and study the branching between the ensuing product channels of the energized radical as a function of its internal rotational and vibrational energy under collision-less conditions. The experiments use a combination of: 1) measurement of product velocity and angular distributions in a crossed laser-molecular beam apparatus, with electron bombardment detection in my lab in Chicago or 2) with tunable vacuum ultraviolet photoionization detection at Taiwan's National Synchrotron Radiation Research Center (NSRRC), and 3) velocity map imaging using state-selective REMPI and single photon VUV ionization of radical intermediates and reaction products. We also employ tunable VUV photoionization detection in our imaging apparatus, using difference frequency four-wave mixing to produce photoionization light tunable from 8 to 10.8 eV. This year of support funded our work to photolytically generate the radical intermediate important in the OH + propene reaction when OH adds to an end carbon. Our other major result this past year was on the photoionization detection of vinoxy radicals. Our experiments at the NSRRC definitively show that vinoxy dissociatively ionizes to both CH 3 + and HCO + , and establishes the absolute partial photoionization cross section of vinoxy to CH 3 + at 10.5 and 11.44 eV. This should allow experimentalists detecting vinoxy radicals produced in bimolecular reactions such as OH + propene to get good branching fractions to that product channel. Finally we initiated studies of the photodissociation of 1-bromo-2-chloroethane and 1,1-bromochloroethane at 193 nm at the NSRRC.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1994

Serendipitous EUV sources detected during the first year of the Extreme Ultraviolet Explorer right angle program

We report the detection of 114 extreme ultraviolet (EUV; 58 - 740 A) sources, of which 99 are new serendipitous sources, based on observations made with the imaging telescopes on board the Extreme Ultraviolet Explorer (EUVE) during the Right Angle Program (RAP). These data were obtained using the survey scanners and the Deep Survey instrument during the first year of the spectroscopic guest observer phase of the mission, from January 1993 to January 1994. The data set consists of 162 discrete pointings whose exposure times are typically two orders of magnitude longer than the average exposure times during the EUVE all-sky survey. Based on these results, we can expect that EUVE will serendipitously detect approximately 100 new EUV sources per year, or about one new EUV source per 10 sq deg, during the guest observer phase of the EUVE mission. New EUVE sources of note include one B star and three extragalactic objects. The B star (HR 2875, EUVE J0729 - 38.7) is detected in both the Lexan/B (approximately 100 A) and Al/Ti/C (approximately 200 A) bandpasses, and the detection is shown not to be a result of UV leaks. We suggest that we are detecting EUV and/or soft x rays from a companion to the B star. Three sources, EUVE J2132+10.1, EUVE J2343-14.9, and EUVE J2359-30.6 are identified as the active galactic nuclei MKN 1513, MS2340.9-1511, and 1H2354-315, respectively.

Mcdonald, K.↗
NASA NTRS1976

Detection of an extreme-ultraviolet source in the Southern sky

The 3700 square degrees around the South Equatorial Pole have been surveyed using a broad-band photometer with peak response at 90 A. One source was detected at about the same intensity as HZ 43. An extrapolation of the results implies that there are about 10 extreme-ultraviolet objects over the whole sky which are as bright as HZ 43. Implications of these results for theories of white dwarf evolution are briefly discussed.

Henry, P.↗
NASA NTRS1990

Flame Detector

Scientific Instruments, Inc. has now developed a second generation, commercially available instrument to detect flames in hazardous environments, typically refineries, chemical plants and offshore drilling platforms. The Model 74000 detector incorporates a sensing circuit that detects UV radiation in a 100 degree conical field of view extending as far as 250 feet from the instrument. It operates in a bandwidth that makes it virtually 'blind' to solar radiation while affording extremely high sensitivity to ultraviolet flame detection. A 'windowing' technique accurately discriminates between background UV radiation and ultraviolet emitted from an actual flame, hence the user is assured of no false alarms. Model 7410CP is a combination controller and annunciator panel designed to monitor and control as many as 24 flame detectors. *Model 74000 is no longer being manufactured.

Source record↗
DOE OSTI2022

The scintillation light detection system of ICARUS-T600: Hardware implementation and early results

The ICARUS-T600 Liquid Argon (LAr) Time Projection Chamber (TPC) is taking data with the Fermilab Booster Neutrino Beam-line (BNB) in the Short Baseline Neutrino (SBN) program to search for a possible LSND-like sterile neutrino signal. A light detection system, based on 360 Hamamatsu R5912-MOD Photo-Multiplier Tubes (PMTs) deployed behind the TPC wire chambers, has been realized to detect vacuum ultraviolet (VUV) photons produced by ionizing particles in LAr. This system is fundamental for the detector operation, providing an efficient trigger and contributing to the 3D reconstruction of events. Moreover, since the TPC is exposed to a huge flux of cosmic rays due to its shallow depths operations, the light detection system allows for the time reconstruction of events, contributing to the identification and to the selection of neutrino interactions within the beam spill gates.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Data vs. MC Comparison of Light Signal from Cosmic Rays in the ICARUS Detectors

Currently, the ICARUS-T600 liquid argon TPC is collecting data exposed to Booster Neutrino and Numi off-axis beams within the SBN program at Fermilab. A light detection system, based on PMTs deployed behind the TPC wire chambers, is in place to detect vacuum ultraviolet photons produced by ionizing particles in LAr. This system is fundamental for the detector operation, providing an efficient trigger and contributing to the 3D reconstruction of events. Moreover, since the TPC is exposed to a huge flux of cosmic rays due to its operations at shallow depths, the light detection system allows for the time reconstruction of events, contributing to the identification and to the selection of neutrino interactions within the beam spill gates. This contribution will primarily focus on the comparative study (data vs. MC) of light signal of cosmic muons to validate the light emulation.

43 PARTICLE ACCELERATORS↗
NASA NTRS2003

Isolation of Purines and Pyrimidines from the Murchison Meteorite

The origin of life on Earth, and possibly on other planets such as Mars, would have required the presence of liquid water and a continuous supply of prebiotic organic compounds. The delivery of organic matter by asteroids, comets, and carbonaceous meteorites could have contributed to the early Earth's prebiotic inventory by seeding the planet with biologically important organic compounds. A wide variety of prebiotic organic compounds have previously been detected in the Murchison CM type carbonaceous chondrite including amino acids, purines and pyrimidines'. These compounds play a major role in terrestrial biochemistry and are integral components of proteins, DNA and RNA. In this study we developed a new extraction technique using sublimation in order to isolate purines and pyrimidines from Murchison2, which is cleaner and more time efficient that traditional methods3. Several purines including adenine, guanine, hypoxanthine and xanthine were positively identified by high performance liquid chromatography and ultraviolet absorption detection in our Murchison extracts. The purines detected in Murchison do not correlate with the distribution of nucleobases found in geological environments on Earth4. Moreover, the abundance of extraterrestrial amino acids and the low level of terrestrial amino acid contaminants found in Murchison', support the idea that the purines in t h s meteorite are extraterrestrial in origin.

Glavin, D. P.↗
NASA NTRS1997

White-light coronal mass ejections: A new perspective from LASCO

More than 275 coronal mass ejections (CMEs) were recorded by the large angle spectroscopic coronagraph (LASCO) from January 1996 through August 1997. Some of the characteristics of 65 of these CMEs, occurring during a three month period (May to July 1997) were quantified. During this time the rate of CME detection was about 0.7 CMEs per day; the distribution of apparent latitudes was clustererd near the equator with an average latitude of 3 deg N; the average width of the CMEs was 49 deg; and the average speed was 324 km/s. The statistical measures and the distributions for these CMEs agree with the existing literature. One new result was the high fraction (plus or minus 35 deg) of CMEs with at least one concave-outward morphological feature, which was considered a possible signature of magnetic disconnection. A new small-scale phenomenon that appears to be the white light counterpart of the extreme ultraviolet microjets detected in the polar coronal holes is described.

St.Cyr, O. C.↗
DOE OSTI2023

Design of a Nanophotonic Hybrid Coupler

This project aims to design and simulate a nanophotonic hybrid coupler for detecting vacuum ultraviolet (VUV) light with higher efficiency. VUV light is of significant interest because of its applications ranging from high energy physics to space science and electronic industry. However, current VUV photodetectors have very low efficiencies because most materials absorb in the VUV region (100-200 nm). To address this challenge, I have designed a plasmonic-dielectric coupler with wavelength shifting properties, enabling high Purcell enhancement and far-field confinement. The coupler consists of a cylindrical cSi resonator on top of a thin ZnO layer, and Ag and SiO2 are used as substrates. Simulations are done using the finite-difference time domain method to solve Maxwell’s equations, and specifically with Meep and Lumerical. The effectiveness of the coupler is characterized by the Purcell factor and far-field radiation. The Purcell factor reaches a maximum near 390 nm and is in the o rder of 10^4. Furthermore, the coupler also allows partial control of the directionality of the far-field radiation. With the presence of the resonator, the radiation is directed towards the coupled metalens. Overall, our design combines the advantages of plasmonic and dielectric couplers, along with the intrinsic wavelength shifting properties of materials to enhance VUV detection significantly, and such a device can be used in, for example, the DUNE project.

Zhou, Jiayang↗
DOE OSTI2022

The electronic set-up for the scintillation light detection system of ICARUS-SBN at Fermilab

The ICARUS-T600 Liquid Argon (LAr) Time Projection Chamber (TPC) is presently used as the far detector of the Short Baseline Neutrino (SBN) program at Fermilab (USA) to search for a possible sterile neutrino signal with the Booster Neutrino Beam (BNB). We discuss a light detection system, based on 360 Hamamatsu R5912-MOD Photo-Multiplier Tubes (PMTs), which has been realized to detect vacuum ultraviolet (VUV) photons produced after the passage of ionizing particles in LAr. High performance electronics allows recording of the PMT signals and provides a fast discrimination for the exploitation of the scintillation light for trigger purposes. This system is fundamental for the TPC operation, contributing to the trigger system and for the 3D reconstruction of events.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗