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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Time-resolved experiments on gas-phase atoms and molecules with XUV and X-ray free-electron lasers

Over the last 20 years, XUV and X-ray free-electron lasers have enabled a wide variety of time-resolved experiments that have dramatically advanced our understanding of ultra-fast molecular dynamics on atomic length scales and femto-second time scales. This review focuses on experimental studies of ultrafast dynamics of atoms and molecules in the gas phase, tracing the development of the field from early proof-of-principle studies to recent pump-probe experiments that elucidate the coupled electronic and nuclear dynamics during photochemical reactions with a temporal resolution that is now extending into the attosecond domain.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2022

Ultrafast probing of charge transfer dynamics with an XUV free-electron laser

We study charge transfer in dissociating molecules of 2-iodopropane (C 3 H 7 I) in a UV pump – XUV probe regime at the SACLA free-electron laser. Signatures of charge transfer from the recently dissociated iodine atom to the neutral propyl radical are observed in recorded 3D ion momentum distributions. This signature has evaded observation in previous related experiments. Detailed analysis of these signatures allows the identification of a region of internuclear separation where charge transfer occurs.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2025

Chemical and Optical Control of Spin Crossover: Ultrafast XUV Spectroscopy of Molecular Magnets in Native Solvation Environments

With support from the US Department of Energy Office of Science, we have developed and utilized extreme ultraviolet (XUV) spectroscopy and sum frequency generation vibrational spectroscopy as probes of charge, spin, and solvation structure and dynamics in molecules and at interfaces. This work is crucial to advancing fundamental understanding of the processes that control the efficiency and speed of energy conversion and information processing in molecules and at interfaces. Accordingly, it has important applications for developing next generation technologies for information storage and processing with increasing data storage density and processing rates as well as developing new methods for efficient energy conversion and storage.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2022

Fragmentation Dynamics of Fluorene Explored Using Ultrafast XUV-Vis Pump-Probe Spectroscopy

We report on the use of extreme ultraviolet (XUV, 30.3 nm) radiation from the Free-electron LASer in Hamburg (FLASH) and visible (Vis, 405 nm) photons from an optical laser to investigate the relaxation and fragmentation dynamics of fluorene ions. The ultrashort laser pulses allow to resolve the molecular processes occurring on the femtosecond timescales. Fluorene is a prototypical small polycyclic aromatic hydrocarbon (PAH). Through their infrared emission signature, PAHs have been shown to be ubiquitous in the universe, and they are assumed to play an important role in the chemistry of the interstellar medium. Our experiments track the ionization and dissociative ionization products of fluorene through time-of-flight mass spectrometry and velocity-map imaging. Multiple processes involved in the formation of each of the fragment ions are disentangled through analysis of the ion images. The relaxation lifetimes of the excited fluorene monocation and dication obtained through the fragment formation channels are reported to be in the range of a few tens of femtoseconds to a few picoseconds.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1974

High angular resolution cosmic X-ray astronomy observations in the energy range 0.15-2 keV and XUV observations of nearby stars from an attitude controlled rocket

The construction of a two dimensional focusing Wolter Type I mirror system for X-ray and XUV astronomical observations from an Astrobee F sounding rocket is described. The mirror design goal will have a one degree field, a 20-arc seconds resolution, an effective area of about 50 sq cm at 1 keV and 10 sq cm at 0.25 keV on axis. A star camera provides aspect data to about 15-arc seconds. Two detectors are placed at the focus with an interchange mechanism to allow a detector change during flight. The following specific developments are reported: (1) position sensitive proportional counter development; (2) channel plate multiplier development; (3) telescope mirror development and payload structure; (4) Australian rocket flight results; (5) Comet Kohoutek He I observation; and (6) Vela, Puppis A, and Gem-Mon bright patch observations.

Garmire, G. P.↗
NASA NTRS1975

XUV results from Skylab

The extreme ultraviolet spectroheliograph of the Skylab-ATM experiment S082A recorded 1000 exposures during the mission, covering the wavelength range from 171 to 335 A or from 315 to 630 A. Each exposure recorded a spectrum of solar images with spatial resolution reaching 2 arc sec. Among the features observed were the chromospheric network, filaments, active regions, XUV bright points, the limb, spicules, prominences, coronal holes, and loops. During the mission, a number of flares were photographed; the images showed the changing form of a flare in different lines from the chromosphere to the corona as well as how this form changed during the course of the flare. The spectral images of a number of eruptive prominences were also recorded.

Tousey, R.↗
NASA NTRS1975

The intensities and profiles of XUV transition zone lines in a quiet sun region compared to a polar coronal hole

The intensities of XUV transition-zone lines from limb spectra of a quiet-sun region and a polar coronal hole are compared. The spectra were obtained with a slit spectrograph on Skylab and cover a region from -12 sec within the limb to 20 sec above it. The lines selected for comparison are formed at temperatures that range from 36,000 to 220,000 K. Lines of the higher-temperature ions, e.g. O v, are significantly less intense in the coronal hole, and lines of lower-temperature ions show little change. Profiles of selected optically thin transition-zone lines from the quiet-sun and coronal-hole spectra are also shown. The lines are broader than expected in ionization equilibrium, and bulk-motion velocities are deduced from the widths of the lines. There appears to be little, if any, statistically significant difference in the velocities obtained from the quiet-sun region and the coronal hole.

Feldman, U.↗
NASA NTRS1975

Limb-brightening curves of XUV transition zone lines in the quiet sun and in a polar coronal hole observed from Skylab

Solar limb-brightening curves are discussed for XUV spectral lines formed in the upper chromosphere and transition zone of a quiet region and a polar coronal hole. The spectra were recorded with a slit spectrograph on Skylab. The lines considered are emitted from ions formed within the temperature range from 10,000 to 220,000 K. The limb-brightening curves cover a region from -4 sec within the limb to +20 sec above it. The data from 0 sec to +20 sec are compared with predictions based on both homogeneous and inhomogeneous models of the transition zone. The limb-brightening curve of the O I line at 1355.6 A indicates that O I is formed in spicules. The limb brightening of the He II line at 1640.4 A is consistent with a temperature of formation between about 40,000 and 90,000 K for He II.

Doschek, G. A.↗
NASA NTRS1976

XUV spectrum of C I observed from Skylab during a solar flare

A list of 193 neutral carbon lines observed in the XUV spectrum of a solar flare between 100 and 2000 A using the normal incidence spectrograph flown on Skylab is presented. Of these, 69 are newly identified lines arising from transitions from upper levels of high quantum number where the quantum number is not less than six. The new lines have allowed the determination of 63 new energy levels. Wavelengths for an additional 109 transitions were calculated by polynomial fitting using reference wavelengths of unblended neutral carbon, Si, N, and S lines emitted in the same atmospheric regions of the flare. The calculated lines falling between 1102 and 1140 A were not observed due to low instrumental efficiency at these wavelengths. The calculated wavelengths are in excellent agreement with those of Johansson (1965). It appears that in solar spectra recombination processes are dominant, enhancing the populations of the high quantum levels relative to the populations of levels with small quantum numbers.

Feldman, U.↗
NASA NTRS1977

Optical contamination - Its prevention in the XUV spectrographs flown by the U.S. Naval Research Laboratory in the Apollo Telescope Mount

During construction and testing of the XUV spectrographs flown in the ATM by the Naval Research Laboratory, many problems associated with optical contamination were encountered. Solving these problems required setting up a contamination prevention program to select the materials used in constructing the instruments and to delineate procedures in assembling, testing, and storing the instruments. A brief description is given of methods of assessing the effects of contamination and of the procedures used to prevent contamination.

Hunter, W. R.↗
NASA NTRS1977

On coronal Fe abundances and temperatures from XUV emission lines

Data obtained by the OSO-7 spectroheliograph on strong XUV lines of five different Fe ions from the outer equatorial corona are presented. Interpretation of the data with a spherically symmetric model atmosphere gives average ion abundances for lines of sight at 0.3 solar radii from the limb. Fe XVI is usually more abundant than Fe XV, XIV, XII and IX, but there are times when Fe XII is more abundant than the other ions. The deviation of measured relative abundances of Fe XII, XIV, and XVI from predictions of ionization equilibrium at one temperature seems to indicate that there are appreciable temperature variations along lines of sight. Element abundances are very uncertain since they appear to depend so heavily on likely but unknown density irregularities along lines of sight.

Nakada, M. P.↗
NASA NTRS1979

Line identification and lifetime measurements in the XUV and soft X-ray regions

A summary of the data acquired concerning line identification and lifetime measurements in the xuv and soft X-ray regions for a variety of both resonance transitions and forbidden transitions in ions of astrophysical interest is provided. Particular attention is called to a few papers which appeared in the Astrophysical Journal. These are of special relevance to specific astrophysical data needs. The many experiments completed in areas related to but somewhat outside the confines of the project title are mentioned.

Sellin, I. A.↗
NASA NTRS1978

The XUV spectroheliometer on SMM

The XUV spectroheliometer for the Solar Maximum Mission (SMM) is described. This instrument is a grazing-incidence polychromatic photoelectric spectrometer illuminated by a grazing-incidence telescope mirror. The wavelength range is 20-1336 A, the spectral resolution is between 0.1 and 0.3 A, and the spatial resolution is 4 arcsec. Simultaneous spectroheliograms in twelve spectral lines are obtained by rastering the instrument at variable rates. The scientific objectives and the mission operations concept are also described.

Reeves, E. M.↗
NASA NTRS1980

CCD camera systems and support electronics for a White Light Coronagraph and X-ray XUV solar telescope

Two instruments, a White Light Coronagraph and an X-ray XUV telescope built into the same housing, share several electronic functions. Each instrument uses a CCD as an imaging detector, but due to different spectral requirements, each uses a different type. Hardware reduction, required by the stringent weight and volume allocations of the interplanetary mission, is made possible by the use of a microprocessor. Most instrument functions are software controlled with the end use circuits treated as peripherals to the microprocessor. The instruments are being developed for the International Solar Polar Mission.

Harrison, D. C.↗