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At least 55 records · Page 3

ExoReL{sup R}: A Bayesian Inverse Retrieval Framework for Exoplanetary Reflected Light Spectra

The high-contrast imaging technique is meant to provide insight into those planets orbiting several astronomical units from their host star. Space missions such as Wide-Field InfraRed Survey Telescope, Habitable Exoplanet Imaging Mission, and Large Ultra-Violet/Optical/InfraRed Surveyor will measure reflected light spectra of cold gaseous and rocky planets. To interpret these observations, we introduce ExoReL{sup R} (Exoplanetary Reflected Light Retrieval), a novel Bayesian retrieval framework to retrieve cloud properties and atmospheric structures from exoplanetary reflected light spectra. As a unique feature, it assumes a vertically nonuniform volume mixing ratio (VMR) profile of water and ammonia, and uses it to construct cloud densities. In this way, clouds and molecular mixture ratios are consistent. We apply ExoReL{sup R} on three test cases: two exoplanets (υ And e and 47 Uma b) and Jupiter. We show that we are able to retrieve the concentration of methane in the atmosphere, and estimate the position of clouds when the signal-to-noise ratio of the spectrum is higher than 15, in line with previous works. Moreover, we described the ability of our model to give a chemical identity to clouds, and we discussed whether or not we can observe this difference in the planetary reflection spectrum. Finally, we demonstrate how it could be possible to retrieve molecular concentrations (water and ammonia in this work) below the clouds by linking the nonuniform VMR profile to the cloud presence. This will help to constrain the concentration of water and ammonia unseen in direct measurements.

79 ASTRONOMY AND ASTROPHYSICS↗

Reducing uncertainties in satellite estimates of aerosol–cloud interactions over the subtropical ocean by integrating vertically resolved aerosol observations

Satellite quantification of aerosol effects on clouds relies on aerosol optical depth (AOD) as a proxy for aerosol concentration or cloud condensation nuclei (CCN). However, the lack of error characterization of satellite-based results hampers their use for the evaluation and improvement of global climate models. We show that the use of AOD for assessing aerosol–cloud interactions (ACIs) is inadequate over vast oceanic areas in the subtropics. Instead, we postulate that a more physical approach that consists of matching vertically resolved aerosol data from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite at the cloud-layer height with Moderate Resolution Imaging Spectroradiometer (MODIS) Aqua cloud retrievals reduces uncertainties in satellite-based ACI estimates. Combined aerosol extinction coefficients (σ) below cloud top (σBC) from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and cloud droplet number concentrations (N d ) from MODIS Aqua yield high correlations across a broad range of σBC values, with σBC quartile correlations ≥0.78. In contrast, CALIOP-based AOD yields correlations with MODIS Nd of 0.54–0.62 for the two lower AOD quartiles. Moreover, σBC explains 41% of the spatial variance in MODIS N d , whereas AOD only explains 17%, primarily caused by the lack of spatial covariability in the eastern Pacific. Compared with σBC, near-surface σ weakly correlates in space with MODIS N d , accounting for a 16% variance. It is concluded that the linear regression calculated from ln(N d )–ln(σBC) (the standard method for quantifying ACIs) is more physically meaningful than that derived from the Nd–AOD pair.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

WASP-117 b: An Eccentric Hot Saturn as a Future Complex Chemistry Laboratory

We present spectral analysis of the transiting Saturn-mass planet WASP-117 b, observed with the G141 grism of the Hubble Space Telescope's (HST) Wide Field Camera 3. We reduce and fit the extracted spectrum from the raw transmission data using the open-source software Iraclis before performing a fully Bayesian retrieval using the publicly available analysis suite TauREx 3.0. We detect water vapor alongside a layer of fully opaque cloud, retrieving a terminator temperature of T{sub term}=833{sub -156}{sup +260} K. In order to quantify the statistical significance of this detection, we employ the atmospheric detectability index (ADI), deriving a value of ADI = 2.30, which provides positive but not strong evidence against the flat-line model. Due to the eccentric orbit of WASP-117 b, it is likely that chemical and mixing timescales oscillate throughout orbit due to the changing temperature, possibly allowing warmer chemistry to remain visible as the planet begins transit, despite the proximity of its point of ingress to apastron. We present simulated spectra of the planet as would be observed by the future space missions such as the Atmospheric Remote-sensing Infrared Exoplanet Large-survey and the James Webb Space Telescope and show that, despite not being able to probe such chemistry with current HST data, these observatories should make it possible in the not too distant future.

79 ASTRONOMY AND ASTROPHYSICS↗

Micropulse Lidar Cloud Mask (MPLCMASK) Value-Added Product for the Fast-Switching Polarized Micropulse Lidar Technical Report

Lidar backscattered signal is a useful tool for identifying vertical cloud structure in the atmosphere in optically thin clouds. Cloud boundaries derived from lidar signals are a necessary input for popular ARM data products, such as the Active Remote Sensing of Clouds (ARSCL) product. An operational cloud boundary algorithm (Wang and Sassen 2001) has been implemented for use with the ARM Micropulse Lidar (MPL) systems. In addition to retrieving cloud boundaries above 500 m, the value-added product (VAP) named Micropulse Lidar Cloud Mask (MPLCMASK) applies lidar-specific corrections (i.e., range-square, background, deadtime, and overlap) as described in Campbell et al. (2002) to the measured backscattered lidar. Depolarization ratio is computed using the methodology developed by Flynn et al. (2007) for polarization-capable MPL systems. The cloud boundaries output from MPLCMASK will be the primary lidar cloud mask for input to the ARSCL product and will be applied to all MPL systems, including historical data sets.

54 ENVIRONMENTAL SCIENCES↗

What Are the Similarities and Differences in Marine Boundary Layer Cloud and Drizzle Microphysical Properties During the ACE–ENA and MARCUS Field Campaigns?

This study compares macrophysical and microphysical properties of single-layered, liquid-dominant MBL clouds from the Measurements of Aerosols, Radiation, and Clouds over the Southern Ocean (MARCUS) (above 60°S) and the ARM East North Atlantic (ENA) site during the Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA) field campaign. A total of 1,136 (16.5% of clouds) and 6,034 5-min cloud samples are selected from MARCUS and ARM ENA in this study. MARCUS clouds have higher cloud-top heights, thicker cloud layers, larger liquid water path, and colder cloud temperatures than ENA. Thinner, warmer MBL clouds at ENA can contain higher layer-mean liquid water content due to higher cloud and ocean surface temperatures along with greater precipitable water vapor (PWV). MARCUS has a higher drizzle frequency rate (71.8%) than ENA (45.1%). Retrieved cloud and drizzle microphysical properties from each field campaign show key differences. MARCUS clouds feature smaller cloud droplets, whereas ENA clouds have larger cloud droplets, especially at the upper region of the cloud. From cloud top to cloud base, drizzle drop sizes increase while number concentrations decrease. Drizzle drop radius and number concentration decrease from cloud base to drizzle base due to net evaporation, and MARCUS' lower specific humidity leads to a higher drizzle base than ENA. In conclusion, the broader surface pressure and lower tropospheric stability (LTS) distributions during MARCUS have demonstrated that there are different synoptic patterns for selected cases during MARCUS with less PWV, while ENA is dominated by high pressure systems with nearly doubled PWV.

54 ENVIRONMENTAL SCIENCES↗

Cloud optical depth and liquid effective radius retrievals from SPHOT zenith radiances

A new three-channel (440, 870, and 1640 nm) retrieval algorithm for cloud optical depth has recently been developed by Christine Chiu and her co-workers [Chiu et al., 2012]. This VAP is to implement the three-channel cloud optical depth retrieval algorithm as an ARM operational VAP. First, simultaneously retrieved cloud optical depth and effective radius datasets will be generated by using the pre-calibrated zenith radiance measurements taken from the ARM Sun-Photometer (SPHOT) and the NASA AERONET and Satellite-based surface albedo derived from MODSI. Finally, the algorithm produces uncertainties along with the retrieval products. This VAP outputs a daily NetCDF file.

54 ENVIRONMENTAL SCIENCES↗

Daytime variation in the aerosol indirect effect for warm marine boundary layer clouds in the eastern North Atlantic

Abstract. Warm boundary layer clouds in the eastern North Atlantic region exhibit significant diurnal variations in cloud properties. However, the diurnal cycle of the aerosol indirect effect (AIE) for these clouds remains poorly understood. This study takes advantage of recent advancements in the spatial resolution of geostationary satellites to explore the daytime variation in the AIE by estimating the cloud susceptibilities to changes in cloud droplet number concentration (Nd). Cloud retrievals for the month of July over 4 years (2018–2021) from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) on Meteosat-11 over this region are analyzed. Our results reveal a significant “U-shaped” daytime cycle in susceptibilities of the cloud liquid water path (LWP), cloud albedo, and cloud fraction. Clouds are found to be more susceptible to Nd perturbations at noon and less susceptible in the morning and evening. The magnitude and sign of cloud susceptibilities depend heavily on the cloud state defined by cloud LWP and precipitation conditions. Non-precipitating thin clouds account for 44 % of all warm boundary layer clouds in July, and they contribute the most to the observed daytime variation. Non-precipitating thick clouds are the least frequent cloud state (10 %), and they exhibit more negative LWP and albedo susceptibilities compared to thin clouds. Precipitating clouds are the dominant cloud state (46 %), but their cloud susceptibilities show minimal variation throughout the day. We find evidence that the daytime variation in LWP and albedo susceptibilities for non-precipitating clouds is influenced by a combination of the diurnal transition between non-precipitating thick and thin clouds and the “lagged” cloud responses to Nd perturbations. The daytime variation in cloud fraction susceptibility for non-precipitating thick clouds can be attributed to the daytime variation in cloud morphology (e.g., overcast or broken). The dissipation and development of clouds do not adequately explain the observed variation in cloud susceptibilities. Additionally, daytime variation in cloud susceptibility is primarily driven by variation in the intensity of cloud response rather than the frequency of occurrence of cloud states. Our results imply that polar-orbiting satellites with an overpass time at 13:30 LT underestimate daytime mean values of cloud susceptibility, as they observe susceptibility daily minima in the study region.

54 ENVIRONMENTAL SCIENCES↗

Deep Convection Initiation, Growth, and Environments in the Complex Terrain of Central Argentina during CACTI

This study characterizes the wide range of deep convective cloud life cycles and their relationships with ambient environments observed during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign near the Sierras de Córdoba (SDC) range in central Argentina. We develop a novel convective cell tracking database for the entire field campaign using C-band polarimetric radar observations. The cell tracking database includes timing, location, area, depth, merge/split information, microphysical properties, collocated satellite-retrieved cloud properties, and sounding-derived environmental conditions. Results show that the SDC exerts a strong control on convection initiation (CI) and growth. CI preferentially occurs east of the SDC ridge during the afternoon, and cells often undergo upscale growth through the evening as they travel eastward toward the plains. Larger and more intense cells tend to occur in more unstable and humid low-level environments, and surface-based cells are stronger than elevated cells. Midtropospheric relative humidity and vertical wind shear also jointly affect the size and depth of the cells. Rapid cell area growth rates exhibit dependence on both large environmental wind shear and low-level moisture. Evolution of convective cell macro- and microphysical properties are strongly influenced by convective available potential energy and low-level humidity, as well as the presence of other cells in their vicinity. This cell tracking database demonstrates a framework that ties measurements from various platforms centering around convective life cycles to facilitate process understanding of factors that control convective evolution.

54 ENVIRONMENTAL SCIENCES↗

EPCAPE Stratiform Cloud Analysis for Radiative Properties Experiment (SCARPE) Field Campaign Report

A unique attribute of the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) is the availability of an elevated secondary measurement site just 5 km from the main U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) Mobile Facility (AMF) deployment on Scripps Pier. Mount Soledad, at 250 m elevation, offers the ability to frequently measure aerosol chemical and microphysical properties within the low-level Eastern Pacific coastal stratiform clouds that the AMF is observing from below. Based on the EPCAPE experiment design to deploy three major systems on Mount Soledad—the scanning radars, the Russell aerosol mobile laboratory, and an ARM microwave radiometer (MWR)—an additional plan was made to deploy a suite of Eppley Laboratory radiometers at this site to measure the radiative response to instantaneous changes in observed aerosol properties and MWR retrieved cloud liquid water path (LWP). This supplemental field campaign was proposed as the Stratiform Cloud Analysis for Radiative Properties Experiment (SCARPE).

54 ENVIRONMENTAL SCIENCES↗

Evidence for the 3D Radiative Effects of Boundary-Layer Clouds From Observations of Direct and Diffuse Surface Solar Fluxes

Numerical experiments have revealed the importance of horizontal transport of light in the presence of clouds (“3D effects”), with consequences for climate, weather, and solar resource availability predictions. Yet, analysis of 3D effects from observations remain sparse because of the difficulty to isolate the effect of horizontal transport in radiation measurements. In this study, we provide observational evidence for 3D effects based on the direct-diffuse partition of surface solar fluxes. It is compared to outputs from the ecRad radiative transfer scheme run on retrieved cloud profiles. Furthermore, the direct-beam calculation takes careful account of the field-of-view of the pyrheliometer to ensure consistency between observed and modeled direct fluxes. Only the solver that accounts for 3D effects is able to reproduce the observed mean direct-diffuse partition as a function of solar zenith angle and cloud cover, in particular at large solar zenith angles where cloud sides intercept most of the direct beam.

54 ENVIRONMENTAL SCIENCES↗

Cloud-atmosphere impacts on the central Arctic surface energy budget (Final Report)

This project investigated how clouds and atmosphere-sea ice interactions shape the central Arctic surface energy budget using observations from the MOSAiC expedition and coordinated model experiments. Analyses focused on three themes. First, a new method applied to thermistor string data revealed that snow thermal conductivity is systematically higher than assumed in most models, strongly influencing conductive heat flux and sea ice growth, especially under clear skies. Second, a full annual cycle of surface energy budget observations, combined with detailed cloud microphysical retrievals, demonstrated how cloud regimes regulate radiative, turbulent, and conductive fluxes, driving seasonal contrasts in sea ice energy balance: in winter, radiative forcing elicits strong turbulent and conductive responses, while in summer excess energy is primarily partitioned into surface melt. Third, these observations were used to evaluate and improve regional and global forecast models. While some models captured key Arctic cloud-radiation states, most exhibited persistent deficiencies in representing liquid-containing clouds, snow-on-sea-ice processes, and flux responses to radiative forcing. Together, these results provide unprecedented benchmarks for understanding coupled Arctic processes, improve parameterizations of snow, sea ice, and cloud interactions, and highlight critical pathways by which atmospheric variability drives sea ice change in a rapidly evolving Arctic system. Lastly, the project was a resounding success, resulting in 38 peer-reviewed publications and dozens of presentations, while also supporting an early career scientist.

54 ENVIRONMENTAL SCIENCES↗

Retrieved Number concentration of Cloud Condensation Nuclei (RNCCN) Value-Added Product (VAP)

The objective of Retrieved Number concentration of Cloud Condensation Nuclei (RNCCN) Value-Added Product (VAP) is to provide the vertical distribution of cloud condensation nuclei (CCN) number concentrations to better represent aerosol indirect effects in climate models. The RNCCN VAP allows to collect a large number of independent samples of vertical CCN measurements at various supersaturation values from the ground. This helps to avoid the high cost of aircraft and increases the temporal distribution of retrieved CCN in the planetary boundary layer. The VAP method is based on Ghan and Collins (2004) and Ghan et al. (2006) proposed parameterizations that retrieve the vertical profiles of CCN directly from the ground level CCN, humidification factor, and in-situ lidar measurements. Further, the VAP accuracy is improved by using the quality controlled data that ensures that the boundary layer is well mixed.

54 ENVIRONMENTAL SCIENCES↗

Arctic Cloud‐Base Ice Precipitation Properties Retrieved Using Bayesian Inference

Abstract Cloud‐climate feedbacks are still the greatest source of uncertainty in current climate projections. Arctic clouds, which are predominantly stratiform and supercooled, often long‐lived, and nearly continuously precipitate ice particles, contribute roughly 10% of the uncertainty attributed to the global cloud feedback. This Arctic cloud uncertainty is driven by incomplete observational and theoretical knowledge required to estimate and explain the state and active processes occurring in those clouds. A focus on ice precipitation properties at Arctic cloud base rather than the surface deconfounds the product of cloud condensate sink processes from the influence of the atmospheric thermodynamic state below cloud base, rendering cloud‐base properties a more appealing target for inference and evaluation of model simulations. Here I describe an inverse model for the estimation of cloud base ice precipitation properties over Utqiagvik, North Slope of Alaska, using the synthesis of ground‐based radar and lidar measurements. By leveraging a Markov Chain Monte Carlo algorithm as the core of the inverse model, a wide range of particle size distributions are sampled, and different combinations of ice habit models are examined, both of which are typically fixed in other retrieval methods. Results show intriguing links between different cloud base thermodynamic and ice precipitation properties. Apparent ice number concentration enhancements at temperatures of −5 and −15°C suggest possible secondary ice production (SIP). The analysis alludes to an overestimation of SIP occurrence and intensity, especially in studies relying only on radar or lidar measurements. Finally, reflectivity‐dependent ice precipitation rate and ice water content parameterizations are presented.

54 ENVIRONMENTAL SCIENCES↗

TWST Cloud Properties (COD, droplet effective radius, and thermodynamic phase). SAIL, AMF2, 2022-2023.

The dataset consists of calibrated zenith shortwave spectral radiances (440-1700 nm) and cloud optical depth (COD) retrievals approximately every second. Retrievals of cloud droplet effective radius and thermodynamic phase are currently done offline, but some of these retrievals are included in the dataset. Effective radius and phase are included for days with periods of sufficiently high COD. Effective radius and phase retrievals in the data set were computed at approximately 5-10 second intervals to reduce computation time. The retrievals can be performed at the full sample rate. The field of view is 0.5 degree.

54 ENVIRONMENTAL SCIENCES↗

Geostationary Satellite Retrievals with Irradiances and Cloud Properties / Processed Data

The Geostationary Operational Environmental Satellite (GOES) records sky brightness temperatures and irradiances at several wavelengths. From these the cloud microphysical and optical properties can be routinely retrieved. These properties are derived using the technique proposed by Minnis et al. 2020, and is similar to the technique used for deriving cloud properties from Moderate Resolution Imaging Spectroradiometer (MODIS) data. The derived GOES properties for the duration of the second Wind Forecasting Improvement Project (WFIP2) within the domain are reported here. Nominally the retrieved dataset has a 30- minute temporal and a 9 km spatial resolution.

17 WIND ENERGY↗

A new classification of satellite-derived liquid water cloud regimes at cloud scale

Clouds are highly variable in time and space, affecting climate sensitivity and climate change. To study and distinguish the different influences of clouds on the climate system, it is useful to separate clouds into individual cloud regimes. In this work we present a new cloud classification for liquid water clouds at cloud scale defined using cloud parameters retrieved from combined satellite measurements from CloudSat and CALIPSO. The idea is that cloud heterogeneity is a measure that allows us to distinguish cumuliform and stratiform clouds, and cloud-base height is a measure to distinguish cloud altitude. The approach makes use of a newly developed cloud-base height retrieval. Using three cloud-base height intervals and two intervals of cloud-top variability as an inhomogeneity parameter provides six new liquid cloud classes. The results show a smooth transition between marine and continental clouds as well as between stratiform and cumuliform clouds in different latitudes at the high spatial resolution of about 20 km. Analysing the micro- and macrophysical cloud parameters from collocated combined MODIS, CloudSat and CALIPSO retrievals shows distinct characteristics for each cloud regime that are in agreement with expectation and literature. This demonstrates the usefulness of the classification.

54 ENVIRONMENTAL SCIENCES↗

Cloud Shortwave Optical Properties

The data set consists of calibrated zenith shortwave spectral radiances (400-950 nm and 940-1665 nm) and cloud optical depth (COD) retrievals every 2 seconds. The field of view is 0.5 degree. Retrievals of cloud droplet effective radius and thermodynamic phase are currently experimental and done offline. Effective radius and phase are not in this data set.

54 ENVIRONMENTAL SCIENCES↗