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Results for “decaying mechanism”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Unitarity of quantum tunneling decay for an analytical exact non-Hermitian resonant-state approach

Highlights: • Foundations of quantum mechanics • Quantum decay • Non-Hermitian Hamiltonian • Unitarity • Resonant state By using an analytical exact non-Hermitian formalism for quantum tunneling decay that involves the expansion of the decaying wave function as a linear combination of resonant states and transient functions associated with the complex poles of the outgoing Green’s function to the problem, it is shown that the integrated decaying probability density in the whole space satisfies unitarity at each value of time.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Ab Initio Calculation of the Contact Operator Contribution in the Standard Mechanism for Neutrinoless Double Beta Decay

Starting from chiral nuclear interactions, we evaluate the contribution of the leading-order contact transition operator to the nuclear matrix element (NME) of neutrinoless double-beta decay, assuming a light Majorana neutrino-exchange mechanism. The corresponding low-energy constant (LEC) is determined by fitting the transition amplitude of the nn → ppe – e – process to a recently proposed synthetic datum. We examine the dependence of the amplitude on similarity renormalization group (SRG) scale and chiral expansion order of the nuclear interaction, finding that both dependences can be compensated to a large extent by readjusting the LEC. We evaluate the contribution of both the leading-order contact operator and standard long-range operator to the neutrinoless double-beta decays in the light nuclei 6,8 He and the candidate nucleus 48 Ca. Furthermore, our results provide the first clear demonstration that the contact term enhances the NME by 43(7)% in 48 Ca, where the uncertainty is propagated from the synthetic datum.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Distinct Mechanisms of Triplet Pair Decay in Amorphous and Crystalline Heteroacene Thin Films

Triplet pairs (TT) in crystalline molecular semiconductors have unique spin properties of interest for quantum information or enhancing solar photoconversion. The population and diffusion dynamics of TT have been the subject of recent studies, both in covalent dimers and in crystalline systems. Here, in this study, we monitor the triplet population in neat polycrystalline and amorphous films of a heteroacene with known TT spectral properties and tunable spin polarization depending on the intermolecular geometry. Transient measurements reveal an anomalous power dependence in polycrystalline films that we attribute to the fast diffusion and interaction of dissociated triplet pairs confined to one-dimensional stacks of strongly coupled molecules. The nongeminate triplet interaction after dephasing facilitates conversion to the triplet 3 TT and eventually T 1 +S 0 . Amorphous films have no power dependence and proceed directly from 1 TT to 3 TT and subsequently T 1 +S 0 via state mixing facilitated by nonparallel geometries and weak exchange coupling.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Numerical Modeling of Air-Blast Suppression as a Function of Explosive-Charge Burial Depth

As a chemical explosion is buried, the mechanism for acoustic wave generation transitions from fully gas-generated at the surface to completely spall-induced at full containment depth. The fully gas-generated and completely spall-induced signals in the acoustic waveform are well described; however, the transition between these two end-members eludes numerical modeling because of the complex phenomena that are involved. The phenomena of crater formation and explosive cloud evolution are simulated using an Eulerian hydrocode that incorporates geomaterials with strength and porosity. Having accurately modeled these phenomena, we can confidently predict the propagation and relative strength of the gas-generated and spall-induced pulses in the recorded acoustic waveform. The numerical predictions agree with observations from the historical Stagecoach experiment as well as modern recordings from the Source Physics Experiment. In particular, the peak pressure p generated by an explosion is initially due to the gas-generated mechanism and decays with scaled depth of burial d s (depth d scaled by the cube-root of explosive yield w 1/3 ) as exp(-d s ) but then transitions near a scaled depth of 6 m/ton 1/3 to the spall-generated mechanism in which the decay is d$_{s}^{-7/4}$. This decay form is related to the strong ground-motion attenuation relationship that affects spall strength. So these results can improve seismoacoustic inverse models for the explosive source that need to account for the gas-generated and spall-induced signals and their effect on peak pressures and other acoustic signal features.

58 GEOSCIENCES↗
DOE OSTI2025

Chemical Interface Damping Revealed by Single-Particle Absorption Spectroscopy

Plasmon-induced interfacial charge separation is a promising way to efficiently extract energetic carriers through direct plasmon decay. This mechanism of charge transfer has been investigated by single-particle scattering spectroscopy, which measures the homogeneous plasmon line width. The line width is broadened by charge transfer, generally known as chemical interface damping. However, conflicting reports exist regarding the effect of chemical interface damping on the corresponding single-particle absorption spectrum, which is needed to accurately determine absolute light conversion efficiencies. This work aims to resolve this question by directly correlating absorption and scattering spectra of individual gold nanorods in the presence and absence of a charge-accepting interface. We find that for TiO 2 coated nanorods, the absorption line width is indeed broadened due to chemical interface damping but is overall narrower than the scattering line width. Here, chemical interface damping is furthermore found to increase with larger resonance energies. The observed differences in line widths between absorption and scattering are elucidated within the context of an analytically tractable model describing the lowest energy optically bright and higher-order optically dark plasmon modes of the nanorod, including bulk, radiative, and chemical interface damping effects. Taken together, these results establish that single-particle absorption spectroscopy is capable of revealing interfacial charge injection by direct plasmon decay.

absorption↗
DOE OSTI2023

Probing the nonexponential decay regime in open quantum systems

The most important law of radioactivity is that of the exponential decay. In the realm of quantum mechanics, however, this decay law is neither rigorous nor fundamental. The deviations from the exponential decay have been observed experimentally at the early stage of a decay process, but there is little evidence for non-exponential behavior at long times. Yet such long-term non-exponentiality is expected theoretically to probe the non-resonant background components of the initial wave function which preserve the structural interference and the memory of how the state was created. In this paper, we propose new observables that can be used for experimental investigations of the post-exponential decay regime, including the decay of threshold resonances, particle correlations in three-body decays, and interference between near-lying resonances. While the specific examples presented in this work pertain to atomic nuclei, the properties of non-exponential decay are generic, i.e., they apply to other many-body open quantum systems, such as hadrons, atoms, molecules, and nanostructures.

6 ≤ A ≤ 19↗
DOE OSTI2023

Spin dynamics in quantum dots on liquid helium

Liquid He-4 is free from magnetic defects, making it an ideal substrate for electrons with long-lived spin states. Such states can serve as qubit states. Here, in this study, we consider the spin states of electrons electrostatically localized in quantum dots on a helium surface. Efficient gate operations in this system require spin-orbit coupling. It can be created by a nonuniform magnetic field from a current-carrying wire, can be turned on and off, and allows one to obtain large electrodipole moment and comparatively fast coupling of spins in neighboring dots. Of central importance is to understand spin decay due to the spin-orbit coupling. We establish the leading mechanism of such decay and show that the decay is sufficiently slow to enable high-fidelity single- and two-qubit gate operations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

R -parity violation axiogenesis

We show that the rotation of the QCD axion field, aided by B–L violation from supersymmetric R-parity violating couplings, can yield the observed baryon abundance. Strong sphaleron processes transfer the angular momentum of the axion field into a quark chiral asymmetry, which R-parity violating couplings convert to the baryon asymmetry of the Universe. We focus on the case of dimensionless R-parity violating couplings with textures motivated by grand unified theories and comment on more general scenarios. The axion decay constant and mass spectrum of supersymmetric particles are constrained by Big Bang nucleosynthesis, proton decay from the R-parity violation, and successful thermalization of the Peccei-Quinn symmetry breaking field. Axion dark matter may be produced by the axion rotation via the kinetic misalignment mechanism for axion decay constants below 10 10 GeV, or by the conventional misalignment mechanism for 10 11-12 GeV. The viable parameter region can be probed by proton decay and axion searches. This scenario may also have connections with collider experiments, including searches for long-lived particles, and observations of gravitational waves.

Beyond Standard Model↗
DOE OSTI2025

Predicting Pulsed-Laser Deposition SrTiO 3 Homoepitaxy Growth Dynamics Using High-Speed Reflection High-Energy Electron Diffraction

Pulsed-laser deposition (PLD) is a powerful technique for growing complex oxides with controlled stoichiometry. To understand growth dynamics therein, it is common to leverage in situ spectroscopies, such as reflection high-energy electron diffraction (RHEED), to monitor surface crystallinity. Most commercial systems rely on video-rate cameras operating at 60-120 Hz that lack sufficient temporal resolution to capture growth dynamics at practical deposition frequencies. Here, a high-speed platform to record in situ dynamics via RHEED at >500 Hz is implemented. An open-source analysis package is designed to fit diffraction spots to 2D Gaussians, allowing single-pulse surface reconstruction kinetics extraction. Using homoepitaxially deposited (001)-oriented SrTiO 3 as a model system, we demonstrate how high-speed RHEED can provide real-time insight into growth processes obscured by slower acquisition systems. By fitting the single-pulse intensity to a set of exponential functions, we observe changes in the characteristic decay time and mechanism correlated to the substrate step width and surface termination. We observe distinct surface effects, with diffraction intensity decaying on lower-energy TiO 2 -terminated surfaces and stabilizing on SrO- or mixed-terminated surfaces. Similarly, using an exponential model, the extracted characteristic time of adatom deposition decreases with increased density of bonding sites associated with mixed termination and narrower step widths. Ultimately, this work shows how increasing RHEED temporal resolution can uncover new insights into growth processes, with practical implications for the design and control of PLD processes. This experimental platform provides new capabilities to enable data-driven machine learning analysis and autonomous control systems to enhance the complexity and fecundity of PLD.

(SrO)↗
DOE OSTI2020

Interference effects for 0 ν β β decay in the left-right symmetric model

Various mechanisms may contribute to neutrinoless double beta decay in the left-right symmetric model. The interference between these mechanisms also contribute to the overall decay rate. The analysis of the contributions of these interference terms is important for disentangling different mechanisms. Here, we study interference effects contributing to the decay rate for neutrinoless double-β decay in the left-right symmetric model. The numerical values for maximum interference for several nuclides are calculated. It is observed that, for most of the interference terms, the contribution is smaller than 20% for all the nuclei considered in the study. However, the interference between the mass mechanisms (light and heavy) and η mechanism is observed to be in the range 30%–50%. The variation of the interference effect with the Q values is also studied.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

The $$\pi f_0(500)$$ decay of the $$a_1(1260)$$

Abstract We evaluate the $$a_1(1260) \rightarrow \pi \sigma (f_0(500))$$ a 1 ( 1260 ) → π σ ( f 0 ( 500 ) ) decay width from the perspective that the $$a_1(1260)$$ a 1 ( 1260 ) resonance is dynamically generated from the pseudoscalar–vector interaction and the $$\sigma $$ σ arises from the pseudoscalar–pseudoscalar interaction. A triangle mechanism with $$a_1(1260) \rightarrow \rho \pi $$ a 1 ( 1260 ) → ρ π followed by $$\rho \rightarrow \pi \pi $$ ρ → π π and a fusion of two pions within the loop to produce the $$\sigma $$ σ provides the mechanism for this decay under these assumptions for the nature of the two resonances. We obtain widths of the order of 13–22 MeV. Present experimental results differ substantially from each other, suggesting that extra efforts should be devoted to the precise extraction of this important partial decay width, which should provide valuable information on the nature of the axial vector and scalar meson resonances and help clarify the role of the $$\pi \sigma $$ π σ channel in recent lattice QCD calculations of the $$a_1$$ a 1 .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2021

Gene family expansions and transcriptome signatures uncover fungal adaptations to wood decay

Because they comprise some of the most efficient wood-decayers, Polyporales fungi impact carbon cycling in forest environment. Despite continuous discoveries on the enzymatic machinery involved in wood decomposition, the vision on their evolutionary adaptation to wood decay and genome diversity remains incomplete. We combined the genome sequence information from 50 Polyporales species, including 26 newly sequenced genomes and sought for genomic and functional adaptations to wood decay through the analysis of genome composition and transcriptome responses to different carbon sources. The genomes of Polyporales from different phylogenetic clades showed poor conservation in macrosynteny, indicative of genome rearrangements. We observed different gene family expansion/contraction histories for plant cell wall degrading enzymes in core polyporoids and phlebioids and captured expansions for genes involved in signalling and regulation in the lineages of white rotters. Furthermore, we identified conserved cupredoxins, thaumatin-like proteins and lytic polysaccharide monooxygenases with a yet uncharacterized appended module as new candidate players in wood decomposition. Given the current need for enzymatic toolkits dedicated to the transformation of renewable carbon sources, the observed genomic diversity among Polyporales strengthens the relevance of mining Polyporales biodiversity to understand the molecular mechanisms of wood decay.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2024

Parity solution to the strong CP problem and a unified framework for inflation, baryogenesis, and dark matter

It has been known for some time that asymptotic parity invariance of weak interactions can provide a solution to the strong CP problem without the need for the axion. Left-right symmetric theories which employ a minimal Higgs sector consisting of a left-handed and a right-handed doublet is an example of such a theory wherein all fermion masses arise through a generalized seesaw mechanism. In this paper we present a way to understand the origin of matter-antimatter asymmetry as well as the dark matter content of the universe in these theories using the Affleck-Dine (AD) leptogenesis mechanism and inflaton decay, respectively. Three gauge singlet fermions are needed for this purpose, two of which help to implement the Dirac seesaw for neutrino masses while the third one becomes the non-thermal dark matter candidate. A soft lepton number breaking term involving the AD scalar field is used to generate lepton asymmetry which suffers no wash-out effects and maintains the Dirac nature of neutrinos. This framework thus provides a unified description of many of the unresolved puzzles of the standard model that require new physics.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2024

Mesoscale interplay among composition heterogeneity, lattice deformation, and redox stratification in single-crystalline layered oxide cathode

Single-crystalline layered oxide materials for lithium-ion batteries are featured by their excellent capacity retention over their polycrystalline counterparts, making them sought-after cathode candidates. Their capacity degradation, however, becomes more severe under high-voltage cycling, hindering many high-energy applications. It has long been speculated that the interplay among composition heterogeneity, lattice deformation, and redox stratification could be a driving force for the performance decay. The underlying mechanism, however, is not well-understood. In this study, we use X-ray microscopy to systematically examine single-crystalline NMC particles at the mesoscale. This technique allows us to capture detailed signals of diffraction, spectroscopy, and fluorescence, offering spatially resolved multimodal insights. Focusing on early high-voltage charging cycles, we uncover heterogeneities in valence states and lattice structures that are inherent rather than caused by electrochemical abuse. These heterogeneities are closely associated with compositional variations within individual particles. Our findings provide useful insights for refining material synthesis and processing for enhanced battery longevity and efficiency.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Recent progress in low energy neutrino scattering physics and its implications for the standard and beyond the standard model physics

Neutrinos continue to provide a testing ground for the structure of the standard model of particle physics as well as hints towards the physics beyond the standard model. Neutrinos of energies spanning over several orders of magnitude, originating in many terrestrial and astrophysical processes, have been detected via various decay and interaction mechanisms. At MeV scales, there has been one elusive process, until a few years ago, known as coherent elastic neutrino-nucleus scattering (CEvNS) that was theoretically predicted over five decades ago but was never observed experimentally. The recent experimental observation of the CEvNS process by the COHERENT collaboration at a stopped pion neutrino source has inspired physicists across many subfields. This has vital implications for nuclear physics, high-energy physics, astrophysics, and beyond. CEvNS, being a low-energy process, provides a natural window to study light, weakly-coupled, new physics in the neutrino sector. In this review, we intend to provide the current status of low energy neutrino scattering physics and its implications for the standard and beyond the standard model physics. We discuss the general formalism of calculating the tree-level CEvNS cross section and present estimated theoretical uncertainties on the CEvNS cross section stemming from different sources. We also discuss the inelastic scattering of tens of MeV neutrinos that have implications for supernova detection in future neutrino experiments. We discuss how the CEvNS experiments can be used as a testing ground for the Standard Model (SM) weak physics as well as in searching for the Beyond the Standard Model (BSM) physics signals. Any deviation from the SM predicted event rate either with a change in the total event rate or with a change in the shape of the recoil spectrum, could indicate new contributions to the interaction cross-section. The SM implications include the study of weak nuclear form factor and weak mixing angle. The BSM studies include non-standard interactions, neutrino electromagnetic properties, and sterile neutrino searches. In conclusion, stopped pion facilities are also a copious source of neutral and changed mesons that allow study of several dark sector physics scenarios such as vector portal models, leptophobic dark matter as well as axion-like particle searches.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Development of Multiplexed Immuno-N-Terminomics to Reveal the Landscape of Proteolytic Processing in Early Embryogenesis of Drosophila melanogaster

Protein expression levels are regulated through both translation and degradation mechanisms. Levels of degradation intermediates, i.e., partially degraded proteins, cannot be distinguished from those of intact proteins by global proteomics analysis, which quantify total protein abundance levels. This study aimed to develop a tool for assessing the aspects of degradation regulation via proteolytic processing through a new multiplexed N-terminomics method involving selective isobaric labeling of protein N-termini and immunoaffinity capture of the labeled N-terminal peptides. Our method allows for not only identification or proteolytic cleavage sites, but also highly multiplexed quantification of proteolytic processing. In this paper, we profiled a number of potential cleavage sites by signal peptidase and provided experimental confirmation of predicted cleavage sites of signal peptide. Furthermore, the present method uniquely represents the landscape of proteomic proteolytic processing rate during early embryogenesis in Drosophila melanogaster, revealing the underlying mechanism of stringent decay regulation of zygotically expressed proteins during early stages of embryogenesis.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗