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At least 55 records · Page 3

Design and performance of a magnetic bottle electron spectrometer for high-energy photoelectron spectroscopy

We describe the design and performance of a magnetic bottle electron spectrometer (MBES) for high-energy electron spectroscopy. Our design features a 2 m long electron drift tube and electrostatic retardation lens, achieving sub-electronvolt (eV) electron kinetic energy resolution for high energy (several hundred eV) electrons with a close to 4π collection solid angle. A segmented anode electron detector enables the simultaneous collection of photoelectron spectra in high resolution and high collection efficiency modes. This versatile instrument is installed at the time-resolved molecular and optical sciences instrument at the Linac Coherent Light Source x-ray free-electron laser (XFEL). In this paper, we demonstrate its high resolution, collection efficiency, and spatial selectivity in measurements where it is coupled to an XFEL source. These combined characteristics are designed to enable high-resolution time-resolved measurements using x-ray photoelectron, absorption, and Auger–Meitner spectroscopy. We also describe the pervasive artifact in MBES time-of-flight spectra that arises from a periodic modulation in electron collection efficiency and present a robust analysis procedure for its removal.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Simulations of muon imaging with the LANL GMT detector for spent nuclear fuel cask content verification

Atmospheric muons are typically high energy, highly penetrating charged particles. They interact with matter primarily through multiple Coulomb scatterings. Muon scattering intensities can be used to characterize the density and atomic number of the matter that they pass through. Previously, the Los Alamos National Laboratory (LANL) muon tomography team performed muon imaging of the partially filled MC-10 spent nuclear fuel (SNF) cask at Idaho National Laboratory (INL). This experiment demonstrated the feasibility of muon imaging for the verification of spent fuel container contents. That original effort used the mini muon tracker array, consisting of two arrays of drift tubes on either side of the SNF cask. The reconstructed image quality was limited by statistics, largely due to low muon flux at high zenith angles. A LANL led team will perform new measurements with a larger array, the Giant Muon Tracker (GMT), to improve data collection rates and statistics. In this work, simulations were performed with the GMT near the partially filled INL MC-10 cask. For more general fuel diversion detection, a full MC-10 cask and casks with a singular missing fuel bundle were also simulated. To understand minimum measurement times needed for missing bundle identification, 100 000 to millions of tracked muons (corresponding to 1.4 days to several weeks measurement time) were analyzed. Simulated images were then analyzed visually and numerically to explore techniques designed to minimize the collection time needed to identify the diversion of fuel in each scenario.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Performance of Michigan sMDT prototype chambers for the HL-LHC ATLAS muon detector upgrade

A new small-diameter Monitored Drift Tube (sMDT) chamber has been developed for the muon spectrometer of the ATLAS experiment to handle the higher collision rates expected at the CERN High Luminosity Large Hadron Collider (HL-LHC). This paper presents measurements of the tracking resolution and hit efficiency of two prototype sMDT chambers constructed at the University of Michigan. Using cosmic-ray muons the sMDT tracking resolution of 103.7 ± 8.1 μm was measured for one chamber and 101.8 ± 7.8 μm for the other, compared with a design resolution of 106 μm. A further tracking resolution improvement to 83.4 ± 7.8 μm was obtained by using new high-gain readout electronics which will be added for HL-LHC. An average tracking efficiency of (98.5 ± 0.2)% was found for both chambers. The methodology used to determine the detector tracking resolution and efficiency, including reconstruction of sMDT data and a Geant4 simulation of the test chamber, is presented in detail.

43 PARTICLE ACCELERATORS↗

The ATLAS experiment at the CERN Large Hadron Collider: a description of the detector configuration for Run 3

The ATLAS detector is installed in its experimental cavern at Point 1 of the CERN Large Hadron Collider. During Run 2 of the LHC, a luminosity of ℒ = 2 × 10 34 cm -2 s -1 was routinely achieved at the start of fills, twice the design luminosity. For Run 3, accelerator improvements, notably luminosity levelling, allow sustained running at an instantaneous luminosity of ℒ = 2 × 10 34 cm -2 s -1 , with an average of up to 60 interactions per bunch crossing. The ATLAS detector has been upgraded to recover Run 1 single-lepton trigger thresholds while operating comfortably under Run 3 sustained pileup conditions. A fourth pixel layer 3.3 cm from the beam axis was added before Run 2 to improve vertex reconstruction and b-tagging performance. New Liquid Argon Calorimeter digital trigger electronics, with corresponding upgrades to the Trigger and Data Acquisition system, take advantage of a factor of 10 finer granularity to improve triggering on electrons, photons, taus, and hadronic signatures through increased pileup rejection. The inner muon endcap wheels were replaced by New Small Wheels with Micromegas and small-strip Thin Gap Chamber detectors, providing both precision tracking and Level-1 Muon trigger functionality. Trigger coverage of the inner barrel muon layer near one endcap region was augmented with modules integrating new thin-gap resistive plate chambers and smaller-diameter drift-tube chambers. Tile Calorimeter scintillation counters were added to improve electron energy resolution and background rejection. Upgrades to Minimum Bias Trigger Scintillators and Forward Detectors improve luminosity monitoring and enable total proton-proton cross section, diffractive physics, and heavy ion measurements. These upgrades are all compatible with operation in the much harsher environment anticipated after the High-Luminosity upgrade of the LHC and are the first steps towards preparing ATLAS for the High-Luminosity upgrade of the LHC. This paper describes the Run 3 configuration of the ATLAS detector.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Commissioning of Extended Electron Beam Ion Source at Brookhaven National Laboratory

Here, the Extended Electron Beam Ion Source (EEBIS) has been installed and commissioned at Brookhaven National Laboratory (BNL) hadron accelerator complex in the spring of 2023. EEBIS has replaced its predecessor, RhicEBIS, which provided ions for BNL hadron facilities for over a decade since 2009. The motivations for the source upgrade are to provide higher intensities of the Au 32+ ion beam for the Relativistic Heavy Ion Collider (RHIC) and to provide of an intense source of polarized 3 He 2+ ions for the future Electron Ion Collider (EIC) at BNL. EEBIS is and will continue to be the primary source for a variety of different ion species for the NASA Space Radiation Laboratory (NSRL) at BNL. EEBIS utilizes two identical, two-meter-long unshielded 5T warm bore superconducting solenoids, and it is operated with electron beam current up to 10 A, providing a high-capacity ion traps to fulfill the requirement for high intensity ion beams. The upstream solenoid contains a “short ion trap” with a length of 95 cm, while the “long ion trap” with a length of 178 cm is located inside the downstream solenoid bore. The main features of EEBIS are: * A Gas injection and ionization cell equipped with a Lorenz pulse valve * High-capacity ZAO non-evaporable getter (NEG) custom linear pumping units * In situ apparatus for pumping speed measurements to monitor NEG activation and saturation * “External drift tube” construction with differential pumping stages to provide space for Lorentz pulse valve and 3 He high-field polarization cell * A Ba oxide electron gun cathode. The design of EEBIS as well as the results of its commissioning and first-year operation are presented and discussed.

43 PARTICLE ACCELERATORS↗

Mitigation of Beam Losses in LANSCE Linear Accelerator

Suppression of beam losses is essential for successful operation of high-intensity accelerator facility. The LANSCE accelerator started routine operation in 1972 as a 0.8 MW average proton beam power facility for meson physics research, and delivered highpower beam for a quarter century. The accelerator currently delivers 100 MeV proton beam to Isotope Production Facility (IPF) and 800 MeV H- beams to various experimental areas. The accelerator is equipped with two independent injectors for H + and H - beams, merging at the entrance of a 201.25 MHz Drift Tube Linac (DTL). The DTL performs acceleration up to the energy of 100 MeV. After the DTL, the Transition Region beamline directs a 100 MeV proton beam to the Isotope Production Facility, while the H - beam is accelerated up to the final energy of 800 MeV in an 805- MHz Coupled Cavity Linac. The H - beams, created with different time structure by a lowenergy chopper, are distributed in the Switch Yard (SY) to four experimental areas: the Lujan Neutron Scattering Center equipped with a Proton Storage Ring (PSR), the Weapons Neutron Research facility (WNR), the Proton Radiography facility (pRad), and the Ultra-Cold Neutron facility (UCN). Multi-beam operation requires careful control of accelerator tune to minimize beam losses. In this paper we review main effects affecting beam losses in LANSCE linear accelerator and discuss methods to reduce them.

43 PARTICLE ACCELERATORS↗

Charged Microdroplets in Air: Characterization and Use in Surface Functionalization and Nanomaterials Preparation (Final Technical Report)

The major theme of this project is the exploration of ions and charged droplets in the open air. The specific goals are (1) focusing ions in the open air, (2) separating and measuring the sizes of charged droplets, (3) examining chemical reactions occurring within droplets, (4) examining chemical reactions occurring between charged droplets and chemical vapors, and (5) characterizing surfaces post droplet deposition. The analysis of ions in the open air greatly simplifies instrumentation as it removes the need for large, costly vacuum pumps. Major strides in this project include the sizing of electrospray droplets using structured illumination microscopy, 3D printed drift tube ion mobility (both standalone and coupled with mass spectrometry), and accelerated Suzuki reactions in Leidenfrost droplets.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

LAMP Manufacturing Survey (Final Report)

This report presents the results of a market manufacturing survey performed for fabricating radiofrequency quadrupoles (RFQ) and Drift Tube Linear Accelerator (DTL) components needed for the Los Alamos Neutron Science Center (LANSCE) Modernization Project (LAMP). A review on existing RFQs and DTLs with their parameters, a summary of specific capabilities needed to manufacture them, the common issues during the fabrication process, their consequences, and resolutions to these problems is presented in this report. The goal of this study is to identify potential collaborators and companies capable of manufacturing the necessary accelerator equipment, while minimizing cost and schedule risks that could impact the future modernization of the LANSCE facility.

43 PARTICLE ACCELERATORS↗

Agilent AgileBioFoundry CRADA (Final Report)

The mission of this CRADA with Agilent was to couple powerful MS platforms (QQQ, IM-QTOF-MS) with Agilent’s novel Ultra-High-Performance Liquid Chromatography (UHPLC) fast metabolomic workflows and perform ABF Machine Learning (ML) to generated datasets. Agilent transferred UHPLC methods to PNNL and LBNL and methods were implemented and demonstrated in both labs, achieving total acquisition times of < 10 min. Metabolites analyzed using Agilent’s shared methods included metabolites from central carbon metabolism, common across hosts, and metabolites unique to engineered strains. Standards were acquired in an UHPLC-Drift Tube Ion Mobility Mass Spectrometer (DTIMS) system for the first time within the context of ABF and methods were optimized based on Agilent’s protocols. Samples from ABF hosts Pseudomonas putida, Aspergillus pseudoterreus, Aspergillus niger and Rhodosporidium toruloides were analyzed using the UHPLC-DTIMS platform for a total of 276 runs. A data analysis workflow compatible with the Experimental Data Depot (EDD) and completely shareable was developed for the acquired UHPLC-DTIMS data. Samples were analyzed using a Data Independent Acquisition Approach (DIA), which for most of the standards provided more transitions therefore increasing detection confidence. Using the data acquired by PNNL, LBNL, and Agilent’s specifications from previous ML projects, SNL applied an ensemble ML strategy to pick the best performing model for automated LC-method selection. Finally, with the contribution of the participant labs and Agilent, SNL developed an Automated Method Selection (AMS) software tool to predict the best liquid chromatography method for analysis of any new molecules of interest. Samples with novel pathways and new metabolite targets of interest are generated at a high pace in the ABF. Therefore, our accomplishment in this CRADA improved the efficiency and accuracy of strain testing by developing and implementing fast analytical methods, robust processing tools, and software for predicting the best methods for UHPLC analysis.

97 MATHEMATICS AND COMPUTING↗

Delivery of H - / H + Beams to Area A

We explore the relative merits of transporting the beam from the H + ion source and from the H - ion source to Area-A for low current applications. Transporting the H - beam to Area-A using the laser neutralization approach has some risk associated with it and will require some development. Alternative method of delivering H - beam to Area-A includes replacing LDBM00 bending magnet with kicker for sharing beam between Line D and modified Line A. Transporting the H + beam to Area-A will have significant impact on the operation the IPF facility and maintaining high pulse rate to IPF will require major modifications to the transition region of the accelerator and Drift Tube Linac.

43 PARTICLE ACCELERATORS↗

LAMP Technical Readiness Evaluation Report (Rev. 1)

An internal preliminary evaluation of Critical Technology Elements (CTEs) for the LANSCE Modernization Project (LAMP) was completed. Corresponding Technical Readiness Levels (TRLs) were also determined for all subsystems using the criteria of DOE G 413.3-4A, Technical Readiness Assessment Guide. The scope of the evaluation was limited to the project Work Breakdown Structure (WBS) elements as defined for the RFQ Injector and Drift Tube Linac (DTL) systems only. Integration of Instrumentation and Controls (I&C) and Safety Systems was not considered, although specific technologies as related to the RFQ and DTL systems were included. Other elements of the project such as Shielding, System Design, Technical Management, and additional facility integration needed to enable off-line testing and pre-installation commissioning were also not evaluated. Each technical subsystem element was evaluated for technical readiness, however, not all were found to meet the criteria for a CTE. Only two subsystem elements were determined to meet the CTE criteria. Their associated TRLs are summarized in the table below. These subsystem elements of the project have the lowest technical readiness due to either being new, novel or modified, requiring additional R&D before being capable of meeting the project Key Performance Parameters (KPPs) and subsystem requirements, or present technology exists but has not yet been demonstrated in a relevant environment. All other subsystems were determined to have a TRL of 8, indicating that actual operating systems exist having similar performance requirements as needed for LAMP. Details of the technical readiness evaluation for each subsystem is given in the following sections of this report.

43 PARTICLE ACCELERATORS↗

Ion Beam Propagation Through the FNAL LEBT

The Fermilab 750keV injector sends 25mA H- beam for 30µs at a rep-rate of 15Hz. The beam transmission through the FNAL injector is currently less than 50% from the ion source to the entrance of the drift tube linac. Recently it was uncovered that the primary loss point is within the region prior to the RFQ which houses the solenoid focal elements that match the beam to the RFQ. Recent diagnostic measurements indicate that the cause of the transmission efficiency could be the non-linear effects of the solenoid elements on the beam. An aperture restriction was placed just upstream of the first solenoid element to restrict the beam size and reduce the non-linear effects of the solenoid element.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Agilent AgileBioFoundry CRADA

NTESS, LBNL, PNNL, and Agilent are collaborating to expand a prototype system that processes hundreds of samples per day by UHPLC-QTOF mass spectrometric-based target methods for both metabolomic and proteomic application sin support the needs of strain optimization. Extending this technology to targeted triple quadrupole and drift tube ion mobility spectrometry mass spectrometric analyses offers direct advantages.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Performance of the Fermilab Linac Injector

The Fermilab Linac injection line consists of a 35 keV magnetron-type H- ion source, two-solenoid Low Energy Beam Transport (LEBT), 201 MHz 4-rod 750 keV Radio Frequency Quadrupole (RFQ), and a Medium Energy Transport (MEBT) containing 4 quadrupoles and a bunching cavity. The injector delivers 25 mA, 48 s pulses to drift-tube Linac at a repetition rate of 15Hz. The transmission efficiency has been lower than expected since commissioning. Recent beam current measurements suggest that the beam is primarily lost upstream of the RFQ exit. Numerical simulations indicate that ions passing through the non-linear field region of the solenoids could produce a beam with an increased emittance resulting in up to 50 % of the LEBT beam current failing to meet the RFQ acceptance. An aperture restriction was installed upstream of the first solenoid to remove these ions. This report describes the results of measurements and simulations as well as the LEBT tuning.

Jones, Daniel C.↗

LAMP Technical Readiness Evaluation Report

An internal preliminary evaluation of Critical Technology Elements (CTEs) for the LANSCE Modernization Project (LAMP) was completed in 2023. This included determining corresponding Technical Readiness Levels (TRLs) for all subsystems using the criteria of DOE G 413.3-4A, Technical Readiness Assessment Guide. This revised report includes a summary of the recent design modifications required to meet the project Key Performance Requirements (KPPs), some of which may reduce technical risk to the project. These recent design modifications include: • Further optimization of the low-energy and medium-energy beam transport regions (LEBT and MEBT, respectively), including relocation of various functional elements (ie choppers, kickers, and bunchers). • An additional H - ion source to separate ion-source function based on beam delivery requirements. • A high-repetition-rate pulsed kicker magnet to select/merge the two H ion beams into a common low-energy beam transport. • Modification and further optimization to a more conventional RFQ design. Performance of the RFQ has been optimized to deliver the required three types of beams while meeting the project KPPs. • The addition of a second chopper in the medium-energy beam transport (MEBT) line to reduce the required pulser voltages. The scope of the evaluation was limited to the project Work Breakdown Structure (WBS) elements as defined for the RFQ Injector and Drift Tube Linac (DTL) systems only. Integration of Instrumentation and Controls (I&C) and Safety Systems was not considered, although specific technologies as related to the RFQ and DTL systems were included. Other elements of the project such as Shielding, System Design, Technical Management, and additional facility integration needed to enable off-line testing and pre-installation commissioning were also not evaluated. Each technical subsystem element was evaluated for technical readiness, however, not all were found to meet the criteria for a CTE. Three subsystem elements were determined to meet the CTE criteria. Their associated TRLs are summarized in the table below. These subsystem elements of the project have the lowest technical readiness due to either being new, novel or modified, requiring additional R&D before being capable of meeting the project Key Performance Parameters (KPPs) and subsystem requirements, or present technology exists but has not yet been demonstrated in a relevant environment. All other subsystems were determined to have a TRL of 8, indicating that actual operating systems exist having similar performance requirements as needed for LAMP. Details of the technical readiness evaluation for each subsystem is given in the following sections of this report.

43 PARTICLE ACCELERATORS↗

MEBT Bunchers: System Design Document (SDD)

The LAMP Medium Energy Beam Transport (MEBT) transfers bunched beam at the energy 3 MeV from RFQ to the Drift-Tube Linac (DTL) entrance. The beam particles (protons or H- ) in the LAMP MEBT have velocity β = v/c = 0.08, where v is the beam velocity, c is the speed of light. The MEBT bunchers keep beam bunches from spreading longitudinally as they propagate through the MEBT, where some unwanted bunches are removed by a chopper to create a required beam pattern. The MEBT bunchers are RF cavities operating at the frequency 201.25 MHz; possible design options were considered in.

43 PARTICLE ACCELERATORS↗

MEBT Chopper System: System Design Document (SDD)

The Medium Energy Beam Transport (MEBT) chopper removes unwanted beam bunches by deflecting them to a target from a bunched beam transported through the MEBT from RFQ to the Drift-Tube Linac (DTL) entrance. The unchopped bunches propagate through the MEBT to DTL, while the deflected bunches are deposited on a target downstream of chopper. The chopper system consists of a deflecting structure, where the beam-deflecting fields are created, and a pulse generator (pulser) that feeds this structure with voltage pulses having the required time pattern. Ideally, the system should turn deflection on and off in the time interval between the bunches to prevent partially chopped / deflected bunches. This usually requires traveling slow-wave chopper structures where the field propagates with the same velocity as the beam, as illustrated in Fig. 1.

43 PARTICLE ACCELERATORS↗

Preliminary Look at the LBEG & MPEG Beam Transmissions between HPSim and Operation Data

This report summarizes recent work on estimating the transmission of LANSCE H- beams from the end of the present DTL to both the PSR stripper foil (LBEG) and WNR target 4 (MPEG). The LBEG beam might be considered a more typical LINAC beam and lends itself to continuous monitoring of transmission through the various stages of the accelerator. For the MPEG, however, the widely-spaced micropulses and lack of the requisite sensitivity current monitors throughout the accelerator make these measurements extremely difficult and more uncertain. Therefore, to assist in estimating the MPEG beam transmission, beam-dynamics simulations using HPSim were employed. These beam transmission estimates from the end of the Drift Tube Linac (DTL) to Target 4 (MPEG) and the PSR stripper foil (LBEG) are vital to determine the charge requirements for LAMP’s front end. In this technote, we demonstrate three major efforts in determining the transmission: (1) Convert the WNR beamline lattice from TRANSPORT to HPSim for use in the simulation; (2) Simulate the optimization process in the Central Control Room (CCR) that brings down the losses by up to a factor of 4000 between the end of the initial physics-based tuneup phase and production beam operation; (3) Analyze operational data to deduce measured transmissions. Table 1 shows the estimated losses with HPSim and operational analysis. Finally, a better measurement and other improvements to refine the results are also proposed.

43 PARTICLE ACCELERATORS↗