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At least 55 records · Page 3

A solution for 40 K interference from K internal to the human body, in an underground high sensitivity whole body counter at the Waste Isolation Pilot Plant, Carlsbad, NM, USA

The objective of the present work is to find a solution for the interference arising from 1461 keV photons emitted by 40 K in natural K internal to the human body in the detection of 241 Am and 210 Pb activities at the level of 37 mBq (1 pCi). The response of a broad energy Ge (BEGe) reference crystal to 1461 keV photons was simulated using GEANT4 code. Simulations were performed for a point source without and with shielding, as well as for a Bottle Manikin Absorption (BOMAB) phantom in the shielded whole-body counting chamber (WBC). The WBC facility is located underground at the Waste Isolation Pilot Plant, Carlsbad, NM, USA. The simulation results were discussed with regards to the interference in detecting the 241 Am and 210 Pb at the level of 37 mBq (1 pCi). The specific conclusion is that the interference counts from 40 K activity at the natural levels present in the human body in typical clinical settings were found to be greater than the 210 Pb and 241 Am signal counts from 37 mBq (1 pCi), when a 38.1 mm diameter, 25.4 mm thick BEGe reference crystal was used. Our solution for minimizing the interference to the desired precision at the specified levels was found by sacrificing the broad energy response of the counting system.

40K gamma-ray interference↗

Statistical characteristics of laser interference and its effect on IR optoelectronic observation systems

We consider statistical characteristics of laser interference recorded in the focal region of an IR optoelectronic observation system under field and out-of-field illumination by laser radiation. The applicability of the analytical description of experimental histograms of the laser interference signal distribution at the photodetector array output using the probability density approximations in the form of gamma distribution and the Gaussian function is substantiated. It is shown that the specific form of these functions is determined both by the mean value (mathematical expectation) of the interference signal and by the characteristic parameter M, which depends on the statistical properties of the laser interference. (laser applications and other issues in quantum electronics)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Ultra-Wideband Communications: Interference Challenges and Solutions

The idea of ultra-wideband (UWB) communications for short ranges (up to a few tens of meters) has been around for nearly three decades. However, despite significant efforts by the industry, UWB deployment has not yet reached its predicted potential. This article, thus, seeks to rectify this situation by providing a practical examination of UWB interference conditions. Through a spectrum survey of today's wireless environments, we explore the interference that UWB devices may face from a perspective of outage probability in both high- and low-rate configurations. We find that by suppressing interference, the outage probability can be reduced by one or more orders of magnitude. In the non-line-of-sight channels, in particular, we find that both interference suppression and bandwidth expansion are required to support the minimum data rates suggested in the IEEE802.15.4 series of standards. Here, we connect these findings to a recently proposed UWB signaling method based on filter banks and show this method fulfills the above requirements for implementing effective UWB systems.

99 - GENERAL AND MISCELLANEOUS↗

Demystifying asynchronous I/O Interference in HPC applications

With increasing complexity of HPC workflows, data management services need to perform expensive I/O operations asynchronously in the background, aiming to overlap the I/O with the application runtime. However, this may cause interference due to competition for resources: CPU, memory/network bandwidth. The advent of multi-core architectures has exacerbated this problem, as many I/O operations are issued concurrently, thereby competing not only with the application but also among themselves. Furthermore, the interference patterns can dynamically change as a response to variations in application behavior and I/O subsystems (e.g. multiple users sharing a parallel file system). Without a thorough understanding, I/O operations may perform suboptimally, potentially even worse than in the blocking case. To fill this gap, here we investigate the causes and consequences of interference due to asynchronous I/O on HPC systems. Specifically, we focus on multi-core CPUs and memory bandwidth, isolating the interference due to each resource. Then, we perform an in-depth study to explain the interplay and contention in a variety of resource sharing scenarios such as varying priority and number of background I/O threads and different I/O strategies: sendfile, read/write, mmap/write underlining trade-offs. The insights from this study are important both to enable guided optimizations of existing background I/O, as well as to open new opportunities to design advanced asynchronous I/O strategies.

97 MATHEMATICS AND COMPUTING↗

Laser-Interference Surface Preparation for Enhanced Coating Adhesion and Adhesive Joining of Multi-Materials (Final Project Report)

This report investigates a laser-interference surface treatment as a non-contact, i.e., without major solid/liquid medium application or abrasion, and non-chemical surface preparation method for aerospace coating systems. It was proposed to use the laser-interference technique to structure surfaces of Al and/or Ti, creating "rough" surfaces with pre-engineered series of ridges and valleys at submicron scale. The science goal of this study was to develop an understanding of the surface microstructure, topology, and physical mechanisms that would improve adhesion and corrosion protection of Al2024-T3. Microstructure analysis indicates that the laser-interference structuring (LIS) was found to reduce the formation of CuMn-rich precipitates in Al 2024-T3 over a 500-800 nm depth from top surface. The X-cut and cross-hatch coating adhesion ratings indicate that the LIS specimens meet the performance requirements in the coating adhesion specifications by having a higher or identical ranking to those specimens prepared with current state-of-the-art chemical conversion or sulfuric acid anodizing. After the ASTM B117 corrosion exposure, it was found that the laser processed specimens exhibited only few blisters. It was found that the corrosion damage was minimized at a laser rastering speed of 4 mm/s, for which only 33% of specimens developed very minor corrosion damage. The ASTM D1654 creepage ratings, used to evaluate corrosion damage along the scribe lines, were found to be at least nine for all coated panels. These results indicate that the laser-interference technique with the additional acetone wiping has the potential to be further developed as a minor chemical surface preparation technique for chromate-containing epoxy primers coatings.

36 MATERIALS SCIENCE↗

Spectrum Interference from Commercial devices in 6 & 7/8 GHz

FCC repurposed spectrum in the 6 GHz band allocated to DOE for commercial use of Wi-Fi 6E/7 in 2020.The 2024 National Spectrum Strategy (NSS) implementation plan is now considering 7/8 GHz band as well for co-existence of commercial devices with federal incumbents such as DOE. This poster summarizes INL’s work on a scientific study on the potential harmful interference caused by the commercial devices in real-world scenarios. It includes research in INL for the following projects funded by DOE: 1) DOE-CIO: Spectrum security for advanced wireless technologies; 2) DOE-OE: 7 GHz Spectrum interference study; 3) DOE-CESER: Harmful interference in 6 GHz from commercial Wi-Fi 6E/7 devices on utility links in the energy sector; 4) DOE/NTIA for NSS Implementation plan: Interference study in 7/8 GHz bands identified in the NSS. 5) NSF: Spectrum Innovation Initiative- National Radio Dynamic Zones (SII-NRDZ).

6 GHz↗

Stress interference in multilayer additive friction stir deposition of AA6061 aluminum

Due to the multilayer deposition nature of metal additive manufacturing processes, each layer being printed experiences the state of thermokinetic and thermomechanical stress that in turn interfere with the state of thermokinetics and thermomechanical stress of subsequently deposited layers. Especially, this multilayer interference significantly affects the resultant properties of the component fabricated using solid-state additive friction stir deposition due to evolution of asymmetric state of planar stress. Due to the lack of comprehensive and suitable in situ diagnosis technique, the complex interference of inter- and multi-layer stresses during additive friction stir deposition was studied in an integrated approach of numerical simulation of fluidic state and experimental probing of stress influenced ultrasonic elastography. The uni-directional and bi-directional layer deposition configurations adopted during additive friction stir deposition result in the generation of constructive and destructive interference of the interlayer stress and hence, asymmetric and symmetric dynamic elasticity distribution respectively within the subsequent layers. With subsequent deposition of additional layers, the odd and even numbers of deposited layers generate asymmetric and nearly symmetric dynamic elasticity distributions.

Yang, Teng↗

Surface chemistry and composition-induced variation of laser interference-based surface treatment of Al alloys

A key limitation for the use of aluminum alloys in multi-material structural components is effective surface cleaning and texturing techniques to improve the quality of structural joints. In this study, the surface and sub-surface chemistries are investigated for a novel surface treatment method using laser interferometry produced by two beams of a pulsed Nd:YAG laser. Surfaces of AA 5128 aluminum alloy were treated using a two-beam laser interference setup, enabling the structuring of the surface at length scales much less than that of the laser beam. Periodic and patterned surface structures were created by the interference power profile through ablation of deposits and debris and melting and re-solidification of the near-surface region during laser-treatment. Chemical changes to the Al alloy surface induced by laser treatment were examined in detail in this study using both x-ray photoelectron spectroscopy (XPS) and scanning Auger microanalysis (SAM) as a function of number of interfering laser shots. XPS surface analysis indicates that this laser technique is effective at cleaning aluminum surfaces. Furthermore, SAM data indicated that there is a compositional-induced variation of Mg due to laser-interference as Mg-rich areas were found in periodic interference-structured ridges.

36 MATERIALS SCIENCE↗

Investigation of potential polyatomic interferences on uranium isotope ratio measurements for the LS-APGD-Orbitrap MS system

The determination of actinide (e.g., U and Pu) content and isotopics is of importance to the nuclear forensics and safeguards communities. However, in the analysis of environmental samples, such as those collected by the International Atomic Energy Agency, uranium measurements can be complicated by isobaric interferences from polyatomic variants of heavy elements (e.g., Pb). This leads to complex, time-consuming sample manipulations (i.e., separations) before determining isotope ratios. An alternative strategy to sample pretreatment is to use high-resolution mass spectrometric platforms during the analysis to fully resolve the uranium isotopes from potential polyatomic interferences, negating the need for prior chemical separation. The liquid sampling - atmospheric pressure glow discharge (LS-APGD) coupled with an Orbitrap mass spectrometer provides a high-resolution (>70,000 m/Δm at m/z 200) inorganic mass spectrometry platform. Further, as a demonstration of the power of this instrumental platform, and indeed, the high-resolution approach in general, uranium isotope ratios were determined in the presence of elemental impurities (e.g., Pb, Pt, Ta, W) commonly encountered with environmental sample swipe analysis, without any prior treatment. Even at elemental impurity concentrations of 1000–5000× relative to uranium, no interference was observed with the 235 U or 238 U signal. In addition, the 235 U/ 238 U isotope ratio for the samples with the concomitants present are within 2 standard deviations of the values obtained without their addition, indicating that these impurities do not impact the determined uranium isotope ratio. These findings represent a significant first step in leveraging the high resolution of the LS-APGD-Orbitrap-MS to overcome isobaric and molecular interferences instead of relying on chemical separations.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

The importance of ion kinetic energy for interference removal in ICP-MS/MS

Here, the effect of ion kinetic energy on gas phase ion reactivity with ICP-MS/MS was investigated in order to explore tuning strategies for interference removal. The collision/reaction gases CO 2 , N 2 O and O 2 were used to observe the ion product distribution for 48 elements using an Agilent tandem ICP-MS (ICP-MS/MS) as a function of reaction gas flow rate (pressure) and ion kinetic energy. The kinetic energy of the incident ion was varied by adjusting the octopole bias (V oct ). The three gases all form oxides (MO + ) as the primary product with differing reaction enthalpies that result in distinct differences in the ion energies required for reaction with product ion distributions that vary with Voct. Consequently, by varying the ion kinetic energy (i.e., V oct ), differences in interference reactivity can be used to achieve maximum separation. Three practical application examples were reported to demonstrate how the ion kinetic energy can be varied to achieve the ideal ion product distribution for interference resolution: CO 2 for the removal of 238 U in Pu analyses, CO 2 for the removal of 40 Ar 16 O vs. 56 Fe, and O 2 for the removal of Sm in Eu analyses, analogous to Pu/Am. The results demonstrate how the starting ion energy defined by V oct is an important factor to fully leverage the utility of any given reaction gas to remove interferences in the mass spectrum using ICP-MS/MS.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Gate-tunable Veselago interference in a bipolar graphene microcavity

The relativistic charge carriers in monolayer graphene can be manipulated in manners akin to conventional optics. Klein tunneling and Veselago lensing have been previously demonstrated in ballistic graphene pn-junction devices, but collimation and focusing efficiency remains relatively low, preventing realization of advanced quantum devices and controlled quantum interference. Here, we present a graphene microcavity defined by carefully-engineered local strain and electrostatic fields. Electrons are manipulated to form an interference path inside the cavity at zero magnetic field via consecutive Veselago refractions. The observation of unique Veselago interference peaks via transport measurement and their magnetic field dependence agrees with the theoretical expectation. We further utilize Veselago interference to demonstrate localization of uncollimated electrons and thus improvement in collimation efficiency. Our work sheds new light on relativistic single-particle physics and provide a new device concept toward next-generation quantum devices based on manipulation of ballistic electron trajectory.

36 MATERIALS SCIENCE↗

Effects of the magnetic field variation on the spin wave interference in a magnetic cross junction

This article reports results of the investigation of the effect of the external magnetic field variation on the spin wave interference in a magnetic cross junction. The experiments were performed using a micrometer scale Y 3 Fe 5 O 12 cross structure with a set of micro-antennas fabricated on the edges of the cross arms. Two of the antennas were used for the spin wave excitation while a third antenna was used for detecting the inductive voltage produced by the interfering spin waves. It was found that a small variation of the bias magnetic field may result in a significant change of the output inductive voltage. The effect is most prominent under the destructive interference condition. The maximum response exceeds 30 dB per 0.1 Oe at room temperature. It takes a relatively small bias magnetic field variation of about 1 Oe to drive the system from the destructive to the constructive interference conditions. The switching is accompanied by a significant, up to 50 dB, change in the output voltage. The obtained results demonstrate a feasibility of the efficient spin wave interference control by an external magnetic field, which may be utilized for engineering novel type of magnetometers and magnonic logic devices.

36 MATERIALS SCIENCE↗

Interference in nonlinear Compton scattering using a Schrödinger-equation approach

The interference between Compton scattering and nonlinear Compton scattering from a two-color field in the X-ray regime is theoretically examined for bound electrons. Here, the underlying phase shifts are analyzed using a perturbative approach in the incoming classical field. The perturbative approach is bench marked with a non-perturbative approach in the classical field. The interference for different combinations of linear polarization of the two fields is examined when the Compton and the nonlinear Compton scattered waves have the same wave vector and polarization. Only two cases exhibit interference. When there is interference, the calculations reveal an intrinsic phase difference between the Compton scattered wave function and the nonlinear Compton scattered wave function of either 0 or pi depending on the scattering angle.

74 ATOMIC AND MOLECULAR PHYSICS↗

Electron interference in atomic ionization by two crossing polarized ultrashort pulses

Formation of geometrically regular interference patterns in the photoelectron momentum distributions (PMDs) corresponding to the photoionization of atoms by two single-color, crossing ultrashort pulses is investigated both analytically and numerically. It is shown that, in contrast to the photoionization by monochromatic pulses, PMDs for the ionization by crossing and co-propagating broadband pulses are essentially different (unless both pulses are linearly polarized), namely, when one pulse is linearly polarized along the propagation direction, ˆk, of the circularly polarized (CP) pulse, then interference maxima (minima) of the ionization probability have the form of three-dimensional single-arm regular spirals which are wound along ˆk. Next, the interference maxima (minima) of the ionization probability by a pair of crossing elliptically polarized pulses have the form of either Newton's rings or two-arm Fermat's spirals, depending on the position of a detection plane. Remarkably, these regular patterns occur only for certain values of the pulse ellipticities, and they become distorted for CP pulses. For both above-mentioned pulse configurations, the features of interference patterns depend on the time delay between pulses, their relative electric field amplitude, and relative carrier-envelope phase. Our predictions, illustrated by the numerical results for the ionization of H and He atoms by two orthogonal pulses, are quite general and we expect them to be valid for the ionization of any randomly oriented atomic or molecular target.

74 ATOMIC AND MOLECULAR PHYSICS↗

Angular interferences of sequentially ionized double-continuum wave packets

Following the recent report of energy and angle interferences in below-threshold photoexcitation Auger processes due to postcollision interactions [Wang and Robicheaux, Phys. Rev. A 98, 013421 (2018)], similar interferences are also found in double-continuum wave packets from a two-step time-delayed photoionization of a two-electron atom. Properties of the interferences are studied in detail with respect to laser pulse time widths, laser frequency chirping, and ionization time delay. Furthermore, the effects of these physical quantities on the resulting interferences are discussed.

74 ATOMIC AND MOLECULAR PHYSICS↗

Interference of Temporally Distinguishable Photons Using Frequency-Resolved Detection

Here, we demonstrate quantum interference of three photons that are distinguishable in time by resolving them in the conjugate parameter frequency. We show that the multiphoton interference pattern in our setup can be manipulated by tuning the relative delays between the photons, without the need for reconfiguring the optical network. Furthermore, we observe that the symmetries of our optical network and the spectral amplitude of the input photons are manifested in the interference pattern. We also demonstrate time-reversed Hong-Ou-Mandel-like interference in the spectral correlations using time-bin entangled photon pairs. By adding a time-varying dispersion using a phase modulator, our setup can be used to realize dynamically reconfigurable and scalable boson sampling in the time domain as well as frequency-resolved multiboson correlation sampling.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Tunable phononic quantum interference induced by two-dimensional metals

Harnessing quantum interference among bosons provides opportunities due to their longer coherence time than fermions. Fano resonance, an example of quantum interference between discrete and continuous states, is marked by an asymmetric lineshape. While photon-based Fano resonance has enabled high-sensitivity molecule sensing, phonon-based Fano resonance remains underexplored because of ineffective interference between discrete phonons and electronic continuum. In this work, we report phonon-based Fano resonance in a graphene/2D Ag/SiC heterostructure, arising from frequency and lifetime matching between discrete and continuous phonons of SiC. The observed Fano asymmetry is tunable over two orders of magnitude, surpassing previously reported phonon-based systems. The 2D Ag layer restructures the interfacial SiC and facilitates resonant scattering to enhance Fano asymmetry, which is unattainable in conventional Ag. We further demonstrated that this Fano resonance allows ultrasensitive molecule detection at the single-molecule level. Our work highlights phonon-based Fano resonance, opening avenues for engineering quantum interference with phonons.

Science & Technology - Other Topics↗

Hydrogen Peroxide Interference in Chemical Oxygen Demand Assessments of Plasma Treated Waters

Plasma-driven advanced oxidation represents a potential technology to safely re-use waters polluted with recalcitrant contaminants by mineralizing organics via reactions with hydroxyl radicals, thus relieving freshwater stress. The process results in some residual hydrogen peroxide, which can interfere with the standard method for assessing contaminant removal. In this work, methylene blue is used as a model contaminant to present a case in which this interference can impact the measured chemical oxygen demand of samples. Next, the magnitude of this interference is investigated by dosing de-ionized water with hydrogen peroxide via dielectric barrier discharge plasma jet and by solution. The chemical oxygen demand increases with increasing concentration of residual hydrogen peroxide. The interference factor should be considered when assessing the effectiveness of plasma to treat various wastewaters.

Groele, Joseph↗