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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Biomass-burning smoke's properties and its interactions with marine stratocumulus clouds in WRF-CAM5 and southeastern Atlantic field campaigns

Abstract. A large part of the uncertainty in climate projections comes from uncertain aerosol properties and aerosol–cloud interactions as well as the difficulty in remotely sensing them. The southeastern Atlantic functions as a natural laboratory to study biomass-burning smoke and to constrain this uncertainty. We address these gaps by comparing the Weather Research and Forecasting with Chemistry Community Atmosphere Model (WRF-CAM5) to the multi-campaign observations ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS), CLARIFY (CLoud–Aerosol–Radiation Interaction and Forcing), and LASIC (Layered Atlantic Smoke Interactions with Clouds) in the southeastern Atlantic in August 2017 to evaluate a large range of the model's aerosol chemical properties, size distributions, processes, and transport, as well as aerosol–cloud interactions. Overall, while WRF-CAM5 is able to represent smoke properties and transport, some key discrepancies highlight the need for further analysis. Observations of smoke composition show an overall decrease in aerosol mean diameter as smoke ages over 4–12 d, while the model lacks this trend. A decrease in the mass ratio of organic aerosol (OA) to black carbon (BC), OA:BC, and the OA mass to carbon monoxide (CO) mixing ratio, OA:CO, suggests that the model is missing processes that selectively remove OA from the particle phase, such as photolysis and heterogeneous aerosol chemistry. A large (factor of ∼2.5) enhancement in sulfate from the free troposphere (FT) to the boundary layer (BL) in observations is not present in the model, pointing to the importance of properly representing secondary sulfate aerosol formation from marine dimethyl sulfide and gaseous SO2 smoke emissions. The model shows a persistent overprediction of aerosols in the marine boundary layer (MBL), especially for clean conditions, which multiple pieces of evidence link to weaker aerosol removal in the modeled MBL than reality. This evidence includes several model features, such as not representing observed shifts towards smaller aerosol diameters, inaccurate concentration ratios of carbon monoxide and black carbon, underprediction of heavy rain events, and little evidence of persistent biases in modeled entrainment. The average below-cloud aerosol activation fraction (NCLD/NAER) remains relatively constant in WRF-CAM5 between field campaigns (∼0.65), while it decreases substantially in observations from ORACLES (∼0.78) to CLARIFY (∼0.5), which could be due to the model misrepresentation of clean aerosol conditions. WRF-CAM5 also overshoots an observed upper limit on liquid cloud droplet concentration around NCLD= 400–500 cm−3 and overpredicts the spread in NCLD. This could be related to the model often drastically overestimating the strength of boundary layer vertical turbulence by up to a factor of 10. We expect these results to motivate similar evaluations of other modeling systems and promote model development to reduce critical uncertainties in climate simulations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Underestimated marine stratocumulus cloud feedback associated with overly active deep convection in models

Cloud feedback remains the largest source of uncertainty in equilibrium climate sensitivity (ECS). Many studies have attempted to narrow uncertainties in cloud feedback and ECS by proposing observable metrics with high skill at predicting future climate, referred to as emergent constraints. These constraints are often associated with clouds, convection, and circulation, and are interrelated. However, physical explanations for these connections remain unclear. Here, we propose a new mechanism relating convection and clouds across multiple climate models. Some models show overly active deep convection on daily timescales in the subtropical low cloud regions, which contributes to weaker subsidence inversion and smaller amounts of low-level clouds. Such models predict smaller shortwave (SW) cloud feedback. Using precipitation frequency in these regions as an emergent constraint, encapsulating this mechanism, models with lower SW cloud feedback (<0.50 W m -2 °C - 1) are found to exhibit erroneously frequent convection. Our results suggest that further improvements in understanding and better modeling of cloud and convective systems are necessary for accurate climate predictions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Reflecting Sunlight: Recommendations for Solar Geoengineering Research and Research Governance

The National Academies of Sciences, Engineering, and Medicine (NASEM) report "Reflecting Sunlight: Recommendations for Solar Geoengineering Research and Research Governance" focused on three atmospheric-based Solar Geoengineering strategies: Stratospheric Aerosol Injection, Marine Cloud Brightening, Cirrus Cloud Thinning. The study recommends that a national (and internationally-coordinated) Solar Geoengineering research program be established and coordinated by the U.S. Global Change Research Program—with a focus on developing information needed by decision makers, not advancing a path to deployment. The study recommends a detailed framework for governance of this research, at both national and international levels. The study also recommends a detailed research agenda for this program, encompassing over a dozen transdisciplinary research topics that can be loosely grouped into the categories of (i) technical dimensions and impacts, (ii) social dimensions, and (iii) context and goals for solar geoengineering research itself.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

Marine Shallow Cloud Adjustments to the Presence of Shortwave-Absorbing Aerosols: Advancing Understanding Through a Combined Analysis of Lasic Datasets and Process Modeling (Final Report)

This is a final report for this award, whose purpose was to support the analysis of data emanating from the LASIC (Layered Atlantic Smoke Interaction with Clouds) campaign. (Layered Atlantic Smoke Interactions with Clouds) is a strategy to improve our understanding of aged carbonaceous aerosol, its seasonal evolution, and the mechanisms by which clouds adjust to the presence of the aerosol. The observational strategy centers on deploying the AMF1 cloud, aerosol, and atmospheric profiling instrumentation to Ascension Island, located within the trade-wind shallow cumulus regime (14.50W, 80S) 3000 km offshore of continental Africa. The location is within the latitude zone of the maximum outflow of aerosol, with the deepening boundary layer known to entrain free-tropospheric smoke. The primary activities for LASIC are: 1) to improve current knowledge on aged biomass burning aerosol and its radiative properties as a function of the seasonal cycle; 2) to use surface-based remote sensing to sensitively interrogate the atmosphere for the relative vertical location of aerosol and clouds; 3) to improve our understanding of the cloud adjustments to the presence of shortwave-absorbing aerosol within the vertical column, both through aerosol-radiation and through aerosol-cloud interactions; 4) to aid low cloud parameterization efforts for climate models. This award serves to further these activities and includes a sub-award to Dr. Pablo Saide at UCLA for activities 3) and 4).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

A robust aerosol impact on clouds along the subtropical to tropical transition

Marine clouds undergo a transition from subtropical stratocumulus (Sc) to shallow cumulus (Cu) and eventually to deep convective (DC) systems as air masses advect from the subtropics towards the deep tropics. How aerosols modulate this Lagrangian cloud evolution remains largely uncertain. Here we use both 5 years of satellite observations mapped along 8 d Lagrangian trajectories and complementary large-eddy simulations from 9 initiation locations across the Northeast Pacific, Southeast Pacific, and Southeast Atlantic. This Lagrangian framework allows us to quantify the aerosol effect and its co-variability with meteorological conditions on cloud microphysics, macrophysics, and top-of-atmosphere radiation through the full Sc-Cu-DC transition. We show that increasing aerosol concentrations leads to deeper and more reflective clouds throughout this cloud transition. Examining the thermodynamic evolution along the trajectory indicates a well-known trend: enhanced moistening near the boundary-layer top and lower free troposphere under polluted conditions, suggesting that part of the co-variability between aerosol and meteorological conditions may be internally driven. The agreement between model simulations and satellite data alongside the multi-basin coherence of the results indicates that aerosols systematically amplify cloud depth and reflectivity during the subtropical–to–tropical cloud transition.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2022

The Shortwave Radiative Flux Response to an Injection of Sea Salt Aerosols in the Gulf of Mexico

We report marine cloud brightening (MCB) has been proposed as a potential means of geoengineering the climate, temporarily providing cooling to offset some of the effects of climate change. Marine sky brightening (MSB), involving the direct scattering of sunlight from sea salt injection into the marine boundary layer, has been proposed as an additional geoengineering method that could work in areas that are not regularly cloudy. Here, we use a regional atmospheric model to simulate MCB and MSB over the Gulf of Mexico and nearby land, a highly populated and economically important region that is not characterized by persistent marine stratocumulus cloud cover. Injection of sea salt in the Aitken mode from a region in the central Gulf of Mexico equivalent to 10.8 Tg yr -1 produces an upwards 8.4 W m -2 radiative flux change across the region at the top of the atmosphere, largely due to cloud property changes. Comparatively, a similar mass injection in the accumulation mode produces a 3.1 W m -2 radiative flux change driven primarily by direct scattering. Injection of even larger particles produces a much smaller radiative flux change. Shortwave flux changes due to clouds are largely driven by an increase in cloud droplet number concentration and an increase in cloud liquid water path (each contributing about 45% to the flux change), with a much lower contribution from cloud fraction changes (10%).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Understanding the causes of satellite–model discrepancies in aerosol–cloud interactions using near-LES simulations of marine boundary layer clouds

Aerosol–cloud interactions (ACI) remain the largest source of uncertainty in model estimates of anthropogenic radiative forcing, primarily because of deficiencies in representing aerosol–cloud microphysical processes that lead to inconsistent cloud liquid water path (LWP) responses to aerosol perturbations between observations and models. To investigate this discrepancy, we conducted a series of large-eddy-scale simulations driven by realistic meteorology over the eastern North Atlantic, and evaluated LWP susceptibility, precipitation processes, and boundary layer thermodynamics using satellite and ground-based observations. Simulated LWP responses show a strong dependence on cloud state. Non-precipitating thin clouds exhibit a modest LWP decrease with increasing cloud droplet number concentration (N d ), consistent in sign but weaker in magnitude than satellite estimates, reflecting enhanced turbulent mixing and evaporation. The largest model-observation discrepancy occurs in non-precipitating thick clouds, where simulated LWP susceptibilities are strongly positive (+0.32) while observations indicate large negative values (−0.69). This discrepancy stems from excessive precipitation driven by underestimated entrainment, overly active accretion, and overly broad drop-size distributions in polluted conditions. While our high-resolution setup mitigates the excessive drizzling common in coarser models and captures key regime transitions, these biases persist – highlighting that improved parameterizations of cloud-top processes, precipitation, and aerosol effects are needed beyond simply increasing model resolution. Additionally, misrepresented moisture inversions in reanalysis introduce a moist bias in cloud-top relative humidity, further amplifying positive LWP susceptibility. Our results also suggest that large negative N d –LWP relationships in observations may reflect internal cloud processes rather than true ACI effects.

Aerosol-cloud interaction↗
DOE OSTI2023

Large-Eddy Simulations of Marine Boundary Layer Clouds Associated with Cold-Air Outbreaks during the ACTIVATE Campaign. Part II: Aerosol–Meteorology–Cloud Interaction

Aerosol effects on micro/macrophysical properties of marine stratocumulus clouds over the western North Atlantic Ocean (WNAO) are investigated using in situ measurements and large-eddy simulations (LES) for two cold-air outbreak (CAO) cases (28 February and 1 March 2020) during the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE). The LES is able to reproduce the vertical profiles of liquid water content (LWC), effective radius r eff and cloud droplet number concentration N c from fast cloud droplet probe (FCDP) in situ measurements for both cases. Furthermore, we show that aerosols affect cloud properties (N c , r eff , and LWC) via the prescribed bulk hygroscopicity of aerosols ($\bar{κ}$) and aerosol size distribution characteristics. N c , r eff , and liquid water path (LWP) are positively correlated to $\bar{κ}$ and aerosol number concentration (N a ) while cloud fractional cover (CFC) is insensitive to $\bar{κ}$ and aerosol size distributions for the two cases. The realistic changes to aerosol size distribution (number concentration, width, and the geometrical diameter) with the same meteorology state allow us to investigate aerosol effects on cloud properties without meteorological feedback. We also use the LES results to evaluate cloud properties from two reanalysis products, ERA5 and MERRA-2. Compared to LES, the ERA5 is able to capture the time evolution of LWP and total cloud coverage within the study domain during both CAO cases while MERRA-2 underestimates them.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) Science Plan

Coastal cities provide the opportunity to characterize marine clouds and the substantial effects of manmade particles on cloud properties and processes. La Jolla lies to the north of San Diego, California, but it is often about a day directly downwind of the major pollution sources located in the ports of Los Angeles and Long Beach. The large dynamic range of aerosol particle concentrations combined with the multi-hour to multi-day persistence of stratocumulus cloud layers makes the site ideal for investigating the seasonal changes in cloud and aerosol properties as well as the quantitative relationships between cloud and aerosol properties.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2026

Drop clustering and drop size correlations from holographic imagery suggest cloud droplet spectral broadening via entrainment-mixing

The question of how droplets rapidly grow large enough to initiate collision-coalescence has persisted for decades. Many theories explaining the production of sufficiently large drops (i.e., those in the “bottleneck” size range; ∼ 25–50 µm diameters) involve drop clustering on millimeter scales. A novel method is introduced to evaluate drop clustering trends particle-by-particle (i.e., the number/proximity of neighboring drops for given droplets; defined as drop clustering fields) which are diagnosed relative to drops within their shared drop environments – in contrast to previous studies which diagnose drop clustering of defined sample volumes, or in terms of absolute length scales. Specifically, this study evaluates the statistical likelihood that drops of a given size are associated with either a significant number of neighboring drops, or are significantly isolated from neighboring drops. Observations are acquired from the HOLODEC during the Cloud System Evolution in the Trades campaign, which sampled subtropical marine clouds. The HOLODEC measures drop size distributions and the 3D spatial coordinates of droplets. Results show drops within the bottleneck size range (diameters of ∼ 25–50 µm) are most likely to be significantly isolated from neighboring drops. This “isolated large drop trend” is primarily observed at subsaturated conditions, suggesting entrainment is the contributing factor. Holograms associated with this trend are more likely to have broader drop size distributions, larger maximum drop sizes and overly regions where precipitation reaches the lowest altitudes from the sampled cloud, suggesting entrainment-mixing drop size distribution broadening is a relevant precipitation-initiation mechanism.

D'Alessandro, John J. [Univ. of Washington, Seattl↗
DOE OSTI2022

Environmental effects on aerosol–cloud interaction in non-precipitating marine boundary layer (MBL) clouds over the eastern North Atlantic

Abstract. Over the eastern North Atlantic (ENA) ocean, a total of 20 non-precipitating single-layer marine boundary layer (MBL) stratus and stratocumulus cloud cases are selected to investigate the impacts of the environmental variables on the aerosol–cloud interaction (ACIr) using the ground-based measurements from the Department of Energy Atmospheric Radiation Measurement (ARM) facility at the ENA site during 2016–2018. The ACIr represents the relative change in cloud droplet effective radius re with respect to the relative change in cloud condensation nuclei (CCN) number concentration at 0.2 % supersaturation (NCCN,0.2 %) in the stratified water vapor environment. The ACIr values vary from −0.01 to 0.22 with increasing sub-cloud boundary layer precipitable water vapor (PWVBL) conditions, indicating that re is more sensitive to the CCN loading under sufficient water vapor supply, owing to the combined effect of enhanced condensational growth and coalescence processes associated with higher Nc and PWVBL. The principal component analysis shows that the most pronounced pattern during the selected cases is the co-variations in the MBL conditions characterized by the vertical component of turbulence kinetic energy (TKEw), the decoupling index (Di), and PWVBL. The environmental effects on ACIr emerge after the data are stratified into different TKEw regimes. The ACIr values, under both lower and higher PWVBL conditions, more than double from the low-TKEw to high-TKEw regime. This can be explained by the fact that stronger boundary layer turbulence maintains a well-mixed MBL, strengthening the connection between cloud microphysical properties and the below-cloud CCN and moisture sources. With sufficient water vapor and low CCN loading, the active coalescence process broadens the cloud droplet size spectra and consequently results in an enlargement of re. The enhanced activation of CCN and the cloud droplet condensational growth induced by the higher below-cloud CCN loading can effectively decrease re, which jointly presents as the increased ACIr. This study examines the importance of environmental effects on the ACIr assessments and provides observational constraints to future model evaluations of aerosol–cloud interactions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Measurements and Analyses to Enable Science for the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE)

Coastal cities provide the opportunity to characterize the substantial effects of manmade particles on marine cloud properties and processes. La Jolla lies to the north of San Diego, California, but it is often about a day directly downwind of the major pollution sources located in the ports of Los Angeles and Long Beach. The large dynamic range of aerosol particle concentrations combined with the multi-hour to multi-day persistence of stratocumulus cloud layers makes the site ideal for investigating the seasonal changes in cloud and aerosol properties as well as the quantitative relationships between cloud and aerosol properties. The Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) characterized the extent, radiative properties, aerosol interactions, and precipitation characteristics of stratocumulus clouds in the Eastern Pacific across all four seasons at two coastal sites in La Jolla. This project was designed to enhance and expand the scientific uses of the ARM AMF1 measurements from EPCAPE. The goal was to ensure meaningful observations were collected that would enable science. The project included the following objectives: (1) Reviewing the ARM AMF1 measurements [ARM, 2021a; b] and circulating a summary of the measurements each week, (2) Comparing AMF1 measurements to those provided by collaborators (including filter measurements at the pier), (3) Collecting and analyzing filter samples from Scripps Pier by Fourier Transform Infrared spectroscopy (FTIR) and X-ray Fluorescence (XRF), (4) Assisting in operations of instruments provided by Guest PIs when possible, and (5) Providing an initial compilation of EPCAPE aerosol and cloud seasonal differences. The expected outcomes of these objectives were enhanced proposals and publications using EPCAPE measurements by helping to identify instrument issues, expanded data access and awareness by distributing weekly plots and related summaries, improved source-related attribution of aerosols with elemental tracers, additional observations provided by Guest PIs, and accelerated ACI studies enabled by the compiled seasonal summaries of aerosol and cloud properties. Three examples of the science enabled by this project are findings that (i) aerosol and cloud aqueous production contributes more than half of sulfate particle mass concentration, (ii) upwind sources make chemical composition very similar at nearby sites despite local differences in meteorology, and (iii) most of the large mass concentration of semi-volatile organic components is co-emitted and co-evaporated with nitrate. Together these findings illustrate how ARM extended field campaigns in coastal regions can be used to constrain ACI processes with direct observations. By using the unique ARM suite of cloud radiative products in addition to the measured aerosol properties at a coastal location, we were able to address the more specific question of which aerosol particles cause how much of the effects on clouds. Identifying this signature in coastal areas provides an opportunity to test the representation of aerosol sources by global models in a range of clean and urban-influenced conditions.

Russell, Lynn [Univ. of California, San Diego, CA ↗
DOE OSTI2020

A Regime-Oriented Approach to Observationally Constraining Extratropical Shortwave Cloud Feedbacks

The extratropical shortwave (SW) cloud feedback is primarily due to increases in extratropical liquid cloud extent and optical depth. Here, we examine the response of extratropical (35°–75°) marine cloud liquid water path (LWP) to a uniform 4-K increase in sea surface temperature (SST) in global climate models (GCMs) from phase 5 of the Coupled Model Intercomparison Project (CMIP5) and variants of the HadGEM3-GC3.1 GCM. Compositing is used to partition data into periods inside and out of cyclones. The response of extratropical LWP to a uniform SST increase and associated atmospheric response varies substantially among GCMs, but the sensitivity of LWP to cloud controlling factors (CCFs) is qualitatively similar. When all other predictors are held constant, increasing moisture flux drives an increase in LWP. Increasing SST, holding all other predictors fixed, leads to a decrease in LWP. The combinations of these changes lead to LWP, and by extension reflected SW, increasing with warming in both hemispheres. Observations predict an increase in reflected SW over oceans of 0.8–1.6 W m -2 per kelvin SST increase (35°–75°N) and 1.2–1.9 W m -2 per kelvin SST increase (35°–75°S). This increase in reflected SW is mainly due to increased moisture convergence into cyclones because of increasing available moisture. The efficiency at which converging moisture is converted into precipitation determines the amount of liquid cloud. Thus, cyclone precipitation processes are critical to constraining extratropical cloud feedbacks

58 GEOSCIENCES↗
DOE OSTI2023

Pluminate: Quantifying aerosol injection behavior from simulation, experimentation and observations

Marine aerosol injections are a key component in further understanding of both the potentials of deliberate injection for marine cloud brightening (MCB), a potential climate intervention (CI) strategy, and key aerosol-cloud interaction behaviors that currently form the largest uncertainty in global climate model (GCM) predictions of our climate. Since the rate of spread of aerosols in a marine environment directly translates to the effectiveness and ability of aerosol injections in impacting cloud radiative forcing, it is crucial to understand the spatial and temporal extent of injected-aerosol effects following direct injection into marine environments. The ubiquity of ship-injected aerosol tracks from satellite imagery renders observational validation of new parameterizations possible in 2D, however, 3D compatible data is more scarce, and necessary for the development of subgrid scale parameterizations of aerosol-cloud interactions in GCMs. This report introduces two novel parameterizations of atmospheric aerosol injection behavior suitable for both 3D (GCM-compatible) and 2D (observation-related) modeling. Their applicability is highlighted using a wealth of different observational data: small and larger scale salt-aerosol injection experiments conducted at SNL, 3D large eddy simulations of ship-injected aerosol tracks and 2D satellite images of ship tracks. The power of experimental data in enhancing knowledge of aerosol-cloud interactions is in particular emphasized by studying key aerosol microphysical and optical properties as observed through their mixing in cloud-like environments.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Maximum Supersaturation in the Marine Boundary Layer Clouds Over the North Atlantic

Abstract The maximum supersaturation ( S x ) in clouds is a key parameter affecting the cloud's microphysical and radiative properties. We investigate the S x of the marine boundary layer clouds by combining airborne and surface observations in the Eastern North Atlantic. The cloud droplet number concentration ( N c ) in the least diluted cloud cores agrees well with the number concentration of particles larger than the Hoppel Minimum (HM) ( N >HM ) below clouds, indicating that the HM represents the average size threshold above which particles are activated to form cloud droplets. The S x values derived from surface observations vary from 0.10% to 0.50% from June 2017 to June 2018, with a clear seasonal variation exhibiting higher values during winter. Most of the S x variance (∼60%) can be explained by the cloud condensation nuclei (CCN) concentration and updraft velocity ( w ), with the CCN concentration playing a more important role than w in explaining the variation of S x . The influence of CCN concentration on S x leads to a buffered response of N c to aerosol perturbations. The response of N c to low aerosol concentration during winter is further buffered by the high w . The global Community Earth System Model (CESM) simulated S x values in the Azores have a positive bias compared to measured S x , likely due to overestimated w and underestimated CCN concentration. The CESM simulated S x exhibits higher values further north over the North Atlantic Ocean, which is attributed to stronger w . The suppression of S x by aerosol is also evident in regions with high CCN concentrations.

54 ENVIRONMENTAL SCIENCES↗