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At least 55 records · Page 3

Aerosol Direct, Indirect, Semidirect, and Surface Albedo Effects from Sector Contributions Based on the IPCC AR5 Emissions for Preindustrial and Present-day Conditions

The anthropogenic increase in aerosol concentrations since preindustrial times and its net cooling effect on the atmosphere is thought to mask some of the greenhouse gas-induced warming. Although the overall effect of aerosols on solar radiation and clouds is most certainly negative, some individual forcing agents and feedbacks have positive forcing effects. Recent studies have tried to identify some of those positive forcing agents and their individual emission sectors, with the hope that mitigation policies could be developed to target those emitters. Understanding the net effect of multisource emitting sectors and the involved cloud feedbacks is very challenging, and this paper will clarify forcing and feedback effects by separating direct, indirect, semidirect and surface albedo effects due to aerosols. To this end, we apply the Goddard Institute for Space Studies climate model including detailed aerosol microphysics to examine aerosol impacts on climate by isolating single emission sector contributions as given by the Coupled Model Intercomparison Project Phase 5 (CMIP5) emission data sets developed for Intergovernmental Panel on Climate Change (IPCC) AR5. For the modeled past 150 years, using the climate model and emissions from preindustrial times to present-day, the total global annual mean aerosol radiative forcing is -0.6 W/m(exp 2), with the largest contribution from the direct effect (-0.5 W/m(exp 2)). Aerosol-induced changes on cloud cover often depends on cloud type and geographical region. The indirect (includes only the cloud albedo effect with -0.17 W/m(exp 2)) and semidirect effects (-0.10 W/m(exp 2)) can be isolated on a regional scale, and they often have opposing forcing effects, leading to overall small forcing effects on a global scale. Although the surface albedo effects from aerosols are small (0.016 W/m(exp 2)), triggered feedbacks on top of the atmosphere (TOA) radiative forcing can be 10 times larger. Our results point out that each emission sector has varying impacts by geographical region. For example, the single sector most responsible for a net positive radiative forcing is the transportation sector in the United States, agricultural burning and transportation in Europe, and the domestic emission sector in Asia. These sectors are attractive mitigation targets.

Bauer, Susanne E.↗

SPEX Airborne Spectropolarimeter Calibration and Performance

To improve our understanding of the complex role of aerosols in the climate system and on air quality, measurements are needed of optical and microphysical aerosol. From many studies, it has become evident that a satellite-based multiangle, multiwavelength polarimeter will be essential to provide such measurements. Here, high accuracy (∼0.003) on the degree of linear polarization (DoLP) measurements is important to retrieve aerosol properties with an accuracy needed to advance our understanding of the aerosol effect on climate. SPEX airborne, a multiangle hyperspectral polarimeter, has been developed for observing and characterizing aerosols from NASA’s high-altitude research aircraft ER-2. It delivers measurements of radiance and DoLP at visual wavelengths with a spectral resolution of 3 and 7–30 nm, respectively, for radiance and polarization, at nine fixed equidistant viewing angles from −56° to +56° oriented along the ground track, and a swath of 7° oriented across-track. SPEX airborne uses spectral polarization modulation to determine the state of linear polarization of scattered sunlight. This technique has been developed in the Netherlands and has been demonstrated with ground-based instruments. SPEX airborne serves as a demonstrator for a family of space-based SPEX instruments that have the ability to measure and characterize atmospheric aerosol by multiangle hyperspectral polarimetric imaging remotely from a satellite platform. SPEX airborne was calibrated radiometrically and polarimetrically using Jet Propulsion Laboratory (JPL) facilities including the Polarization Stage Generator-2 (PSG-2), which is designed for polarimetric calibration and validation of the Airborne Multiangle SpectroPolarimetric Imager (AirMSPI). Using the PSG-2, the accuracy of the SPEX airborne DoLP measurements in the laboratory setup is found to be 0.002–0.004. Radiometric calibration is realized with an estimated accuracy of 4%. In 2017, SPEX airborne took part in the “Aerosol Characterization from Polarimeters and Lidar” campaign on the ER-2 that included four polarimeters and two lidars. Polarization measurements of SPEX airborne and the coflying Research Scanning Polarimeter (RSP), recorded during the campaign, were compared and display root-mean-square (RMS) differences ranging from 0.004 (at 555 nm) up to 0.02 (at 410 nm). For radiance measurements, excellent agreement between SPEX airborne and RSP is obtained with an RMS difference of ∼4%. The lab- and flight-performance values for polarization are similar to those recently published for AirMSPI, where also an intercomparison with RSP was made using data from field campaigns in 2013. The intercomparison of radiometric and polarimetric data both display negligible bias. The in-flight comparison results provide verification of SPEX airborne’s capability to deliver high-quality data.

Aerosols↗

TPSAS-NF1676L-34796-DND

The recently completed 2015-2017 EVS-2 mission NAAMES (The North Atlantic Aerosols and Marine Ecosystems Study) provides a unique set of airborne remote sensing and ship-based in situ measurements in a remote and under-sampled region of the Earth?s ocean. The NASA SABOR (Ship-Aircraft Bio-Optical Research) campaign was conducted during the summer of 2014, also in the Atlantic Ocean, out of the Chesapeake Bay and in the eastern coastal region of the United States. For both campaigns, the NASA GISS Research Scanning Polarimeter, a multi-angle, multi-spectral polarimeter measured the upwelling polarized radiances from aircraft. And for both campaigns, ship-based in situ measurements of the ocean were collected jointly with the aircraft measurements. We present results from the new RSP-MAPP (1) that is based on optimal estimation and that can retrieve simultaneous aerosol microphysical properties (including effective radius, single-scattering albedo, and real refractive index) and ocean color products using accurate radiative transfer, Mie calculations, and the DP (Detritus Plankton) series of accurate, numerically efficient ocean bio-optical models. The RSP-MAPP algorithm was applied to data collected during SABOR and NAAMES to retrieve aerosol microphysics and ocean products for all Aerosols-Above-Ocean (AAO) scenes. The RSP-MAPP products are compared against i) collocated aerosol extinction and backscatter profiles collected by the NASA LaRC airborne High Spectral Resolution Lidar (HSRL-1), including lidar depth profiles of the ocean diffuse attenuation coefficient and the hemispherical backscatter coefficient, and ii) collocated ship-based in situ measurements of the ocean.

Snorre Stamnes↗

Self-limiting physical and chemical effects in volcanic eruption clouds

One-dimensional aerosol microphysical and photochemical models are used to study the chemistry of stratospheric volcanic clouds. The results indicate that the aerosol microphysical processes of condensation and coagulation produce larger particles as the SO2 injection rate is increased. Larger particles have a smaller optical depth per unit mass and settle out of the stratosphere at a faster rate than smaller ones, restricting the total number of particles in the stratosphere. The microphysical processes moderate the impact of volcanic clouds on the earth's radiation budget and climate, suggesting that volcanic effects may be self limiting. It is noted that the injection of HCl into the stratosphere, which could lead to large ozone changes, is limited by a cold trap effect in which HCl and water vapor condense on ash particles in the rising volcanic plume and fall out as ice.

Pinto, Joseph P.↗

Remote Sensing of Aerosol Optical and Microphysical Properties using Polarization and Lidar Techniques

Tropospheric aerosols cause a substantial forcing of the terrestrial climate, but the magnitude of this forcing remains largely unknown. This explains the significant interest of the climate community to the prospect of measuring key aerosol properties from space using advanced remote sensing techniques. It has been known for a long time that polarization of the scattered light is much more sensitive to the aerosol microphysics than the scattered intensity. It is, therefore, not surprising that the most recent addition to the New Polar Orbiting Operational Environmental Satellite System (NPOESS) payload is the so-called Aerosol Polarimetry Sensor (APS). The main objective of this instrument is to measure the aerosol and cloud properties with accuracy and coverage sufficient for a reliable estimate of the direct and indirect aerosol forcings of climate. Accordingly, the first part of this lecture course will focus on describing the basic concept of the APS, the physical principles of polarization data analyses, and the results already obtained with an aircraft version of the APS. Polar stratospheric clouds (PSCs) represent another poorly understood aerosol component of the terrestrial atmosphere which affects the climate by supporting chemical reactions destroying the ozone layer. The high altitude of the PSCs and their predominant occurrence in high latitude and polar regions make it very difficult to study PSCs using conventional in situ techniques. Most of the information that we have about this type of clouds has been gathered using ground-based polarization lidars. The second part of the course will focus on explaining the physical principles of the polarization lidar technique and describing retrievals of PSC particle microphysical characteristics by converting I multispectral lidar measurements of the backscattered intensity and depolarization.

Mishchenko, Michael↗

Improvement of Stratospheric Aerosol Extinction Retrieval from OMPS/LP Using a New Aerosol Model

The Ozone Mapping and Profiler Suite Limb Profiler (OMPS/LP) has been flying on the Suomi National Polar-orbiting Partnership (S-NPP) satellite since October 2011. It is designed to produce ozone and aerosol vertical profiles at 2-kilometer vertical resolution over the entire sunlit globe. Aerosol extinction profiles are computed with Mie theory using radiances measured at 675 nanometers. The operational Version 1.0 (V1.0) aerosol extinction retrieval algorithm assumes a bimodal lognormal aerosol size distribution (ASD) whose parameters were derived by combining an in situ measurement of aerosol microphysics with the Stratospheric Aerosol and Gas Experiment (SAGE II) aerosol extinction climatology. Internal analysis indicates that this bimodal lognormal ASD does not sufficiently explain the spectral dependence of LP-measured radiances. In this paper we describe the derivation of an improved aerosol size distribution, designated Version 1.5 (V1.5), for the LP retrieval algorithm. The new ASD uses a gamma function distribution that is derived from Community Aerosol and Radiation Model for Atmospheres (CARMA)-calculated results. A cumulative distribution fit derived from the gamma function ASD gives better agreement with CARMA results at small particle radii than bimodal or unimodal functions. The new ASD also explains the spectral dependence of LP-measured radiances better than the V1.0 ASD. We find that the impact of our choice of ASD on the retrieved extinctions varies strongly with the underlying reflectivity of the scene. Initial comparisons with collocated extinction profiles retrieved at 676 nanometers from the SAGE III instrument on the International Space Station (ISS) show a significant improvement in agreement for the LP V1.5 retrievals. Zonal mean extinction profiles agree to within 10 percent between 19 and 29 kilometers, and regression fits of collocated samples show improved correlation and reduced scatter compared to the V1.0 product. This improved agreement will motivate development of more sophisticated ASDs from CARMA results that incorporate latitude, altitude and seasonal variations in aerosol properties.

Ozone Mapping Profiler Suite Limb Profiler (OMPS/L↗

Development of a global model for atmospheric backscatter at CO2 wavelengths

Computer graphics software was developed to examine in detail the simulated variations of aerosol size distribution due to gravitational sedimentation effects. This examination contributes to understanding the effect of aerosol microphysical processes occurring in an aerosol plume which undergoes transport in the atmosphere. Results are presented in graphical form. Future research directions are outlined.

Source record↗

Development of a global model for atmospheric backscatter at CO2 wavelengths

Work on the following tasks is reported briefly: (1) to investigate the effect of aerosol microphysical processes, occurring in an aerosol plume which undergoes transport in the atmosphere, on its beta sub CO2 value and (2) to examine experimentally measured size distributions for the free troposphere, fit bimodal log-normal models with different retractive indices for the two modes, and calculate beta sub CO2.

Source record↗

Simulating the Volcanic Sulfate Aerosols From the 1991 Eruption of Cerro Hudson and Their Impact on the 1991 Ozone Hole

The Chilean volcano Cerro Hudson erupted between August 8th and 15th, 1991, injecting between 1.7 and 2.9 Tg of SO2 into the upper troposphere and lower stratosphere. We simulate this injection using the GEOS Earth system model with detailed sulfur chemistry and sectional aerosol microphysics, focusing on the resulting aerosols and their contribution to the 1991 Antarctic Austral Springtime ozone hole. The simulations show a column ozone deficit (12 DU) in the Southern Hemisphere vortex collar region. The majority of this effect is between 10 and 20 km and due to heterogeneous chemistry. The model shows a 26% decrease in ozone from background levels at these altitudes, compared with in-situ observations of a 50% decrease. Above 20 km, the dynamical response to the eruption also causes lower ozone values, a novel modeling result. This experiment highlights potential interactions between proposed solar radiation management geoengineering aerosols and volcanic eruptions.

aerosols↗

Lower stratospheric aerosols at a tropical latitude station

A pulsed ruby lidar has been in regular operation at the tropical station Trivandrum (8 deg 33 sec N, 76 deg 57 sec E) since October 1986. The lidar data were analyzed to obtain monthly mean aerosol extinction at lower stratospheric altitudes. The monthly mean variation of aerosol extinction shows a peak in March to April with a trough in the winter months. This behavior is compared with that of temperature at the same altitude, obtained from balloonsonde measurements at the same station. It is found that there is a negative correlation between the two with high extinction values corresponding to low temperature values and vice versa. This is attributed to the stratospheric aerosol microphysical processes. The association of stratospheric aerosol extinction with the tropopause altitude and temperature was studied along with the implications of these results.

Krishnamurthy, B. V.↗

Inversion of multiangular polarimetric measurements from the ACEPOL campaign: an application of improving aerosol property and hyperspectral ocean color retrievals

NASA's Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) mission, scheduled for launch in the time frame of late 2022 to early 2023, will carry the Ocean Color Instrument (OCI), a hyperspectral scanning radiometer, and two multiangle polarimeters (MAPs), the UMBC Hyper-Angular Rainbow Polarimeter 2 (HARP2) and the SRON Spectro-Polarimeter for Planetary EXploration one (SPEXone). One purpose of the PACE MAPs is to better characterize aerosol properties, which can then be used to improve atmospheric correction for the retrieval of ocean color in coastal waters. Though this is theoretically promising, the use of MAP data in the atmospheric correction of colocated hyperspectral ocean color measurements have not yet been well demonstrated. In this work, we performed aerosol retrievals using the MAP measurements from the Research Scanning Polarimeter (RSP) and demonstrate its application to the atmospheric correction of hyperspectral radiometric measurements from SPEX airborne. Both measurements were collected on the same aircraft from the Aerosol Characterization from Polarimeter and Lidar (ACEPOL) field campaign in 2017. Two cases over ocean with small aerosol loading (aerosol optical depth ∼0.04) are identified including colocated RSP and SPEX airborne measurements and Aerosol Robotic Network (AERONET) ground-based observations. The aerosol retrievals are performed and compared with two options: one uses reflectance measurement only and the other uses both reflectance and polarization. It is demonstrated that polarization information helps reduce the uncertainties of aerosol microphysical and optical properties. The retrieved aerosol properties are then used to compute the contribution of atmosphere and ocean surface for atmospheric correction over the discrete bands from RSP measurements and the hyperspectral SPEX airborne measurements. The water-leaving signals determined this way are compared with both AERONET and Moderate Resolution Imaging Spectroradiometer (MODIS) ocean color products for performance analysis. The results and lessons learned from this work will provide a basis to fully exploit the information from the unique combination of sensors on PACE for aerosol characterization and ocean ecosystem research.

Meng Gao↗

Development of a global model for atmospheric backscatter at CO2 wavelengths

The effect of aerosol microphysical processes on the backscatter from an aerosol plume undergoing long-range atmospheric transport was studied. A numerical model which examines the effects of coagulation and sedimentation on an aerosol size distribution is under development and the initial results for a single homogeneous layer were obtained. Use was made of the SAGE/SAM II data set to study the global variation of aerosol concentration and, hence, to predict the variation of Beta sub CO2. Computer programs were written to determine the mean, median, and the probability distribution of the measured aerosol extinction as a function of altitude, latitude and geographical conditions. The first data sets analyzed in this way are under study. Data was used to study aerosol behavior over the U.S.A. and the Pacific Ocean.

Kent, G. S.↗

The Turning Point of the Aerosol Era

Over the CMIP6 historical period (1850–2014), aerosols provided the largest negative forcing compared to all other climate forcings via their ability to absorb or scatter solar radiation and alter clouds. Aerosols played an important role in counterbalancing warming by greenhouse gases (GHGs). Here we study aerosol forcing trends in the CMIP6 simulations of the NASA Goddard Institute for Space Studies (GISS) ocean-atmosphere ModelE version 2.1 (GISS-E2.1-G) using a fully coupled atmospheric composition configuration, including interactive gas-phase chemistry, and either an aerosol microphysical (MATRIX) or a mass-based aerosol (OMA) module. Simulations of the CMIP6 historical period are analyzed as well as four Shared Socioeconomic Pathway (SSP) future scenarios for 2015–2100: SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5. The main conclusion of this study is that aerosol forcing in the GISS model has reached its turning point, switching from globally increasing to a decreasing trend in the first decade of the 21st century. This result is robust, independent of which aerosol module or SSP scenario is used. Non-linear aerosol-cloud interactions dominate as a forcing agent over aerosol-radiation interactions. Aerosols' ability to counterbalance GHG forcing on the global scale is today at a level comparable to that at the beginning of the last century. In the 1980s, the decade of largest global aerosol loads, aerosols balanced up to 80% of GHG forcing. As a consequence, global warming of the last decades, which is primarily driven by greenhouse gases, has been augmented by the effect of decreasing aerosol cooling in our model. By the end of this century, following the SSP scenarios, aerosols will only counterbalance 0%–20% of GHG forcing, depending on model and on scenario.

Aerosol forcing↗

Simultaneous Aerosol and Ocean Polarimeter Products Using Coupled Atmosphere-Ocean Vector Radiative Transfer and Neural Networks: The PACE-MAPP Algorithm

We describe the PACE-MAPP algorithm that simultaneously retrieves aerosol and ocean optical parameters using multiangle and multi-channel polarimeter measurements from the SPEXone, Hyper-Angular Rainbow Polarimeter 2 (HARP2), and Ocean Color Instrument (OCI) instruments onboard the NASA Plankton, Aerosol, Cloud, ocean Ecosystem (PACE) observing system PACE-MAPP is adapted from the Research Scanning Polarimeter (RSP) Microphysical Aerosol Properties from Polarimetry (RSP-MAPP) algorithm. A key feature of the MAPP family of algorithms is the use of a coupled vector radiative transfer model such that the atmosphere and ocean are always considered together as one system. Consequently, conservation of energy ensures that negative water-leaving radiances do not occur. PACE-MAPP uses optimal estimation to simultaneously characterize the optical and microphysical properties of aerosol and ocean constituents, find the optimal solution, and reliably account for the uncertainties of each parameter. This coupled approach, together with multiangle, multi-channel polarimeter measurements, will enable retrievals of aerosol and water properties across the Earth’s oceans. The PACE-MAPP algorithm provides aerosol and ocean products for both the open ocean and coastal areas and is designed to be accurate, modular, and efficient by using fast neural networks that replace the time-consuming vector radiative transfer calculations. We provide an overview of the PACE-MAPP framework and also describe its modular components including its aerosol and hydrosol models, ocean bio-optical models, and thin cirrus model.

Snorre Stamnes↗

Historical evidence for a connection between volcanic eruptions and climate change

The times of historical volcanic aerosol clouds were compared with changes in atmospheric temperatures on regional, hemispheric, and global scales. These involve either a direct comparison of individual significant eruption years with temperature records, or a comparison of eruption years with composited temperature records for several years before and after chosen sets of eruptions. Some studies have challenged the connection between individual eruptions and climate change. Mass and Portman (1989) recently suggested that the volcanic signal was present, but smaller than previously thought. In a study designed to test the idea that eruptions could cause small changes in climate, Hansen and other (1978) chose one of the best monitored eruptions at the time, the 1963 eruption of Agung volcano on the island of Bali. Using a simple radiation-balance model, in which an aerosol cloud in the tropics was simulated, this basic pattern of temperature change in the tropics and subtropics was reproduced. There may be natural limits to the atmospheric effects of any volcanic eruption. Self-limiting physical and chemical effects in eruption clouds were proposed. Model results suggest that aerosol microphysical processes of condensation and coagulation produce larger aerosols as the SO2 injection rate is increased. The key to discovering the greatest effects of volcanoes on short-term climate may be to concentrate on regional temperatures where the effects of volcanic aerosol clouds can be amplified by perturbed atmospheric circulation patterns, especially changes in mid-latitudes where meridional circulation patterns may develop. Such climatic perturbations can be detected in proxy evidence such as decreases in tree-ring widths and frost damage rings in climatically sensitive parts of the world, changes in treelines, weather anomalies such as unusually cold summers, severity of sea-ice in polar and subpolar regions, and poor grain yields and crop failures.

Rampino, Michael R.↗

Organic Aerosol Volatility Parameterizations and Their Impact on Atmospheric Composition and Climate

Despite their importance and ubiquity in the atmosphere, organic aerosols are still very poorly parameterized in global models. This can be explained by two reasons: first, a very large number of unconstrained parameters are involved in accurate parameterizations, and second, a detailed description of semi-volatile organics is computationally very expensive. Even organic aerosol properties that are known to play a major role in the atmosphere, namely volatility and aging, are poorly resolved in global models, if at all. Studies with different models and different parameterizations have not been conclusive on whether the additional complexity improves model simulations, but the added diversity of the different host models used adds an unnecessary degree of variability in the evaluation of results that obscures solid conclusions. Aerosol microphysics do not significantly alter the mean OA vertical profile or comparison with surface measurements. This might not be the case for semi-volatile OA with microphysics.

Aerosols↗

Potential impact of aerosols on convective clouds revealed by Himawari-8 observations over different terrain types in eastern China

Convective clouds are common and play a major role in Earth's water cycle and energy balance; they may even develop into storms and cause severe rainfall events. To understand the convective cloud development process, this study investigates the impact of aerosols on convective clouds by considering the influence of both topography and diurnal variation in radiation. By combining texture analysis, clustering, and thresholding methods, we identify all convective clouds in two warm seasons (May–September, 2016/17) in eastern China based on Himawari-8 Level 1 data. Having large diurnally resolved cloud data together with surface meteorological and environmental measurements, we investigate convective cloud properties and their variation, stratified by elevation and diurnal change. We then analyze the potential impact of aerosol on convective clouds under different meteorological conditions and topographies. In general, convective clouds tend to occur preferentially under polluted conditions in the morning, which reverses in the afternoon. Convective cloud fraction first increases then decreases with aerosol loading, which may contribute to this phenomenon. Topography and diurnal meteorological variations may affect the strength of aerosol microphysical and radiative effects. Updraft is always stronger along the windward slopes of mountains and plateaus, especially in northern China. The prevailing southerly wind near the foothills of mountains and plateaus is likely to contribute to this windward strengthening of updraft and to bring more pollutant into the mountains, thereby strengthening the microphysical effect, invigorating convective clouds. By comparison, over plain, aerosols decrease surface heating and suppress convection by blocking solar radiation reaching the surface.

clouds↗

Potential impact of aerosols on convective clouds revealed by Himawari-8 observations over different terrain types in Eastern China

Convective clouds are common and play a major role in Earth’s water cycle and energy balance; they may even develop into storms and cause severe rainfall events. To understand the convective cloud development process, this study investigates the impact of aerosols on convective clouds by considering the influence of both topography and diurnal variation of radiation. By combining texture analysis, clustering and thresholding methods, we identify all convective clouds in two warm seasons (May-September, 2016-2017) in eastern China based on Himawari-8 Level 1 data. Having a large diurnally resolved cloud data together with surface meteorological and environmental measurements, we investigate convective cloud properties and their variation, stratified by elevation and diurnal change. We then analyze the potential impact of aerosol on convective clouds under different meteorological conditions and topographies. In general, convective clouds tend to occur preferentially under polluted conditions in the morning, which reverses in the afternoon. Convective cloud fraction first increases then decreases with aerosol loading, which may contribute to this phenomenon. Topography and diurnal meteorological variations may affect the strength of aerosol microphysical and radiative effects. Updraft is always stronger along the windward slopes of mountains and plateaus, especially in northern China. The prevailing southerly wind near the foothills of mountains and plateaus is likely to contribute to this windward strengthening of updraft and to bring more pollutant into the mountains, thereby strengthening the microphysical effect, invigorating convective clouds. By comparison, over plain, aerosols decrease surface heating and suppresses convection by blocking solar radiation reaching the surface.

Tianmeng Chen↗