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DOE OSTI2025

Demonstration of a Novel Radiochemical Mix Diagnostic for Fusion Implosions at the National Ignition Facility

Mixing of the ablator material into the fuel of an inertial confinement fusion implosion reduces compression and enhances radiative losses, preventing ignition. Here, we describe a novel use of charged-particle radiochemistry to measure the ablator mix in contact with the fusion hot spot. The capsule uses a graded Be-Cr layer to increase the confinement of the hot spot. 52 Mn and 51 Cr isotopes are collected from the implosion and counted, and the ratio is related to the amount of Cr mixed into the hot spot. Thus, a new diagnostic to determine the degradation due to mix on fusion implosions has been developed.

MacLaren, S. A. [Lawrence Livermore National Labor↗

DOE OSTI2022

Co-optimized Mixed-Mode Engine and Fuel Demonstrator for Improved Fuel Economy while Meeting Emissions Requirements

Progressively increasing regulatory demands on fuel economy and future global emission standards have led to a focus on advanced engine development to improve overall engine efficiency and fulfill emission requirements. Low temperature combustion (LTC) and gasoline compression ignition (GCI) are promising technologies to achieve these goals and have the advantage of using existing refinery infrastructure and subsequent economies of scale for a robust energy supply. By applying spark ignition (SI) for cold start, LTC for low load operations, and GCI for medium to high load operations, a multimode GCI engine concept was proposed and the fuel formation was co-optimized to maximize fuel economy improvement potential while maintaining ULEV 70 emissions standards. HATCI has successfully demonstrated the feasibility of this multimode GCI engine concept, and confirmed the fuel economy improvement over the baseline SI engine by simulating the FTP75 vehicle drive cycle. In this report, the technical approaches, multimode engine control, and engine test results of both steady state and transitions, CFD modeling, fuel testing, and FTP75 drive cycle simulation results are summarized, followed with technical challenges observed, and recommendations for possible follow-up studies.

02 PETROLEUM↗

DOE OSTI2022

Qualification of ANSI/HPS N13.1-2011 Mixing Criteria by Computational Fluid Dynamics Modeling for the 3430 Building Fan Addition and Increased Ventilation Capacity

Additional ventilation capacity has been designed for the 3430 Building filtered exhaust stack system. The updated system will increase the number of fans from two to three and include new ductwork with a larger diameter to integrate the new fan into the existing stack. Stack operations will involve running various fan combinations at any given time. The air monitoring system of the existing two-fan stack previously was found to comply with the American National Standards Institute/Health Physics Society (ANSI/HPS) N13.1-1999 standard. Full-scale, three-dimensional computational fluid dynamics (CFD) modeling was used to evaluate the modified three-fan system for compliance with the ANSI/HPS N13.1-2011 standard, which essentially is equivalent to the ANSI/HPS N13.1-1999 standard. The four mixing criteria evaluated are 1) flow angle, 2) velocity, 3) gas tracer, and 4) particle tracer. Benchmarking of the CFD modeling methodology showed good agreement with previous testing used to qualify the stack, and modeling of the existing two-fan system showed good agreement with test data collected from the 3430 Building stack. Modeling was performed to develop a suitable three-fan design. Initial modeling of the three-fan design and basic ductwork showed that flow angles and velocity uniformity were acceptable; however, the gas tracer and particle tracer mixing results were not acceptable. To meet ANSI/HPS N13.1-2011 criteria, an air blender was added to the stack design.

42 ENGINEERING↗

DOE OSTI2022

Qualification of ANSI/HPS N13.1-2011 Mixing Criteria by Computational Fluid Dynamics Modeling for the 3430 Building Fan Addition and Increased Ventilation Capacity

42 ENGINEERING↗

DOE OSTI2024

Controlling radioisotope proportions when randomly sampling from Dirichlet distributions in PyRIID

As machine learning models for radioisotope quantification become more powerful, likewise the need for high-quality synthetic training data grows as well. For problem spaces that involve estimating the relative isotopic proportions of various sources in gamma spectra it is necessary to generate training data that accurately represents the variance of proportions encountered. In this report, we aim to provide guidance on how to target a desired variance of proportions which are randomly when using the PyRIID Seed Mixer, which samples from a Dirichlet distribution. We provide a method for properly parameterizing the Dirichlet distribution in order to maintain a constant variance across an arbitrary number of dimensions, where each dimension represents a distinct source template being mixed. We demonstrate that our method successfully parameterizes the Dirichlet distribution to target a specific variance of proportions, provided that several conditions are met. This allows us to follow a principled technique for controlling how random mixture proportions are generated which are then used downstream in the synthesis process to produce the final, noisy gamma spectra.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2024

Qualification of Mixing Criteria by Computational Fluid Dynamics Modeling for the 325 Building Stack Revision

Additional ventilation capacity has been designed for the 325 Building filtered exhaust stack system. The four (4) existing main facility exhaust fans are past the end of their useful life. The fans are being replaced to provide additional exhaust capacity for future growth and to provide a more robust system. Stack operations will involve running various fan combinations at any given time. The air monitoring system of the existing stack previously was found to comply with the American National Standards Institute/Health Physics Society (ANSI/HPS) N13.1-1999 standard. Full-scale, three-dimensional computational fluid dynamics (CFD) modeling was used to evaluate the modified four-fan system for compliance with the ANSI/HPS N13.1-2021 standard, which essentially is equivalent in mixing requirements to the ANSI/HPS N13.1-1999 standard (and ANSI/HPS N13.1-2011). The four mixing criteria evaluated are 1) flow angle, 2) velocity, 3) gas tracer, and 4) particle tracer. In addition to the evaluating the modified four-fan system a temporary single fan stack configuration was also evaluated with CFD modeling. The temporary stack is planned to be used while the four-fan system is being modified. Modeling of the modified four-fan design and temporary ductwork showed that flow angles, velocity uniformity, gas tracer, and particle tracer were acceptable.

42 ENGINEERING↗

DOE OSTI2022

On the Spectral Evolution of Hot White Dwarf Stars. II. Time-dependent Simulations of Element Transport in Evolving White Dwarfs with STELUM

White dwarf stars are subject to various element transport mechanisms that can cause their surface composition to change radically as they cool, a phenomenon known as spectral evolution. In this paper, we undertake a comprehensive theoretical investigation of the spectral evolution of white dwarfs. First, we introduce STELUM, a new implementation of the stellar evolutionary code developed at the Université de Montréal. We provide a thorough description of the physical content and numerical techniques of the code, covering the treatment of both stellar evolution and chemical transport. Then, we present two state-of-the-art numerical simulations of element transport in evolving white dwarfs. Atomic diffusion, convective mixing, and mass loss are considered simultaneously as time-dependent diffusive processes and are fully coupled to the cooling. We first model the PG 1159-DO-DB-DQ evolutionary channel: a helium-, carbon-, and oxygen-rich PG 1159 star transforms into a pure-helium DB white dwarf due to gravitational settling and then into a helium-dominated, carbon-polluted DQ white dwarf through convective dredge-up. We also compute for the first time the full DO-DA-DC evolutionary channel: a helium-rich DO white dwarf harboring residual hydrogen becomes a pure-hydrogen DA star through the float-up process and then a helium-dominated, hydrogen-bearing DC star due to convective mixing. We demonstrate that our results are in excellent agreement with available empirical constraints. In particular, our DO-DA-DC simulation perfectly reproduces the lower branch of the bifurcation observed in the Gaia color–magnitude diagram, which can therefore be interpreted as a signature of spectral evolution.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1974

An examination of injector/combustor design effects on scramjet performance

Description of a simplified one-dimensional treatment of fuel injection for supersonic combustor performance analysis. Representative mixing efficiency variations for both parallel and cross-stream injection are obtained, and approximate means for estimating the length required for complete mixing are demonstrated. Comparisons of calculated and measured data show good agreement.

Anderson, G. Y.↗

NASA NTRS1976

Formation of ferrobasalt at east Pacific midocean spreading centers

A numerical modeling using a least squares petrologic mixing program demonstrates that ridge ferrobasalts from three east Pacific regions are generated from normal midocean ridge balsalt by crystal fractionation of plagioclase, clinopyroxene, and minor olivine at shallow mantle depths. Clinopyroxene is an important fractionating phase in this model in contrast to most previously proposed fractionation models. Calculations demonstrate that the ferrobasalts represent a much smaller percentage of residual liquid than has previously been proposed. Implications of extensive shallow crystal fractionation for the determination of depths of magma generation are discussed. The different fields on an anorthite-olivine-hypersthene ternary diagram for basalts from east Pacific fast and moderate spreading ridges can be explained by variable degrees of shallow crystal fractionation rather than by different depths of magma generation as suggested by Bass (1971) and Scheidegger (1973).

Clague, D. A.↗

NASA NTRS1981

An advective model for two-dimensional transport of stratospheric trace species

A parameterization of two-dimensional transport is applied to photochemical models of stratospheric trace species. It is shown that in a first approximation, tracer transport in the meridional plane may be treated as an advective rather than a diffusive process. The concept of residual mean meridional circulation (Andrews and McIntyre, 1976; Boyd, 1976) is used in the model and shown to be a modified Eulerian mean, a good approximation to the Lagrangian mean motion. A simple example in which the equilibrium distribution is computed for a tracer with a uniform tropospheric source and a stratospheric sink proportional to the local mixing ratio demonstrates the potential of the proposed parameterization. The resulting distribution is found to agree qualitatively with the observed stratospheric distribution of trace species whose sources are in the troposphere.

Holton, J. R.↗

NASA NTRS1993

Strontium and oxygen isotope study of M-1, M-3 and M-4 drill core samples from the Manson impact structure, Iowa: Comparison with Haitian K-T impact glasses

Strontium and oxygen isotope analyses were performed on 8 samples from the M-1, M-3, and M-4 cores recently drilled at the Manson impact structure. The samples were three elastic sedimentary rocks (of probable Cretaceous age) which occurred as clasts within the sedimentary clast breccia, two samples of crystalline rock breccia matrix, and three samples of dolomite and limestone. The Sr-87/Sr-86 (corrected to 65 Ma) ratios were much higher than those in impact glasses from the Haitian Cretaceous-Tertiary (K-T) boundary. Isotope mixing calculations demonstrate that neither the silicate or carbonate rocks analyzed from the Manson crater, or mixtures of these rocks are appropriate source materials for the Haitian impact glasses. However, the Sr-87/Sr-86 (65Ma) ratio and delta O-18 value of the Ca-rich Haitian glasses are well reproduced by mixtures of Si-rich Haitian glass with platform carbonate of K-T age.

Blum, Joel D.↗

NASA NTRS2001

Traveling Magnetic Field Applications for Materials Processing in Space

Including the capability to induce a controlled fluid flow in the melt can significantly enrich research on solidification phenomena in a microgravity environment. The traveling magnetic field (TMF) is a promising technique to achieve this goal and is the aim of our ground-based project. In this presentation we will discuss new theoretical as well as experimental results recently obtained by our group. In particular, we experimentally demonstrated efficient mixing of metal alloys in long tubes subjected to TMF during processing. Application of this technique can be an elegant solution to ensure melt homogenization prior to solidification in a microgravity environment where natural convection is generally absent. Results of our theoretical work on TMF induced flows, such as convection control in Bridgman as well as in the Traveling Heater method, will be presented. Possible applications of TMF on board the ISS will also be discussed.

Motakef, S.↗

NASA NTRS2001

Traveling Magnetic Field Applications for Materials Processing in Space

Including the capability to induce a controlled fluid flow in the melt can significantly enrich research on solidification phenomena in a microgravity environment. The traveling magnetic field (TMF) is a promising technique to achieve this goal and is the aim of our ground-based project. In this presentation we will discuss new theoretical as well as experimental results recently obtained by our group. In particular, we experimentally demonstrated efficient mixing of metal alloys in long tubes subjected to TMF during processing. Application of this technique can provide an elegant solution to ensure melt homogenization prior to solidification in a microgravity environment where natural convection is generally absent. Results of our experimental work of applying the TMF technique to alloy melts will be presented. Possible applications of TMF on board the International Space Station will also be discussed.

Grugel, R. N.↗

NASA NTRS2004

Measurements of Infrared and Acoustic Source Distributions in Jet Plumes

The aim of this investigation was to use the linear phased array (LPA) microphones and infrared (IR) imaging to study the effects of advanced nozzle-mixing techniques on jet noise reduction. Several full-scale engine nozzles were tested at varying power cycles with the linear phased array setup parallel to the jet axis. The array consisted of 16 sparsely distributed microphones. The phased array microphone measurements were taken at a distance of 51.0 ft (15.5 m) from the jet axis, and the results were used to obtain relative overall sound pressure levels from one nozzle design to the other. The IR imaging system was used to acquire real-time dynamic thermal patterns of the exhaust jet from the nozzles tested. The IR camera measured the IR radiation from the nozzle exit to a distance of six fan diameters (X/D(sub FAN) = 6), along the jet plume axis. The images confirmed the expected jet plume mixing intensity, and the phased array results showed the differences in sound pressure level with respect to nozzle configurations. The results show the effects of changes in configurations to the exit nozzles on both the flows mixing patterns and radiant energy dissipation patterns. By comparing the results from these two measurements, a relationship between noise reduction and core/bypass flow mixing is demonstrated.

Agboola, Femi A.↗

NASA NTRS2007

Spacecraft Fire Detection: Smoke Properties and Transport in Low-Gravity

Results from a recent smoke particle size measurement experiment conducted on the International Space Station (ISS) are presented along with the results from a model of the transport of smoke in the ISS. The experimental results show that, for the materials tested, a substantial portion of the smoke particles are below 500 nm in diameter. The smoke transport model demonstrated that mixing dominates the smoke transport and that consequently detection times are longer than in normal gravity.

Urban, David L.↗

DOE OSTI2021

Storage Requirements for Grid Integration of Marine Renewable Energy - a Parametric Study

Marine resources such as waves and tides house immense potential to serve as energy-rich sources of renewable power generation. They are known to be highly available,persistent and predictable in nature. Therefore, these can serve as one of the critical components for a primarily renewable energy-driven, resilient and robust future power grid. Although some inherent temporal characteristics of these resources lend themselves favorably to potential grid applications, the inclusion of storage allows the benefits and value streams to become realized more fully. In this paper, we present a framework for assessing impact of marine energy resources inclusion on the overall load generation balance and its impact on the relevant storage requirements to obtain the desired level of renewable energy penetration. From this study, we can critically infer two main points - (a) the relative storage requirements for grid operations with and without marine energy, and (b) the avoided cost of storage by including marine energy into the generation mix. We demonstrate our framework for two different locations across the United States.

Hanif, Sarmad↗

DOE OSTI2020

Concentration and Recovery of Rare Earth Elements from Eastern US Coal Refuse

Recent studies funded by the US Department of energy have shown that coal and coal byproducts contain elevated contents of Rare Earth Elements (REEs), making them a potential resource for these critical materials. The approach employed in this research focused on the concentration and extraction of REEs from fine coal refuse derived from various preparation plants in the Appalachian coal basin of the United States. Initial efforts in this research focused on the identification and characterization of REEs in various fine coal refuse streams from nine distinct industrial preparation plants in Appalachia. The average REE content in these materials was determined to be approximately 200 ppm, but the REE content showed a strong correlation to the aluminum content, suggesting that the REEs are closely associated with the clay minerals present in the refuse. Given the relatively low REE concentrations, initial efforts sought to concentrate the REEs through decarbonization and dispersive liberation steps. In these tests, high-shear agitation in the presence of a polyelectrolyte, followed by sedimentation was able to isolate the REE-enriched fine clay particles from siliceous gangue minerals. Following the dispersive liberation step, all samples were found to have an REE content greater than 300 ppm, a benchmark used for many initial exploratory studies. In one case, the REE content was increased by more than 125%. Subsequent extraction tests initially utilized a direct ion-exchange leaching approach with ammonium sulfate as lixiviant. In all cases, the simple ion-exchange leaching process failed to recover significant quantities of rare earth elements, ultimately suggesting that the REEs in fine coal waste may be passivated or bound in a colloidal phase. To access this colloidal phase, several alternative approaches were evaluated, including leaching with alternative ion-exchange lixiviants, reductive leaching, gas-purged leaching, and others. The approach that showed the most promise was strong alkaline pretreatment, followed by ion-exchange leaching with ammonium sulfate at pH 4. A combination of strong alkali and high-temperatures treatment successfully liberated the REEs, converting them to a form amenable to ion-exchange leaching. The highest REE recovery achieved with this method was determined to be 39%. Lastly, bench-scale solvent extraction tests were used to further concentrate REEs in the leach solution and demonstrate that mixed rare earth concentrates can be successfully produced from fine coal refuse.

01 COAL, LIGNITE, AND PEAT↗

NASA NTRS1997

Structure of the Compressible Reacting Mixing Layer: A Linear Stability Analysis

Previous investigations have demonstrated that a mixing layer in compressible reacting conditions can develop two instability modes in addition to the more common central mode, which exists unaccompanied in incompressible non-reacting flows. These 'outer' modes were shown in the investigations of Planche and Reynolds to have a detrimental effect on mixing and combustion efficiency and therefore their presence has important consequences for applications of supersonic combustion. Results from a parametric study of the compressible reacting mixing layer's regime space using a linear stability technique will be discussed. The purpose is to develop a more complete understanding behind the effects of compressibility, heat release and the density, equivalence and velocity ratios on the amplification rate and structure of each instability mode.

Day, M. J.↗