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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3

Correlated Signal Analysis for Nuclear Emergency Response

In the context of nuclear emergency response (NER) scenarios, the critical task is to quickly identify a "black box" as a potential threat, as failing to do so could have catastrophic consequences. Techniques for passive assay of a “black box” typically include gamma-ray spectroscopy and neutron coincidence/multiplicity counting. However, there are significant challenges associated with these type of measurements. First, the presence of intervening materials can obstruct the detection of relevant signatures. Second, the presence of strong non-fission neutron sources, like (α, n) emitters, can add uncertainties to the neutron multiplicity analysis. In our LDRD-MFR Phase II work, a portable neutron spectrometer, called the Compact Fast Neutron Spectrometer (CFNS), was developed for NER applications. The CFNS system leverages information-rich neutron energy spectra to derive actionable information. This work investigates the use of correlated signals in the CFNS from special nuclear material (SNM) to characterize physical properties, such as intervening shielding material and fission to non-fission neutron contributions. In this report, the Phase II results from bulk SNM measurements at the National Criticality Experiments Research Center (NCERC) are briefly discussed along with the motivation for this work. Afterwards, simulations using the MCNPX-PoliMi transport code are discussed, which were used to expand our correlated signal study. Signal triggered analysis for neutron multiplicity extraction will also be discussed. Lastly, the use neutron-photon correlations for intervening material identification are shown, along with the use of correlated neutron energy spectra for α-ratio extraction.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

ECAR: Baseline Characterization Database Verification Report – PCEA Billet 01D3-35

The purpose of this engineering calculations and analysis report (ECAR) is to present data collected in the Baseline Graphite Characterization Program, which is directly tasked with supporting the Idaho National Laboratory’s (INL’s) research and development efforts on the Advanced Reactor Technologies (ART) Program. This program populates a comprehensive database that reflects the baseline properties of nuclear-grade graphite with regard to individual grade, billet, and position within individual billets. The physical- and mechanical-property information collected will be transferred to the Nuclear Data Management and Analysis System (NDMAS), and that database will help populate the handbook of property data available to member nations of the Generation-IV International Forum. Transfer of these data from the applicable technical lead to the dissemination databases available to other end users requires a full review of the test procedures and data-collection efforts through an analysis of the multiple summary spreadsheets and values being collected. This report represents the analysis for PCEA Billet 01D3-35 and facilitates release of associated data to the NDMAS custodians.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Smaller and faster: a review of conventional and nanocalorimetry techniques for determining thermophysical properties of nuclear materials

Thermal analysis of nuclear materials is critical for the advancement of nuclear technology. The heat effects associated with heat capacity, phase transformation, and radiation damage can be measured with conventional calorimeters. However, conventional calorimetric techniques are often restricted in terms of heating rate and sample mass, especially when studying the limited amounts of materials subject to extreme conditions. In this review, we summarize conventional calorimetric studies of critical thermophysical and thermochemical properties of pure actinide metals (U, Np, Am, Pu), fast reactor metallic fuel alloy systems (U–Zr, U–Pu–Zr, Pu–U, Pu–Zr), and actinide oxides that are primary constituents or transmutation products in light water reactor fuel rods (U–O, Np–O, Am–O, Pu–O, Pu–U–O). Adiabatic and drop calorimetry have been the primary techniques used for these studies, however the development of fast scanning calorimetry using micro-electro-mechanical-based systems allows determination of thermodynamic properties from smaller sample masses. We report recent investigations that leverage the fast heating rates of nanocalorimetry by itself or combined with other characterization techniques. Furthermore, we then discuss opportunities for nanocalorimetry to provide solutions to some of the technical challenges inherent in thermal analysis of nuclear materials, namely a reduction in sample activity, emulating heating transients, investigation of phase evolution in irradiated samples, and characterization of radiation damage evolution. Nanocalorimetry has the potential to significantly advance the understanding of thermophysical properties in nuclear materials and thus accelerate the development of nuclear technology.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Characterization of Urbix Resources Natural Flake Graphite Material for Nuclear Applications (CRADA NFE-18-07340 Final Report)

Urbix Resources is a company specializing in graphite powder processing and purification. Urbix is looking to become the first domestic supplier of nuclear-grade graphite in the United States. This has led to a Cooperative Research and Development Agreement (CRADA) being established between the Oak Ridge National Laboratory (ORNL) and Urbix Resources, with the goal of characterizing a purified graphite feedstock supplied by Urbix Resources. The resulting data will then be used to determine the viability of a large-scale nuclear graphite production and qualification campaign. These characterization methods have been performed on the as-received graphite feedstock, a heat-treated batch of the feedstock, a milled batch of the feedstock, and a nuclear-grade graphite powder historically used in fuel production. The data from the heat-treated and milled feedstock will determine how different processing methods affect the powder’s physical properties, whereas the data from the nuclear grade graphite will provide information about the characteristics of a graphite previously accepted for nuclear applications. All of these powders have been characterized individually and as part of a resin-graphite blend (herein referred to as matrix) that has been used in past fuel experiments. The results of these experiments show that the Urbix powder and nuclear-grade graphite powder display notably different properties from one another in many cases, but this discrepancy may have been the result of the typical particle size of each powder. This hypothesis is supported by tests conducted on the milled powder, which showed a closer resemblance in properties to the nuclear-grade graphite than the as-received powder. The method for pressing the graphite matrix also had a noticeable effect on the measured properties.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Nuclear-matter saturation and symmetry energy within Δ -full chiral effective field theory

Nuclear saturation and the symmetry energy are key properties of low-energy nuclear physics that depend on fine details of the nuclear interaction. The equation of state around saturation is also an important anchor for extrapolations to higher densities and studies of neutron stars. Here we develop a unified statistical framework that uses realistic nuclear forces to link the theoretical modeling of finite nuclei and infinite nuclear matter. We construct fast and accurate emulators for nuclear-matter observables and employ an iterative history-matching approach to explore and reduce the enormous parameter domain of Δ -full chiral interactions. We perform rigorous uncertainty quantification and find that model calibration including O 16 observables gives saturation predictions that are more precise than those that only use few-body data. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Design and Technical Study of Neutrino Detector Spacecraft

A neutrino detector is proposed to be developed for use on a space probe in close orbit of the Sun. The detector will also be protected from radiation by a tungsten shield Sun shade, active veto array and passive cosmic shielding. With the intensity of solar neutrinos substantially greater in a close solar orbit than on the Earth only a small 250 kg detector is needed. It is expected that this detector and space probe studying the core of the Sun, its nuclear furnace and particle physics basic properties will bring new knowledge beyond what is currently possible for Earth bound solar neutrino detectors.

Design and Technical Study↗

Baseline Characterization Database Verification Report - PCEA Billet 01S8-9

The purpose of this engineering calculations and analysis report (ECAR) is to present data collected in the Baseline Graphite Characterization Program, which is directly tasked with supporting the Idaho National Laboratory's (INL's) research and development efforts on the Advanced Reactor Technologies (ART) Program. This program populates a comprehensive database that reflects the baseline properties of nuclear-grade graphite with regard to individual grade, billet, and position within individual billets. The physical- and mechanical-property information being collected will be transferred to the Nuclear Data Management and Analysis System (NDMAS), and that database will help populate the handbook of property data available to member nations of the Generation-IV International Forum. Transfer of these data from the applicable technical lead to the dissemination databases available to other end users requires a full review of the test procedures and data-collection efforts through an analysis of the multiple summary spreadsheets and values being collected. This report represents the analysis for PCEA Billet 01S8-9 and facilitates release of associated data to the NDMAS custodians.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

The conductive propagation of nuclear flames. I - Degenerate C + O and O + Ne + Mg white dwarfs

The paper determines the physical properties - speed, width, and density structure - of conductive burning fronts in degenerate carbon-oxygen (C + O) and oxygen-neon-magnesium (O + Ne + Mg) compositions for a grid of initial densities and compositions. The dependence of the physical properties of the flame on the assumed values of nuclear reaction rates, the nuclear reaction network employed, the thermal conductivity, and the choice of coordinate system are investigated. The occurrence of accretion-induced collapse of a white dwarf is found to be critically dependent on the velocity of the nuclear conductive burning front and the growth rate of hydrodynamic instabilities. Treating the expanding area of the turbulent burning region as a fractal whose tile size is identical to the minimum unstable Rayleigh-Taylor wavelength, it is found, for all reasonable values of the fractal dimension, that for initial C + O or O + Ne + Mg densities above about 9 x 10 exp 9 g/cu cm the white dwarf should collapse to a neutron star.

Timmes, F. X.↗

Dense Nuclear Matter Equation of State from Heavy-Ion Collisions

The nuclear equation of state (EOS) is at the center of numerous theoretical and experimental efforts in nuclear physics, motivated by its crucial role in our understanding of the properties of nuclear matter found on Earth, in neutron stars, and in neutron-star mergers. With advances in microscopic theories for nuclear interactions, the availability of experiments probing nuclear matter under conditions not reached before, and the advent of multi-messenger astronomy, the next decade will bring new opportunities for determining the nuclear matter EOS.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Emulating ab initio computations of infinite nucleonic matter

We construct efficient emulators for the computation of the infinite nuclear matter equation of state. These emulators are based on the subspace-projected coupled-cluster method for which we here develop a new algorithm called small-batch voting to eliminate spurious states that might appear when emulating quantum many-body methods based on a non-Hermitian Hamiltonian. The efficiency and accuracy of these emulators facilitate a rigorous statistical analysis within which we explore nuclear matter predictions for > 10 6 different parametrizations of a chiral interaction model with explicit Δ -isobars at next-to-next-to leading order. Constrained by nucleon-nucleon scattering phase shifts and bound-state observables of light nuclei up to He 4 , we use history matching to identify nonimplausible domains for the low-energy coupling constants of the chiral interaction. Within these domains we perform a Bayesian analysis using sampling and importance resampling with different likelihood calibrations and study correlations between interaction parameters, calibration observables in light nuclei, and nuclear matter saturation properties. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A probabilistic inverse prediction method for predicting plutonium processing conditions

In the past decade, nuclear chemists and physicists have been conducting studies to investigate the signatures associated with the production of special nuclear material (SNM). In particular, these studies aim to determine how various processing parameters impact the physical, chemical, and morphological properties of the resulting special nuclear material. By better understanding how these properties relate to the processing parameters, scientists can better contribute to nuclear forensics investigations by quantifying their results and ultimately shortening the forensic timeline. This paper aims to statistically analyze and quantify the relationships that exist between the processing conditions used in these experiments and the various properties of the nuclear end-product by invoking inverse methods. In particular, these methods make use of Bayesian Adaptive Spline Surface models in conjunction with Bayesian model calibration techniques to probabilistically determine processing conditions as an inverse function of morphological characteristics. Not only does the model presented in this paper allow for providing point estimates of a sample of special nuclear material, but it also incorporates uncertainty into these predictions. This model proves sufficient for predicting processing conditions within a standard deviation of the observed processing conditions, on average, provides a solid foundation for future work in predicting processing conditions of particles of special nuclear material using only their observed morphological characteristics, and is generalizable to the field of chemometrics for applicability across different materials.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Gamma Irradiation Facility

Gamma irradiation is a process that uses Cobalt60 radionuclide produced artificially in nuclear reactors to irradiate a variety of items using gamma radiation. A key characteristic of gamma irradiation is its high penetration capability and the fact that it can modify physical, chemical, and biological properties of the irradiated materials.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Actinide Radiation Chemistry and Used Nuclear Fuel Reprocessing

Although the actinides boast many unique physical and chemical properties, their inherent susceptibility to radioactive decay—and subsequent consequences of radiation-induced chemistry—are what make them truly interesting and challenging elements to understand. From a closed nuclear fuel cycle perspective, the ability to predict and control the effects of actinide-driven radiolysis is critical for the design, development, and deployment of advanced used nuclear fuel reprocessing strategies and technologies. The absorption of ionizing radiation from actinide decay leads to the formation of a variety of transient and steady-state radicals, ions, and molecular radiolysis products that can lead to significant changes in a reprocessing solvent system’s physical and chemical properties, which ultimately limits that process’ efficiency and longevity. Presented here is an overview of recent advances in actinide radiation chemistry as it applied to used nuclear fuel reprocessing.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

SNEWPY: A Data Pipeline from Supernova Simulations to Neutrino Signals

Current neutrino detectors will observe hundreds to thousands of neutrinos from a Galactic supernovae, and future detectors will increase this yield by an order of magnitude or more. With such a data set comes the potential for a huge increase in our understanding of the explosions of massive stars, nuclear physics under extreme conditions, and the properties of the neutrino. However, there is currently a large gap between supernova simulations and the corresponding signals in neutrino detectors, which will make any comparison between theory and observation very difficult. SNEWPY is an open-source software package which bridges this gap. The SNEWPY code can interface with supernova simulation data to generate from the model either a time series of neutrino spectral fluences at Earth, or the total time-integrated spectral fluence. Data from several hundred simulations of core-collapse, thermonuclear, and pair-instability supernovae is included in the package. This output may then be used by an event generator such as sntools or an event rate calculator such as SNOwGLoBES. Additional routines in the SNEWPY package automate the processing of the generated data through the SNOwGLoBES software and collate its output into the observable channels of each detector. In this paper we describe the contents of the package, the physics behind SNEWPY, the organization of the code, and provide examples of how to make use of its capabilities.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

High-resolution laser system for the S 3 -Low Energy Branch

Here, in this paper we present the first high-resolution laser spectroscopy results obtained at the GISELE laser laboratory of the GANIL-SPIRAL2 facility, in preparation for the first experiments with the S 3 -Low Energy Branch. Studies of neutron-deficient radioactive isotopes of erbium and tin represent the first physics cases to be studied at S 3 . The measured isotope-shift and hyperfine structure data are presented for stable isotopes of these elements. The erbium isotopes were studied using the 4f 12 6s 2 3 H 6 → 4f 12 ( 3 H)6s6p J = 5 atomic transition (415 nm) and the tin isotopes were studied by the 5s 2 5p 2 ( 3 P 0 ) → 5s 2 5p6s( 3 P 1 ) atomic transition (286.4 nm), and are used as a benchmark of the laser setup. Additionally, the tin isotopes were studied by the 5s 2 5p6s( 3 P 1 ) → 5s 2 5p6p( 3 P 2 ) atomic transition (811.6 nm), for which new isotope-shift data was obtained and the corresponding field-shift F 812 and mass-shift M 812 factors are presented.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Exploring the Strong Interaction of Three-Body Systems at the LHC

Deuterons are atomic nuclei composed of a neutron and a proton held together by the strong interaction. Unbound ensembles composed of a deuteron and a third nucleon have been investigated in the past using scattering experiments, and they constitute a fundamental reference in nuclear physics to constrain nuclear interactions and the properties of nuclei. In this work, K + -d and p-d femtoscopic correlations measured by the ALICE Collaboration in proton-proton (pp) collisions at $\sqrt{s}$ = 13 TeV at the Large Hadron Collider (LHC) are presented. It is demonstrated that correlations in momentum space between deuterons and kaons or protons allow us to study three-hadron systems at distances comparable with the proton radius. The analysis of the K + -d correlation shows that the relative distances at which deuterons and protons or kaons are produced are around 2 fm. The analysis of the p-d correlation shows that only a full three-body calculation that accounts for the internal structure of the deuteron can explain the data. In particular, the sensitivity of the observable to the short-range part of the interaction is demonstrated. These results indicate that correlations involving light nuclei in pp collisions at the LHC will also provide access to any three-body system in the strange and charm sectors.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Probing transverse momentum dependent structures with azimuthal dependence of energy correlators

We study the azimuthal angle dependence of the energy-energy correlators $\langle \mathcal{E}\left({\widehat{n}}_{1}\right)\mathcal{E}\left({\widehat{n}}_{2}\right)\rangle $ in the back-to-back region for e + e - annihilation and deep inelastic scattering (DIS) processes with general polarization of the proton beam. We demonstrate that the polarization information of the beam and the underlying partons from the hard scattering is propagated into the azimuthal angle dependence of the energy-energy correlators. In the process, we define the Collins-type EEC jet functions and introduce a new EEC observable using the lab-frame angles in the DIS process. Furthermore, we extend our formalism to explore the two-point energy correlation between hadrons with different quantum numbers ${\mathbb{S}}_{i}$ in the back-to-back limit $\langle {\mathcal{E}}_{{\mathbb{S}}_{1}}\left({\widehat{n}}_{1}\right){\mathcal{E}}_{{\mathbb{S}}_{2}}\left({\widehat{n}}_{2}\right)\rangle $. We find that in the Operator Product Expansion (OPE) region the nonperturbative information is entirely encapsulated by a single number. Using our formalism, we present several phenomenological studies that showcase how energy correlators can be used to probe transverse momentum dependent structures.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Temperature-Dependent Speciation of Ni(II) in Molten Chloride, Bromide, and Iodide Salts

Understanding the fundamental speciation and local structure of metal cations─such as nickel, which is present as a corrosion product─in molten salt media is essential for assessing their impact on the thermal and physical properties of salts used for advanced nuclear energy applications. In this study, we employed an integrated approach of combining X-ray absorption spectroscopy (XAS), UV–vis spectroscopy, and ab initio molecular dynamics (AIMD) to investigate the halide-dependent speciation of divalent nickel ions, Ni(II), in LiCl–KCl, LiBr–KBr, and LiI–KI eutectic salt mixtures from room temperature to 600 °C. Our findings show that both halide type and temperature significantly influence the local coordination of nickel in these molten salt systems. A notable aspect of Ni(II) speciation in LiI–KI salts is the formation of a polyiodide species. In conclusion, our findings provide critical insights into metal ion speciation in molten salt systems, enhancing our understanding of the factors that govern the physicochemical properties of these complex fluids.

36 MATERIALS SCIENCE↗