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DOE OSTI2025

Modelling Thomson Scattering in a Hydrogen Plasma at Stellar Interior Conditions Using the Hypernetted‐Chain Approach

Under the extreme conditions found in small stars, where electron degeneracy and Coulomb coupling are significant, accurate modeling of Thomson scattering is crucial for determining opacity, a primary quantity for stellar energy transport. We use hypernetted-chain calculations, incorporating quantum pseudopotentials and electron-exchange effects to obtain the electron–electron static structure factor to calculate the Thomson scattering transport cross-section for conditions prevailing in the interior of small stars. These results are compared to those from average-atom simulations and analytical calculations. Our findings support laboratory astrophysics experiments aimed at benchmarking opacity models for stellar interiors, particularly for red dwarf stars, and help to bridge theoretical models with observations.

ICF↗

DOE OSTI2022

Characterization of a 1D-imaging high-energy x-ray backlighter driven by the National Ignition Facility Advanced Radiographic Capability laser

Plastic deformation of samples compressed to Mbar pressures at high strain rates at the National Ignition Facility (NIF) forms the basis of ongoing material strength experiments in conditions relevant to meteor impacts, geophysics, armor development, and inertial confinement fusion. Hard x-ray radiography is the primary means of measuring the evolution of these samples, typically employing a slit-collimated high-Z microdot driven by the NIF laser to generate >40 keV x rays [E. Gumbrell et al., Rev. Sci. Instrum. 89, 10G118 (2018) and C. M. Huntington et al., Rev. Sci. Instrum. 89, 10G121 (2018)]. Alternatively, a dysprosium “micro-flag” target driven by the Advanced Radiographic Capability laser (~2 kJ, 10 ps) can deliver significantly higher spatiotemporal resolution [M. P. Hill et al., Rev. Sci. Instrum. 92, 033535 (2021)], especially in high-opacity samples. Here, initial experiments revealed problematic brightness and spectral gradients from this source, but by radiographing a set of diamond-turned, 105 µm-thick Pb test objects and supported by simulations using the 3D Monte Carlo code GEANT4, these geometry-dependent gradients across the field of view are quantified and mitigation strategies are assessed. In addition to significantly enhancing the modulation transfer function compared to the existing system, image stacking from multiple layers of image plate is shown to almost double the signal to noise ratio that will reduce uncertainties in future dynamic strength experiments.

47 OTHER INSTRUMENTATION↗

DOE OSTI2025

Solar fusion III: New data and theory for hydrogen-burning stars

In stars that lie on the main sequence in the Hertzsprung-Russell diagram, like our Sun, hydrogen is fused to helium in a number of nuclear reaction chains and series, such as the proton-proton chain and the carbon-nitrogen-oxygen cycles. Precisely determined thermonuclear rates of these reactions lie at the foundation of the standard solar model. This review, the third decadal evaluation of the nuclear physics of hydrogen-burning stars, is motivated by the great advances made in recent years by solar neutrino observatories, putting experimental knowledge of the proton-proton (𝑝⁢𝑝)-chain neutrino fluxes in the few-percent precision range. The basis of the review is a one-week community meeting held in July 2022 in Berkeley, California, and many subsequent digital meetings and exchanges. The relevant reactions of solar and stellar hydrogen burning are reviewed here from both theoretical and experimental perspectives. Recommendations for the state of the art of the astrophysical 𝑆 factor and its uncertainty are formulated for each of them. Furthermore, several other topics of paramount importance for the solar model are reviewed as well: recent and future neutrino experiments, electron screening, radiative opacities, and current and upcoming experimental facilities. In addition to reaction-specific recommendations, general recommendations are also formed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2021

Time-dependent density functional theory applied to average atom opacity

We focus on studying the opacity of iron, chromium, and nickel plasmas at conditions relevant to experiments carried out at Sandia National Laboratories. In this work, we calculate the photoabsorption cross sections and subsequent opacity for plasmas using linear-response time-dependent density functional theory (TD-DFT). Our results indicate that the physics of channel mixing accounted for in linear-response TD-DFT leads to an increase in the opacity in the bound-free quasicontinuum, where the Sandia experiments indicate that models underpredict iron opacity. However, the increase seen in our calculations is only in the range of 5%–10%. Further, we do not see any change in this trend for chromium and nickel. This behavior indicates that channel mixing effects do not explain the trends in opacity observed in the Sandia experiments.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2018

Iron X-ray Transmission at Temperature Near 150 eV Using the National Ignition Facility: First Measurements and Paths to Uncertainty Reduction

Discrepancies exist between theoretical and experimental opacity data for iron, at temperatures 180–195 eV and electron densities near 3 × 1022/cm3, relevant to the solar radiative-convective boundary. Another discrepancy, between theory and helioseismic measurements of the boundary’s location, would be ameliorated if the experimental opacity is correct. To address these issues, this paper details the first results from new experiments under development at the National Ignition Facility (NIF), using a different method to replicate the prior experimental conditions. In the NIF experiments, 64 laser beams indirectly heat a plastic-tamped rectangular iron-magnesium sample inside a gold cavity. Another 64 beams implode a spherical plastic shell to produce a continuum X-ray flash which backlights the hot sample. An X-ray spectrometer records the transmitted X-rays, the unattenuated X-rays passing around the sample, and the sample’s self-emission. From these data, X-ray transmission spectra are inferred, showing Mg K-shell and Fe L-shell X-ray transitions from plasma at a temperature of ~150 eV and electron density of ~8 × 1021/cm3. These conditions are similar to prior Z measurements which agree better with theory. The NIF transmission data show statistical uncertainties of 2–10%, but various systematic uncertainties must be addressed before pursuing quantitative comparisons. The paths to reduction of the largest uncertainties are discussed. Once the uncertainty is reduced, future NIF experiments will probe higher temperatures (170–200 eV) to address the ongoing disagreement between theory and Z data.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Jupiter Laser Facility Annual Report, FY 2025

Dear JLF community, I cannot believe I am now entering my third year as JLF director — time definitely flies when you are having fun! FY25 was another pivotal year for the Jupiter Laser Facility, marked by both scientific achievement and growing visibility for our community. Building on the successful reopening and refurbishment of the facility, we continued to demonstrate how JLF drives innovation in high energy density and fusion energy science, laser technology, and workforce development. Across Janus, Titan, and COMET, users executed a diverse portfolio of experiments, from dynamic compression and opacity measurements to laser plasma interactions, laboratory astrophysics, and advanced diagnostics. These efforts are highlighted in this report, including the development of new probes that capture the time evolution of plasmas on a single shot, and diagnostics and platforms that are already impacting experiments at NIF and other large facilities. JLF continues to serve as both a testbed for new ideas and a bridge to larger scale campaigns. FY25 also showcased the broader role of JLF within the Laboratory and the national HED science ecosystem. The NIF JLF User Groups Meeting in February brought nearly 180 participants to Livermore and highlighted the scientific progress made during JLF’s first full year of renewed operations. JLF research and users were recognized with Director’s Institutional Awards and Early and Mid Career awards, underscoring the quality and impact of the work performed here. Our team also contributed prominently to national conversations about laser safety, plasma physics, and inertial fusion energy through invited talks, conferences, and professional society leadership. JLF’s integration with LaserNetUS deepened this year as well. We launched a new technical exchange program across LaserNetUS facilities and kicked it off with a JLF team visit to the BELLA Center at Lawrence Berkeley National Laboratory. These exchanges are strengthening operations, sharing best practices, and improving the user experience across the network. Filming for the LaserNetUS “Behind the Scenes” series and participation in the annual LaserNetUS meeting further increased the visibility of our facility and our users. At the same time, JLF continues to play a central role in ambitious new programs, such as the Big Aperture Thulium laser effort funded through one of the DOE Office of Science Microelectronics Science Research Centers, which will use JLF infrastructure to explore next generation high rep rate lasers for EUV and x-ray source development. A core part of our mission remains training the next generation of scientists. In FY25, we welcomed another cohort of summer students, who joined experimental teams on Titan and presented their research at LLNL’s student poster symposium and national inertial fusion energy meetings. JLF users and early career scientists showcased their work at conferences across the country, highlighting experiments performed at the facility. These hands on experiences, and the mentoring provided by our staff and user teams, are central to JLF’s identity as a true user facility. Finally, FY25 reinforced JLF’s role as a focal point for partnerships and outreach. We hosted visits from international collaborators, science leaders, and we shared the story of the facility through venues such as the Big Ideas Lab podcast. These interactions help connect our work to a broader scientific and policy audience and open new pathways for collaboration. As we look ahead, the combination of refurbished hardware, new capabilities like STILETTO and enhanced short pulse performance on Titan, strong partnerships across LLNL and LaserNetUS, and a growing user community positions JLF for an even more ambitious program in the coming years. I am deeply grateful to our technical and operations staff for their dedication, to our LLNL partners for their continued support, and to our users for bringing bold, creative ideas to the facility. I look forward to more experiments, capabilities, partnerships, and groundbreaking science in the years to come! With brightest regards, Félicie Albert, JLF Director.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS2004

Chondrule Crystallization Experiments

Given the great diversity of chondrules, laboratory experiments are invaluable in yielding information on chondrule formation process(es) and for deciphering their initial conditions of formation together with their thermal history. In addition, they provide some critical parameters for astrophysical models of the solar system and of nebular disk evolution in particular (partial pressures, temperature, time, opacity, etc). Most of the experiments simulating chondrules have assumed formation from an aggregate of solid grains, with total pressure of no importance and with virtually no gain or loss of elements from or to the ambient environment. They used pressed pellets attached to wires and suffered from some losses of alkalis and Fe.

Hweins, R. H.↗

NASA NTRS1993

The role of atmospheric heat transport in the seasonal carbon dioxide cycle

We have carried out numerical experiments with a general circulations model (GCM) and energy balance model of the martian atmosphere to define the importance of heat transported to the polar regions in determining the amount of CO2 condensed on the surface during the fall and winter seasons and the amount sublimated during the spring and summer seasons. In so doing, we performed both sensitivity experiments, in which the dust opacity was varied over the full range of its observed values, and annual simulations, in which the dust opacity varied continuously with seasonal data, in accord with measurements taken at the Viking landers. Dust opacity represents the key variable for determining the contribution of atmospheric heat advection to the energy budget in the polar regions. The amount of heat advected to the winter polar regions increases monotonically as the dust opacity at low and middle latitudes increases. However, the increase is sharpest between optical depths of 0 and 1 tends to level off at still higher optical depths. Heat advection is more important at times of CO2 condensation than CO2 sublimation, since the temperature gradients are much steeper in the winter hemisphere than in the summer hemisphere. Because dust opacity is much higher during northern winter than during southern winter, atmospheric heat advection reduces the amount of CO2 that condenses in the north by a much larger factor than it does in the south.

Pollack, James B.↗

DOE OSTI2023

Radiation burnthrough measurements to infer opacity at conditions close to the solar radiative zone–convective zone boundary

Recent measurements at the Sandia National Laboratory of the x-ray transmission of iron plasma have inferred opacities much higher than predicted by theory, which casts doubt on modeling of iron x-ray radiative opacity at conditions close to the solar convective zone-radiative zone boundary. An increased radiative opacity of the solar mixture, in particular iron, is a possible explanation for the disagreement in the position of the solar convection zone-radiative zone boundary as measured by helioseismology and predicted by modeling using the most recent photosphere analysis of the elemental composition. In this report we present data from radiation burnthrough experiments, which do not support a large increase in the opacity of iron at conditions close to the base of the solar convection zone and provide a constraint on the possible values of both the mean opacity and the opacity in the x-ray range of the Sandia experiments. The data agree with opacity values from current state-of-the-art opacity modeling using the CASSANDRA opacity code.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Deep learning for NLTE spectral opacities

Computer simulations of high energy density science experiments are computationally challenging, consisting of multiple physics calculations including radiation transport, hydrodynamics, atomic physics, nuclear reactions, laser–plasma interactions, and more. To simulate inertial confinement fusion (ICF) experiments at high fidelity, each of these physics calculations should be as detailed as possible. However, this quickly becomes too computationally expensive even for modern supercomputers, and thus many simplifying assumptions are made to reduce the required computational time. Much of the research has focused on acceleration techniques for the various packages in multiphysics codes. In this work, we explore a novel method for accelerating physics packages via machine learning. The non-local thermodynamic equilibrium (NLTE) package is one of the most expensive calculations in the simulations of indirect drive inertial confinement fusion, taking several tens of percent of the total wall clock time. We explore the use of machine learning to accelerate this package, by essentially replacing the physics calculation with a deep neural network that has been trained to emulate the physics code. Overall, we demonstrate the feasibility of this approach on a simple problem and perform a side-by-side comparison of the physics calculation and the neural network inline in an ICF Hohlraum simulation. We show that the neural network achieves a 10× speed up in NLTE computational time while achieving good agreement with the physics code for several quantities of interest.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2022

Development of an Enhanced Radiation Physics Toolset for Modeling Spectral and Imaging Signatures in the Warm Dense Matter Experiments

Radiative and atomic processes in plasmas play a critical role in a wide variety of high energy density laboratory plasma (HEDLP) experiments. The emission, absorption, and transport of radiation can strongly affect the overall energetics and evolution of such plasmas. In addition, radiation-based diagnostics – including imaging, spectroscopy, and absolute flux measurements – are widely used to determine key features of HEDLPs. To advance our understanding of HEDLP science, it is vital to have high-fidelity computational physics tools that have well-tested radiation physics modeling, and that are readily accessible to researchers in the HEDLP community. Simulations play an extremely important role for planning and designing the experiments, as well as for post-experiment data analysis. Prism Computational Sciences develops software that is used by National Laboratories and universities (including five members of LaserNetUS network). Prominent examples of such research efforts include z-pinch and short-pulse laser experiments designed to study the basic physics of photoionized plasmas and photoionization fronts, as well as their application to astrophysical plasmas. The main effort was dedicated to the development of non-equilibrium equation-of-state (EOS) models within the HELIOS-CR code, a hydrodynamics code with inline collisional-radiative atomic kinetics. Gas cell experiments on Z and Omega demonstrated the importance of non-equilibrium effects on atomic kinetics in photoionized plasmas. Recent proof-of-principle experiments on Omega EP confirmed the advantages of using a short-pulse laser to create an intense radiation drive, leading to additional experiments being proposed. Photoionization front experiments at LLE also emphasizes the importance of radiation and atomic physics. In both studies, HELIOS-CR simulations played a crucial role in computing non-equilibrium opacities and ionization distributions. A newly developed non-LTE EOS model will help addressing possible non-equilibrium effects, on for example specific heat, and their influence in plasma evolution. Prism also implemented support for open-source atomic data generated by the Flexible Atomic Code. This allows researchers to generate custom atomic tables and use them within the complex framework of simulation tools developed by Prism. The ability to use open-source atomic data would be extremely valuable for hydrodynamics and spectroscopic simulations that include high-Z materials, e.g., picosecond x-ray pulse generation experiments. Support for new atomic structures was fully implemented, and the data can be used by all simulation tools developed at Prism: radiation-hydrodynamics, imaging and spectroscopy, EOS and opacity. The development resulted in a significant fidelity enhancement to the simulations tools developed by Prism that are currently used in other cutting-edge experiments including: opacity measurement experiments performed to both understand the basic radiative and atomic properties of plasmas as well as provide data for more accurately modeling the internal structure of the Sun and other stars, high-intensity short-pulse laser experiments performed to develop short-wavelength light sources for use as backlighters and to investigate fast ignition concepts for inertial fusion energy; capsule implosion experiments designed to develop inertial fusion as an energy source, etc.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Measurement of mix at the fuel–ablator interface in indirectly driven capsule implosions on the National Ignition Facility

The interface between the capsule ablator and fuel ice layer is susceptible to hydrodynamic instabilities. The subsequent mixing of hot ablator material into the ice reduces fuel compression at stagnation and is a candidate for reduced capsule performance. The ability to diagnose ice–ablator mix is critical to understanding and improving stability at this interface. Combining the crystal backlighter imager with the single line of sight camera on the National Ignition Facility (NIF) allows direct measurement of ice–ablator mix by providing multiple quasi-monochromatic radiographs of layered capsule implosions per experiment with high spatial (∼12 μm) and temporal (∼35 ps) resolution. The narrow bandwidth of this diagnostic platform allows radiography of the inner edge of the capsule limb close to stagnation without capsule self-emission contaminating the data and removes opacity uncertainties typically associated with the spectral content of the radiograph. Analysis of radiographic data via a parameterized forward-fitting Abel inversion technique provides measurements of the distribution of mix mass inwards from the ice–ablator interface. The sensitivity of this mix measurement technique was demonstrated by applying it to layered experiments in which the stability of the ice–ablator interface was expected to vary significantly. Additional experiments suggest that high-density carbon capsules that employ a buried-layer dopant profile suffer from mixing at the innermost doped–undoped interface. Data from these experiments suggest that opacity models used in hydrodynamic simulations of NIF experiments can potentially over-predict the opacity of doped capsules. LLNL-JRNL-850535-DRAFT.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

NASA NTRS1996

Development of a solar-cell dust opacity measurement instrument for Mars Pathfinder

The atmosphere of Mars has a considerable load of suspended dust. Over time, this dust is deposited out of the atmosphere. The mechanism and the temporal and geographical variation of this deposition are not well characterized. Measurements of settling rates and dust properties are of considerable scientific interest. Atmospheric dust affects the atmospheric solar absorption and thus the heat balance of Mars, as well as serving as nucleation sites for water and CO2 frost. Knowledge of dust properties is of critical interest to design and prediction of the lifetime and power output of solar arrays, and also to design of mechanical mechanisms and radiators. An instrument has been designed and fabricated to measure the dust accumulation during the course of the Mars Pathfinder rover mission. The solar-cell coverglass transmission experiment will measure the change in optical opacity of a transparent coverglass as dust settles on the surface, and a quartz crystal monitor will measure the mass deposited.

Geoffrey A. Landis↗

DOE OSTI2020

Progress toward NIF opacity measurements

The opacities of iron and other mid-Z elements help to regulate the transport of energy in the sun. Recent experiments on the Sandia National Laboratories Z machine have shown large discrepancies between the measured and calculated opacities of iron at certain solar conditions. To replicate these opacity measurements a platform is being developed on the National Ignition Facility to measure the opacities of iron and other elements at the same conditions as in the Z experiments. The NIF platform consists of a hohlraum to heat the opacity sample to the desired conditions, a separate backlighter to radiograph the sample, and a spectrometer to give the spectrally resolved opacity. Not only must the opacity be measured but the temperature and density of the sample must also be accurately determined. This platform has now produced its first iron transmission measurements. Overall, these measurements will be presented along with plans for future measurements and details on how the measurements will be improved.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

NASA NTRS2005

Overview of the Spirit Mars Exploration Rover Mission to Gusev Crater: Landing Site to Backstay Rock in the Columbia Hills

Spirit landed on the floor of Gusev Crater and conducted initial operations on soil covered, rock-strewn cratered plains underlain by olivine-bearing basalts. Plains surface rocks are covered by wind-blown dust and show evidence for surface enrichment of soluble species as vein and void-filling materials and coatings. The surface enrichment is the result of a minor amount of transport and deposition by aqueous processes. Layered granular deposits were discovered in the Columbia Hills, with outcrops that tend to dip conformably with the topography. The granular rocks are interpreted to be volcanic ash and/or impact ejecta deposits that have been modified by aqueous fluids during and/or after emplacement. Soils consist of basaltic deposits that are weakly cohesive, relatively poorly sorted, and covered by a veneer of wind blown dust. The soils have been homogenized by wind transport over at least the several kilometer length scale traversed by the rover. Mobilization of soluble species has occurred within at least two soil deposits examined. The presence of mono-layers of coarse sand on wind-blown bedforms, together with even spacing of granule-sized surface clasts, suggest that some of the soil surfaces encountered by Spirit have not been modified by wind for some time. On the other hand, dust deposits on the surface and rover deck have changed during the course of the mission. Detection of dust devils, monitoring of the dust opacity and lower boundary layer, and coordinated experiments with orbiters provided new insights into atmosphere-surface dynamics.

Arvidson, R. E.↗

NASA NTRS1983

Saturn's pole - geometric correction based on voyager UVS and radio occultations

Measurements of of the opacity of Saturn's rings acquired during occultation experiments at radio (3.6 cm) and ultraviolet wavelengths were initially reduced to radial position rho using a standard pole vector. Common features in the two data sets from this reduction were offset by distances Delta rho(i). These offsets have been attributed to an error in the pole direction. Because the viewing geometries were quite different for the two experiments, the set of differences of Delta rho(i) provides a sensitive measure of corrections needed to refine the Saturn pole direction. The new standard pole vector in 1950.0 coordinates has right ascension alpha = 38.409 + or - 0.016 deg and declination delta = 83.324 + or - 0.002 deg.

Simpson, R. A.↗

NASA NTRS1998

Modeling Molecular Opacities Using Galileo Probe Observations

Data from the Net Flux Radiometer (NFR) experiment on the Galileo mission has been successfully collected and analyzed through 1996. As data was received, the best available laboratory spectroscopic data and was used in the reduction procedure. Since then newer and more accurate spectroscopic data has become available. During this agreement, research efforts focused on re-analysis of certain aspects of the data which benefited from recent improvements in spectroscopic databases, and from a more exact treatment of certain aspects of the physical theory of line shape and line broadening. In addition, a brief survey was completed of the available information, both theoretical and observational, of the absorption, reflection and transmission spectra of the atmospheres of the various types of planets that could reasonably be expected to occur in other solar systems.

Freedman, Richard S.↗

NASA NTRS1998

Modeling Molecular Opacities using Galileo Probe Observations

Freedman, Richard S.↗