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At least 55 records · Page 3

Radiative impact of aerosols generated from biomass burning

Atmospheric aerosol particles play a vital role in the Earth's radiative energy budget. They exert a net cooling influence on climate by directly reflecting the solar radiation to space and by modifying the shortwave reflective properties of clouds. Each year, increasing amounts of aerosol particles are released into the atmosphere due to biomass burning, dust storms, forest fires, and volcanic activity. These particles significantly perturb the radiative balance on local, regional, and global scales. While the detection of aerosols over water is a well established procedure, the detection of aerosols over land is often difficult due to the poor contrast between the aerosols and the underlying terrain. In this study, we use textural measures in order to detect aerosols generated from biomass burning over South America, using AVHRR data. The regional radiative effects are then examined using ERBE data. Preliminary results show that the net radiative forcing of aerosols is about -36 W/sq m.

Christopher, Sundar A.↗

Observations of Smoke Aerosol from Biomass Burning in Mexico: Effect of Particle Aging on Radiative Forcing and Remote Sensing

We take advantage of the May 1998 biomass burning event in Southern Mexico to test the global applicability of a smoke aerosol size model developed from data observed in South America. The Mexican event is an unique opportunity to observe well-aged, residual smoke. Observations of smoke aerosol size distribution made from vertical profiles of airborne in situ measurements show an inverse relationship between concentration and particle size that suggests the aging process continues more than a week after the smoke is separated from its fire sources. The ground-based radiometer retrievals show that the column-averaged, aged, Mexican smoke particles are larger (diameter = 0.28 - 0.33 micrometers) than the mean smoke particles in South America (diameter = 0.22 - 0.30 micrometers). However, the difference (delta - 0.06 micrometer) translates into differences in backscattering coefficient of only 4-7% and an increase of direct radiative forcing of only 10%.

Remer, Lorraine A.↗

Numerical investigation of alpha particle confinement under the perturbation of neoclassical tearing modes and toroidal field ripple in CFETR

The confinement of alpha particles in burning plasma is a key issue in fusion reactor design, including particle interaction with instabilities. Here, we include two topics: the effect of neoclassical tearing modes (NTMs) and toroidal field ripple on alpha particle loss, and the assessment of particle redistribution under an NTM with a reduced model. We consider Chinese fusion engineering test reactor parameters, the alpha particle distribution given by TRANSP/NUBEAM and the NTM perturbation function given by the initial value code TM1. We show that the synergistic effect of the NTM and ripple is negligible; the particle loss fraction does not change with increasing NTM amplitude. Only passing particles are affected by the mode particle resonance, producing profile flattening but no increased loss because only trapped particles are influenced by ripple. To study alpha particle profile flattening, the work adopts an innovative method of phase vector rotation to determine regions of good and broken Kolmogorov–Arnold–Moser surfaces and equilibrates the particle density according to local stochasticity.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Optical properties of aerosol emissions from biomass burning in the tropics, BASE-A

Ground-based and airborne measurements of biomass-burning smoke particle optical properties, obtained with a view to aerosol-absorption properties, are presented as a function of time and atmospheric height. The wavelength dependence of the optical thickness can be explained by a log-normal size distribution, with particles' effective radius varying between 0.1 and 0.2 microns. The strong correlation noted between aerosol particle profile and CO profile indicates that smoke particulates constitute a good tracer for emission trace gases from tropical biomass burning.

Holben, Brent N.↗

Radiative Effects of Aerosols Generated from Biomass Burning, Dust Storms, and Forest Fires

Atmospheric aerosol particles, both natural and anthropogenic, are important to the earth's radiative balance. They scatter the incoming solar radiation and modify the shortwave reflective properties of clouds by acting as Cloud Condensation Nuclei (CCN). Although it has been recognized that aerosols exert a net cooling influence on climate (Twomey et al. 1984), this effect has received much less attention than the radiative forcings due to clouds and greenhouse gases. The radiative forcing due to aerosols is comparable in magnitude to current anthropogenic greenhouse gas forcing but opposite in sign (Houghton et al. 1990). Atmospheric aerosol particles generated from biomass burning, dust storms and forest fires are important regional climatic variables. A recent study by Penner et al. (1992) proposed that smoke particles from biomass burning may have a significant impact on the global radiation balance. They estimate that about 114 Tg of smoke is produced per year in the tropics through biomass burning. The direct and indirect effects of smoke aerosol due to biomass burning could add up globally to a cooling effect as large as 2 W/sq m. Ackerman and Chung (1992) used model calculations and the Earth Radiation Budget Experiment (ERBE) data to show that in comparison to clear days, the heavy dust loading over the Saudi Arabian peninsula can change the Top of the Atmosphere (TOA) clear sky shortwave and longwave radiant exitance by 40-90 W/sq m and 5-20 W/sq m, respectively. Large particle concentrations produced from these types of events often are found with optical thicknesses greater than one. These aerosol particles are transported across considerable distances from the source (Fraser et al. 1984). and they could perturb the radiative balance significantly. In this study, the regional radiative effects of aerosols produced from biomass burning, dust storms and forest fires are examined using the Advanced Very High Resolution Radiometer (AVHRR) Local Area Coverage (LAC) data and the instantaneous scanner ERBE data from the NOAA-9 and NOAA-10 satellites.

Christopher Sundar A.↗

Using the Black Carbon Particle Mixing State to Characterize the Lifecycle of Biomass Burning Aerosols

The lifecycle of black carbon (BC)-containing particles from biomass burns is examined using aircraft and surface observations of BC mixing state for plume ages from ~15 minutes to 10 days. Because BC is non-volatile and chemically inert, changes in the mixing state of BC-containing particles are driven solely by changes in particle coating, which is mainly secondary organic aerosol (SOA). The coating mass initially increases rapidly (k = 0.84 hr-1), then remains growth relatively constant for 1 to 2 days as plume dilution no longer supports further growth, then decreases slowly until only ~30 % of the maximum coating mass remains after 10 days, (kloss = 0.011 hr-1). The mass ratio of coating-to-core for a BC-containing particle with a 100 nm mass- equivalent diameter BC core reaches a maximum of ~20 after a few hours and drops to ~5 after 10 days of aging. The initial increase in coating mass can be used to determine SOA formation rates. The slow loss of coating material, not captured in global models, comprises the dominant fraction of the lifecycle of these particles. Coating-to-core mass ratios of BC particles in the stratosphere are much greater than those in the free troposphere indicating a different lifecycle.

54 ENVIRONMENTAL SCIENCES↗

Energetic particle transport in 3D equilibrium. Final report

In this project, we have further developed the state-of-the-art fusion simulation code, gyrokinetic toroidal code (GTC), for studying the energetic particle (EP) transport in the 3D equilibrium. We have applied the new capabilities to simulate the EP transport by the Alfven eigenmodes in stellarators and by 3D magnetic islands in tokamaks. As part of V&V efforts for 3D capability, the 3D capabilities of GTC have been applied to study thermal transport in stellarators and tokamak with 3D magnetic fields by microturbulence, which could cause additional EP loss. Effects magnetic islands on neoclassical bootstrap current have also been studied. The computational capability developed and physics learned in this project are in support of fusion SciDAC Center for Integrated Simulation of Energetic Particles in Burning Plasmas (ISEP). During this project, the PI has supervised 6 postdoctoral researchers and 4 PhD students at the University of California, Irvine. A complete list of 49 publications and 23 invited talks partially supported by this grant since 7/2015 appears at the end of this report. Five key publications closely related to this project are highlighted in this report.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Overview of fast particle experiments in the first MAST Upgrade experimental campaigns

Abstract MAST-U is equipped with on-axis and off-axis neutral beam injectors (NBI), and these external sources of super-Alfvénic deuterium fast-ions provide opportunities for studying a wide range of phenomena relevant to the physics of alpha-particles in burning plasmas. The MeV range D-D fusion product ions are also produced but are not confined. Simulations with the ASCOT code show that up to 20% of fast ions produced by NBI can be lost due to charge exchange (CX) with edge neutrals. Dedicated experiments employing low field side (LFS) gas fuelling show a significant drop in the measured neutron fluxes resulting from beam-plasma reactions, providing additional evidence of CX-induced fast-ion losses, similar to the ASCOT findings. Clear evidence of fast-ion redistribution and loss due to sawteeth (ST), fishbones (FB), long-lived modes (LLM), Toroidal Alfvén Eigenmodes (TAE), Edge Localised Modes (ELM) and neoclassical tearing modes (NTM) has been found in measurements with a Neutron Camera (NCU), a scintillator-based Fast-Ion Loss Detector (FILD), a Solid-State Neutral Particle Analyser (SSNPA) and a Fast-Ion Deuterium- α (FIDA) spectrometer. Unprecedented FILD measurements in the range of 1–2 MHz indicate that fast-ion losses can be also induced by the beam ion cyclotron resonance interaction with compressional or global Alfvén eigenmodes (CAEs or GAEs). These results show the wide variety of scenarios and the unique conditions in which fast ions can be studied in MAST-U, under conditions that are relevant for future devices like STEP or ITER.

Physics↗

Ignition and combustion characteristics of metallized propellants

Over the past six months, experimental investigations were continued and theoretical work on the secondary atomization process was begun. Final shakedown of the sizing/velocity measuring system was completed and the aluminum combustion detection system was modified and tested. Atomizer operation was improved to allow steady state operation over long periods of time for several slurries. To validate the theoretical modeling, work involving carbon slurry atomization and combustion was begun and qualitative observations were made. Simultaneous measurements of aluminum slurry droplet size distributions and detection of burning aluminum particles were performed at several axial locations above the burner. The principle theoretical effort was the application of a rigid shell formation model to aluminum slurries and an investigation of the effects of various parameters on the shell formation process. This shell formation model was extended to include the process leading up to droplet disruption, and previously developed analytical models were applied to yield theoretical aluminum agglomerate ignition and combustion times. The several theoretical times were compared with the experimental results.

Mueller, D. C.↗

Trace impurity transport in multi-species plasmas with large particle fluxes

A burning fusion plasma has a large inwards flux of fuel and outwards flux of ash. Existing impurity transport theories do not account for a steady-state environment of such large fluxes. In this paper, we extend classical transport theory to account for a background of such fluxes. In a mainly two-ion species magnetized plasma, with oppositely directed density gradients maintained by oppositely directed sources of the two species, trace impurity ions are shown to align with the larger mass ions. This unexpected behavior is derived analytically and simulated numerically using the MITNS (Multiple-Ion Transport Numerical Solver) code. Overall, the result suggests a potential advantage of edge-fueled p-B11 fusion in extracting high-Z impurities, and possible applications in plasma-based separation methods.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

SiC particles from asymptotic giant branch stars - Mg burning and the s-process

The question of whether isotopically anomalous SiC particles found in meteorites originate in AGB stars is addressed. It is shown that if the peak helium shell flash temperatures of massive (6-9 solar masses) stars are about 10 percent larger than they are normally assumed to be, alpha particle reactions with the magnesium will become significant. Then the (Mg-29)(alpha, n)Si-29 reaction produces a large excess of Si-29. With a light element nuclear reaction network, the evolution of the silicon isotopic composition during AGB evolution is calculated. It is found that the experimentally determined correlation between excess Si-29 and excess Si-30 in SiC particles from carbonaceous chondrites can indeed be naturally produced in this way. It is suggested that if the large isotopically anomalous SiC particles carrying nearly pure-process krypton and xenon do indeed originate in AGB stars, those stars were massive and had peak shell flash temperatures near 450 KM.

Brown, Lawrence E.↗

Particle Shape, Size, and Composition from Satellites

The MISR Research Aerosol (RA) retrieval algorithm produces (A) aerosol amount (optical depth – AOD), (B) an aerosol size constraint (Angstrom Exponent) (C) fraction of non-spherical particles, and (D) particle light-absorption (SSA). Near the Camp fire source region the particles tend to be large (low Angstrom Exponent) and non-spherical particles, probably from burning in the town of Paradise. Aerosols are smaller and more spherical downwind, probably as the plume mixes with smoke from burning forest.

aerosol↗

Ignition of metals and alloys by high-velocity particles

The ignition of metals and alloys by impacting high-velocity particles in gaseous oxygen was investigated. A convergent/divergent nozzle was used to accelerate the flowing oxygen, which in turn accelerated the particles to velocities greater than 305 m/s (1000 ft/s). The test sample (target) was placed at the end of the chamber in the flow path. Aluminum 6061, type 316 stainless steel, type 304 stainless steel, and Inconel 718 were ignited with 1600-micron aluminum 2017 particles at elevated temperatures and pressures whereas Monel 400 could not be ignited. The ignition susceptibility of metals and alloys appeared to increase as the inlet pressure, sample temperature, and particle size were increased. Type 304 stainless steel particles required more extreme conditions for ignition of materials than similar sized aluminum particles. The results indicated that ignition and subsequent burning of the particles were required for ignition of the target materials with the possible exception of aluminum 6061.

Benz, F. J.↗

Effects of aerosol from biomass burning on the global radiation budget

An analysis is made of the likely contribution of smoke particles from biomass burning to the global radiation balance. These particles act to reflect solar radiation directly; they also can act as cloud condensation nuclei, increasing the reflectivity of clouds. Together these effects, although uncertain, may add up globally to a cooling effect as large as 2 watts per square meter, comparable to the estimated contribution to sulfate aerosols. Anthropogenic increases of smoke emission thus may have helped weaken the net greenhouse warming from anthropogenic trace gases.

Penner, Joyce E.↗

Field intercomparison of ice nucleation measurements: the Fifth International Workshop on Ice Nucleation Phase 3 (FIN-03)

Abstract. The third phase of the Fifth International Ice Nucleation Workshop (FIN-03) was conducted at the Storm Peak Laboratory in Steamboat Springs, Colorado, in September 2015 to facilitate the intercomparison of instruments measuring ice-nucleating particles (INPs) in the field. Instruments included two online and four offline measurement systems for INPs, which are a subset of those utilized in the laboratory study that comprised the second phase of FIN (FIN-02). The composition of the total aerosols was characterized using the Particle Analysis by Laser Mass Spectrometry (PALMS) and Wideband Integrated Bioaerosol Sensor (WIBS) instruments, and aerosol size distributions were measured by a laser aerosol spectrometer (LAS). The dominant total particle compositions present during FIN-03 were composed of sulfates, organic compounds, and nitrates, as well as particles derived from biomass burning. Mineral-dust-containing particles were ubiquitous throughout and represented 67 % of supermicron particles. Total WIBS fluorescing particle concentrations for particles with diameters of > 0.5 µm were 0.04 ± 0.02 cm−3 (0.1 cm−3 highest; 0.02 cm−3 lowest), typical of the warm season in this region and representing ≈ 9 % of all particles in this size range as a campaign average. The primary focus of FIN-03 was the measurement of INP concentrations via immersion freezing at temperatures > −33 °C. Additionally, some measurements were made in the deposition nucleation regime at these same temperatures, representing one of the first efforts to include both mechanisms within a field campaign. INP concentrations via immersion freezing agreed within factors ranging from nearly 1 to 5 times on average between matched (time and temperature) measurements, and disagreements only rarely exceeded 1 order of magnitude for sampling times coordinated to within 3 h. Comparisons were restricted to temperatures lower than −15 °C due to the limits of detection related to sample volumes and very low INP concentrations. Outliers of up to 2 orders of magnitude occurred between −25 and −18 °C; a better agreement was seen at higher and lower temperatures. Although the 5–10 factor agreement of INP measurements found in FIN-03 aligned with the results of the FIN-02 laboratory comparison phase, giving confidence in progress of this measurement field, this level of agreement still equates to temperature uncertainties of 3.5 to 5 °C that may not be sufficient for numerical cloud modeling applications that utilize INP information. INP activity in the immersion-freezing mode was generally found to be an order of magnitude or more, making it more efficient than in the deposition regime at 95 %–99 % water relative humidity, although this limited data set should be augmented in future efforts. To contextualize the study results, an assessment was made of the composition of INPs during the late-summer to early-fall period of this study inferred through comparison to existing ice nucleation parameterizations and through measurement of the influence of thermal and organic carbon digestion treatments on immersion-freezing ice nucleation activity. Consistent with other studies in continental regions, biological INPs dominated at temperatures of > −20 °C and sometimes colder, while arable dust-like or other organic-influenced INPs were inferred to dominate below −20 °C.

54 ENVIRONMENTAL SCIENCES↗