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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
NASA NTRS1985

Hexagonal uniformly redundant arrays for coded-aperture imaging

Uniformly redundant arrays are used in coded-aperture imaging, a technique for forming images without mirrors or lenses. This technique is especially important for the high energy X-ray and gamma-ray region above 20 kev. In this technique, a mask consisting of opaque (closed) and trasparent (open) areas is placed between the photon sources to be imaged and a position sensitive detector or a detector array. Each source casts a shadow pattern of the mask or aperture onto the detector. This shadow pattern may be viewed as an encoded signal for that source direction. If each possible source code is unique, the detected composite of overlapping shadow patterns may be decoded to produce an image of the source distribution.

Finger, M. H.↗
NASA NTRS1988

Intercalibration of the hard X-ray spectrometers on the PVO and ICE (ISEE-3) spacecraft

The energetic photon spectrometers aboard the ICE and PVO (Pioneer Venus Orbiter) are described briefly, and the procedure for their in-flight calibrations is discussed. Successful intercalibration of these two instruments led to stereoscopic observations of 100 keV-2 MeV photon sources in solar flares and the study of the directivity and height structure of these sources. The impulsive hard X-ray source is found to extend from the chromosphere to the corona, the brightness of the source decreasing rapidly with increase in height above the chromosphere. The analysis so far indicates no systematic directivity for the hard X-ray source. The observations are consistent with energetic electrons accelerated in the corona propagating downward toward the chromosphere. However, when avaraged over the duration of an impulsive hard X-ray flare, the 'beaming' of electrons is found to be small in most flares.

Kane, S. R.↗
NASA NTRS1989

Gamma ray bursts from magnetospheric plasma oscillations

Neutron star Magnetospheric Plasma Oscillations (MPO), can account for the energetics, decay time scale, and spectra of typical Gamma Ray Bursts (GRBs). The soft photon source is likely to be due to backwarming of the reprocessing boundary by the incipient gamma rays. It is shown that the observed fraction of bursts displaying low energy absorption features may be understood in the context of an MPO model. Moreover, it is found that GRB spectra should display these cyclotron lines about 18 percent of the time, which is consistent with the KONUS and Ginga sets of data.

Melia, Fulvio↗
NASA NTRS1989

The probability of detecting absorption features in gamma-ray burst spectra

It has recently been suggested that several mechanisms for the primary release of energy in gamma-ray bursts may result in the excitation of magnetospheric plasma oscillations (MPO) above the polar cap of a neutron star. The basic MPO idea is refined by determining the soft photon source (which damps the particle motion via inverse Compton scattering interactions) self-consistently by means of a Monte Carlo simulation for the deposition of back-scattered gamma-ray energy below the stellar photosphere. The observed fraction of bursts displaying low-energy absorption features may be understood in the context of a model wherein the overall spectrum changes with inclination angle due to the superposition of several components with different angular distributions. GRB spectra should display these cyclotron lines about 18 percent of the time, which is consistent with the KONUS and Ginga sets of data.

Melia, F.↗
NASA NTRS1990

Gamma-ray bursts from magnetospheric plasma oscillations

Relativistic, (neutron star) magnetospheric plasma oscillations, damped by inverse Compton scatterings with the ambient radiation field, can account for the energetics, decay time scale, and spectra of typical gamma-ray bursts (GRBs). The dissipation time scale tau depends on the energy of the perturbation, and that tau of about 1 sec for W(burst) is about 10 to the 36th ergs. Several plausible mechanisms for 'loading' the magnetosphere, all of which might be contributing to the GRB phenomenon are discussed. The soft photon source is likely due to backwarming of the reprocessing boundary (i.e., the stellar surface and possibly an accretion disk) by the incipient gamma-rays, which is consistent with the Ginga observation of a slowly decaying, low-energy X-ray component in some bursts.

Melia, Fulvio↗
NASA NTRS1992

Cyclotron resonant scattering in gamma-ray bursts - Further analysis of GB880205

We have extended our previous work by exploring several plane-parallel slab geometries to model the formation of cyclotron line features. We calculated the Compton temperature T(C) as a function of column density Ne for each of the new geometries. We then fit the resulting spectra to GB880205 exactly as described in Wang et al. (1989). The results show that the addition of column depth below the photon source plane leads to a modest improvement in chi-squared which, although not statistically significant, is pleasing because these geometries are more physically realistic.

Freeman, P. E.↗
NASA NTRS1994

Searching for hard X-ray directivity during the rise, peak, and decay phases of solar flares

We have identified 72 large solar flares (peak counting rates more than 1000 counts/s) observed by Hard X-ray Burst Spectroscopy (HXRBS) on-board the Solar Maximum Mission (SMM). Using a database of these flares, we have studied hard X-ray (50-850 keV) spectral center-to-limb variation and its evolution with time. The major results are the following: (1) During the rise phase, the center-to-limb spectral variation is small, with a hardness of delta delta = 0.02 +/- 0.25, and a statistical significance of 0.1 sigma. (2) During the peak phase, the center-to-limb variation is delta delta = 0.13 +/- 0.13, with a statistical significance of 1 sigma. (3) During the decay phase, the center-to-limb variation changes to softening. The softness is relatively large with delta delta = -0.25 +/- 0.21, and a statistical significance of 1.2 sigma. (4) The linear least-squares fits to the spectral center-to-limb variations do not have slopes significantly different from zero during all those three phases. (5) The center events and limb events spectral distributions are shown to be not different by using Kolmogorov-Smirnov two-samples test. (6) The fraction of events detected near the limb is marginally consistent with that expected from isotropically emitting flares. (7) On average, flares evolve as soft-hard-soft. These results suggest that there is no statistically significant evidence for hard X-ray directivity during the rise, peak, and decay phases of solar flares. The hard X-ray radiation pattern at those energies is almost isotropic during all those phases. This lack of directivity (or anisotropy) found in this study is not in agreement with the results discovered by Vestrand et al. (1987) in which they found energetic photon source is anisotropic, using SMM Gamma-Ray Spectrometer (GRS) data at a much higher energy band of 0.3-1 MeV. If we want to interpret the results of Vestrand et al. (1987) and our present results in a self-consistent way, we must conclude that at energies of greater than 50 keV, the Compton backscattering suppresses the hard X-ray anisotropy sufficiently so that no significant directivity can be measured during the rise, peak, and decay phases of solar flares. during the rise, peak, and decay phases of solar flares.

Li, Peng↗
NASA NTRS1995

Phase lags in Cygnus X-1

Coronae of hot electrons are ubiquitous features in models of the inner regions of accreting black holes and nonmagnetic neutron stars. The scattering optical depth of these coronae inferred from observations is often tau approximately 3, so the energy spectrum of the disk in these regions is likely masked by the spectrum of upscattered photons in the corona and some of the disk properties are thus obscured. Observations of the dependence on not available with the energy spectrum. In our picture, the disk emission is modeled as a photon source injected into a Comptonizing corona; Comptonization may also occur in the disk, but for our purposes the disk emission is simply an input to the corona. We show that, contrary to some claims, the functional dependence of lag on Fourier frequency emerges intact from transit through the corona, modulo a multiplicative factor (which may in principle be negative, so that a phase lag can be changed to a phase lead), even if the properties of the corona vary with time. We also show that any frequency dependence of the lag due to variation in the corona itself is only second order in the amplitude of the variation, and cannot exceed the transit time approximately ms of the corona; thus, the lags of up to 0.1 s seen in several black hole candidates come from lags in the emission from the disk. Finally, we predict that plots of the time lag versus Fourier frequency in black hole candidates should have a 'shelf' of constant lag equal to the coronal lag (approximately 1 ms), with the constant being proportional to In (E(sub 2)/E(sub 1)) for the lag between energies E(sub 2) and E(sub 1). The lack of such a shelf in current observations of several galactic black hole candidates constraints the radii of the coronae to be R less than or approximately = 10(exp 8) tau cm.

Miller, M. Coleman↗
NASA NTRS2002

X-Ray and Electrostatic Levitation Undercooling Studies in Ti-Zr-Ni Quasicrystals Forming Alloys

The first undercooling nucleation measurements of electrostatic-levitated droplets of TiZrNi alloys that form the icosahedral quasicrystal phase (i-phase) are presented. The reduced undercooling for crystallization decreases with an increasing polytetrahedral order of the primary solidifying phase, supporting the existence of a developing icosahedral short-range order in the undercooled liquid. X-ray diffraction measurements made at the Advance Photon Source on levitated liquid droplets of these alloys at their liquidus temperatures, however, show no evidence for increased icosahedral order. This suggests that significant ordering only occurs below the melting temperature.

Rogers, J. R.↗
NASA NTRS2004

The X-ray Polarimetry Explorer (XPE)

We present details of a Thomson scattering polarimeter suitable for a small-explorer- class mission. Termed XPE, for X-Ray Polarimetry Explorer, the instrument consists of a beryllium scattering cone surrounded by an annular multiwire proportional counter which registers the energy and position of scattered source photons. The polarimeter is sensitive over an energy range of 7-27 keV and will achieve 3% minimum detectable polarization of Her X-1 in a 1/2-day observation, and cover a 30-target core observation program, at the same sensitivity level, in approximately 8 months.

Ramsey, Brian↗
NASA NTRS2003

An Overview of the Materials Science Research at the Marshall Space Flight Center Electrostatic Levitator Facility and Recent CDDF Efforts

Containerless processing is an important tool for materials research. The freedom from a crucible allows processing of liquid materials in a metastable undercooled state, as well as allowing processing of high temperature and highly reactive melts. Electrostatic levitation (ESL) is a containerless method which provides a number of unique advantages, including the ability to process non-conducting materials, the ability to operate in ultra-high vacuum or at moderate gas pressure (approx. = 5 atm), and the decoupling of positioning force from sample heating. ESL also has the potential to reduce internal flow velocities below those possible with electromagnetic, acoustic, or aero-acoustic techniques. In electrostatic levitation, the acceleration of gravity (or residual acceleration in reduced gravity) is opposed by the action of an applied electric field on a charged sample. Microgravity allows electrostatic levitation to work even more effectively. The ESL facility at NASA s Marshall Space Flight Center is in use for materials research and thermophysical property measurement by a number of different internal and external investigators. Results from the recent CDDF studies on the high energy X-ray beamline at the Advanced Photon Source of Argonne National Laboratory will be presented. The Microgravity Research Program supports the facility.

Source record↗
NASA NTRS2004

Micro-XANES Measurements on Experimental Spinels and the Oxidation State of Vanadium in Spinel-Melt Pairs

Spinel can be a significant host phase for V as well as other transition metals such as Ni and Co. However, vanadium has multiple oxidation states V(2+), V(3+), V(4+) or V(5+) at oxygen fugacities relevant to natural systems. We do know that D(V) spinel/melt is correlated with V and TiO2 content and fO2, but the uncertainty of the oxidation state under the range of natural conditions has made elusive a thorough understanding of D(V) spinel/melt. For example, V(3+) is likely to be stable in spinels, based on exchange with Al in experiments in the CaO-MgO-Al2O3-SiO2 system. On the other hand, it has been argued that V(4+) will be stable across the range of natural oxygen fugacities in nature. In order to gain a better understanding of D(V) spinel/melt we have equilibrated spinel-melt pairs at controlled oxygen fugacities, between HM to NNO, where V is present in the spinel at natural levels (approx. 300 ppm V). These spinel-melt pairs were analyzed using micro-XANES at the Advanced Photon Source at Argonne National Laboratory. The new results will be used together with spinel compositional data (Ti, V content) and oxygen fugacity, to unravel the effects of these variables on D(V) spinel/melt.

Righter, K.↗
NASA NTRS2005

Micro-XANES Measurements on Experimental Spinels and the Oxidation State of Vanadium in Coexisting Spinel and Silicate Melt

Spinel can be a significant host phase for V which has multiple oxidation states V(sup 2+), V(sup 3+), V(sup 4+) or V(sup 5+) at oxygen fugacities relevant to natural systems. The magnitude of D(V) spinel/melt is known to be a function of composition, temperature and fO2, but the uncertainty of the oxidation state under the range of natural conditions has made elusive a thorough understanding of D(V) spinel/melt. For example, V(sup 3+) is likely to be stable in spinels, based on exchange with Al in experiments in the CaO-MgO-Al2O3-SiO2 system. On the other hand, it has been argued that V(sup 4+) will be stable across the range of natural oxygen fugacities in nature. In order to build on our previous work in more oxidized systems, we have carried out experiments at relatively reducing conditions from the FMQ buffer to 2 log fO2 units below the IW buffer. These spinel-melt pairs, where V is present in the spinel at natural levels (approx. 300 ppm V), were analyzed using an electron microprobe at NASA-JSC and micro- XANES at the Advanced Photon Source at Argonne National Laboratory. The new results will be used together with previous results to understand the valence of V in spinel-melt systems across 12 orders of magnitude of oxygen fugacity, and with application to natural systems.

Righter, K.↗
NASA NTRS2006

Floating the Ball: Advances in the Technology of Electrostatic Levitation

Electrostatic Levitation (ESL) is an emerging technology. The MSFC ESL is a NASA facility that supports investigations of refractory solids and melts. The facility can be used to process a wide variety of materials including metals, alloys, ceramics, glasses and semiconductors. Containerless processing via ESL provides a high-purity environment for the study of high temperature materials and access to metastable states. Scientific topics investigated in the facility include nucleation, undercooling, metastable state formation and metallic glass formation. Additionally, the MSFC ESL provides data for the determination of phase diagrams, time-temperature-transition diagrams, viscosity, surface tension, density, heat capacity and creep resistance. In order to support a diverse research community, the MSFC ESL facility has developed a number of technical capabilities, including a portable system for in situ studies of structural tran$hrmations during processing at the high-energy X-ray beamline at the Advanced Photon Source of Argonne National Laboratory. The capabilities of the MSFC ESL facilities will be discussed and selected results of materials processing and characterization studies will be presented.

Rogers, Jan R.↗
NASA NTRS2007

GRBs: The Most Distant Signposts in our Universe

Gamma-Ray Bursts (GRBs) are the most powerful photon sources in the Universe, rivaled only by supernovae in the magnitude of their energy release. In 1997 GRB were found to originate in host galaxies at cosmological distances, revealing the total energy of their explosions to be an astounding approx.10(exp 52) - 10(exp 53)ergs. GRB durations span over five orders of magnitude, ranging from milliseconds to thousands of seconds. The underlying sources of the energy release remain, however, unknown. Leading candidates are mergers, either of two neutron stars or of a black hole and a neutron star, and core collapses of very massive stars, called "collapsars". To date the furthest GRB galaxy has been found at a cosmological redshift of 6.29, very close to the most distant quasar (at z=6.4). Since the Swift satellite continues to observe these phenomena at a rate of approx.120 per year, and with the upcoming launch of GLAST with two burst instruments on board, we will be able to use GRBs as beacons to probe very high redshifts. Thus bursts found at 6<z<20 can be efficient probes of the intergalactic medium, the first (population III) stars and the early stages of galaxy formation.

Kouveliotou, Chryssa↗
NASA NTRS2008

Experimental Constraints on the Partitioning and Valence of V and Cr in Garnet and Coexisting Glass

A series of experiments with garnet and coexisting melt have been carried out across a range of oxygen fugacities (near hematite-magnetite (HM) to below the iron-wustite (IW) buffers) at 1.7 GPa to study the partitioning and valence of Cr and V in both phases. Experiments were carried out in a non end loaded piston cylinder apparatus, and the run products were analyzed with electron microprobe and xray absorption near edge structure (XANES) analysis at beamline 13-ID at the Advanced Photon Source of Argonne National Lab. The valence of vanadium and chromium were determined using the position and intensity of the Ka pre-edge peaks, calibrated on a series of Cr and Vbearing standard glasses. This technique has been applied to V and Cr in glasses and V in spinels previously, and in these isotropic phases there are no orientational effects on the XANES spectra (Righter et al., 2006, Amer. Mineral. 91, 1643-1656). We also now demonstrate this to be true for V and Cr in garnet. Also, previous work has shown that V has a higher valence in the glass (or melt) than in the coexisting spinel. This is also true for V in garnet-glass pairs in this study. Vanadium valence in garnets varies from 2.7 below the IW buffer to 3.7 near HM, and for coexisting glass it varies from 3.2 to 4.3. Vanadium valence measured in some natural garnets from mantle localities indicates V in the more reduced range at 2.5. Comparisons will be made between fO2 estimated from V valence and other methods for garnet-bearing mantle samples. In contrast, Cr valence measured in garnet and coexisting glass for all experimental and natural samples is 2.9- 3.0, suggesting that the valence of Cr does not vary within either phase across a large fO2 range. These results demonstrate that while V varies from 2+ to 3+ to 4+ in garnet-melt systems, Cr does not, and this will ultimately affect the partitioning behavior of these two elements in natural systems. Garnet/melt D(Cr) are between 12 and 17 across this range of fO2, whereas D(V) has the highest partition coefficient approx.3, near the IW buffer where the valence of V is almost entirely 3+.

Righter, K.↗
NASA NTRS2008

Role of Hf on Phase Formation in Ti45Zr(38-x)Hf(x)Ni17 Liquids and Solids

Hafnium and zirconium are very similar, with almost identical sizes and chemical bonding characteristics. However, they behave differently when alloyed with Ti and Ni. A sharp phase formation boundary near 18-21 at.% Hf is observed in rapidly-quenched and as-cast Ti45Zr38-xHfxNi17 alloys. Rapidly-quenched samples that contain less than 18 at.% Hf form the icosahedral quasicrystal phase, whiles samples containing more than 21 at.% form the 3/2 rational approximant phase. In cast alloys, a C14 structure is observed for alloys with Hf lower than the boundary concentration, while a large-cell (11.93 ) FCC Ti2Ni-type structure is found in alloys with Hf concentrations above the boundary. To better understand the role of Hf on phase formation, the structural evolution with supercooling and the solidification behavior of liquid Ti45Zr38-xHfxNi17 alloys (x=0, 12, 18, 21, 38) were studied using the Beamline Electrostatic Levitation (BESL) technique using 125keV x-rays on the 6ID-D beamline at the Advanced Photon Source, Argonne National Laboratory. For all liquids primary crystallization was to a BCC solid solution phase; interestly, an increase in Hf concentration leads to a decrease in the BCC lattice parameter in spite of the chemical similarity between Zr and Hf. A Reitveld analysis confirmed that as in the cast alloys, the secondary phase that formed was the C14 below the phase formation boundary and a Ti2Ni-type structure at higher Hf concentrations. Both the liquidus temperature and the reduced undercooling change sharply on traversing the phase formation boundary concentration, suggesting a change in the liquid structure. Structural information from a Honeycutt-Anderson index analysis of reverse Monte Carlo fits to the S(q) liquid data will be presented to address this issue.

Wessels, V.↗
NASA NTRS2011

Silica-Titania Composite (STC)'s Performance in the Photocatalytic Oxidation of Polar VOCs

The objective of this paper is to determine the performance of a Silica-Titania Composite (STC) in the photocatalytic oxidation (PCO) of polar VOCs for potential applications in trace contaminant control within space habitats such as the ISS and CEV Orion. Tests were carried out in a bench scale STC-packed annular reactor under continuous illumination by either a UV-C germicidal lamp(lambda (sub max) = 254 nm) or UV-A fluorescent BLB (lambda(sub max) = 365 nm) for the removal of ethanol (a predominant polar VOC in the ISS cabin). The STC's performance was evaluated in terms of the ethanol mineralization rate, mineralization efficiency, and the extent of its oxidation intermediate (acetaldehyde) formation in response to the type of light source (photon energy and photon flux) and relative humidity (RH) implemented. Results demonstrated that acetaldehyde was the only quantifiable intermediate in the effluent under UV illumination, but was not found in the dark adsorption experiments. The mineralization rate increased with an increase in photon energy (UV-C greater than UV-A), even though both lamps were adjusted to emit the same incident photon flux, and also increased with increasing photon flux. However, photonic efficiency decreased as the photon flux increased. More importantly, a higher photon flux gave rise to a lower effluent acetaldehyde concentration. The effect of RH on PCO was complex and intriguing because it affected both physical adsorption and photocatalytic oxidation. In general, increasing RH caused a decrease in adsorption capacity for ethanol and reduced the mineralization efficiency with a concomitant higher acetaldehyde evolution rate. The effect of RH was less profound than that of photon flux.

Levine, Lanfang H.↗