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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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48 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Validation of energetic particle transport models for time-dependent integrated simulations of burning plasmas (Final ST Report)

The major goal of this project is to deliver a suite of validated energetic particle (EP) modeling tools for time-dependent integrated tokamak simulations (with the code TRANSP) that can be used for modeling plasma discharges featuring a substantial EP content, such as burning plasmas. During FY20, issues were resolved with an energetic particle transport model called TGLF-EP, with improvements made to the TGLF-EP workflow, generation of input files, and interpretation of runs on the NERSC supercomputing cluster. The recipient also gave input on simulations with the code TRANSP to reproduce the reference JET discharge, and assessed the accuracy and uncertainties of the simulated B field, current evolution, thermal plasma profiles, stored energy, etc. Input was also given on interpretation of fast-ion instability calculations and recommendations for modifications to JET afterglow discharge for the upcoming DT campaign.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

2D-imaging of absolute OH and H 2 O 2 profiles in a He–H 2 O nanosecond pulsed dielectric barrier discharge by photo-fragmentation laser-induced fluorescence

We report pulsed dielectric barrier discharges (DBD) in He–H 2 O and He–H 2 O–O 2 mixtures are studied in near atmospheric conditions using temporally and spatially resolved quantitative 2D imaging of the hydroxyl radical (OH) and hydrogen peroxide (H 2 O 2 ). The primary goal was to detect and quantify the production of these strongly oxidative species in water-laden helium discharges in a DBD jet configuration, which is of interest for biomedical applications such as disinfection of surfaces and treatment of biological samples. Hydroxyl profiles are obtained by laser-induced fluorescence (LIF) measurements using 282 nm laser excitation. Hydrogen peroxide profiles are measured by photo-fragmentation LIF (PF-LIF), which involves photo-dissociating H 2 O 2 into OH with a 212.8 nm laser sheet and detecting the OH fragments by LIF. The H 2 O 2 profiles are calibrated by measuring PF-LIF profiles in a reference mixture of He seeded with a known amount of H 2 O 2 . OH profiles are calibrated by measuring OH-radical decay times and comparing these with predictions from a chemical kinetics model. Two different burst discharge modes with five and ten pulses per burst are studied, both with a burst repetition rate of 50 Hz. In both cases, dynamics of OH and H 2 O 2 distributions in the afterglow of the discharge are investigated. Gas temperatures determined from the OH-LIF spectra indicate that gas heating due to the plasma is insignificant. The addition of 5% O 2 in the He admixture decreases the OH densities and increases the H 2 O 2 densities. The increased coupled energy in the ten-pulse discharge increases OH and H 2 O 2 mole fractions, except for the H 2 O 2 in the He–H 2 O–O 2 mixture which is relatively insensitive to the additional pulses.

hydrogen peroxide↗
DOE OSTI2022

Origin of Intense Electron Heating in Relativistic Blast Waves

The modeling of gamma-ray burst afterglow emission bears witness to strong electron heating in the precursor of Weibel-mediated, relativistic collisionless shock waves propagating in unmagnetized electron–ion plasmas. In this Letter, we propose a theoretical model, which describes electron heating via a Joule-like process caused by pitch-angle scattering in the decelerating, self-induced microturbulence and the coherent charge-separation field induced by the difference in inertia between electrons and ions. The emergence of this electric field across the precursor of electron–ion shocks is confirmed by large-scale particle-in-cell (PIC) simulations. Integrating the model using a Monte Carlo-Poisson method, we compare the main observables to the PIC simulations to conclude that the above mechanism can indeed account for the bulk of electron heating.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Ion fluxes and memory effects in an Ar–O 2 modulated radiofrequency-driven atmospheric pressure plasma jet

In this work we used molecular beam mass spectrometry to characterize ion fluxes produced by a modulated radiofrequency (RF)-driven atmospheric pressure plasma jet operating in a homogeneous gas environment (Ar + 1% O 2 ). The influence of the RF modulation frequency (100 Hz to 20 kHz) on the ion fluxes was investigated by time-resolved measurements, and the lifetimes of the dominant ions, O 2 + , NO + , O − , O 2 − and O 3 − , were found to be 28 ± 2, 117 ± 8, 7.3 ± 0.4, 17 ± 1 and 23 ± 2 μs, respectively. The absolute ion densities in the near afterglow region were found to be of the order of 1011 cm−3. Significant differences in the dynamics of the positive and negative ions were found; these are explained by the presence of electrons at similar densities in the afterglow produced by electron detachment reactions from negative ions due to the large concentrations of atomic oxygen and singlet delta oxygen. Transitions in ion flux dynamics for different modulation frequencies and at the startup of the plasma were analyzed together with intensified charge coupled device images recording the plasma propagation in order to assess the dynamics of plasma plume propagation and how it is impacted by ‘memory effects’. Quantitative measurements of the ion densities enabling these memory effects are reported. The results in this paper highlight the tremendous impact of memory effects on plasma propagation and the corresponding pre-ionization.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Time-resolved measurements of HO 2 radical in a heated plasma flow reactor

Time-resolved, absolute HO 2 number density in diluted H 2 –O 2 –Ar, CH 4 –O 2 -Ar, and C 2 H 4 –O 2 –Ar mixtures excited by a repetitive ns pulse discharge in a heated plasma flow reactor is measured by Cavity Ringdown Spectroscopy (CRDS). The experimental results are obtained at $\textit{T}$ = 300-600 K and $\textit{P}$ = 130 Torr, both during the discharge pulse burst and in the afterglow. In this work, the HO 2 number density is inferred from the CRDS data using a spectral model exhibiting good agreement with previous measurements of absolute HO 2 absorption cross sections. In the room-temperature H 2 –O 2 mixture, as well as in CH 4 –O 2 and C 2 H 4 –O 2 mixtures over the entire temperature range studied, HO2 is generated only during the discharge burst and decays in the afterglow. However, in the H 2 –O 2 mixture at elevated temperatures, $\textit{T}$ = 400-600 K, HO 2 persists in the afterglow up to 10 ms after the discharge burst, comparable with the flow residence time in the reactor. Comparison with kinetic modeling shows that the sustained reactivity after the source of radicals is turned off is due to a chain propagation / hydrogen oxidation process, which dominates the radical recombination reactions. The kinetic modeling predictions are in good agreement with the relative HO 2 number density measured in all three mixtures, although the model underpredicts the absolute number densities in H 2 –O 2 at $\textit{T}$ = 400-600 K by up to a factor of two. Detection of the sustained low-temperature reactivity in H 2 –O 2 , initiated by the radical generation in the plasma, suggests that the plasma excitation may also affect kinetics of oxidation and reforming of fuels exhibiting low-temperature chemistry below hot ignition point.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Measurements of atoms and metastable species in N 2 and H 2 –N 2 nanosecond pulse plasmas

We report time-resolved, absolute number densities of metastable N 2 (A 3 Σ u + , v = 0, 1) molecules, ground state N 2 and H atoms, and rotational–translational temperature have been measured by tunable diode laser absorption spectroscopy and two-photon absorption laser-induced fluorescence in diffuse N 2 and N 2 –H 2 plasmas during and after a nanosecond pulse discharge burst. Comparison of the measurement results with the kinetic modeling predictions, specifically the significant reduction of the N 2 (A 3 Σ u + ) populations and the rate of N atom generation during the burst, suggests that these two trends are related. The slow N atom decay in the afterglow, on a time scale longer than the discharge burst, demonstrates that the latter trend is not affected by N atom recombination, diffusion to the walls, or convection with the flow. This leads to the conclusion that the energy pooling in collisions of N 2 (A 3 Σ u + ) molecules is a major channel of N 2 dissociation in electric discharges where a significant fraction of the input energy goes to electronic excitation of N 2 . Additional measurements in a 1% H 2 –N 2 mixture demonstrate a further significant reduction of N 2 (A 3 Σ u + , v = 0, 1) populations, due to the rapid quenching by H atoms accumulating in the plasma. Comparison with the modeling predictions suggests that the N 2 (A 3 Σ u + ) molecules may be initially formed in the highly vibrationally excited states. The reduction of the N 2 (A 3 Σ u + ) number density also diminishes the contribution of the energy pooling process into N2 dissociation, thus reducing the N atom number density. The rate of N atom generation during the burst also decreases, due to its strong coupling to N 2 (A 3 Σ u + , v) populations. On the other hand, the rate of H atom generation, produced predominantly by the dissociative quenching of the excited electronic states of N 2 by H 2 , remains about the same during the burst, resulting in a nearly linear rise in the H atom number density. Comparison of the kinetic model predictions with the experimental results suggests that the yield of H atoms during the quenching of the excited electronic state of N 2 by molecular H 2 is significantly less than 100%. The present results quantify the yield of N and H atoms in high-pressure H 2 –N 2 plasmas, which have significant potential for ammonia generation using plasma-assisted catalysis

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Microphysics of Relativistic Collisionless Electron-ion-positron Shocks

Abstract We perform particle-in-cell simulations to elucidate the microphysics of relativistic weakly magnetized shocks loaded with electron-positron pairs. Various external magnetizations σ ≲ 10 −4 and pair-loading factors Z ± ≲ 10 are studied, where Z ± is the number of loaded electrons and positrons per ion. We find the following: (1) The shock becomes mediated by the ion Larmor gyration in the mean field when σ exceeds a critical value σ L that decreases with Z ± . At σ ≲ σ L the shock is mediated by particle scattering in the self-generated microturbulent fields, the strength and scale of which decrease with Z ± , leading to lower σ L . (2) The energy fraction carried by the post-shock pairs is robustly in the range between 20% and 50% of the upstream ion energy. The mean energy per post-shock electron scales as E ¯ e ∝ Z ± + 1 − 1 . (3) Pair loading suppresses nonthermal ion acceleration at magnetizations as low as σ ≈ 5 × 10 −6 . The ions then become essentially thermal with mean energy E ¯ i , while electrons form a nonthermal tail, extending from E ∼ Z ± + 1 − 1 E ¯ i to E ¯ i . When σ = 0, particle acceleration is enhanced by the formation of intense magnetic cavities that populate the precursor during the late stages of shock evolution. Here, the maximum energy of the nonthermal ions and electrons keeps growing over the duration of the simulation. Alongside the simulations, we develop theoretical estimates consistent with the numerical results. Our findings have important implications for models of early gamma-ray burst afterglows.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Modeling of the effects of non-equilibrium excitation and electrode geometry on H 2 /air ignition in a nanosecond plasma discharge

In this work, we present the results of two-dimensional modeling of the effects of non-equilibrium excitation and electrode geometry on H 2 /air ignition in a nanosecond plasma discharge. A multiscale adaptive reduced chemistry solver for plasma assisted combustion (MARCS-PAC) based on PASSKEy discharge modeling package and compressible multi-component reactive flow solver ASURF+ is developed and validated. This model is applied to simulate the impact of non-equilibrium plasma excitation and electrode geometry and heat loss on the dynamics of the discharge from streamer to spark and ignition kernel development in a H 2 /air mixture with a pair of cylindrical electrodes. The results show that the plasmagenerated species (N 2 (A), N 2 (B), N 2 (a'), N 2 (C), O( 1 D), O and H) in the spark and afterglow significantly accelerate the ignition kernel development. The increase of discharge voltage at the same total discharge energy promotes the non-equilibrium active species production. It is found that the production of electronically excited species at higher reduced electric field strength is more efficient in enhancing ignition in comparison to the vibrational excitation and heating. Moreover, the 2D simulation clearly reveals that the electric field and active species distribution are highly non-uniform. The streamers are initiated at the sharp outer edges of the negative and positive electrodes by a strong electric field while the electric field is much weaker at the centerline of the electrodes. Furthermore, the simulations reveal that the ignition enhancement is sensitive to the variation of electrode shape, diameter, and gap size due to the changes of electric field distribution and location of streamer formation. A cylindrical electrode produces a larger discharge volume and ignition kernel than the parabolic and spherical electrodes, when the discharge is localized near the axis of the gap. It is found that there is a non-monotonic dependence of ignition kernel size on the electrode diameter and inter-electrode distance. The increase of electrode diameter and gap size above the optimal conditions leads to the reduction of ignition kernel volume, due to the decrease of active species concentration and gas temperature. At a larger electrode surface area and electrode diameter as well as smaller electrode gap size, the heat loss to electrode plays a greater role in reducing the ignition kernel size and slowing ignition kernel development. This work provides insights and guidance to understand the kinetic enhancement of non-equilibrium plasma and the effects of electrode geometries on ignition for the optimization ignitors in advanced engines.

42 ENGINEERING↗
DOE OSTI2020

A computational study of the thermodynamic conditions leading to autoignition in nanosecond pulsed discharges

Nanosecond pulsed discharges have attracted the attention of engine manufacturers due to the possibility of attaining distributed ignition sites that accelerate burn rates while resulting in very little electrode erosion. Multidimensional modeling tools currently capture the electrical structure of such discharges accurately, but resolving the chemical structure remains a challenging problem owing to the disparity of time-scales in streamer propagation (nanoseconds) and ignition phenomena (microseconds). The purpose of this study is to extend multidimensional results towards resolving the chemical structure in the wake of streamers (or the afterglow) by using a batch reactor model. This can afford the use of very detailed chemical kinetic information. The full non-equilibrium nature of the electrons is taken into account, along with fast gas heating, shock wave propagation, and thermal diffusion. The results shed light on ignition phenomena brought about by such discharges.

ignition, plasma, kinetics↗
DOE OSTI2024

Long-term Evolution of Relativistic Unmagnetized Collisionless Shocks

Abstract We study a relativistic collisionless electron–positron shock propagating into an unmagnetized ambient medium using 2D particle-in-cell simulations of unprecedented duration and size. The shock generates intermittent magnetic structures of increasingly larger size as the simulation progresses. Toward the end of our simulation, at around 26,000 plasma times, the magnetic coherence scale approaches λ ∼ 100 plasma skin depths, both ahead and behind the shock front. We anticipate a continued growth of λ beyond the time span of our simulation, as long as the shock accelerates particles to increasingly higher energies. The post-shock field is concentrated in localized patches, which maintain a local magnetic energy fraction ε B ∼ 0.1. Particles randomly sampling the downstream fields spend most of their time in low field regions ( ε B ≪ 0.1) but emit a large fraction of the synchrotron power in the localized patches with strong fields ( ε B ∼ 0.1). Our results have important implications for models of gamma-ray burst afterglows.

Astronomy & Astrophysics↗
DOE OSTI2021

A Computational Study of the Thermodynamic Conditions Leading to Autoignition in Nanosecond Pulsed Discharges

Nanosecond pulsed discharges have attracted the attention of engine manufacturers due to the possibility of attaining distributed ignition sites that accelerate burn rates while resulting in very little electrode erosion. Multidimensional modeling tools currently capture the electrical structure of such discharges accurately, but resolving the chemical structure remains a challenging problem owing to the disparity of time-scales in streamer propagation (nanoseconds) and ignition phenomena (microseconds). The purpose of this study is to extend multidimensional results toward resolving the chemical structure in the wake of streamers (or the afterglow) by using a batch reactor model (BRM). This can afford the use of very detailed chemical kinetic information. The full nonequilibrium nature of the electrons is taken into account, along with fast gas heating, shock wave propagation, and thermal diffusion. The results shed light on ignition phenomena brought about by such discharges.

42 ENGINEERING↗
DOE OSTI2022

Emission phases of implosion sources for x-ray absorption fine structure spectroscopy

At the Laboratory for Laser Energetics' Omega Laser Facility, thin plastic shells were directly driven with ∼20 kJ resulting in a time-integrated x-ray yield of ∼1012 ph/eV/sr at 7 keV. Using temporally, spatially, and spectrally discriminating diagnostics, three x-ray emission phases were identified: corona emission produced by the laser ablation of the shell, core stagnation, and afterglow emission due to the expanding hot material after stagnation. The newly measured corona and afterglow emission phases account for ∼25% of the total x-ray signal and produce x-ray emission at a different time or larger radius than previously considered. The resulting implications of this additional emission for x-ray absorption fine structure spectroscopy are discussed. Finally, improvements to the laser drive intensity and uniformity produced a factor-of-2 increase in total x-ray emission while decreasing the size of the stagnated core.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗