Search NASA⌕ Search

SEARCH · Search NASA

Results for “positron annihilation”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
NASA NTRS1973

Positron annihilation radiation from neutron stars

Balloon observations of a low energy flux line at 2 x 0.001 photons cm/2 s/1 from the galactic center region around 470 keV are interpreted as the positron annihilation radiation that occurs on the surface of old neutron stars and is redshifted by their gravitational fields. An astrophysical model is formulated to explain the observed flux that provides for about 0.2 neutron stars per 3 x 10 to the 49th power cubic meters assuming that the disk thickness is about 1.5 x 10 to the 19th power meters.

Borner, G. A.↗
NASA NTRS1978

Detection of 511 keV positron annihilation radiation from the galactic center direction

A balloon-borne gamma ray telescope with an approximately 130 cu cm high purity germanium detector was flown over Australia to detect sharp spectral features from the galactic center direction. A 511 keV positron annihilation line was observed at a flux level of (1.21 plus or minus 0.22) x (10/cu cm) photons/sec/sp cm. Suggestive evidence for the detection of the three-photon positronium continuum is presented. The possible origin of the positrons is discussed.

Leventhal, M.↗
NASA NTRS1984

Search for 511 keV electron-positron annihilation radiation from mildly active galaxies using the HEAO 3 gamma-ray spectrometer

The HEAO 3 spacecraft's gamma-ray spectrometer has been used to obtain upper limits to the 511-keV electron-positron annihilation line flux from seven galaxies: M 81/M 82, NGC 4278, M 104, NGC 6500, NGC 2911, and NGC 262. These appear to contain scaled-up versions of the radio source in the galactic center, and their nonthermal activity appears to be confined to the central regions, implying that energetic particles produced in these nuclei do not escape into the low density regions of interstellar or intergalactic space. On the basis of the scaling law adopted, six of these seven galaxies should have been detected above the upper limits obtained for narrow 511 keV emission. Explanations are adduced which account for the scaling law's failure to predict the correct level of radiation annihilation.

Marscher, A. P.↗
NASA NTRS1994

Morphology of Thermoset Polyimides by Positron Annihilation Spectroscopy

Thermoset polyimides have great potential for successfully meeting tough stress and temperature challenges in the advanced aircraft development program. However, studies of structure/property relationships in these materials have not been very successful so far. Positron annihilation spectroscopy has been used to investigate free volumes and associated parameters. It has been noted that the free volume correlates well with the molecular weight, cross-link density and thermal coefficient of expansion of these materials. Currently no other techniques are available for direct measurement of these parameters. Experimental results and their interpretations will be discussed.

Ranganathaiah, C.↗
NASA NTRS1984

Effect of metal ions on positron annihilation characteristics in metal ion containing epoxies

In the course of developing improved moisture-resistant epoxy resins, two different types of epoxy resins containing variable mole ratios of chromium ions per polymer repeat unit were developed. Positron annihilation characteristics have been investigated in these resins as a function of their metal ion content. In both cases, the presence of metal ions reduces the lifetime as well as the intensity of the long life component. The long life component intensity reduction is considerably more pronounced than the lifetime reduction. These results have been discussed in terms of increased unpaired electron density at Ps formation sites due to the presence of chromium ions in the matrix.

Singh, J. J.↗
NASA NTRS1990

Fatigue damage in superalloys determined using Doppler broadening positron annihilation

Axial fatigue specimens of three superalloys, Inconel 718, Incoloy 903 and Haynes 188, were machined from solution-heat-treated material and artificially aged. They were subjected to cyclic loading for a selected number of cycles after which the S parameter was determined using Doppler broadening positron annihilation. Initially, the S parameter decreased, followed by a large increase and a subsequent decline leading to fracture. This has been interpreted as the removal of residual vacancies, the introduction of new defects by cyclic loading, and, finally, a clustering of the defects as microcracks which grow to cause failure.

Hoeckelman, Donald↗
DOE OSTI2024

Dynamic Scaling Analysis of Accelerated Irradiation Testing on Additive Manufacturing Materials by Positron Annihilation

The timely applications of Additive Manufacturing (AM) materials in nuclear environments require accelerated irradiation tests, mainly ion irradiation to enable rapid prototyping. Low dose ion irradiation would cause sub-nanostructure changes by generation of lattice defects, vacancies, vacancy clusters and voids and void swelling caused by cellular dislocations. Positron Annihilation Lifetime (PAL), a novel technology, sensitive towards sub-nanostructure morphology with high accuracy (about 10-7 vacancy per atom), supported by Transition Electron Microscope (TEM) would be applied to identify the type and total size of the defects. The subsequent PAL measurements and TEM surface studies would be followed by PAL analysis that includes sophisticated trapping model. The PAS results would become an input to dynamic scaling analysis (that predicts radiation effects from low dose studies for high dose effects), which incorporate mean-field theory model. The final effect is an in-depth understanding of the microstructure evolution of AM materials under ion irradiation which can be extrapolated to the studies of neutron irradiation, since ion-irradiation takes less time and do not cause the irradiation hazard. The working hypothesis is that PAL technology, that have excellent sensitivity to low-defect concentration would help to identify ion-induced material damage on the atomic and nano-scale level, which then could be extrapolated to understand the neutron damage better.

accelerated irradiation testing↗
NASA NTRS2005

INTEGRAL/SPI Observations of Electron-Positron Annihilation Radiation from our Galaxy

The spectrometer on INTEGRAL (SPI) is a coded-aperture gamma-ray telescope with moderate angular resolution (3 deg) and superior energy resolution (2 keV at 511 kev). One of it's principal science goals is the detailed study of 511 keV electron-positron annihilation from our Galaxy. The origin of this radiation remains a mystery, however current morphological studies suggest an older stellar population. There has also been recent speculation on the possibility of the existence of light (< 100 MeV) dark matter particles whose annihilation or decay could produce the observed 511 keV emission. In this paper we summarize the current results from SPI, compare them with previous results and discuss their implication on possible models for the production of the annihilation radiation.

Teegarden, B. J.↗
DOE OSTI2020

Defect accommodation in off-stoichiometric (SrTiO 3 ) n SrO Ruddlesden–Popper superlattices studied with positron annihilation spectroscopy

he low dielectric loss underlying the record performance of strained (SrTiO 3 ) n SrO Ruddlesden–Popper films as tunable microwave dielectrics was postulated to arise from (SrO) 2 faults accommodating local non-stoichiometric defects. Here, we explore the effect of non-stoichiometry on (SrTiO 3 ) n SrO using positron annihilation lifetime spectroscopy on a composition series of 300 nm thick n = 6 (Sr 1+δ TiO 3 ) n SrO thin films. These films show titanium-site vacancies across the stoichiometry series, with evidence that TiO x vacancy complexes dominate. Little change in defect populations is observed across the series, indicating the ability of Ruddlesden–Popper phases to accommodate ± 5% off-stoichiometry. This ability for defect accommodation is corroborated by scanning transmission electron microscopy with electron energy loss spectroscopy.

Physics↗
NASA NTRS1991

GRIS observations of positron annihilation radiation from the Galactic center

In the present Gamma-Ray Imaging Spectrometer (GRIS) observations, the 511 keV line has been spectrally resolved and the Galactic plane and center components have been independently measured. These data, in combination with those from other narrow-field observations in the 1980s, support the two-component model of the positron annihilation source. A strong hard-X-ray continuum was detected in the Galactic plane observation; this 'diffuse' continuum component solves the mystery as to why wide-field instruments have detected such high continuum emission from the Galactic center, in virtue of its source contributions.

Gehrels, N.↗
NASA NTRS1973

Positron-annihilation radiation from neutron stars.

Matter accreted on the surfaces of neutron stars consists of energetic particles of a few tens to one or two hundred MeV per nucleon, depending on the neutron-star mass. In addition to heat, such particles produce nuclear reactions with the surface material. It is proposed that the recently observed 473 plus or minus 30 keV spectral feature from the galactic center is gravitationally redshifted positron-annihilation radiation produced at the surfaces of neutron stars. The principal observational tests of the model would be the detection of nuclear gamma-ray lines from the galactic center.

Ramaty, R.↗
DOE OSTI2022

Identifying Redox Orbitals and Defects in Lithium-Ion Cathodes with Compton Scattering and Positron Annihilation Spectroscopies: A Review

Reduction-oxidation (redox) reactions that transfer conduction electrons from the anode to the cathode are the fundamental processes responsible for generating power in Li-ion batteries. Electronic and microstructural features of the cathode material are controlled by the nature of the redox orbitals and how they respond to Li intercalation. Thus, redox orbitals play a key role in performance of the battery and its degradation with cycling. We unravel spectroscopic descriptors that can be used to gain an atomic-scale handle on the redox mechanisms underlying Li-ion batteries. Our focus is on X-ray Compton Scattering and Positron Annihilation spectroscopies and the related computational approaches for the purpose of identifying orbitals involved in electrochemical transformations in the cathode. This review provides insight into the workings of lithium-ion batteries and opens a pathway for rational design of next-generation battery materials.

Nokelainen, Johannes (ORCID:0000000328857850)↗
DOE OSTI2020

Positron annihilation lifetime spectroscopy study of polyvinylpyrrolidone‐added polyvinylidene fluoride membranes: Investigation of free volume and permeation relationships

ABSTRACT Polyvinylidene fluoride (PVDF) membranes were prepared via the phase inversion method from casting solutions containing PVDF, dimethylformamide (DMF), and polyvinylpyrrolidone (PVP) as pore former. PVP was used in the casting solution in a range of 0–5 wt % and extracted. The effect on membranes of using PVP in the casting process was analyzed by X‐ray diffraction, differential scanning calorimetry, scanning electron microscopy, viscosity, and water permeability techniques. With an increase of PVP from 0 to 5 wt %, the PVDF casting solution viscosities increased from 858 to 1148 cP; the resulting PVDF membrane thickness increased; and the crystallinity of PVDF membranes decreased from 40.0 to 33.3%, which indicates that the addition of PVP inhibits the degree of crystallization in the PVDF membranes. SEM results revealed the shape and size of macropores in the membranes; these macropores changed after PVP addition to the casting solutions. The impact of structural changes on free‐volume properties was evaluated using positron annihilation lifetime spectroscopy (PALS) studies. PALS analysis indicated no effect on the average radius (~3.4 Å) of membrane free‐volume holes from the addition of PVP to the casting solution. However, the percentage of o ‐Ps pick‐off annihilation intensity, I 3 , increased from 1.7 to 5.1% with increased PVP content. Further, increasing the PVP content from 0.5 to 5% resulted in an increased final pure water permeability flux. For instance, the 210 min flux for a 14% PVDF + 0.5% PVP membrane was found to be 3.3 times greater than a control membrane having the same PVDF concentration. © 2020 Wiley Periodicals, Inc. J. Polym. Sci. 2020 , 58 , 589–598

Eren, Bilge↗
NASA NTRS2008

Asymmetric 511 keV Positron Annihilation Line Emission from the Inner Galactic Disk

A recently reported asymmetry in the 511 keV gamma-ray line emission from the inner galactic disk is unexpected and mimics an equally unexpected one in the distribution of LMXBs seen at hard X-ray energies. A possible conclusion is that LMXBs are an important source of the positrons whose annihilation gives rise to the line. We will discuss these results, their statistical significance and that of any link between the two. The implication of any association between LMXBs and positrons for the strong annihilation radiation from the galactic bulge will be reviewed.

Skinner, Gerry↗
NASA NTRS2005

INTEGRAL/SPI Limits on Electron-Positron Annihilation Radiation from the Galactic Plane

The center of our Galaxy is a known strong source of electron-positron 511- keV annihilation radiation. Thus far, however, there have been no reliable detections of annihilation radiation outside of the central radian of our Galaxy. One of the primary objectives of the INTEGRAL (INTErnational Gamma-RAy Astrophysics Laboratory) mission, launched in Oct. 2002, is the detailed study of this radiation. The Spectrometer on INTEGRAL (SPI) is a high resolution coded-aperture gamma-ray telescope with an unprecedented combination of sensitivity, angular resolution and energy resolution. We report results from the first 10 months of observation. During this period a significant fraction of the observing time was spent in or near the Galactic Plane. No positive annihilation flux was detected outside of the central region (|l| greater than 40 degrees) of our Galaxy. In this paper we describe the observations and data analysis methods and give limits on the 511-keV flux.

Teegarden, B. J.↗
NASA NTRS1987

Positron annihilation at the Galactic center

The efficiency of production of positrons by gamma-gamma interaction under conditions which may occur in the Galactic center. Their annihilation line and three-photon annihilation continuum contribute to the emitted radiation. If a geometrical model is assumed, it will be possible to determine the parameters of the gamma-ray source region. By comparing the computed spectra to observations, a rough estimate is made using extant data.

Carrigan, B. J.↗