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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Abundant ammonia and nitrogen-rich soluble organic matter in samples from asteroid (101955) Bennu

Organic matter in meteorites reveals clues about early Solar System chemistry and the origin of molecules important to life, but terrestrial exposure complicates interpretation. Samples returned from the B-type asteroid Bennu by the Origins, Spectral Interpretation, Resource Identification, and Security–Regolith Explorer mission enabled us to study pristine carbonaceous astromaterial without uncontrolled exposure to Earth’s biosphere. Here we show that Bennu samples are volatile rich, with more carbon, nitrogen and ammonia than samples from asteroid Ryugu and most meteorites. Nitrogen-15 isotopic enrichments indicate that ammonia and other N-containing soluble molecules formed in a cold molecular cloud or the outer protoplanetary disk. We detected amino acids (including 14 of the 20 used in terrestrial biology), amines, formaldehyde, carboxylic acids, polycyclic aromatic hydrocarbons and N-heterocycles (including all five nucleobases found in DNA and RNA), along with ~10,000 N-bearing chemical species. All chiral non-protein amino acids were racemic or nearly so, implying that terrestrial life’s left-handed chirality may not be due to bias in prebiotic molecules delivered by impacts. The relative abundances of amino acids and other soluble organics suggest formation and alteration by low-temperature reactions, possibly in NH 3 -rich fluids. Bennu’s parent asteroid developed in or accreted ices from a reservoir in the outer Solar System where ammonia ice was stable.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2025

Building wet planets through high-pressure magma–hydrogen reactions

Close-in transiting sub-Neptunes are abundant in our Galaxy. Planetary interior models based on their observed radius–mass relationship suggest that sub-Neptunes contain a discernible amount of either hydrogen (dry planets) or water (wet planets) blanketing a core composed of rocks and metal. Water-rich sub-Neptunes have been believed to form farther from the star and then migrate inwards to their present orbits. Here we report experimental evidence of reactions between warm, dense hydrogen fluid and silicate melt that release silicon from the magma to form alloys and hydrides at high pressures. We found that oxygen liberated from the silicate melt reacts with hydrogen, producing an appreciable amount of water up to a few tens of weight per cent, which is much greater than previously predicted based on low-pressure ideal gas extrapolation. Consequently, these reactions can generate a spectrum of water contents in hydrogen-rich planets, with the potential to reach water-rich compositions for some sub-Neptunes, implying an evolutionary relationship between hydrogen-rich and water-rich planets. Therefore, detection of a large amount of water in exoplanet atmospheres may not be the optimal evidence for planet migration in the protoplanetary disk, calling into question the assumed link between composition and planet formation location.

Horn, H. W. [Arizona State University, Tempe, AZ (↗
DOE OSTI2020

Molecular growth upon ionization of van der Waals clusters containing HCCH and HCN is a pathway to prebiotic molecules

The growth mechanisms of organic molecules in an ionizing environment such as the interstellar medium are not completely understood. Here we examine by means of ab initio molecular dynamics (AIMD) simulations and density functional theory (DFT) computations the possibility of bond formation and molecular growth upon ionization of van der Waals clusters of pure HCN clusters, and mixed clusters of HCN and HCCH, both of which are widespread in the interstellar medium. Ionization of van der Waals clusters can potentially lead to growth in low temperature and low-density environments. Our results show, that upon ionization of the pure HCN clusters, strongly bound stable structures are formed that contain N∙∙∙H bonds, and growth beyond pairwise HCN molecules is seen only in a small percentage of cases. In contrast, mixed clusters, where HCCH is preferentially ionized over HCN, can grow up to 3 or 4 units long with new carbon–carbon and carbon–nitrogen covalent bonds. Moreover, cyclic molecules formed, such as the radical cation of pyridine, which is a prebiotic molecule. The results presented here are significant as they provide a feasible pathway for molecular growth of small organic molecules containing both carbon and nitrogen in cold and relatively denser environments such as in dense molecular clouds but closer to the photo-dissociation regions, and protoplanetary disks. In the mechanism we propose, first, a neutral van der Waals cluster is formed. Once the cluster is formed it can undergo photoionization which leads to chemical reactivity without any reaction barrier.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

The formation and structure of iron-dominated planetesimals

Metal-rich asteroids and iron meteorites are considered core remnants of differentiated planetesimals and/or products of oxygen-depleted accretion. Investigating the origins of iron-rich planetesimals could provide key insights into planet formation mechanisms. Using differentiation models, we evaluate the interior structure and composition of representative-sized planetesimals (~200 km diameter), while varying oxygen fugacity and initial bulk meteoritic composition. Under the oxygen-poor conditions that likely existed early in the inner regions of the Solar System and other protoplanetary disks, core fractions remain relatively consistent across a range of bulk compositions (CI, H, EH, and CBa). Some of these cores could incorporate significant amounts of silicon (10–30 weight%) and explain the metal fractions of Fe-rich bodies in the absence of mantle stripping. Conversely, planetesimals forming under more oxidizing conditions, such as beyond snow lines, could exhibit smaller cores, enriched in carbon, sulfur (>1 wt%), and oxides. Sulfur-rich cores, like those formed from EH and H bulk compositions, could remain partly molten, sustain dynamos, and even drive sulfur-rich volcanism. Additionally, bodies with high carbon contents, such as CI compositions, can form graphitic outer layers. These variations highlight the importance of initial formation conditions in shaping planetesimal structures. Future missions, such as NASA’s Psyche mission, offer an opportunity to measure the relative abundances of key elements (Fe, Ni, Si, and S) necessary to distinguish among formation scenarios and structure models for Fe-rich and reduced planetesimals.

meteorites↗
DOE OSTI2021

Fossil records of early solar irradiation and cosmolocation of the CAI factory: A reappraisal

Calcium-aluminum–rich inclusions (CAIs) in meteorites carry crucial information about the environmental conditions of the nascent Solar System prior to planet formation. Based on models of 50V– 10 Be co-production by in-situ irradiation, CAIs are considered to have formed within ~0.1 AU from the proto-Sun. Here, we present vanadium (V) and strontium (Sr) isotopic co-variations in fine- and coarse-grained CAIs and demonstrate that kinetic isotope effects during partial condensation and evaporation best explain V isotope anomalies previously attributed to solar particle irradiation. We also report initial excesses of 10 Be and argue that CV CAIs possess essentially a homogeneous level of 10 Be, inherited during their formation. Based on numerical modeling of 50V–10Be co-production by irradiation, we show that CAI formation during protoplanetary disk build-up likely occurred at greater heliocentric distances than previously considered, up to planet-forming regions (~1AU), where solar particle fluxes were sufficiently low to avoid substantial in-situ irradiation of CAIs.

58 GEOSCIENCES↗
DOE OSTI2022

Ryugu's nucleosynthetic heritage from the outskirts of the Solar System

Little is known about the origin of the spectral diversity of asteroids and what it says about conditions in the protoplanetary disk. Here we show that samples returned from Cb­type asteroid Ryugu have Fe isotopic anomalies indistinguishable from Ivuna­type (CI) chondrites, which are distinct from all other carbonaceous chondrites. Iron isotopes, therefore, demonstrate that Ryugu and CI chondrites formed in a reservoir that was different from the source regions of other carbonaceous asteroids. Growth and migration of the giant planets destabilized nearby planetesimals and ejected some inwards to be implanted into the Main Belt. In this framework, most carbonaceous chondrites may have originated from regions around the birthplaces of Jupiter and Saturn, while the distinct isotopic composition of CI chondrites and Ryugu may reflect their formation further away in the disk, owing their presence in the inner Solar System to excitation by Uranus and Neptune

58 GEOSCIENCES↗
DOE OSTI2022

Oxygen isotopes of anhydrous primary minerals show kinship between asteroid Ryugu and comet 81P/Wild2

The extraterrestrial materials returned from asteroid (162173) Ryugu consist predominantly of low-temperature aqueously formed secondary minerals and are chemically and mineralogically similar to CI (Ivuna-type) carbonaceous chondrites. Here, we show that high-temperature anhydrous primary minerals in Ryugu and CI chondrites exhibit a bimodal distribution of oxygen isotopic compositions: 16 O-rich (associated with refractory inclusions) and 16 O-poor (associated with chondrules). Both the 16 O-rich and 16 O-poor minerals probably formed in the inner solar protoplanetary disk and were subsequently transported outward. The abundance ratios of the 16 O-rich to 16 O-poor minerals in Ryugu and CI chondrites are higher than in other carbonaceous chondrite groups but are similar to that of comet 81P/Wild2, suggesting that Ryugu and CI chondrites accreted in the outer Solar System closer to the accretion region of comets.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Astronomical context of Solar System formation from molybdenum isotopes in meteorite inclusions

Calcium-aluminum–rich inclusions (CAIs) in meteorites are the first solids to have formed in the Solar System, defining the epoch of its birth on an absolute time scale. This provides a link between astronomical observations of star formation and cosmochemical studies of Solar System formation. We show that the distinct molybdenum isotopic compositions of CAIs cover almost the entire compositional range of material that formed in the protoplanetary disk. We propose that CAIs formed while the Sun was in transition from the protostellar to pre–main sequence (T Tauri) phase of star formation, placing Solar System formation within an astronomical context. Our results imply that the bulk of the material that formed the Sun and Solar System accreted within the CAI-forming epoch, which lasted less than 200,000 years.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

HD 191939: Three Sub-Neptunes Transiting a Sun-like Star Only 54 pc Away

We present the discovery of three sub-Neptune-sized planets transiting the nearby and bright Sun-like star HD 191939 (TIC 269701147, TOI 1339), a K {sub s} = 7.18 mag G8 V dwarf at a distance of only 54 pc. We validate the planetary nature of the transit signals by combining 5 months of data from the Transiting Exoplanet Survey Satellite with follow-up ground-based photometry, archival optical images, radial velocities, and high angular resolution observations. The three sub-Neptunes have similar radii (R{sub b}=3.42{sub −0.11}{sup +0.11}, R{sub c}=3.23{sub −0.11}{sup +0.11}, and R{sub d}=3.16{sub −0.11}{sup +0.11} R{sub ⊕}), and their orbits are consistent with a stable, circular, and coplanar architecture near mean-motion resonances of 1:3 and 3:4 (P {sub b} = 8.88, P {sub c} = 28.58, and P {sub d} = 38.35 days). The HD 191939 system is an excellent candidate for precise mass determinations of the planets with high-resolution spectroscopy due to the host star’s brightness and low chromospheric activity. Moreover, the system’s compact and near-resonant nature can provide an independent way to measure planetary masses via transit timing variations while also enabling dynamical and evolutionary studies. Finally, as a promising target for multiwavelength transmission spectroscopy of all three planets’ atmospheres, HD 191939 can offer valuable insight into multiple sub-Neptunes born from a protoplanetary disk that may have resembled that of the early Sun.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

MIRC-X: A Highly Sensitive Six-telescope Interferometric Imager at the CHARA Array

Michigan InfraRed Combiner-eXeter (MIRC-X) is a new highly sensitive six-telescope interferometric imager installed at the CHARA Array that provides an angular resolution equivalent of up to a 330 m diameter baseline telescope in J- and H-band wavelengths ((λ/(2B))∼0.6 mas). We upgraded the original Michigan InfraRed Combiner (MIRC) instrument to improve sensitivity and wavelength coverage in two phases. First, a revolutionary sub-electron noise and fast-frame-rate C-RED ONE camera based on an SAPHIRA detector was installed. Second, a new-generation beam combiner was designed and commissioned to (i) maximize sensitivity, (ii) extend the wavelength coverage to J band, and (iii) enable polarization observations. A low-latency and fast-frame-rate control software enables high-efficiency observations and fringe tracking for the forthcoming instruments of the CHARA Array. Since mid-2017, MIRC-X has been offered to the community and has demonstrated best-case H-band sensitivity down to 8.2 correlated magnitude. MIRC-X uses single-mode fibers to coherently combine the light from six telescopes simultaneously with an image-plane combination scheme and delivers a visibility precision better than 1%, and closure phase precision better than 1°. MIRC-X aims at (i) imaging protoplanetary disks, (ii) detecting exoplanets with precise astrometry, and (iii) imaging stellar surfaces and starspots at an unprecedented angular resolution in the near-infrared. In this paper, we present the instrument design, installation, operation, and on-sky results, and demonstrate the imaging capability of MIRC-X on the binary system ι Peg. The purpose of this paper is to provide a solid reference for studies based on MIRC-X data and to inspire future instruments in optical interferometry.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2020

Revisiting the Architecture of the KOI-89 System

While high stellar obliquities observed in exoplanetary systems may be attributed to processes that tilt the planetary orbits, it is also possible that they reflect misalignments between protoplanetary disks and stellar spins. This latter hypothesis predicts the presence of coplanar multiplanetary systems misaligned with their central stars. Here we reevaluate the evidence of such an architecture that has been claimed for the KOI-89 system. An early-type star, KOI-89 has one validated transiting planet, KOI-89.01/Kepler-462b (period 84.7 days, radius 3.0 R {sub ⊕}), and one transiting planet candidate, KOI-89.02 (period 207.6 days, radius 4.0 R {sub ⊕}), where the latter exhibits transit timing variations (TTVs). A previous modeling of the stellar gravity-darkening effect in the transit light curves inferred a high stellar obliquity of ≈70°. We perform photodynamical modeling of the Kepler transit light curves and use the resulting constraints on the orbital configuration and transit times to update the gravity-darkened transit model. As a result, we find no firm evidence for the gravity-darkening effect in the transit shapes and conclude that stellar obliquity is not constrained by the data. Given the evidence for low orbital eccentricities from the dynamical analysis, the system architecture can thus be consistent with many other multitransiting systems with flat, near-circular orbits aligned with the stellar spin. We find that the TTVs imparted on its neighbor imply that KOI-89.01 has a mass ≳20 M {sub ⊕}. This would render it one of the densest known sub-Neptunes, mostly composed of a solid core. Lower masses are possible if the TTVs are instead due to an unseen third planet.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

The TW Hya Rosetta Stone Project. I. Radial and Vertical Distributions of DCN and DCO{sup +}

Molecular D/H ratios are frequently used to probe the chemical past of solar system volatiles. Yet it is unclear which parts of the solar nebula hosted an active deuterium fractionation chemistry. To address this question, we present 0."2–0."4 Atacama Large Millimeter/submillimeter Array (ALMA) observations of DCO{sup +} and DCN 2–1, 3–2, and 4–3 toward the nearby protoplanetary disk around TW Hya, taken as part of the TW Hya Rosetta Stone project, augmented with archival data. DCO{sup +} is characterized by an excitation temperature of ~40 K across the 70 au radius pebble disk, indicative of emission from a warm, elevated molecular layer. Tentatively, DCN is present at even higher temperatures. Both DCO{sup +} and DCN present substantial emission cavities in the inner disk, while in the outer disk the DCO{sup +} and DCN morphologies diverge: most DCN emission originates from a narrow ring peaking around 30 au, with some additional diffuse DCN emission present at larger radii, while DCO{sup +} is present in a broad structured ring that extends past the pebble disk. Based on a set of simple parametric disk abundance models, these emission patterns can be explained by a near-constant DCN abundance exterior to the cavity, and an increasing DCO{sup +} abundance with radius. In conclusion, the ALMA observations reveal an active deuterium fractionation chemistry in multiple disk regions around TW Hya, but not in the cold planetesimal-forming midplane and in the inner disk. More observations are needed to explore whether deuterium fractionation is actually absent in these latter regions, and if its absence is a common feature or something peculiar to the old TW Hya disk.

36 MATERIALS SCIENCE↗
DOE OSTI2021

An Asymmetric Dust Ring around a Very Low Mass Star ZZ Tau IRS

We present Atacama Large Millimeter/submillimeter Array (ALMA) gas and dust observations at band 7 (339 GHz: 0.89 mm) of the protoplanetary disk around a very low mass star ZZ Tau IRS with a spatial resolution of 025. The {sup 12}CO J = 3 → 2 position–velocity diagram suggests a dynamical mass of ZZ Tau IRS of ∼0.1–0.3 M {sub ☉}. The disk has a total flux density of 273.9 mJy, corresponding to an estimated mass of 24–50 M {sub ⊕} in dust. The dust emission map shows a ring at r = 58 au and an azimuthal asymmetry at r = 45 au with a position angle of 135°. The properties of the asymmetry, including radial width, aspect ratio, contrast, and contribution to the total flux, were found to be similar to the asymmetries around intermediate mass stars (∼2 M {sub ☉}) such as MWC 758 and IRS 48. This implies that the asymmetry in the ZZ Tau IRS disk shares a similar origin with others, despite the star being ∼10 times less massive. Our observations also suggest that the inner and outer parts of the disk may be misaligned. Overall, the ZZ Tau IRS disk shows evidence of giant planet formation on a ∼10 au scale at a few megayears. If confirmed, it will challenge existing core accretion models in which such planets have been predicted to be extremely hard to form around very low mass stars.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2020

Meso-scale Instability Triggered by Dust Feedback in Dusty Rings: Origin and Observational Implications

High spatial resolution observations of protoplanetary disks by ALMA have revealed many substructures that are providing interesting constraints on disk physics as well as dust dynamics, both of which are essential for understanding planet formation. We carry out high-resolution, 2D global hydrodynamic simulations, including the effects of dust feedback, to study the stability of dusty rings. When the ring edges are relatively sharp and the dust surface density becomes comparable to the gas surface density, we find that dust feedback enhances the radial gradients of both the azimuthal velocity profile and the potential vorticity profile at the ring edges. This eventually leads to instabilities on meso-scales (spatial scales of several disk scale heights), causing dusty rings to be populated with many compact regions with highly concentrated dust densities. We also produce synthetic dust emission images using our simulation results and discuss the comparison between simulations and observations.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2021

Stellar Rotation of T Tauri Stars in the Orion Star-forming Complex

We present a large-scale study of stellar rotation for T Tauri stars in the Orion star-forming complex. We use the projected rotational velocity ($v\sin (i)$) estimations reported by the APOGEE-2 collaboration as well as individual masses and ages derived from the position of the stars in the HR diagram, considering Gaia-EDR3 parallaxes and photometry plus diverse evolutionary models. We find an empirical trend for $v\sin (i)$ decreasing with age for low-mass stars (0.4M ⊙ < M $\star$ < 1.2M ⊙ ). Our results support the existence of a mechanism linking $v\sin (i)$ to the presence of accreting protoplanetary disks, responsible for regulating stellar rotation on timescales of about 6 Myr, which is the timescale in which most of the T Tauri stars lose their inner disk. Our results provide important constraints to models of rotation in the early phases of evolution of young stars and their disks.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Stellar Outbursts and Chondrite Composition

Abstract The temperatures of observed protoplanetary disks are not sufficiently high to produce the accretion rate needed to form stars, nor are they sufficient to explain the volatile depletion patterns in CM, CO, and CV chondrites and terrestrial planets. We revisit the role that stellar outbursts, caused by high-accretion episodes, play in resolving these two issues. These outbursts provide the necessary mass to form the star during the disk lifetime and provide enough heat to vaporize planet-forming materials. We show that these outbursts can reproduce the observed chondrite abundances at distances near 1 au. These outbursts would also affect the growth of calcium-aluminum-rich inclusions and the isotopic compositions of carbonaceous and noncarbonaceous chondrites.

Astronomy & Astrophysics↗
DOE OSTI2024

Phase and Morphology of Water-ice Grains Formed in a Cryogenic Laboratory Plasma

Abstract Grains of ice are formed spontaneously when water vapor is injected into a weakly ionized laboratory plasma in which the background gas has been cooled to cryogenic temperatures comparable to those of deep space. These ice grains are levitated indefinitely within the plasma so that their time evolution can be observed under free-floating conditions. Using microscope imaging, ice grains are shown to have a spindle-like fractal structure and grow over time. Both crystalline and amorphous phases of ice are observed using Fourier transform infrared spectroscopy. A mix of crystalline and amorphous grains coexists under certain thermal conditions, and a linear mixing model is used on the ice absorption band surrounding 3.2 μ m to examine the ice phase composition and its temporal stability. The extinction spectrum is also affected by inelastic scattering as grains grow, and characteristic grain radii are obtained from Mie scattering theory and compared to size measurements from direct imaging. Observations are used to compare possible ice nucleation mechanisms, and it is concluded that nucleation is likely catalyzed by ions, as ice does not nucleate in the absence of plasma and impurities are not detected. Ice grain properties and infrared extinction spectra show similarity to observations of some astrophysical ices observed in protoplanetary disks, implying that the fractal morphology of the ice and observed processes of homogeneous ice nucleation could occur as well in such astrophysical environments with weakly ionized conditions.

Astronomy & Astrophysics↗
DOE OSTI2020

Isotopic Evolution of the Inner Solar System Inferred from Molybdenum Isotopes in Meteorites

The fundamentally different isotopic compositions of non-carbonaceous (NC) and carbonaceous (CC) meteorites reveal the presence of two distinct reservoirs in the solar protoplanetary disk that were likely separated by Jupiter. However, the extent of material exchange between these reservoirs, and how this affected the composition of the inner disk, are not known. Here we show that NC meteorites display broadly correlated isotopic variations for Mo, Ti, Cr, and Ni, indicating the addition of isotopically distinct material to the inner disk. The added material resembles bulk CC meteorites and Ca–Al-rich inclusions in terms of its enrichment in neutron-rich isotopes, but unlike the latter materials is also enriched in s-process nuclides. The comparison of the isotopic composition of NC meteorites with the accretion ages of their parent bodies reveals that the isotopic variations within the inner disk do not reflect a continuous compositional change through the addition of CC dust, indicating an efficient separation of the NC and CC reservoirs and limited exchange of material between the inner and outer disk. Instead, the isotopic variations among NC meteorites more likely record a rapidly changing composition of the disk during infall from the Sun's parental molecular cloud, where each planetesimal locks the instant composition of the disk when it forms. Here, a corollary of this model is that late-formed planetesimals in the inner disk predominantly accreted from secondary dust that was produced by collisions among pre-existing NC planetesimals.

58 GEOSCIENCES↗