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Experimental laser system features polarization feedback scheme maintaining frequency lock. Generates light at wavelength of 369.4 nanometers by second-harmonic generation from 738.8-nanometers laser diode. System prototype of source of 369.4-nanometers radiation used to optically pump 2S1/2 ' 2P1/2 transition in 171Yb+ ions in lightweight, low-power trapped-ion frequency-standard apparatus.
Data obtained from the electric field induced second harmonic generation (EFISH) and Kurtz Powder Methods will be provided to MSFC for further refinement of their method. A theoretical model for predicting the second-order nonlinearities of organic salts is being worked on. Another task is the synthesis of a number of salts with various counterions. Several salts with promising SHG activities and new salts will be tested for the presence of two crystalline forms. The materials will be recrystallized from dry and wet solvents and compared for SHG efficiency. Salts that have a high SHG efficiency and no tendency to form hydrates will be documented. The synthesis of these materials are included in this report. A third task involves method to aid in the growth of large, high quality single crystals by solution processes. These crystals will be characterized for their applicability in the fabrication of devices that will be incorporated into optical computers in future programs. Single crystals of optimum quality may be obtained by crystal growth in low-gravity. The final task is the design of a temperature lowering single crystal growth apparatus for ground based work. At least one prototype will be built.
A system (36, 98) for determining the linearity of an RF detector (46, 106). A first technique involves combining two RF signals from two stable local oscillators (38, 40) to form a modulated RF signal having a beat frequency, and applying the modulated RF signal to a detector (46) being tested. The output of the detector (46) is applied to a low frequency spectrum analyzer (48) such that a relationship between the power levels of the first and second harmonics generated by the detector (46) of the beat frequency of the modulated RF signal are measured by the spectrum analyzer (48) to determine the linearity of the detector (46). In a second technique, an RF signal from a local oscillator (100) is applied to a detector (106) being tested through a first attenuator (102) and a second attenuator (104). The output voltage of the detector (106) is measured when the first attenuator (102) is set to a particular attenuation value and the second attenuator (104) is switched between first and second attenuation values. Further, the output voltage of the detector (106) is measured when the first attenuator (102) is set to another attenuation value, and the second attenuator (104) is again switched between the first and second attenuation values. A relationship between the voltage outputs determines the linearity of the detector (106).
Second-order nonlinear optical processes including second-harmonic generation, optical rectification, and difference-frequency generation associated with intersubband transitions in wurtzite GaN/AlGaN quantum well (QW) are investigated theoretically. Taking into account the strain-induced piezoelectric (PZ) effects, we solve the electronic structure of the QW from coupled effective-mass Schrodinger equation and Poisson equation including the exchange-correlation effect under the local-density approximation. We show that the large PZ field in the QW breaks the symmetry of the confinement potential profile and leads to large second-order susceptibilities. We also show that the interband optical pump-induced electron-hole plasma results in an enhancement in the maximum value of the nonlinear coefficients and a redshift of the peak position in the nonlinear optical spectrum. By use of the difference-frequency generation, THz radiation can be generated from a GaN/Al(0.75)Ga(0.25)N with a pump laser of 1.55 micron.
Holographic interferometry with UV light from KDP crystal generating second harmonic of Q switched ruby laser red output, noting optical path length sensitivity
Intensity correlations in optical parametric noise and second harmonic generation measured by two photon delayed coincidence counting
The theory and recent applications of waves in periodic structures are reviewed. Both the Floquet and coupled waves approach are analyzed in some detail. The theoretical part of the paper includes wave propagation in unbounded and bounded active or passive periodic media, wave scattering from periodic boundaries, source radiation (dipole, Cerenkov, transition, and Smith-Purcell) in periodic media, and pulse transmission through a periodic slab. The applications part covers the recent development in a variety of fields: distributed feedback oscillators, filters, mode converters, couplers, second-harmonic generators, deflectors, modulators, and transducers in the fields of integrated optics and integrated surface acoustics. Work on insect compound eyes, mechanical structures, ocean waves, pulse compressions, temperature waves, and cholesteric liquid crystals, and particles interaction with crystals is briefly reviewed, especially in the case of zeolite crystals and superlattices. Recent advances in fabrication techniques for very fine gratings are also covered.
The scattered signal excited by nonlinear mixing of two plane waves normally incident on an infinitely long column of plasma is investigated. A general solution is obtained for the polarization in which the electric field vectors of the waves are perpendicular to the column axis and the column is assumed to be radically inhomogeneous. This general theory is then applied to the special cases of the inhomogeneous column in the long-wavelength limit, and the homogeneous column both for the general case and in the long-wavelength limit. It is determined that dipole and quadrupole components should predominate in the polar radiation pattern for the long-wavelength case. The special case of second harmonic generation due to a single incident wave is analyzed in detail. Nonlinear scattering coefficients are computed, and the corresponding polar radiation patterns are determined. The findings of this study are employed to evaluate the feasibility of observing nonlinear scattering from meteor trails.
The squeezing spectra for the output fields of several intracavity nonlinear optical systems are obtained. It is shown that at critical points, e.g., the turning points for optical bistability, the threshold for parametric oscillation, and the self-pulsing instability in second-harmonic generation, perfect squeezing in the output field is, in principle, possible.
Diode-laser-pumped Nd:YLF lasers are demonstrated at 1.047 microns with less than 1-mW thresholds and internal quantum efficiencies approaching 70 percent. Operation at 1.053 microns has also been achieved. Intracavity second-harmonic generation using MgO:LiNbO3 has generated up to 145-micro-W output at 523.6 nm for 30.1 mW of diode-laser pump power.
The rapid improvement in diode laser pump sources has led to the recent progress in diode laser pumped solid state lasers. To date, electrical efficiencies of greater than 10 percent were demonstrated. As diode laser costs decrease with increased production volume, diode laser and diode laser array pumped solid state lasers will replace the traditional flashlamp pumped Nd:YAG laser sources. The use of laser diode array pumping of slab geometry lasers will allow efficient, high peak and average power solid state laser sources to be developed. Perhaps the greatest impact of diode laser pumped solid state lasers will be in spectroscopic applications of miniature, monolithic devices. Single-stripe diode-pumped operation of a continuous-wave 946 nm Nd:YAG laser with less than 10 m/w threshold was demonstrated. A slope efficiency of 16 percent near threshold was shown with a projected slope efficiency well above a threshold of 34 percent based on results under Rhodamine 6G dye-laser pumping. Nonlinear crystals for second-harmonic generation of this source were evaluated. The KNbO3 and periodically poled LiNbO3 appear to be the most promising.
Single-stripe diode-laser-pumped operation of a continuous-wave 946-nm Nd:YAG laser with less than 10-mW threshold has been demonstrated. A slope efficiency of 16 percent near threshold was shown with a projected slope efficiency well above a threshold of 34 percent based on results under Rhodamine 6G dye-laser pumping. Nonlinear crystals for second-harmonic generation of this source were evaluated. KNbO3 and periodically poled LiNbO3 appear to be the most promising.
Recent progress in the development of highly efficient coherent optical sources is reviewed. This work focusses on nonlinear frequency conversion of the highly coherent output of the Non-Planar Ring Laser Oscillators developed earlier in the program, and includes high efficiency second harmonic generation and the operation of optical parametric oscillators for wavelength diversity and tunability.
Kilometer wavelength radiation, measured from distant positions over the North Pole and over the Earth's equator, was compared to the area of discrete aurora imaged by several low-altitude spacecraft. Through correlative studies of auroral kilometric radiation (AKR) with about two thousand auroral images, a stereoscopic view of the average auroral acceleration region was obtained. A major result is that the total AKR power increases as the area of the discrete auroral oval increases. The implications are that the regions of parallel potentials or the auroral plasma cavities, in which AKR is generated, must possess the following attributes: (1) they are shallow in altitude and their radial position depends on wavelength, (2) they thread flux tubes of small cross section, (3) the generation mechanism in them reaches a saturation limit rapidly, and (4) their distribution over the discrete auroral oval is nearly uniform. The above statistical results are true for large samples collected over a long period of time (about six months). In the short term, AKR frequently exhibits temporal variations with scales as short as three minutes (the resolution of the averaged data used). These fluctuations are explainable by rapid quenchings as well as fast starts of the electron cyclotron maser mechanism. There were times when AKR was present at substantial power levels while optical emissions were below instrument thresholds. A recent theoretical result may account for this set of observations by predicting that suprathermal electrons, of energies as low as several hundred eV, can generate second harmonic AKR. The indirect observations of second harmonic AKR require that these electrons have mirror points high above the atmosphere so as to minimize auroral light emissions. The results provide evidence supporting the electron cyclotron maser mechanism.
Recent progress in the development of highly efficient coherent optical sources was reviewed. This work has focused on nonlinear frequency conversion of the highly coherent output of the non-planar ring laser oscillators developed earlier in the program, and includes high efficiency second harmonic generation and the operation of optical parametric oscillators for wavelength diversity and tunability.
The variation of the anion counterion in the presently formulated organic salts, whose cation possesses large molecular hyperpolarizability, will in many cases yield materials with large powder second-harmonic generation efficiencies. The highest such efficiency is three orders of magnitude greater than that of the urea used as a reference compound. It is demonstrated that such nonconventional donors as Br(-) and the pyrenyl moiety can be incorporated into molecules which, in the requisite crystallographic environment, will exhibit substantial bulk susceptibilities.
Laser development, high efficiency, high power second harmonic generation, operation of optical parametric oscillators for wavelength diversity and tunability, and studies in coherent communications are reviewed.
A series of organometallic and organic salts, in which the cation has been designed to have a large molecular hyperpolarizability, has been prepared. Variation of the counterion (anion) in many cases leads to materials with large powder second harmonic generation (SHG) efficiencies, the highest of which is roughly 2000 times that of a urea reference.