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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
NASA NTRS2010

Highly Conductive Multifunctional Graphene Polycarbonate Nanocomposites

Graphene nanosheet bisphenol A polycarbonate nanocomposites (0.027 2.2 vol %) prepared by both emulsion mixing and solution blending methods, followed by compression molding at 287 C, exhibited dc electrical percolation threshold of approx.0.14 and approx.0.38 vol %, respectively. The conductivities of 2.2 vol % graphene nanocomposites were 0.512 and 0.226 S/cm for emulsion and solution mixing. The 1.1 and 2.2 vol % graphene nanocomposites exhibited frequency-independent behavior. Inherent conductivity, extremely high aspect ratio, and nanostructure directed assembly of the graphene using PC nanospheres are the main factors for excellent electrical properties of the nanocomposites. Dynamic tensile moduli of nanocomposites increased with increasing graphene in the nanocomposite. The glass transition temperatures were decreased with increasing graphene for the emulsion series. High-resolution electron microscopy (HR-TEM) and small-angle neutron scattering (SANS) showed isolated graphene with no connectivity path for insulating nanocomposites and connected nanoparticles for the conductive nanocomposites. A stacked disk model was used to obtain the average particle radius, average number of graphene layers per stack, and stack spacing by simulation of the experimental SANS data. Morphology studies indicated the presence of well-dispersed graphene and small graphene stacking with infusion of polycarbonate within the stacks.

Yoonessi, Mitra↗
NASA NTRS1981

Small-angle approximation to the transfer of narrow laser beams in anisotropic scattering media

The broadening and the signal power detected of a laser beam traversing an anisotropic scattering medium were examined using the small-angle approximation to the radiative transfer equation in which photons suffering large-angle deflections are neglected. To obtain tractable answers, simple Gaussian and non-Gaussian functions for the scattering phase functions are assumed. Two other approximate approaches employed in the field to further simplify the small-angle approximation solutions are described, and the results obtained by one of them are compared with those obtained using small-angle approximation. An exact method for obtaining the contribution of each higher order scattering to the radiance field is examined but no results are presented.

Box, M. A.↗
NASA NTRS1975

Brillouin-scattering measurements of the acoustic absorption coefficient in liquid CS2

High-resolution Brillouin spectra were recorded for light scattered at small angles from liquid CS2. The use of a single-mode He-Ne laser, locked in frequency to a Fabry-Perot interferometer, permitted measurements of line widths of the order of 10 MHz for frequencies in the range 300-1000 MHz. These measurements extend previous Brillouin line-width measurements at higher frequencies into the region where relaxation effects are dominant and connect the optical measurements with lower-frequency acoustical data.

Coakley, R. W.↗
NASA NTRS1985

Experimental characterization of fatigue crack tip processes

Many analytical models have been proposed to describe the physical processes attendant to a fatigue crack tip, as well as the rate at which fatigue cracks grow. By applying advanced experimental methods (such as electron channeling, stereoimaging, and in-situ cyclic loading in an SEM) to a broad range of structural materials, it has been shown that it is possible to critically assess the physical assumptions incorporated into the models. Refinements in existing models and the development of new ones have resulted. New insights into materials' behavior are providing guidelines for improving the fatigue resistance of structural alloys. In the near future, even more advanced experimental methods, such as high temperature SEM stages and small angle neutron scattering, will be available to study creep/fatigue interactions in metals and ceramics.

Lankford, J.↗
NASA NTRS1994

Powder agglomeration in a microgravity environment

This is the final report for NASA Grant NAG3-755 entitled 'Powder Agglomeration in a Microgravity Environment.' The research program included both two types of numerical models and two types of experiments. The numerical modeling included the use of Monte Carlo type simulations of agglomerate growth including hydrodynamic screening and molecular dynamics type simulations of the rearrangement of particles within an agglomerate under a gravitational field. Experiments included direct observation of the agglomeration of submicron alumina and indirect observation, using small angle light scattering, of the agglomeration of colloidal silica and aluminum monohydroxide. In the former class of experiments, the powders were constrained to move on a two-dimensional surface oriented to minimize the effect of gravity. In the latter, some experiments involved mixture of suspensions containing particles of opposite charge which resulted in agglomeration on a very short time scale relative to settling under gravity.

Cawley, James D.↗
NASA NTRS1994

Surfactant-based critical phenomena in microgravity

The objective of this research project is to characterize by experiment and theoretically both the kinetics of phase separation and the metastable structures produced during phase separation in a microgravity environment. The particular systems we are currently studying are mixtures of water, nonionic surfactants, and compressible supercritical fluids at temperatures and pressures where the coexisting liquid phases have equal densities (isopycnic phases). In this report, we describe experiments to locate equilibrium isopycnic phases and to determine the 'local' phase behavior and critical phenomena at nearby conditions of temperature, pressure, and composition. In addition, we report the results of preliminary small angle neutron scattering (SANS) experiments to characterize microstructures that exist in these mixtures at different fluid densities.

Kaler, Eric W.↗
NASA NTRS1996

Isopycnic Phases and Structures in H2O/CO2/Ethoxylated Alcohol Surfactant Mixtures

Ternary mixtures of H2O and CO2 with ethoxylated alcohol (C(i)E(j)) surfactants can form three coexisting liquid phases at conditions where two of the phases have the same density (isopycnic phases). Isopycnic phase behavior has been observed for mixtures containing the surfactants C8E5, C10E6, and C12E6, but not for those mixtures containing either C4E1 or CgE3. Pressure-temperature (PT) projections for this isopycnic three-phase equilibrium were determined for H2O/CO2/C8E5 and H2O/CO2/C10E6 mixtures at temperatures from approximately 25 to 33 C and pressures between 90 and 350 bar. As a preliminary to measuring the microstructure in isopycnic three component mixtures, phase behavior and small angle neutron scattering (SANS) experiments were performed on mixtures of D2O/CO2/ n-hexaethyleneglycol monododecyl ether (C12E6) as a function of temperature (25-31 C), pressure (63.1-90.7 bar), and CO2 composition (0-3.9 wt%). Parameters extracted from model fits of the SANS spectra indicate that, while micellar structure remains essentially unchanged, critical concentration fluctuations increase as the phase boundary and plait point are approached.

Paulaitis, Michael E.↗
NASA NTRS1996

Polymer-Induced Depletion Interaction and Its Effect on Colloidal Sedimentation in Colloid-Polymer Mixtures

In this paper we focus on the polymer-induced depletion attraction and its effect on colloidal sedimentation in colloid-polymer mixtures. We first report a small angle neutron scattering (SANS) study of the depletion effect in a mixture of hard-sphere-like colloid and non-adsorbing polymer. Then we present results of our recent sedimentation measurements in the same colloid-polymer mixture. A key parameter in controlling the sedimentation of heavy colloidal particles is the interparticle potential U(tau), which is the work required to bring two colloidal particles from infinity to a distance tau under a give solvent condition. This potential is known to affect the average settling velocity of the particles and experimentally one needs to have a way to continuously vary U(tau) in order to test the theory. The interaction potential U(tau) can be altered by adding polymer molecules into the colloidal suspension. In a mixture of colloid and non-adsorbing polymer, the potential U(tau) can develop an attractive well because of the depletion effect, in that the polymer chains are expelled from the region between two colloidal particles when their surface separation becomes smaller than the size of the polymer chains. The exclusion of polymer molecules from the space between the colloidal particles leads to an unbalanced osmotic pressure difference pushing the colloidal particles together, which results in an effective attraction between the two colloidal particles. The polymer-induced depletion attraction controls the phase stability of many colloid-polymer mixtures, which are directly of interest to industry.

Tong, Penger↗
NASA NTRS1999

A New Instrument for Measurement of the Solar Aureole Radiance Distribution from Unstable Platforms

A novel imaging solar aureole radiometer, which can obtain absolute radiometric measurements of the solar aureole when operated on an unstable platform is described. A CCD array is used to image the aureole, while a neutral density occulter on a long pole blocks the direct solar radiation. This ensures accurate direction registration as the sun appears in acquired images, and the total circumsolar region is measured simultaneously. The imaging nature of this instrument along with a special triggering device permit acquisition of the circumsolar sky radiance within 7.5 degrees of the center of the solar disk, and within 1 degree of the edge of the solar disk. This innovation makes possible for the first time, reliable and accurate radiometric measurements of the solar aureole from unstable mobile platforms such as ships. This allows determination small angle atmospheric scattering. The instrument has been used in field studies of atmospheric aerosols and will be used in satellite validation and calibration campaigns.

Ritter, Joseph M.↗
NASA NTRS1999

Drop Breakup in Fixed Bed Flows as Model Stochastic Flow Fields

We examine drop breakup in a class of stochastic flow fields as a model for the flow through fixed fiber beds and to elucidate the general mechanisms whereby drops breakup in disordered, Lagrangian unsteady flows. Our study consists of two parallel streams of investigation. First, large scale numerical simulations of drop breakup in a class of anisotropic Gaussian fields will be presented. These fields are generated spectrally and have been shown in a previous publication to be exact representations of the flow in a dilute disordered bed of fibers if close interactions between the fibers and the drops are dynamically unimportant. In these simulations the drop shape is represented by second and third order small deformation theories which have been shown to be excellent for the prediction of drop breakup in steady strong flows. We show via these simulations that the mechanisms of drop breakup in these flows are quite different than in steady flows. The predominant mechanism of breakup appears to be very short lived twist breakups. Moreover, the occurrence of breakup events is poorly predicted by either the strength of the local flow in which the drop finds itself at breakup, or the degree of deformation that the drop achieves prior to breakup. It is suggested that a correlation function of both is necessary to be predictive of breakup events. In the second part of our research experiments are presented where the drop deformation and breakup in PDMS/polyisobutylene emulsions is considered. We consider very dilute emulsions such that coalescence is unimportant. The flows considered are simple shear and the flow through fixed fiber beds. Turbidity, small angle light scattering, dichroism and microscopy are used to interrogate the drop deformation process in both flows. It is demonstrated that breakup at very low capillary numbers occurs in both flows but larger drop deformation occurs in the fixed bed flow. Moreover, it is witnessed that breakup in the bed occurs continuously during flow and apparently with uniform probability through the bed length. The drop deformations witnessed in our experiments are larger than those predicted by the numerical simulations, and future plans to investigate these differences are discussed.

Shaqfeh, Eric S. G.↗
NASA NTRS2019

Searching for Lunar Horizon Glow With the Lunar Orbiter Laser Altimeter

We present the results of a 2-year-long systematic campaign to monitor the lunar dust exosphere for enhancements in dust concentration at altitudes < 20 km both during and outside of major meteor stream periods. We utilize the radiometric capabilities of the Lunar Orbiter Laser Altimeter Laser Ranging telescope onboard the Lunar Reconnaissance Orbiter to search for forward-scattered sunlight from exospheric dust grains, called lunar horizon glow (LHG). Specifically, we test the hypothesis that major meteor streams can produce LHG similar to what was measured in Apollo 15 coronal photography. Assuming a one-dimensional exponential vertical dust profile and a dust grain radius r ~ 0:1 μm, we derive an upper limit of ~ 10(exp -11) g cm(exp -2) on the overlying column dust mass density near the terminator during stream periods, a limit roughly 10 times lower than inferred from Apollo 15. Recent studies at altitudes ~ 1 - 20 km outside of major meteor streams and at higher altitudes during streams placed limits on the density of similarly-sized grains ~ 100 - 1000 times lower than Apollo 15. Our results show that Apollo 15-like LHG, if real, is also a rare occurrence at altitudes < 20 km during major meteor stream periods. This study is the first to quantitatively constrain the role of meteor streams in producing Apollo 15-like LHG at altitudes < 20 km and small forward scattering angles, and further narrows the properties of any similar high-altitude LHG and the conditions under which it can occur.

M K Barker↗
NASA NTRS2020

Nuclear Fusion Reactions in Deuterated Metals

Nuclear fusion reactions of D-D are examined in an environment comprised of high density cold fuel embedded in metal lattices in which a small fuel portion is activated by hot neutrons. Such an environment provides for enhanced screening of the Coulomb barrier due to conduction and shell electrons of the metal lattice, or by plasma induced by ionizing radiation (γ quanta). We show that neutrons are far more efficient than energetic charged particles, such as light particles (e−, e+) or heavy particles (p, d, α) in transferring kinetic energy to fuel nuclei (D) to initiate fusion processes. It is well-known that screening increases the probability of tunneling through the Coulomb barrier. Electron screening also significantly increases the probability of large- versus small-angle Coulomb scattering of the reacting nuclei to enable subsequent nuclear reactions via tunneling. This probability is incorporated into the astrophysical factor S(E). Aspects of screening effects to enable calculation of nuclear reaction rates are also evaluated, including Coulomb scattering and localized heating of the cold fuel, primary D-D reactions, and subsequent reactions with both the fuel and the lattice nuclei. The effect of screening for enhancement of the total nuclear reaction rate is a function of multiple parameters including fuel temperature and the relative scattering probability between the fuel and lattice metal nuclei. Screening also significantly increases the probability of interaction between hot fuel and lattice nuclei increasing the likelilhood of Oppenheimer-Phillips processes opening a potential route to reaction multiplication. We demonstrate that the screened Coulomb potential of the target ion is determined by the nonlinear Vlasov potential and not by the Debye potential. In general, the effect of screening becomes important at low kinetic energy of the projectile. We examine the range of applicability of both the analytical and asymptotic expressions for the well-known electron screening lattice potential energy Ue, which is valid only for E >> Ue (E is the energy in the center of mass reference frame). We demonstrate that for E ≤ Ue, a direct calculation of Gamow factor for screened Coulomb potential is required to avoid unreasonably high values of the enhancement factor f (E) by the analytical—and more so by the asymptotic—formulas.

Vladimir Pines↗
NASA NTRS1980

Spectral scattering properties of turbid waters

River water samples have been examined for optical scattering properties at wavelengths between 400 and 800 nm. Scattering coefficients were calculated from measurements of beam attenuation and absorption coefficients and are observed to vary with wavelength. At a fixed wavelength, the scattering coefficient is influenced by both phytoplankton concentration (as indicated by chlorophyll a) and suspended solids concentration. Measurements of small angle volume-scattering function indicate that the phase function at an angle of 1.5 deg is not constant for turbid waters and varies with both wavelength and beam attenuation coefficient. These data differ from previously published results for relatively clear oceanic and coastal waters. Caution is required when attempting to estimate scattering coefficient values from single-angle measurements of volume-scattering function.

Whitlock, C. H.↗
NASA NTRS1973

An Approximate Equation For The Multiply Scattered Contribution to A Lidar Return

An approximate equation is developed which describes the contribution of Nth order scattering to a lidar return. This development assumes a homogeneous scattering medium characterized by a scattering function sharply peaked in the forward direction and relatively insensitive to angle near the backscatter direction. The derivation includes the effects of finite divergence of the transmitted laser beam, finite receiver field of view, finite separation between the laser and the receiver and nonparallel system alignment. The derivation presented uses small angle approximations to reduce the time dependent multiple scattering problem to a time independent form which is then solved with techniques previously developed for multiple small angle nuclear scattering.

Eloranta, Edwin W.↗
NASA NTRS1976

Effects of multiple scattering on light pulses reflected by turbid atmospheres

Multiple scattering contributions to lidar returns from turbid atmospheres are derived by means of an analytical theory. It is assumed that scattering takes place mainly at small angles except for one event that scatters the light backward. The phase functions are approximated by the sum of Gaussian functions of the scattering angle in both the forward and backward directions. The three-dimensional radiative transfer equation is transformed to a one-dimensional problem by means of Fourier transforms. Neumann solutions to the transformed equation of radiative transfer are then found. A number of examples are presented for cloud, fog and haze models. The results are found to be in satisfactory agreement with results obtained from the Monte Carlo analysis of Kunkel (1974) and the theory of light pulses doubly scattered by turbid atmospheres which was developed by Eloranta (1972).

Weinman, J. A.↗
NASA NTRS1993

Processing of semicrystalline polymers

Our research group has been interested in the processing-structure-property relationships in semicrystalline polymers and blends for many years. In situ real time x ray scattering at elevated temperatures is being used to monitor the development of structure. An ongoing collaboration with Dr. Malcolm Capel at the Brookhaven National Synchrotron Light Source allows the performance of real time wide and small angle x ray scattering to study the phase transformations in semicrystalline polymers. The first part of my presentation will be about our recent use of x ray scattering to study blends of poly(ethylene terephthalate) with polyarylates. The purpose of the next portion of the presentation is to show how we may study effects of self-deformation of polymers during processing in the gravity environment, using real time x ray scattering. In this way, how processing stresses alter the microstructure of semicrystalline polymers was learned, and ultimately microgravity processing strategies that will result in more uniform morphology in these polymers is hoped to be developed.

Cebe, Peggy↗
NASA NTRS2007

Coupling of Multiple Coulomb Scattering with Energy Loss and Straggling in HZETRN

The new version of the HZETRN deterministic transport code based on Green's function methods, and the incorporation of ground-based laboratory boundary conditions, has lead to the development of analytical and numerical procedures to include off-axis dispersion of primary ion beams due to small-angle multiple Coulomb scattering. In this paper we present the theoretical formulation and computational procedures to compute ion beam broadening and a methodology towards achieving a self-consistent approach to coupling multiple scattering interactions with ionization energy loss and straggling. Our initial benchmark case is a 60 MeV proton beam on muscle tissue, for which we can compare various attributes of beam broadening with Monte Carlo simulations reported in the open literature.

Mertens, Christopher J.↗