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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 55 records · Page 3
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Fission In R-process Elements (FY20 Q2 Quarterly Report)

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Fission In R-process Elements (Q4 FY2020 Quarterly Report)

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Fission In R-process Elements (Q1 FY2021)

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r -process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Fission In R-Process Elements

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Fission In R-process Elements (FIRE) - Quarterly Report (Q2FY22)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Fission In R-process Elements (FIRE)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Fission In R-process Elements (FIRE) (NA-22 Quarterly Report, Q4FY22)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for fission work, BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Measurement of the prompt fission neutron spectrum from 800 keV to 10 MeV for 240 Pu(sf) and for the 240 Pu($n,f$) reaction induced by neutrons of energy from 1–20 MeV

Here, the presence of 240 Pu in nuclear fuels for reactors has resulted in high uncertainties in the results of reactor and nuclear transmutation calculations because of deficiencies in 240 Pu-related nuclear data. Specifically for the prompt fission neutron spectrum (PFNS) of 240 Pu, there is only one neutron-induced, (n,f), measurement at 0.85 MeV incident neutron energy and only one complete spontaneous fission, (sf), measurement. This limited availability of data does not sufficiently guide nuclear data evaluations of these quantities. Here we report on a measurement of both the 240 Pu(sf) and the 240 Pu(n,f) PFNS, both over the emitted neutron energy range of 0.79–10.0 MeV, and from incident neutron energies of 1.0–20.0 MeV for the (n,f) reaction. Measurements were made with a hemispherical array of liquid scintillators at the high-energy Los Alamos Neutron Science Center white neutron source at the Weapons Neutron Research facility as part of the joint LANL-LLNL Chi-Nu experimental campaign to measure actinide fission neutron spectra. These measurements are the first of their kind, and provide clear experimental evidence for second-chance fission, third chance fission, and pre-equilibrium neutron emission processes in neutron-induced fission of 240 Pu, and are the first ever measurements above 1 MeV incident neutron energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Measurement of the Prompt Fission Neutron Spectrum from 800 keV to 10 MeV for 240 Pu($sf$) and for the 240 Pu($n,f$) Reaction Induced by Neutrons of Energy from 1-20 MeV

The presence of 240 Pu in nuclear fuels for reactors has resulted in high uncertainties in the results of reactor and nuclear transmutation calculations because of deficiencies in 240 Pu-related nuclear data. Specifically for the prompt fission neutron spectrum (PFNS) of 240 Pu, there is only one neutron-induced, ($n,f$), measurement at 0.85 MeV incident neutron energy and only one complete spontaneous fission, ($sf$), measurement. This limited availability of data does not sufficiently guide nuclear data evaluations of these quantities. Here we report on a measurement of both the 240 Pu($sf$) and the 240 Pu($n,f$) PFNS, both over the emitted neutron energy range of 0.79–10.0 MeV, and from incident neutron energies of 1.0–20.0 MeV for the ($n,f$) reaction. Measurements were made with a hemispherical array of liquid scintillators at the high-energy Los Alamos Neutron Science Center white neutron source at the Weapons Neutron Research facility as part of the joint LANL-LLNL Chi-Nu experimental campaign to measure actinide fission neutron spectra. These measurements are the first of their kind, and provide clear experimental evidence for second-chance fission, third-chance fission, and pre-equilibrium neutron emission processes in neutron-induced fission of 240 Pu, and are the first ever measurements above 1 MeV incident neutron energy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Constraining the impact of chlorine as a neutron absorber in next-gen fast reactor designs

The role of chlorine as a neutron poison and as a seed for producing radioactive waste in nuclear systems has driven a renewed interest to improve its nuclear data uncertainties. Additionally, basic and applied science programs that use CLYC (Cs 2 LiYCl 6 :Ce) detectors for neutron spectroscopy and monitoring are also very sensitive to any change in chlorine nuclear data for simulations of the detector response. In this work, sensitivities relevant for these different applications are addressed through simulations of the efficiency of CLYC detectors in a fast fission spectrum when applying new chlorine nuclear data as input. These simulations are validated by an experimental measurement using CLYC detectors coupled to an ionization chamber loaded with a 252 Cf spontaneous fission source. The results are then used to obtain the first reliable direct measurement of the 35 Cl(n,p 0 ) and summed Cl(n,p+n,α) fission spectrum average cross sections, found to be 54.7(32) and 105.0(98) mb, respectively. The results are within uncertainty of calculated fission spectrum averaged cross sections based on recently re-evaluated chlorine nuclear data, which confirm recent impact studies performed for the Molten Chloride Reactor Experiment. Meanwhile, there currently exists only one published criticality benchmark experiment that is sufficiently sensitive to chlorine nuclear data. Discrepancies are found with this set of criticality safety benchmarks, which are more sensitive to thermal and epithermal neutron energies than the energies, above 100 keV, tested in this current work. Hence, there is still a need to re-evaluate the chlorine nuclear data at lower energies to assess these discrepancies. Interpretation of the data from future “faster” criticality benchmarks, which are needed for next-gen fast reactor designs, benefit from the improved constraints on the chlorine nuclear data validated in this work.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Absolute mass calibration of fission product distributions measured with the E-$v$ method

The mass calibration of fission product distributions measured with the energy–velocity (E-v) method constitutes a technical challenge. The energy loss of the fission fragments in the various dead layers of the spectrometer and other sources of pulse-height defects of the energy detectors are a significant source of systematic uncertainty in the mass calculations used to determine the measured fission product yields. Here, in this study, the absolute calibration of the fission mass distributions is accomplished by measuring prompt γ-rays in coincidence with the fission fragments. This allows for the direct calibration of the mass spectra and eliminates any dependence on potentially complicated energy corrections. The first test measurement was performed at the Los Alamos Neutron Science Center employing the SPectrometer for Ion DEtermination in fission Research (SPIDER). SPIDER is a 2E-2v spectrometer designed for measuring independent fission product yields from neutron-induced fission. In this test, the single-arm SPIDER (E-v) system and an array of 252 Cf sources were used. The single-arm system consisted of two time pick-off detectors for measuring the time-of-flight of the fission fragments and a double-sided silicon strip detector (DSSD) for measuring the kinetic energy. Characteristic γ-rays from fission fragments were detected using three high-purity germanium (HPGe) detectors. For the mass calibration, γ–mass coincidence events from twelve product isotopes were used. The measured FPYs from 252 Cf spontaneous fission were found to be in excellent agreement with the evaluated data after applying the absolute mass calibration. From the γ–mass coincidence events, the mass resolution of the system was also extracted. An average mass resolution of ~1.4 AMU (FWHM) for the light fragments and ~2.4 AMU (FWHM) for the heavy fragments were found. This was the first in-situ calibration and characterization of the SPIDER spectrometer, which paves the way for high-quality FPY measurements with this instrument.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2020

Fission In R-process Elements - FY2020

The goal of the FIRE topical collaboration in nuclear theory is to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This will be achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration is composed of LLNL (lead) and LANL for work on nuclear data (ground-state properties, fission, β-decay), BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities receive funds from the DOE Office of Science, while national laboratories receive funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2022

Fission In R-process Elements (FIRE)

The goal of the FIRE topical collaboration in nuclear theory was to determine the astrophysical conditions of the rapid neutron capture process (r-process), which is responsible for the formation of heavy elements. This was achieved by including in r-process simulations the most advanced models of fission (spontaneous, neutron-induced, β-delayed) that have been developed at LLNL and LANL. The collaboration was composed of LLNL (lead) and LANL for work on nuclear data (ground-state properties, fission, β-decay), BNL for nuclear data management, and the university of Notre Dame and North Carolina State University for r-process simulations. Under DOE/NNSA agreement, both universities received funds from the DOE Office of Science, while national laboratories received funds directly from NA221.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Fission and the r -process nucleosynthesis of translead nuclei in neutron star mergers

In this report we study the impact of fission on the production and destruction of translead nuclei during the r-process nucleosynthesis occurring in neutron-star mergers. Abundance patterns and rates of nuclear energy production are obtained for different ejecta conditions using three sets of stellar reaction rates, one of which is based on microscopic and consistent calculations of nuclear masses, fission barriers, and collective inertias. We show that the accumulation of fissioning material during the r process can strongly affect the free neutron abundance after the r-process freeze-out. This leads to a significant impact on the abundances of heavy nuclei that undergo α decay or spontaneous fission, affecting the radioactive energy production by the ejecta at timescales relevant for kilonova emission.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Fission fragment decay simulations with the CGMF code

The CGMF code implements the Hauser-Feshbach statistical nuclear reaction model to follow the de-excitation of fission fragments by successive emissions of prompt neutrons and γ rays. The Monte Carlo technique is used to facilitate the analysis of complex distributions and correlations among the prompt fission observables. Starting from initial configurations for the fission fragments in mass, charge, kinetic energy, excitation energy, spin, and parity, Y(A,Z,KE,U,J,π), CGMF samples neutron and γ-ray probability distributions at each stage of the decay process, conserving energy, spin and parity. Nuclear structure and reaction input data from the RIPL3 library are used to describe fission fragment properties and decay probabilities. Characteristics of prompt fission neutrons, prompt fission γ rays, and independent fission yields can be studied consistently. Correlations in energy, angle and multiplicity among the emitted neutrons and γ rays can be easily analyzed as a function of the emitting fragments. Finally, in its current version, CGMF is limited to certain spontaneous fission reactions on Pu and Cf isotopes, as well as neutron-induced fission reactions up to 20 MeV on U, Np, and Pu isotopes.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2025

Level structure of light neutron-rich La isotopes beyond the 𝑁 = 82 shell closure

Here, the high spin excited states of Lanthanum isotopes 140–143 La, above the 𝑁 = 82 closed shell, were populated in fission reactions. The prompt 𝛾-ray transitions were measured using two complementary methods: (a) in coincidence with the isotopically identified fragments produced in the fission of the 238 U + 9 Be system using the Variable Mode Spectrometer (VAMOS++) and the Advanced Gamma Tracking Array (AGATA) spectrometer, and (b) high statistics threefold 𝛾−𝛾−𝛾 and fourfold 𝛾−𝛾−𝛾−𝛾 coincidence data from the spontaneous fission of 252 Cf using the Gammasphere. This work reports the first identification of a pair of parity doublet structures in 143 La and the new high spin level structure in 140–142 La from prompt 𝛾-ray spectroscopy. The level structures are interpreted in terms of the systematics of neighboring odd-𝑍 nuclei above the 𝑍 = 50 shell closure and large-scale shell model calculations. The present results indicate the presence of stable octupole deformation in 143 La. The excitation energy pattern and their comparison with neighboring isotones, moving away from the 𝑁 = 82 closed shell, point towards a transition from single-particle structures to an alternating parity rotational band structure in the La isotopic chain.

Navin, A. [Centre National de la Recherche Scienti↗