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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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NASA NTRS1989

Fluorescence from photoexcitation of C2H2 at 50-106 nm

The photoabsorption and fluorescence cross sections of C2H2 were measured in the 50-106 nm region using synchrotron radiation as a light source. Fluorescence observed at several excitation wavelengths was dispersed to identify the fluorescing species that are excited C2H, C2, CH, H, and possibly C2H2. The photodissociation process of C2H2 leading to the formation of fluorescing species is discussed. The C2 (C-A) emission observed at 92.3 and 95.5 nm is produced by the molecular elimination process associated with superexcited state(s). Fluorescence spectra from the two-photon excitation of C2H2 at 157.5 and 193 nm were also observed and compared with those of single-photon excitation at the equivalent excitation energies.

Han, J. C.↗

NASA NTRS1991

NO(gamma) emission by energy transfer from NO(+) (a) to NO

Ultraviolet emission produced by photoexcitation of NO at 50-80 nm is observed using synchrotron radiation as a light source. The emission increases at an excitation wavelength corresponding to the ionization potential of the NO(+) (a) state. The emission spectra at several excitation wavelengths are dispersed and identified to be mainly the NO(gamma) band. The dependence of emission intensity on gas pressure and delay time indicates that the emission is produced by a secondary reaction, which is attributed to the energy transfer from NO(+) (a) to NO.

Ma, Guang↗

NASA NTRS1992

Quantitative photoabsorption and fluorescence spectroscopy of benzene, naphthalene, and some derivatives at 106-295 nm

Photoabsorption and fluorescence cross sections of benzene, (o-, m-, p-) xylenes, naphthalene, 1-methylnaphthalene, and 2-ethylnaphthalene in the gas phase are measured at 106-295 nm using synchrotron radiation as a light source. Fluorescences are observed from the photoexcitation of benzene and xylenes at 230-280 nm and from naphthalene and its derivatives at 190-295 nm. The absolute fluorescence cross section is determined by calibration with respect to the emission intensity of the NO(A-X) system, for which the fluorescence quantum yield is equal to 1. To cross-check the current calibration method, the quantum yield of the SO2(C-X) system at 220-230 nm was measured since it is about equal to 1. The current quantum-yield data are compared with previously published values measured by different methods.

Suto, Masako↗

NASA NTRS1991

Photoabsorption and photoionization cross sections of NH3, PH3, H2S, C2H2, and C2H4 in the VUV region

Using synchrotron radiation as a continuum light source, the photoabsorption and photoionization cross sections of NH3, PH3, H2S, C2H2, and C2H4 have been measured from their respective ionization thresholds to 1060 A. The vibrational constants associated with the nu(2) totally symmetric, out-of-plane bending vibration of the ground electronic state of PH3(+) have been obtained. The cross sections and quantum yields for producing neutral products through photoexcitation of these molecules in the given spectral regions have also been determined. In the present work, autoionization processes were found to be less important than dissociation and predissociation processes in NH3, PH3, and C2H4. Several experimental techniques have been employed in order to examine the various possible systematic errors critically.

Xia, T. J.↗

NASA NTRS1982

Fluorescence yields from photodissociation of OCS at 1060-1240 A

The cross sections for the production of fluorescence (3000-8000 A) from excited photofragments of OCS were determined in order to gain a better understanding of the role of carbonyl sulfide in interstellar photochemistry. Synchrotron radiation was used as the light source for the measurements in the 1060-1240 A region, as it is suitable for measuring the absorption cross section in the structured region. It was found that the quantum yields for the production of various CO triplet states are less than 1.5% at the observed excitation photon wavelengths.

Lee, L. C.↗

NASA NTRSDate not supplied

In Situ Synchrotron Micro-CT of Microballoon-Filled RTV Silicone During Thermal Decomposition

This work investigates the thermal decomposition of microballoon-filled room-temperature-vulcanizing (RTV) silicone using time-resolved synchrotron micro-CT at the Advanced Light Source. In situ imaging of constrained and unconstrained samples captures the evolution of the internal microstructure during heating, including material expansion, microballoon and void growth, tearing, pyrolysis, shrinkage, and increasing porosity. The measurements provide new insight into the mechanisms governing RTV degradation and generate three-dimensional data for future quantitative analysis and material-response model development.

TPS↗

NASA NTRS1989

Photoabsorption and photodissociation of molecules important in the interstellar medium

Photoabsorption and fluorescence cross sections of molecules important in the interstellar medium were measured in the 90 to 200 nm region using synchrotron radiation, excimer laser, and condensed discharge lamps as light sources. The quantitative spectroscopic data are currently needed for the modeling of formation and destruction rates of molecules by the interstellar radiation field. Fluorescences from excited photofragments produced by vacuum ultraviolet radiation of molecules are dispersed to identify the emitting species. The fluorescence data are useful for the identification of emission sources in interstellar clouds.

Lee, Long C.↗

NASA NTRS1990

Role of the methylene amidogen (H2CN) radical in the atmospheres of Titan and Jupiter

The methylene amidogen (H2CN) radical can be shown to be an important intermediate in models for the formation of HCN (via N + CH3) and the recombination of H to H2 (via H + HCN) on Titan as well as in models for the formation of HCN (via NH2 + C2H3) in the atmosphere of Jupiter. Experiments in our laboratory in a discharge flow system with mass spectrometric detection of both reactants and products have established that the major product channel (90 percent for the reaction N + CH3 is that leading to H2CN + H. The same result was obtained for N + CD3 yields D2CN + D. The rate constant for the reaction D + D2CN yields DCN + D2 was measured for the first time and k(298 K) greater than 7 x 10(exp -11) cu cm/s was found. The same result was obtained for the H atom reaction. This is the final step in the reaction sequence leading to HCN on both Titan and Jupiter and to formation of H2 from H on Titan. The first measurement of the ionization potentials for H2CN and D2CN was also made. From electron impact studies I.P. = (9.6 + or - 1.0) eV was obtained for both radicals. An upperlimit of I.P. less than 11.6 eV came from observations of the H2CN radical by photoionization mass spectrometry using an Ar resonance lamp (106.7 nm). Further photoionization experiments are planned using synchrotron radiation plus monochromator as a tunable vacuum UV light source.

Nesbitt, F. L.↗

NASA NTRS1988

Photoabsorption and phototdissociation of molecules important in the interstellar medium

The photoabsorption and photodissociation cross sections of interstellar molecules and radicals were measured in the 90 to 200 nm region using synchrotron radiation, F sub 2 laser, excimer lasers, and discharge lamps as light sources. These data are currently needed for determining the formation and destruction rates of molecules and radicals by the interstellar radiation field.

Lee, Long C.↗

NASA NTRS1982

On the nature of 2 gamma bursts with spectral evolutions observed by the Konus experiment

Several unique features of the evolving spectra of the April 2, 1979B, and November 11, 1979 gamma-ray bursts observed by the Konus experiment can be used to determine a number of critical parameters of the sources, within the context of the thermal synchrotron model, including their luminosity distance. These results shed much light on the origin of these events and possibly gamma bursts in general.

Liang, E. P.↗

NASA NTRS1983

On the nature of two gamma bursts with spectral evolutions observed by the KONUS experiment

Liang, E. P.↗

NASA NTRS1978

Polarized vacuum ultraviolet and X-radiation

The most intense source of polarized vacuum UV and X radiation is synchrotron radiation, which exhibits a degree of partially polarized light between about 80-100%. However, the radiation transmitted by vacuum UV monochromators can also be highly polarized. The Seya-Namioka type of monochromator can produce partially polarized radiation between 50-80%. For certain experiments it is necessary to know the degree of polarization of the radiation being used. Also, when synchrotron radiation and a monochromator are combined the polarization characteristic of both should be known in order to make full use of these polarization properties. The polarizing effect of monochromators (i.e., diffraction gratings) have been measured at the Seya angle and at grazing angles for various spectral orders. Experimental evidence is presented which shows that the reciprocity law holds for polarization by reflection where the angle of incidence and diffraction are unequal. These results are reviewed along with the techniques for measuring the degree of polarization.

Samson, J. A. R.↗

NASA NTRS1994

Radio continuum polarimetric imaging of high redshift radio galaxies

Multifrequency images of total and polarized radio continuum emission from the two high redshift radio galaxies 0902+343 (z = 3.40) and 0647+415 (4C 41.17, z = 3.80) are presented. These images represent the most sensitive polarimetric study of high redshift ratio galaxies to date. The emission from both galaxies is substantially polarized, up to 30% in some regions, and both sources sit behind deep 'Faraday screens,' producing large rotation measures, over 10(exp 3) rad/sq. m in magnitude, and large rotation measure gradients across the sources. Such large rotation measures provide further evidence that high redshift radio galaxies are situated in very dense environments. Drawing the analogy to a class of low redshift powerful radio galaxies with similarly large rotation measures, we suggest that 0902+343 and 0647+415 are situated at the centers of dense, x-ray 'colling flow' clusters, and that the cluster gas is substantially magnetized. The remarkable similarity between the optical and radio morphologies of 0647+415 on scales as small as 0.1 sec is presented. We consider, and reject, both synchrotron and inverse Compton radiation as possible sources of the optical emission. We also consider both scattering of light out of a 'cone' of radiation from an obscured nucleus, and jet-induced star formation, and find that both models encounter difficulties in explaining this remarkably close radio-optical alignment. High resolution spectral index images reveal compact, flat spectrum components in both sources. We suggest that these components are the active nuclei of the galaxies. Lastly, high resolution images of 0902+343 show that the southernmost component forms a 'ring' of 0.2 sec radius. We discuss the possibility that this ring is the result of gravitational lensing, along the lines proposed by Kochanek & Lawrence (1990).

Carilli, C. L.↗

NASA NTRS1975

The solar-flare infrared continuum

Potential sources of infrared (1 micron to 1 mm) continuum in solar flares are considered. Several mechanisms should produce detectable fluxes: in the 350 micron window for ground-based observations, impulsive emission will arise in synchrotron radiation from 1-10 MeV electrons, and possibly thermal (free-free) continuum from the source of the white-light flare; the hot flare plasma responsible for soft X-ray emission will also emit detectable fluxes of free-free continuum in the largest flares. At shorter wavelengths the dominant infrared emission will come from the H alpha flare itself. Observations in the infrared wavelengths will help to complete the picture of flare structure in both the impulsive and gradual phases.

Ohki, K.↗

NASA NTRS1972

The optical properties of platinum and gold in the vacuum ultraviolet

The optical constants of platinum and gold thin films have been determined in the spectral region of 40 to 200 nm by reflection measurements. The highly polarized continuum of synchrotron radiation emitted by the 240-MeV electron storage ring at the Physical Sciences Laboratory of the University of Wisconsin was used as a light source for the spectrum below 120 nm, while a windowless discharge lamp coupled to a normal incidence monochromator provided a source for the longer wavelengths. Optical constants were determined by a computer program based on iterative solutions to the Fresnel equations for reflection as a function of the angle of incidence.

Linton, R. C.↗

NASA NTRS2022

Hunting extreme BL Lacertae blazars with Fermi-Large Area Telescope

The emission of very-high-energy (VHE) photons (⁠E > 100 GeV⁠) in blazars is closely connected to the production of ultra-relativistic particles and the role of these γ-ray sources as cosmic particle accelerators. This work focuses on a selection of 22 γ-ray objects from the 2BIGB catalogue of high-synchrotron-peaked sources, which are classified as blazar candidates of uncertain type in the 4FGL-DR2 catalogue. We study these sources by means of a re-analysis of the first 10 yr of γ-ray data taken with the Fermi-Large Area Telescope, including the attenuation by the extragalactic background light. Their broad-band spectral energy distributions are also evaluated, using multiwavelength archival data in the radio, optical, and X-ray bands, in terms of one-zone synchrotron-self-Compton models, adding an external Compton component when needed. Out of this analysis, we identify 17 new extreme high-synchrotron-peaked (EHSP) candidates and compare their physical parameters with those of prototypical EHSP blazars. Finally, the resulting models are used to assess their detectability by the present and future generation of ground-based Imaging Atmospheric Cherenkov Telescopes. We find two VHE candidates within the reach of the current and next generation of Cherenkov telescopes: J0847.0−2336 and J1714.0−2029.

M Nievas Rosillo↗

NASA NTRS1992

Near-infrared images of the nuclear region of NGC 5128

High-resolution near-infrared images of NGC 5128 (Centaurus A) are presented, which probe the optically obscured nuclear region. The images show a central source at K (2.23 microns) and 3.26 microns. This central object is not prominent in the shorter wavelength images at J and H (1.23 and 1.65 micron, respectively), probably due to high extinction. The color images (H - K and J - H) provide evidence for a steep gradient in extinction across the array field. The images indicate three components: a red, variable, compact nucleus; the diffuse elliptical galaxy starlight; and a blue extension to the NE. The nucleus has decreased in flux density by a factor of 2.5 over less than about 5 yr at 3.26 microns. However, current spectral constraints on the nuclear source at near-infrared wavelengths cannot definitively determine the relative contributions from the known ratio synchrotron source (AGN) and from various possible dust-enshrouded thermal sources. The blue spot, approximately 7.6 +/- 0.1 arcsec NE of the nucleus appears to be a hole in the extinction, possibly enhanced by scattered light from the active galactic nucleus.

Turner, Paula C.↗

NASA NTRS2003

Probing for Pulsars: An XMM Study of the Composite SNRS G327.1-1.1 and CTA1

The subject grant is for analysis of XMM data from the supernova remnant CTA1. Our investigation centered on the study of the compact source Rx 50007.0+7302 that, based on our previous observations, appears to be a neutron star powering a wind nebula in the remnant interior. This compact source has also been suggested as the counterpart of the EGRET source 2EG J0008+7307. The analysis of the data from the compact source is complete. We find that the spectrum of the source is well described by a power law with the addition of a soft thermal component that may correspond to emission from hot polar cap regions or to cooling emission from a light element atmosphere over the entire star. There is evidence of extended emission on small spatial scales which may correspond to structure in the underlying synchrotron nebula. Extrapolation of the nonthermal emission component to gamma-ray energies yields a flux that is consistent with that of 2EG J0008+7307, thus strengthening the proposition that there is a gamma-ray emitting pulsar at the center of CTA 1. Our timing studies with the EPIC pn data revealed no evidence for pulsations, however; we set an upper limit of 61% on the pulsed fraction from this source. The results from this study were presented in a poster at the recent IAU Symposium in Sydney, Australia. A paper summarizing these results, entitled "Xray Observations of the Compact Source in CTA 1" (Slane et al.) has been submitted for publication in the Astrophysical Journal.

Slane, Patrick↗