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DOE OSTI2022

Neutron-upscattering enhancement of the triple-alpha process

Abstract The neutron inelastic scattering of carbon-12, populating the Hoyle state, is a reaction of interest for the triple-alpha process. The inverse process (neutron upscattering) can enhance the Hoyle state’s decay rate to the bound states of 12 C, effectively increasing the overall triple-alpha reaction rate. The cross section of this reaction is impossible to measure experimentally but has been determined here at astrophysically-relevant energies using detailed balance. Using a highly-collimated monoenergetic beam, here we measure neutrons incident on the Texas Active Target Time Projection Chamber (TexAT TPC) filled with CO 2 gas, we measure the 3 α -particles (arising from the decay of the Hoyle state following inelastic scattering) and a cross section is extracted. Here we show the neutron-upscattering enhancement is observed to be much smaller than previously expected. The importance of the neutron-upscattering enhancement may therefore not be significant aside from in very particular astrophysical sites (e.g. neutron star mergers).

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2022

Manifestation of postcollision interaction in Krypton LMN Auger spectra following K-shell photoionization

In this work, we report on an experimental and theoretical study of post-collision interaction (PCI) effects on L 2 -M 4,5 N 2,3 Auger electrons measured above the Kr K-edge in which L 2 vacancies are primarily generated by KL 2 x-ray emission. Such cascade processes, in which a deep inner-shell vacancy decays first by x-ray emission followed by Auger electron emission, is a strong decay mode in heavy atoms. The L 2 -M 4,5 N 2,3 Auger electron peak is observed to become increasingly asymmetric with a shifting peak maximum as the absorbed x-ray energy approaches the K-shell ionization threshold. This is attributed to PCI energy exchanges of the Auger electron with the 1s photoelectron. To model the PCI effects, we have applied a semiclassical approach modified to account for the combined lifetimes of the K and L 2 hole states. In addition, our analysis treats several closely spaced Auger transitions with final ionic states having different terms and angular momenta.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2023

Scrambling and quantum chaos indicators from long-time properties of operator distributions

Scrambling is a key concept in the analysis of nonequilibrium properties of quantum many-body systems. Most studies focus on its characterization via out-of-time-ordered correlation (OTOC) functions, particularly through the early-time decay of the OTOC. However, scrambling is a complex process which involves operator spreading and operator entanglement, and a full characterization requires one to access more refined information on the operator dynamics at several timescales. In this work we analyze operator scrambling by expanding the target operator in a complete basis and studying the structure of the expansion coefficients treated as a coarse-grained probability distribution in the space of operators. Here we study different features of this distribution, such as its mean, variance, and participation ratio, for the Ising model with longitudinal and transverse fields, kicked collective spin models, and random circuit models. We show that the long-time properties of the operator distribution display common features across these cases and discuss how these properties can be used as a proxy for the onset of quantum chaos. Finally, we discuss the connection with OTOCs and analyze the cost of probing the operator distribution experimentally using these correlation functions.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2024

Measurements of the branching fractions of semileptonic D s + decays via e + e − → D s * + D s * −

We measure the absolute branching fractions of semileptonic D s + decays via the e + e − → D s * + D s * − process using e + e − collision data corresponding to an integrated luminosity of 10.64 fb − 1 collected by the BESIII detector at center-of-mass energies between 4.237 and 4.699 GeV. The branching fractions are B ( D s + → η e + ν e ) = ( 2.35 ± 0.11 stat ± 0.10 syst ) % , B ( D s + → η ′ e + ν e ) = ( 0.82 ± 0.09 stat ± 0.04 syst ) % , B ( D s + → ϕ e + ν e ) = ( 2.21 ± 0.16 stat ± 0.11 syst ) % , B ( D s + → f 0 ( 980 ) e + ν e , f 0 ( 980 ) → π + π − ) = ( 0.15 ± 0.02 stat ± 0.01 syst ) % , B ( D s + → K 0 e + ν e ) = ( 0.24 ± 0.0 4 stat ± 0.0 1 syst ) % , and B ( D s + → K * 0 e + ν e ) = ( 0.19 ± 0.0 3 stat ± 0.0 1 syst ) % . These results are consistent with those measured via the e + e − → D s * ± D s ∓ process by BESIII and CLEO. Using two-parameter series expansion, the hadronic transition form factors of D s + → η e + ν e , D s + → η ′ e + ν e , and D s + → K 0 e + ν e are determined to be f + η ( 0 ) = 0.442 ± 0.02 2 stat ± 0.01 7 syst , f + η ′ ( 0 ) = 0.557 ± 0.06 2 stat ± 0.02 4 syst , and f + K 0 ( 0 ) = 0.677 ± 0.09 8 stat ± 0.02 3 syst . Published by the American Physical Society 2024

Ablikim, M.↗

DOE OSTI2021

FVCOM-ICM4.0

FVCOM-ICM is a water quality model that simulates the influence of nutrients and carbon pollution on biogeochemical oceanographic processes such as phytoplankton primary productivity, nutrient consumption, mineralization, decay and settling of particulate organic matter and computes resulting dissolved oxygen (DO) concentrations and pH levels. An “offline” approach of coupling Finite Volume Coastal Ocean Model (FVCOM) hydrodynamic solutions to CE-QUAL-ICM biogeochemical model was used. FVCOM and CE-QUAL-ICM are public domain Fortran Codes that were developed independently by US Army Corps of Engineers and University of Massachusetts. PNNL developed FVCOM-ICM that has the ability to conduct water quality calculations using a previously computed hydrodynamic solution. The biogeochemical calculations using CE-QUAL-ICM kinetics are conducted over the same finite-volume mesh and in the FVCOM framework.

Khangaonkar, Tarang↗

DOE OSTI2026

Geant4 RApid Pair Production Application (GRAPPA) v1.0.0

GRAPPA is a Geant4 application that simulates the interaction of an incoming particle beam (typically electron or photons) with an High-Z material. Particles are generated at a certain energy and interact with a solid target. The product of this interaction is detected and saved on file. The application implements a basic target that is just a simple box, and it accepts complex target descriptions via GDML files. The user has the freedom to set detectors to capture the desired particles. This application enables studying processes such as antiparticle production, muon generation, and atomic decay.

Terzani, Davide [Lawrence Berkeley National Labora↗

DOE OSTI2021

Using Grover's search algorithm to characterize the Rigetti Quantum Computing Platform

Performance of the Rigetti quantum computing platform was tested during the period of time from 12/16/2019 to 05/18/2020. The Grover's search (GS) algorithm was used as a testing tool, in particular, 3- and 4-level versions of the algorithm. As a result, a number of hardware issues were revealed, so the algorithm was split to smaller blocks and individual gates, and all of them were tested separately. The fidelity decay was found to be due to both decoherent processes and coherent errors of the native hardware gates. These errors were estimated from RX gate benchmarks and were in a form of extra rotation of the quantum state. As a consequence of that, performance of the algorithm was shown to be strongly dependent on the native gate decomposition of the program. Suggestions and possible improvements of the future Rigetti runs are made based on the obtained observations.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2025

Benchmark Exercise Report for Experimental Study of Bubble Scrubbing in Sodium Pool

Mechanistic source term (MST) analyses are likely to be an important part of advanced reactor licensing applications. For the purpose, an MST analysis code applicable to newly introduced advanced reactors, called SRT (Simplified Radionuclide Transport) code, has been developed by Argonne National Laboratory. SRT can track overall behaviors of radionuclides especially in metal fuel-based sodium fast reactors (SFRs) and microreactors. Throughout the simulation, migration inside fuel pins before failure, interaction with coolant (for SFR), removal/leakage in cover gas and containment (or confinement), and environmental dose impacts are considered alongside radioactive decay for short-lived nuclides. Among the postulated process, pool scrubbing phenomenon, especially under sodium pool condition, has been identified as high importance with limited supportive data. The phenomenon plays a crucial role in assessing the degree of radiological impacts as radioactive aerosols or vapors are efficiently and effectively removed during the process. To provide validation basis for SRT in assessing pool scrubbing performance inside sodium pools, the University of Wisconsin-Madison performed tests including extensive parametric effects. Separate effect tests were conducted to directly evaluate the SRT models and to estimate degree of contribution by each contributing factor. Specifically, bubble size, aerosol size, aerosol density, aerosol concentration, pool depth, system temperature, and bubble swarm effects were considered. According to the parametric effects, decontamination performance enhances with decreasing bubble size, large density, and deeper pool height. Aerosol concentration provides no effect for the whole range of interest, and pool temperature variation shows minor effects under the considered temperature condition. When multiple bubbles are injected generating a bubble swarm condition, DF performance further enhances by bubble interactions and turbulence characteristics. The measurement shows the exceptional importance of aerosol size range considered, with the lowest decontamination, where most radionuclides are expected to escape.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

NASA NTRS1971

Locating the magnetospheric ring current

Protons are studied in the global depression of the earth's horizontal magnetic field. It is shown that 10 to 100 keV protons dominate ring current energetics in two preferred regions of cyclotron instability, which serve as stable trapping boundaries for ring current protons. The only apparent means of removing this stably trapped belt of particles are considered to be by charge exchange interactions, or by outward expansion of the plasmapause to erode the ring current. Both of these processes require about two days, which is the characteristic decay period of the main phase depression. Questions whose answers are necessary to formulate a quantitative theory of geomagnetic storms which relates main phase depression to solar wind parameters are included.

Thorne, R. M.↗

NASA NTRS1977

A search for helium ions in the recovery phase of a magnetic storm

Data from an energetic ion mass spectrometer experiment on the low-latitude polar-orbiting satellite 1971-89A were examined for evidence of helium ions in the region of the ring current during the recovery phase of the December 17-18, 1971 magnetic storm. The principal precipitating ion species with energies between 0.7 and 12 keV were observed to be O+ and H+. No evidence for He+ was obtained. Inferences about the composition of the trapped population are made on the basis of simultaneous observations in the equatorial plane by Explorer 45. Coordinated observations with Explorer 45 and the Fritz Peak Observatory during the period of a stable auroral red arc have provided some information on the ionospheric and magnetospheric processes associated with the arc. A comparison of charge exchange and precipitation lifetimes during the recovery phase of the December 17-18 storm has shown both processes to be of comparable importance as ring current decay mechanisms in the energy range of the observations.

Sharp, R. D.↗

NASA NTRS1984

Ablation effects in oxygen-lead fragmentation at 2.1 GeV/nucleon

The mechanism of particle evaporation was used to examine ablation effects in the fragmentation of 2.1 GeV/nucleon oxygen nuclei by lead targets. Following the initial abrasion process, the excited projectile prefragment is assumed to statistically decay in a manner analogous to that of a compound nucleus. The decay probabilities for the various particle emission channels are calculated by using the EVAP-4 Monte Carlo computer program. The input excitation energy spectrum for the prefragment is estimated from the geometric ""clean cut'' abrasion-ablation model. Isotope production cross sections are calculated and compared with experimental data and with the predictions from the standard geometric abrasion-ablation fragmentation model.

Townsend, L. W.↗

NASA NTRS1990

Resonant Alfven wave heating of the plasma sheet boundary layer

The exchange of energy between the plasma mantle and the plasma sheet boundary layer (PSBL) is examined with a one-dimensional magnetotail model. The energy exchange occurs via Poynting flux generated by the localized mode conversion of a surface wave to an Alfven wave. This Poynting flux propagates through the lobe and into the PSBL where it is absorbed by two processes. The first arises from a gradient in the plasma beta causing a smooth absorption of Poynting flux. The second process results from the localized mode conversion of the decaying surface wave to an Alfven wave, causing a localized absorption of energy. A numerical solution of the linearized ideal MHD equations is obtained by assuming an adiabatic equation of state.

Harrold, B. G.↗

NASA NTRS1994

Applications of SAR Measurements in Ocean-Ice Atmosphere Interaction Studies

The difficulty in observing the polar sea-ice cover and its influence on the atmospheric and oceanic boundary layer is the ephemerality of active geophysical prosesses. Identifying timescales of sea-ice formation, change and decay, is the key to successful measurement of these processes.

sea-ice formation microwave radar imaging SAR↗

DOE OSTI2026

Standard Candles for Supernova Neutrino Detection at DUNE

The Deep Underground Neutrino Experiment (DUNE) far detector is sensitive to $\mathcal{O}(10)$ MeV electron neutrinos through $ν_e$ charged-current reaction with argon. This capability is a unique window into the $ν_e$ component of a Galactic core-collapse supernova flux. Extracting the properties of the supernova spectrum is, however, limited by the poorly-known $ν_e$-Ar cross section. We propose a data-driven strategy that leverages $^8$B solar neutrinos and muon-decay-at-rest neutrinos as standard candles for this process. These calibration samples constrain both the low-energy and high-energy components of the cross section relevant for supernova detection. Our method reduces the reliance on nuclear models, which can bias the extraction of the spectral parameters by as much as 300$\%$.

Cheng, Ting [Fermilab]↗

DOE OSTI2026

Gamma-ray signatures of 𝑟-process radioactivity from the collapse of magnetized white dwarfs

We predict the gamma-ray line emission from 𝑟-process nuclei synthesized in the ejecta of the accretion-induced collapse (AIC) of a magnetized, rapidly rotating white dwarf. Using ejecta from a two-dimensional general-relativistic neutrino-magnetohydrodynamic simulation, further evolved with a radiation-hydrodynamics code coupled to an in situ nuclear reaction network, we construct angle-dependent gamma-ray spectra in the 0.01–10 MeV band via composition-dependent ray tracing through the ejecta. The emission between ∼1 and 10 d is dominated by 132 I (𝑡 1/2 = 2.3 h), continuously replenished by the decay of its parent 132 Te (𝑡 1/2 = 3.2 d), with additional contributions from 131 I, 133 Xe, and 132 Te . At 𝑡 ≳ 20 d, 56 Co (from 56 Ni decay) becomes the primary emitter. The simultaneous presence of 𝑟 process and iron-peak gamma-ray lines is distinctive of AIC ejecta and absent in binary neutron star mergers, where iron-peak nuclei are generally not synthesized. Comparing with the 3⁢𝜎 continuum sensitivities of planned MeV gamma-ray telescopes (COSI, AMEGO-X, e-ASTROGAM, GRAMS, GammaTPC), we find the brightest 𝑟-process lines detectable to ∼10 Mpc by GammaTPC and GRAMS, with the signal approaching their sensitivity threshold at 30 Mpc. As a result, the 𝑟-process spectral features survive time integration over ∼30 d exposures, demonstrating robustness against the long observation times required by gamma-ray detectors.

Nuclear reactions↗

DOE OSTI2022

Magnetized laser–plasma interactions in high-energy-density systems: Parallel propagation

In this study, we investigate parametric processes in magnetized plasmas, driven by a large-amplitude pump light wave. Our focus is on laser–plasma interactions relevant to high-energy-density (HED) systems, such as the National Ignition Facility and the Sandia MagLIF concept. We present a self-contained derivation of a “parametric” dispersion relation for magnetized three-wave interactions, meaning the pump wave is included in the equilibrium, similar to the unmagnetized work of Drake et al., Phys. Fluids 17, 778 (1974). For this, we use a multi-species plasma fluid model and Maxwell's equations. The application of an external B field causes right- and left-polarized light waves to propagate with differing phase velocities. This leads to Faraday rotation of the polarization, which can be significant in HED conditions. Phase-matching and linear wave dispersion relations show that Raman and Brillouin scattering have modified spectra due to the background B field, though this effect is usually small in systems of current practical interest. We study a scattering process we call stimulated whistler scattering, where a light wave decays to an electromagnetic whistler wave (ω≲ω ce ) and a Langmuir wave. This only occurs in the presence of an external B field, which is required for the whistler wave to exist.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Shedding light on charmonium

We investigate E1 radiative transitions within charmonium in a relativistic approach based on light-front QCD. In quantum field theory, two sets of processes are pure E1: χ c 0 → J / ψ γ ( ψ → χ c 0 γ ) and h c → η c γ ( η c ′ → h c γ ), both involving the P -wave charmonia. We compute the E1 radiative decay widths as well as the corresponding transition form factors of various processes including those involving 2 P states. These observables provide an access to the microscopic structures of the P -wave charmonium. We show that our parameter-free predictions are in excellent agreement with the experimental measurements as well as lattice simulations whenever available. Published by the American Physical Society 2024

Astronomy & Astrophysics↗

DOE OSTI2023

Atmosphere–Ocean Coupled Energy Budgets of Tropical Convective Discharge–Recharge Cycles

An energy budget combining atmospheric moist static energy (MSE) and upper ocean heat content (OHC) is used to examine the processes impacting day-to-day convective variability in the tropical Indian and western Pacific Oceans. Feedbacks arising from atmospheric and oceanic transport processes, surface fluxes, and radiation drive the cyclical amplification and decay of convection around suppressed and enhanced convective equilibrium states, referred to as shallow and deep convective discharge–recharge (D–R) cycles, respectively. The shallow convective D–R cycle is characterized by alternating enhancements of shallow cumulus and stratocumulus, often in the presence of extensive cirrus clouds. The deep convective D–R cycle is characterized by sequential increases in shallow cumulus, congestus, narrow deep precipitation, wide deep precipitation, a mix of detached anvil and altostratus and altocumulus, and once again shallow cumulus cloud types. Transitions from the shallow to deep D–R cycle are favored by a positive “column process” feedback, while discharge of convective instability and OHC by mesoscale convective systems (MCSs) contributes to transitions from the deep to shallow D–R cycle. Variability in the processes impacting MSE is comparable in magnitude to, but considerably more balanced than, variability in the processes impacting OHC. Variations in the quantity of atmosphere–ocean coupled static energy (MSE + OHC) result primarily from atmospheric and oceanic transport processes, but are mainly realized as changes in OHC. MCSs are unique in their ability to rapidly discharge both lower-tropospheric convective instability and OHC.

54 ENVIRONMENTAL SCIENCES↗