Search NASA⌕ Search

SEARCH · Search NASA

Results for “MULTIPLE SCATTERING”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 541 records · Page 30

Exact Rayleigh scattering calculations for use with the Nimbus-7 Coastal Zone Color Scanner

The radiance reflected from a plane-parallel atmosphere and flat sea surface in the absence of aerosols has been determined with an exact multiple scattering code to improve the analysis of Nimbus-7 CZCS imagery. It is shown that the single scattering approximation normally used to compute this radiance can result in errors of up to 5 percent for small and moderate solar zenith angles. A scheme to include the effect of variations in the surface pressure in the exact computation of the Rayleigh radiance is discussed. The results of an application of these computations to CZCS imagery suggest that accurate atmospheric corrections can be obtained for solar zenith angles at least as large as 65 deg.

Gordon, Howard R.↗

Approximation for Horizontal Photon Transport in Cloud Remote Sensing Problems

The effect of horizontal photon transport within real-world clouds can be of consequence to remote sensing problems based on plane-parallel cloud models. An analytic approximation for the root-mean-square horizontal displacement of reflected and transmitted photons relative to the incident cloud-top location is derived from random walk theory. The resulting formula is a function of the average number of photon scatterings, and particle asymmetry parameter and single scattering albedo. In turn, the average number of scatterings can be determined from efficient adding/doubling radiative transfer procedures. The approximation is applied to liquid water clouds for typical remote sensing solar spectral bands, involving both conservative and non-conservative scattering. Results compare well with Monte Carlo calculations. Though the emphasis is on horizontal photon transport in terrestrial clouds, the derived approximation is applicable to any multiple scattering plane-parallel radiative transfer problem. The complete horizontal transport probability distribution can be described with an analytic distribution specified by the root-mean-square and average displacement values. However, it is shown empirically that the average displacement can be reasonably inferred from the root-mean-square value. An estimate for the horizontal transport distribution can then be made from the root-mean-square photon displacement alone.

Plantnick, Steven↗

High-Efficiency Solar-To-Fuel Photoelectrochemistry in Disordered Photonic Glass Electrodes (Final Technical Report)

This project investigated how photonic glass (PG) photoelectrodes—disordered arrangements of dielectric scatterers—can serve as scalable, tunable platforms for light trapping in photoelectrochemical (PEC) solar-to-fuel systems. By leveraging disorder-driven optical phenomena such as multiple scattering resonances and light localization, PG structures offer an alternative to conventional photonic crystals and inverse opals that require high structural precision. The scientific goals were to twofold: (1) develop approaches to predictive models for high performance PG electrodes based on light absorption simulations, and (2) fabricate, characterize, and optimize PG-based photoelectrodes for solar-to-hydrogen and solar-to-fuel photoelectrochemical applications. To overcome the complexity of ensemble optical simulations for disordered materials, the researchers developed a machine-learning-accelerated emulation of all configurations in the design space. With this approach, PG photoelectrodes based on a TiO2 semiconductor were designed to enhance PEC currents of up to one hundred times higher than the equivalent ultra-thin film photoanodes and several times higher than the equivalent photonic crystal. The research also explored integrated systems for electrochemical hydrogen production based on replacing water oxidation with the specific glycerol oxidation electrocatalysis. Overall, the project outlined an approach to a simple-to-fabricate photoelectrode system to drive photoelectrochemical reactions relevant to solar photochemical energy conversion.

14 SOLAR ENERGY↗

A New Method for Estimating the Single Scattering Phase Functions of Regolith Grains

Hapke's photometric model has been widely used in solar system remote sensing applications for nearly two decades. Recently, Hapke extended his model to describe the coherent-backscatter opposition effect and multiple-scattering by particles with anisotropic single particle phase functions (SPPF's). A practical difficulty for retrieving Hapke's model parameters from typical planet, satellite, and asteroid photometry data sets is that the model employs a large number of adjustable parameters (at least eight) that can be reliably constrained only for a small number of planetary data sets in which both disk-resolved and whole-disk observations are available from opposition to very large phase angles. The present work aims to reduce the number of adjustable parameters and preserve (or even enhance) the model's accuracy and usefulness by expressing Hapke's parameters in terms of more fundamental physical properties on which they mutually depend. The most difficult part of this task, described here, is to develop a simple method for computing the effective SPPF for structurally complex regolith grains from optical constants, grain-size distribution, and average regolith porosity. The development of light-scattering models for irregularly shaped particles is a large, complex subject and many sophisticated methods, such as Discrete Dipole Approximation (DDA) and Monte-Carlo simulations, have been explored elsewhere. Many of these methods are computationally intensive and probably impractical for routine substitution in Hapke's model. Here, progress is reported in developing a practical, semi-empirical method for estimating the directional scattering behavior (i.e. SPPF) of irregular regolith grains. The method employs Optical Transfer Function (OTF) techniques to model how the structural complexity of regolith particles broaden and attenuate the angular distribution of scattered light relative to that expected from ideal spherical particles of equivalent size and composition.

Helfenstein, P.↗

Elastic proton scattering off nonzero spin nuclei

In recent years, we constructed a microscopic optical potential (OP) for elastic nucleon-nucleus ( NA ) scattering using modern approaches based on chiral theories for the nucleon-nucleon ( NN ) interaction. The OP was derived at first order of the spectator expansion in Watson multiple scattering theory and its final expression was a folding integral between the NN t matrix and the nuclear density of the target. Two- and three-body forces are consistently included both in the target and in the projectile description. The purpose of this work is to apply our microscopic OP to nuclei characterized by a ground state of spin-parity quantum numbers J π ≠ 0 + . We extended our formalism to include the spin of the target nucleus. The full amplitudes of the NN reaction matrix are retained in the calculations starting from two- and three-body chiral forces. The microscopic OP can be applied in the energy range 100 ≤ E ≤ 350 MeV. Finally, we show a remarkable agreement with experimental data for the available observables and, simultaneously, provide reliable estimates for the theoretical uncertainties. This work paves the way toward a full microscopic approach to inelastic NA scattering, showing that the derivation of optical potentials between states with J π ≠ 0 + is completely under control.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Isothermal, Compton-heated coronae above accretion disks

The structure of Compton-heated coronae above accretion disks is studied here by using analytic and numerical approaches are used here to determine the direct and scattered radiation reaching the base of the corona for a range of central source luminosities. It is found that the outer region of the corona is unaffected by multiple scattering in the interior, provided that the luminosity of the central source is sufficient below the Eddington limit. How attenuation and scattering by the corona affects the strength of chromospheric emission lines is determined, as is the condition for which the irradiation due to the central source exceeds the locally generated flux from the disk. Finally, it is shown that the stability analysis for irradiated accretion disks of Tuchman et al. is not substantially altered by the corona.

Ostriker, Eve C.↗

Recent studies of the optical properties of dust and cloud particles in the Mars atmosphere and the interannual frequency of global dust storms

The results of research with two distinctly separate sets of observations yield new information on the optical properties of particulate scatterers in the Mars atmosphere, and on the interannual variability of the abundance of such scatterers in the Mars atmosphere. The first set of observations were taken by the IRTM (Infrared Thermal Mapper) instrument onboard the Viking Orbiters, during the period 1976 to 1980. Several hundred emission phase function (EPF) sequences were obtained over the Viking mission, in which the IRTM visual brightness channel observed the same area of surface/atmosphere as the spacecraft passed overhead. The 1 to 2 percent accuracy of calibration and the phase-angle coverage that characterizes these data make them ideally suited to determining both the optical depths and optical properties of dust and cloud scatterers in the Mars atmosphere versus latitude, longitude, seasons (L sub s), and surface elevation over the extended period of Viking observations. The EPF data were analyzed with a multiple scattering radiative transfer code to determine dust single scattering albedos which are distinctly higher than indicated by the Viking Lander observations. The second set of observations regard ground-based observations of the 1.3 to 2.6 mm rotational transitions of CO in the Martian atmosphere. The low-to-mid latitude average of the atmospheric temperature profile (0 to 70 km altitude) were derived from a number of such observations over the 1980 to 1990 period.

Clancy, R. T.↗

Hard jet substructure in a multistage approach

We present predictions and postdictions for a wide variety of hard jet-substructure observables using a multistage model within the framework. The details of the multistage model and the various parameter choices are described in []. A novel feature of this model is the presence of two stages of jet modification: a high-virtuality phase [modeled using the modular all twist transverse-scattering elastic-drag and radiation model ()], where modified coherence effects diminish medium-induced radiation, and a lower virtuality phase [modeled using the linear Boltzmann transport model ()], where parton splits are fully resolved by the medium as they endure multiple scattering induced energy loss. Energy-loss calculations are carried out on event-by-event viscous fluid dynamic backgrounds constrained by experimental data. The uniform and consistent descriptions of multiple experimental observables demonstrate the essential role of modified coherence effects and the multistage modeling of jet evolution. Using the best choice of parameters from [], and with no further tuning, we present calculations for the medium modified jet fragmentation function, the groomed jet momentum fraction z g and angular separation r g distributions, as well as the nuclear modification factor of groomed jets. These calculations provide accurate descriptions of published data from experiments at the Large Hadron Collider. Furthermore, we provide predictions from the multistage model for future measurements at the BNL Relativistic Heavy Ion Collider. Published by the American Physical Society 2024

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Scattering and absorption from poly-dispersed aerosols

Results from numerical computations of the diffuse sky radiances and degree of polarization are given. These results were obtained by solving the equation of radiative transfer in the formulation of Eschelbach. In these computations, multiple scattering and absorption by aerosol particles were considered. In addition, results from experimental measurements of the complex refractive index of aerosol samples at different relative humidities are presented. From the radiation flux divergences which were computed based on the determined properties of atmospheric aerosol particles, atmospheric heating rates were derived which were found to be comparable to the heating rates by water vapor.

Bullrich, K.↗

Light scattering study of highly absorptive, non-fractal, hematite aggregates

In this paper, we present measurements of the scattered light intensity by aerosolized hematite aggregate particles. The measurements were made at a wavelength of 532 nm in the scattering angle range from 0.32° to 157°. Hematite has high values of the real and imaginary parts of the refractive index m = n + iκ = 3 + i0.5 at the studied wavelength. Scanning electron micrographs (SEM) indicated that the particles were aggregates whereas the optical microscope pictures showed that the aerosol had a bimodal distribution with effective mean diameters of roughly 1 and 10 µm. This is consistent with the light scattering results which displayed two Guinier regimes. The aggregates were composed of smaller grains with an approximate size of 200 nm. Ultra Small-Angle X-ray Scattering (USAXS) indicate that the aggregates were uniform and non-fractal. Mie calculations for a sphere equivalent to the aggregate size were compared to the experimentally observed results. The observed results showed an enhanced backscattering, whereas the Mie calculations did not due to the large imaginary part of the refractive index. Hematite aggregates were simulated by assuming they were composed of spherical monomers inside a spherical volume. Then the light scattering was calculated using the T-matrix method for these simulated aggregates. The calculated results show an enhanced backscattering. We present a dimensional analysis to estimate the extent of multiple scattering within the aggregate and find a correlation between the average number of scattering events within the aggregate and the enhancement in the backscattering.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Modeling, Performance Assessment, and Nodal Data Analysis of TRISO-Fueled Systems with Shift

This technical report documents several enhancements to the Shift Monte Carlo (MC) code under the US Department of Energy (DOE) Nuclear Energy Advanced Modeling and Simulation (NEAMS) program in fiscal year (FY) 2022. Performance enhancements were added to Shift specifically for tristructural isotropic (TRISO)–fueled reactor systems and guided based on performance analysis in FY 2021. For the pebble performance model developed in previous studies, the runtime improved by ~ 91× compared to the original model and ~ 2× compared to the user-optimized model. Compared to Serpent, Shift is ~ 3× slower if Serpent delta-tracking is enabled but ~ 2× faster when delta-tracking is disabled. The multigroup cross section generation was improved through simplifying tally input definitions, porting several post-processing tally operations from Python scripts into the Shift code base, and accounting for production reactions in the scattering multiplicity. Progress was also made on two emerging capabilities: (1) the development of Titan (a Shift reactor physics user interface) and (2) initial investigation into path-length tallies for computing multigroup scattering matrices.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Asymmetry parameters of the phase function for densely packed scattering grains

Spatial correlation among densely packed particles can substantially change their single-scattering properties, thus making questionable the applicability of the independent scattering approximation in calculations of light scattering by planetary regoliths. The same problem arises in geophysics in light scattering computations for snow, frosts, and bare soil. In this paper, we use a dense-medium light-scattering theory based on the introduction of the static structure factor to calculate asymmetry parameters of the phase function for densely packed particles with real refractive indices 1.31 and 1.66, approximating water ice and soil particles, respectively, and imaginary refractive indices 0, 0.01, and 0.3. For sparsely distributed, independently scattering grains, the calculated asymmetry parameters are always positive and always larger than those for densely packed particles. For densely packed grains, the asymmetry parameters may be negative but only for radius-to-wavelength ratios from about 0.1 to about 0.4. With decreasing particle size, the calculated asymmetry parameters tend to zero independently of the compaction state. In the geometrical optics regime, the asymmetry parameters for densely packed scatterers are positive and very close to those for independently scattering grains. These results may have important implications for remote sensing of the Earth and solid planetary surfaces. In particular, it is demonstrated that negative asymmetry parameters derived with some approximate multiple-scattering theories may be physically irrelevant and can be the result of using an inaccurate bidirectional reflection function combined with the ill-conditionally of the inverse scattering problem.

Mishchenko, Michael I.↗

Which nuclear data can be validated with LLNL pulsed-sphere experiments?

It is shown here that 14-MeV D+T LLNL pulsed-sphere experiments bring complementary information into the process of validating nuclear data compared to experiments that are traditionally used for this purpose—such as critical assemblies. To be more specific, the 14-MeV D+T LLNL pulsed-sphere neutron-leakage spectra enable to validate scattering and fission nuclear data up to 15 MeV (compared to approximately up to 5 MeV when using criticality experiments) and employ to this end simple compound targets containing only few isotopes. In this work, sensitivity profiles of the spectra to nuclear data are calculated in order to understand in detail which isotopes, observables, and energy ranges of nuclear data contribute significantly to their simulation. These profiles are presented for a few selected spheres containing 16 O, 12 C, 56 Fe, and 239 Pu. It is shown that the neutron-leakage spectra of spheres containing light elements are mostly sensitive to elastic- and inelastic-scattering cross sections on discrete levels and corresponding angular distributions. Spheres of structural materials are sensitive to elastic- and inelastic-scattering cross sections, including scattering on discrete levels and the continuum, and double-differential cross sections. Actinide spheres are also strongly sensitive to the fission observables, in particular to the total-fission neutron spectrum. Thin spheres (in which neutrons experience on average less than one scatter) are mostly sensitive to data near the elastic peak, in the energy range from 12–15 MeV, while thicker ones can be sensitive to data at lower incident-neutron energies due to multiple-scattering effects. This information is brought together with simulations of 71 pulsed-sphere neutron-leakage spectra using the ENDF/B-VII.1 and ENDF/B-VIII.0 nuclear-data libraries. This analysis highlights ENDF/B-VIII.0 data that could be further investigated for potential shortcomings ( 6 Li, 12 C, 16 O, 24-26 Mg, 27 Al, 48 Ti, 56 Fe, and 208 Pb) or are likely reliable ( 1,2 H, 7 Li, 9 Be, 14 N, 235,238 U, and 239 Pu) as indicated by validating with LLNL pulsed-sphere experiments.

14-MeV D+T LLNL pulsed-sphere neutron-leakage spec↗

Re-Analysis of the Solar Phase Curves of the Icy Galilean Satellites

Re-analysis of the solar phase curves of the icy Galilean satellites demonstrates that the quantitative results are dependent on the single particle scattering function incorporated into the photometric model; however, the qualitative properties are independent. The results presented here show that the general physical characteristics predicted by a Hapke model (B. Hapke, 1986, Icarus 67, 264-280) incorporating a two parameter double Henyey-Greenstein scattering function are similar to the predictions given by the same model incorporating a three parameter double Henyey-Greenstein scattering function as long as the data set being modeled has adequate coverage in phase angle. Conflicting results occur when the large phase angle coverage is inadequate. Analysis of the role of isotropic versus anisotropic multiple scattering shows that for surfaces as bright as Europa the two models predict very similar results over phase angles covered by the data. Differences arise only at those phase angles for which there are no data. The single particle scattering behavior between the leading and trailing hemispheres of Europa and Ganymede is commensurate with magnetospheric alterations of their surfaces. Ion bombardment will produce more forward scattering single scattering functions due to annealing of potential scattering centers within regolith particles (N. J. Sack et al., 1992, Icarus 100, 534-540). Both leading and trailing hemispheres of Europa are consistent with a high porosity model and commensurate with a frost surface. There are no strong differences in predicted porosity between the two hemispheres of Callisto, both are consistent with model porosities midway between that deduced for Europa and the Moon. Surface roughness model estimates predict that surface roughness increases with satellite distance from Jupiter, with lunar surface roughness values falling midway between those measured for Ganymede and Callisto. There is no obvious variation in predicted surface roughness with hemisphere for any of the Galilean satellites.

Domingue, Deborah↗

Polarimetric signatures of a canopy of dielectric cylinders based on first and second order vector radiative transfer theory

Complete polarimetric signatures of a canopy of dielectric cylinders overlying a homogeneous half space are studied with the first and second order solutions of the vector radiative transfer theory. The vector radiative transfer equations contain a general nondiagonal extinction matrix and a phase matrix. The energy conservation issue is addressed by calculating the elements of the extinction matrix and the elements of the phase matrix in a manner that is consistent with energy conservation. Two methods are used. In the first method, the surface fields and the internal fields of the dielectric cylinder are calculated by using the fields of an infinite cylinder. The phase matrix is calculated and the extinction matrix is calculated by summing the absorption and scattering to ensure energy conservation. In the second method, the method of moments is used to calculate the elements of the extinction and phase matrices. The Mueller matrix based on the first order and second order multiple scattering solutions of the vector radiative transfer equation are calculated. Results from the two methods are compared. The vector radiative transfer equations, combined with the solution based on method of moments, obey both energy conservation and reciprocity. The polarimetric signatures, copolarized and depolarized return, degree of polarization, and phase differences are studied as a function of the orientation, sizes, and dielectric properties of the cylinders. It is shown that second order scattering is generally important for vegetation canopy at C band and can be important at L band for some cases.

Tsang, Leung↗

An Innovative Concept for Spacebased Lidar Measurement of Ocean Carbon Biomass

Beam attenuation coefficient, c, provides an important optical index of plankton standing stocks, such as phytoplankton biomass and total particulate carbon concentration. Unfortunately, c has proven difficult to quantify through remote sensing. Here, we introduce an innovative approach for estimating c using lidar depolarization measurements and diffuse attenuation coefficients from ocean color products or lidar measurements of Brillouin scattering. The new approach is based on a theoretical formula established from Monte Carlo simulations that links the depolarization ratio of sea water to the ratio of diffuse attenuation Kd and beam attenuation C (i.e., a multiple scattering factor). On July 17, 2014, the CALIPSO satellite was tilted 30Âdeg off-nadir for one nighttime orbit in order to minimize ocean surface backscatter and demonstrate the lidar ocean subsurface measurement concept from space. Depolarization ratios of ocean subsurface backscatter are measured accurately. Beam attenuation coefficients computed from the depolarization ratio measurements compare well with empirical estimates from ocean color measurements. We further verify the beam attenuation coefficient retrievals using aircraft-based high spectral resolution lidar (HSRL) data that are collocated with in-water optical measurements.

Hu, Yongxiang↗

Evaluating Light Rain Drop Size Estimates from Multiwavelength Micropulse Lidar Network Profiling

This paper investigates multiwavelength retrievals of median equivolumetric drop diameter D(sub 0) suitable for drizzle and light rain, through collocated 355-/527-nm Micropulse Lidar Network (MPLNET) observations collected during precipitation occurring 9 May 2012 at the Goddard Space Flight Center (GSFC) project site. By applying a previously developed retrieval technique for infrared bands, the method exploits the differential backscatter by liquid water at 355 and 527 nm for water drops larger than approximately 50 micrometers. In the absence of molecular and aerosol scattering and neglecting any transmission losses, the ratio of the backscattering profiles at the two wavelengths (355 and 527 nm), measured from light rain below the cloud melting layer, can be described as a color ratio, which is directly related to D(sub 0). The uncertainty associated with this method is related to the unknown shape of the drop size spectrum and to the measurement error. Molecular and aerosol scattering contributions and relative transmission losses due to the various atmospheric constituents should be evaluated to derive D(sub 0) from the observed color ratio profiles. This process is responsible for increasing the uncertainty in the retrieval. Multiple scattering, especially for UV lidar, is another source of error, but it exhibits lower overall uncertainty with respect to other identified error sources. It is found that the total error upper limit on D(sub 0) approaches 50%. The impact of this retrieval for long-term MPLNET monitoring and its global data archive is discussed.

light-rain drop size estimates↗

Errors induced by the neglect of polarization in radiance calculations for Rayleigh-scattering atmospheres

Although neglecting polarization and replacing the rigorous vector radiative transfer equation by its approximate scalar counterpart has no physical background, it is a widely used simplification when the incident light is unpolarized and only the intensity of the reflected light is to be computed. We employ accurate vector and scalar multiple-scattering calculations to perform a systematic study of the errors induced by the neglect of polarization in radiance calculations for a homogeneous, plane-parallel Rayleigh-scattering atmosphere (with and without depolarization) above a Lambertian surface. Specifically, we calculate percent errors in the reflected intensity for various directions of light incidence and reflection, optical thicknesses of the atmosphere, single-scattering albedos, depolarization factors, and surface albedos. The numerical data displayed can be used to decide whether or not the scalar approximation may be employed depending on the parameters of the problem. We show that the errors decrease with increasing depolarization factor and/or increasing surface albedo. For conservative or nearly conservative scattering and small surface albedos, the errors are maximum at optical thicknesses of about 1. The calculated errors may be too large for some practical applications, and, therefore, rigorous vector calculations should be employed whenever possible. However, if approximate scalar calculations are used, we recommend to avoid geometries involving phase angles equal or close to 0 deg and 90 deg, where the errors are especially significant. We propose a theoretical explanation of the large vector/scalar differences in the case of Rayleigh scattering. According to this explanation, the differences are caused by the particular structure of the Rayleigh scattering matrix and come from lower-order (except first-order) light scattering paths involving right scattering angles and right-angle rotations of the scattering plane.

Mishchenko, M. I.↗