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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 541 records · Page 30

Global characterization of a laser-generated neutron source

Laser-driven neutron sources are routinely produced by the interaction of laser-accelerated protons with a converter. They present complementary characteristics to those of conventional accelerator-based neutron sources (e.g. short pulse durations, enabling novel applications like radiography). We present here results from an experiment aimed at performing a global characterization of the neutrons produced using the Titan laser at the Jupiter Laser Facility (Livermore, USA), where protons were accelerated from 23 $\mathrm {\mu }$ m thick plastic targets and directed onto a LiF converter to produce neutrons. For this purpose, several diagnostics were used to measure these neutron emissions, such as CR-39, activation foils, time-of-flight detectors and direct measurement of $^7{\rm Be}$ residual activity in the LiF converters. The use of these different, independently operating diagnostics enables comparison of the various measurements performed to provide a robust characterization. These measurements led to a neutron yield of $2.0\times 10^{9}$ neutrons per shot with a modest angular dependence, close to that simulated.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Neutrons produced by known energies of ions abundant in space

Particle accelerator radiation measurements are applied to the problem of calculating biological dose from radiation produced in the walls of a spacecraft by various ions in space. Neutrons, one of the products of the interactions of energetic ions with matter, are usually quite penetrating and have large values of Q.F. or R.B.E. Ions of helium, boron, carbon, nitrogen, and oxygen were accelerated and directed onto target materials of copper or tantalum. The secondary neutron production was determined. Studies were made of the angular distribution and an inferred neutron spectrum was calculated from activities of threshold reaction detectors.

Wadman, W. W., III↗

Pulsar disk systems

It is proposed that radio pulsars have the same basic physical features as X-ray pulsars. Specifically, it is suggested that active radio pulsars are rotating neutron stars surrounded by fossil disks left over from the collapse event and that energy is extracted from the rotation of the neutron star by interaction with the disk to produce pulsar luminosity. Attention is given to a model in which the neutron star acts as a unipolar generator (or Faraday disk dynamo) and the disk acts as a load. The self-excitation of the disk/pulsar system is considered along with aspects of disk persistence, pulsed emission, and magnetically field aligned currents to the disk. An investigation is conducted regarding the possibility of a deposition of material in the form of a disk about a pulsar, taking into account questions concerning disk survival. It is found that there are some promising features regarding a disk system.

Michel, F. C.↗

Instrumental background in balloon-borne gamma-ray spectrometers and techniques for its reduction

Instrumental background in balloon-borne gamma-ray spectrometers is presented. The calculations are based on newly available interaction cross sections and new analytic techniques, and are the most detailed and accurate published to date. Results compare well with measurements made in the 20 keV to 10 MeV energy range by the Goddard Low Energy Gamma-ray Spectrometer (LEGS). The principal components of the continuum background in spectrometers with GE detectors and thick active shields are: (1) elastic neutron scattering of atmospheric neutrons on the Ge nuclei; (2) aperture flux of atmospheric and cosmic gamma rays; (3) beta decays of unstable nuclides produced by nuclear interactions of atmospheric protons and neutrons with Ge nuclei; and (4) shield leakage of atmospheric gamma rays. The improved understanding of these components leads to several recommended techniques for reducing the background.

Gehrels, N.↗

The Electron Calorimeter (ECAL) Long Duration Balloon Experiment

Accurate measurements of the cosmic ray electron energy spectrum in the energy region 50 GeV to greater than 1 TeV may reveal structure caused by the annihilation of exotic dark matter particles and/or individual cosmic ray sources. Here we describe a new long duration balloon (LDB) experiment, ECAL, optimized to directly measure cosmic ray electrons up to several TeV. ECAL includes a double layer silicon matrix, a scintillating optical fiber track imager, a neutron detector and a fully active calorimeter to identify more than 90% of the incident electrons with an energy resolution of about 1.7% while misidentifying only 1 in 200,000 protons and 0.8% of secondary gamma rays as electrons. Two ECAL flights in Antarctica are planned for a total exposure of 50 days with the first flight anticipate for December 2009.

Guzik, T. G.↗

Quantifying concentration distributions in redox flow batteries with neutron radiography

Abstract The continued advancement of electrochemical technologies requires an increasingly detailed understanding of the microscopic processes that control their performance, inspiring the development of new multi-modal diagnostic techniques. Here, we introduce a neutron imaging approach to enable the quantification of spatial and temporal variations in species concentrations within an operating redox flow cell. Specifically, we leverage the high attenuation of redox-active organic materials (high hydrogen content) and supporting electrolytes (boron-containing) in solution and perform subtractive neutron imaging of active species and supporting electrolyte. To resolve the concentration profiles across the electrodes, we employ an in-plane imaging configuration and correlate the concentration profiles to cell performance with polarization experiments under different operating conditions. Finally, we use time-of-flight neutron imaging to deconvolute concentrations of active species and supporting electrolyte during operation. Using this approach, we evaluate the influence of cell polarity, voltage bias and flow rate on the concentration distribution within the flow cell and correlate these with the macroscopic performance, thus obtaining an unprecedented level of insight into reactive mass transport. Ultimately, this diagnostic technique can be applied to a range of (electro)chemical technologies and may accelerate the development of new materials and reactor designs.

Science & Technology - Other Topics↗

Solar-geophysical data number 499, March 1986. Part 1: (Prompt reports). Data for February 1986, January 1986 and late data

Solar-Geophysical Data Number 499, March 1986, Part 1 (Prompt Reports); Data for February 1986, January 1986 and Late Data, contains the following: Detailed index for 1985 to 1986; Data for February 1986--(IUWDS alert periods (Advance and worldwide), Solar activity indices, Solar flares, Solar radio emission, Vostok inferred interplanetary magnetic field polarity, Stanford mean solar magnetic field); data for January 1986--(Solar active regions, Sudden ionospheric disturbances, Solar radio spectral observations, Cosmic ray measurements by neutron monitor, Geomagnetic indices, Radio propagation indices); Late data-(Solar active regions, Solar radio spectral observations Culgoora, Cosmic ray measurements by neutron monitor, Calcium plage data).

Coffey, H. E.↗

Validation and demonstration of the AEFC as a practical safeguards tool for inventory verification

The Advanced Experimental Fuel Counter (AEFC) is a nondestructive assay (NDA) instrument designed to determine the residual fissile mass in irradiated fuel assemblies for safeguards verification purposes. This is done by actively interrogating an assembly with a neutron source and measuring the total (Singles) and correlated (Doubles) neutron count rates resulting from induced fissions in the irradiated nuclear fuel and relating those rates to the residual fissile mass using calibration curves. Comprehensive NDA measurements of the irradiated fuel inventory at Israeli Research Reactor 1 (IRR-1) were taken with the AEFC to validate a set of previously developed calibration curves. During the campaign, measurements were acquired of 32 standard fuel assemblies and three control assemblies in just nine days. This is a significant majority of the research reactor's irradiated fuel inventory and the largest data set gathered by the AEFC to date. Many of the fuel assemblies measured during the campaign had much shorter cooling times than those assemblies previously measured with the instrument. Calibration curves developed from previous AEFC deployments were used to determine the residual 235 U mass in the measured standard fuel assemblies. The results of the campaign demonstrated that the AEFC can be used to estimate the 235 U mass remaining in a large number of irradiated fuel assemblies with 1%–5% uncertainty in a reasonable amount of time despite operating in a high dose environment.

98 NUCLEAR DISARMAMENT, SAFEGUARDS, AND PHYSICAL P↗

Crystal activation experiment MA-151

The crystal activation experiment consisted of two sample packages that were flown in the command module and returned to earth for analysis of the radioactivity induced in them during the flight. The objective of the experiment was to define the background caused by detector activation that interferes when gamma radiation is measured in the 0.02- to 10-megaelectronvolt range from earth orbit. Preliminary results show that the activation of the NaI(Tl) crystal was a factor of 3 below that from a similar measurement on Apollo 17. The identification of certain species and the level of activation observed show an important contribution from the interactions of thermal and energetic neutrons produced as secondaries in the spacecraft. That the activation was reduced by only a factor of 3 compared with the Apollo 17 experiment, despite the geomagnetically shielded orbit, possibly indicates more efficient secondary neutron production by the more energetic cosmic rays.

Trombka, J. I.↗

Testing the Activation Analysis for Fusion in OpenMC

OpenMC is a community-developed Monte Carlo neutron and photon transport simulation code. It can perform fission simulations such as fixed-source, k-eigenvalue, and subcritical multiplication calculations on models built using either a constructive solid geometry or CAD representation. To explore the use of OpenMC for fusion activation analysis, a detailed model of the Fusion Neutronics Science Facility (FNSF) was first developed for comparisons against an existing SERPENT model. A 90-degree model of FNSF in Standard-Triangle-Language (STL) CAD format was converted to Constructive Solid Geometry (CSG) using each code's built-in functions, and the geometries were validated by ensuring no cells overlapped and no particles were lost during simulations. The neutron fluxes were calculated and compared for multiple components close to the plasma. The results show differences mostly below 1% in fluxes and averaged 8% for activity and decay heat. Here, the work described in this study tests the CAD-based geometry using the DagMC toolkit in OpenMC and compares the activation analysis of OpenMC to SERPENT code.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Alternatives to NIST Cf-252 Iirradiations for Transfer Calibration of S-32 Neutron Monitors

Gas-flow proportional counting systems are used by the Radiation Metrology Laboratory (RML) at Sandia National Laboratories for reactor fluence monitoring with the 32 S(n,p) 32 P reaction. Calibration of these systems has traditionally been accomplished by fluence-transfer irradiations at the NIST 252 Cf facility. Such calibrations have become increasingly difficult as the NIST 252 Cf source decayed to unusable levels. To minimize the risk to the testing programs from an inability to properly calibrate these systems, the RML has developed two alternative calibration techniques: 1) development and implementation of certified 32 P sources for activity calibrations and subsequent calculation of neutron fluence, and 2) direct counting of non-certified reactor-irradiated sulfur pellets by liquid scintillation counting to determine 32 P activity for the subsequent calibration of gas-flow proportional counters. Preliminary comparisons show that the several calibration methods are capable of overall uncertainties within about 5 percent.

Vehar, David W.↗

Activation of Insulation in Low Power Nuclear Experiments

Nuclear experiments aim to test new designs, procedures, and materials. Similar to conventional power reactors, potential sources of worker exposure to radiation is a primary concern. One such concern is the insulation materials that are used in or near the reactor, which can often create dust when being handled. If this material receives a substantial neutron dose, then it can become activated, which can pose a health risk if inhaled or ingested. This analysis looked at the activation of, and conservative dose estimates from, industrial grade insulations that may be used in a reactor experiment.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Analysis of Second Target Station Target Removal Dose Rates

The Second Target Station (STS) project at Oak Ridge National Laboratory’s spallation neutron source is a crucial initiative for maintaining U.S. leadership in neutron sciences. The STS aims to create the world’s brightest pulsed cold neutron source, enabling cutting-edge research across various scientific disciplines. To ensure safe and efficient maintenance operations, understanding the effects of shutdown dose rates from activated components within the STS target systems is essential. This study establishes a computational framework for calculating decay gamma sources and subsequent shutdown dose rates utilizing advanced methods to account for all activation channels, including high-energy interactions down to thermal neutron capture. This study describes a novel integration of multiple tools and provides an effective means of analyzing activation and shutdown dose rates at spallation neutron facilities. A custom-developed script automates the decay gamma source generation process, ensuring proper sampling during the variance reduction phase, which is critical for accurate predictions of shutdown dose rates.

Transmutation↗

Fusion Neutron Generator

The proposed code, named FROG (Fusion neutron Generator) is built upon the open-source particle transport Monte Carlo toolkit Geant4. Geant4 provides C++ classes that can be leveraged to build application-specific codes dealing with the transport of particles through matter. Geant4-based codes are applied in high-energy particle physics experiments, medical applications, shielding, and space applications for example. The FROG code allows the user to define the geometry of a neutron converter device shaped as a hollow cylinder, where a neutron breeding material such as lithium deuteride (LiD) is cladded by two concentric cylinders. Such neutron converter is then placed inside a regular nuclear fission reactor, where thermal neutrons will react with the neutron breeder material (typically, Lithium 6), and through a series of reactions, will generate high-energy neutrons – neutrons whose kinetic energy are around 14 MeV. The hollowed central portion can hold a specimen that will be bombarded by high-energy neutrons created inside the neutron breeding material. Figuratively speaking, this type of device transforms neutrons from thermal (~0.625 eV) to fusion (~14 MeV) energies and is sometimes termed “fusion-to-thermal neutron converters” in the literature. The code consists of C++ source file compiled and linked to generate an executable. The user can select the dimensions of the converter (radius, length, and thickness of the breeder material), the breeder material type, the cladding material, and the specimen material that will be activated or irradiated. As input, the neutron flux for a specific location inside a reactor, for instance, positions in ATR, is required. As output, the code predicts the number of high-energy neutrons produced, the total neutron flux and fluence as well as its detailed spectrum. The physics involved in such device is very complex, as it requires modeling neutron transport, light-ion (tritons) transport, as well as fusion reactions. The Geant4 toolkit provides the required physical models.

Martin, NicholasP. [Idaho National Laboratory (INL↗

An Active Learning-Based Streaming Pipeline for Reduced Data Training of Structure Finding Models in Neutron Diffractometry

Structure determination workloads in neutron diffractometry are computationally expensive and routinely require several hours to many days to determine the structure of a material from its neutron diffraction patterns. The potential for machine learning models trained on simulated neutron scattering patterns to significantly speed up these tasks have been reported recently. However, the amount of simulated data needed to train these models grows exponentially with the number of structural parameters to be predicted and poses a significant computational challenge. To overcome this challenge, we introduce a novel batch-mode active learning (AL) policy that uses uncertainty sampling to simulate training data drawn from a probability distribution that prefers labelled examples about which the model is least certain. We confirm its efficacy in training the same models with ∼ 75% less training data while improving the accuracy. We then discuss the design of an efficient stream-based training workflow that uses this AL policy and present a performance study on two heterogeneous platforms to demonstrate that, compared with a conventional training workflow, the streaming workflow delivers ∼ 20% shorter training time without any loss of accuracy.

Wang, Tianle [Brookhaven National Laboratory (BNL)↗

Improved Spacecraft Materials for Radiation Protection

Methods by which radiation shielding is optimized need to be developed and materials of improved shielding characteristics identified and validated. The galactic cosmic rays (GCR) are very penetrating and the energy absorbed by the astronaut behind the shield is nearly independent of shield composition and even the shield thickness. However, the mix of particles in the transmitted beam changes rapidly with shield material composition and thickness. This results in part from the breakup of the high-energy heavy ions of the GCR which make contributions to biological effects out of proportion to their deposited energy. So the mixture of particles in the radiation field changes with shielding and the control of risk contributions from dominant particle types is critical to reducing the hazard to the astronaut. The risk of biological injury for a given particle type depends on the type of biological effect and is specific to cell or tissue type. Thus, one is faced with choosing materials which may protect a given tissue against a given effect but leave unchanged or even increase the risk of other effects in the same tissue or increase the risks to other adjacent tissues of a different type in the same individual. The optimization of shield composition will then be tied to a specific tissue and risk to that tissue. Such peculiarities arise from the complicated mixture of particles, the nature of their biological response, and the details of their interaction with material constituents. Aside from the understanding of the biological response to specific components, one also needs an accurate understanding of the radiation emerging from the shield material. This latter subject has been a principal element of this project. In the past ten years our understanding of space radiation interactions with materials has changed radically, with a large impact on shield design. For example, the NCRP estimated that only 2 g/sq cm. of aluminum would be required to meet the annual 500 mSv limit for the exposure of the blood forming organs (this limit is strictly for LEO but can be used as a guideline for the Mars mission analysis). The current estimates require aluminum shield thicknesses above 50 g/sq cm., which is impractical. In such a heavily shielded vehicle, the neutrons produced throughout the vehicle also contribute significantly to the exposure and this demands greater care in describing the angular dependence of secondary particle production processes. As such the continued testing of databases and transport procedures in laboratory and spaceflight experiments has continued. This has been the focus of much of the last year's activity and has resulted in improved neutron prediction capability. These new methods have also improved our understanding of the surface environment of Mars. The Mars 2003 NRA HEDS related surface science requirements were driven by the need to validate predictions on the upward flux of neutrons produced in the Martian regolith and bedrock made by the codes developed under this project. The codes used in the surface environment definition are also being used to look at in situ resources for the development of construction material for Martian surface facilities. For example, synthesis of polyimides and polyethylene as binders of regolith for developing basic structural elements has been studied and targets built for accelerator beam testing of radiation shielding properties. Preliminary mechanical tests have also been promising. Improved spacecraft materials have been identified (using the criteria reported by this project at the last conference) as potentially important for future shielding materials. These are liquid hydrogen, hydrogenated nanofibers, liquid methane, LiH, Polyethylene, Polysulfone, and Polyetherimide (in order of decreasing shield performance). Some of the materials are multifunctional and are required for other onboard systems. We are currently preparing software for trade studies with these materials relative to the Mars Reference Mission as required in the project's final year.

Wilson, John W.↗

Neutron-capture Cl-36, Ca-41, Ar-36, and Sm-150 in large chondrites: Evidence for high fluences of thermalized neutrons

We have measured significant concentrations of Cl-36, Ca-41, Ar-36 from decay of Cl-36, and Sm-150 produced from the capture of thermalized neutrons in the large Chico L6 chondrite. Activities of Cl-36 and Ca-41, corrected for a high-energy spallogenic component and a terrestrial age of approximately 50 ka, give average neutron-capture production rates of 208 atoms/min/g-Cl and 1525 atoms/min/kg-Ca, which correspond to thermal neutron (n) fluxes of 6.2 n/sq cm/s and 4.3 n/sq cm/s, respectively. If sustained for the approximately 65 Ma single-stage, cosmic ray exposure age of Chico, these values correspond to thermal neutron fluences of approximately 1.3 x 10(exp 16) and 0.8 x 10(exp 16) n/sq cm for Cl-36 and Ca-41, respectively. Stepwise temperature extraction of Ar in Chico impact melt shows Ar-36/Ar-38 ratios as large as approximately 9. The correlation of high Ar-36/Ar-38 with high Cl/Ca phases in neutron-irradiated Chico indicates that the excess Ar-36 above that expected from spallation is due to decay of neutron-produced Cl-36. Excess Ar-36 in Chico requires a thermal neutron fluence of 0.9-1.7 x 10(exp 16) n/sq cm. Decreases in Sm-149/Sm-152 due to neutron-capture by Sm-149 correlate with increases in Sm-150/Sm-152 for three samples of Chico, and one of the Torino H-chondrite. The 0.08% decrease in Sm-149 shown by Chico corresponds to a neutron fluence of 1.23 x 10(exp 16) n/sq cm. This fluence derived from Sm considers capture of epithermal neutrons and effects of chemical composition on the neutron energy distribution. Excess Ar-36 identified in the Arapahoe, Bruderheim, and Torino chondrites and the Shallowater aubrite suggest exposure to neutron fluences of approximately 0.2-0.2 x 10(exp 16) n/sq cm. Depletion of Sm-149 in Torino and the LEW86010 angrite suggest neutron fluences of 0.8 x 10(exp 16) n/sq cm and 0.25 x 10(exp 16) n/sq cm, respectively. Neutron fluences of approximately 10(exp 16) n/sq cm in Chico are almost as large as those previously observed for some lunar soils. Consideration of exposure ages suggests that the neutron flux in Chico may have been greater than that in many lunar soils.

Bogard, D. D.↗