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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 541 records · Page 30
All sourcesNASA NTRSDOE OSTI
DOE OSTI2010

Rotational dependence of the proton-transfer reaction HBr{sup +}+ CO{sub 2}{yields} HOCO{sup +}+ Br. II. Comparison of HBr{sup +} ({sup 2}{Pi}{sub 3/2}) and HBr{sup +} ({sup 2}{Pi}{sub 1/2})

The effects of reactant ion rotational excitation on the exothermic proton-transfer reactions of HBr{sup +}({sup 2}{Pi}{sub 1/2}) and DBr{sup +}({sup 2}{Pi}{sub 1/2}), respectively, with CO{sub 2} were studied in a guided ion beam apparatus. Cross sections are presented for collision energies in the center of mass system E{sub c.m.} in the range of 0.23 to 1.90 eV. The HBr{sup +}/DBr{sup +} ions were prepared in a state-selective manner by resonance enhanced multiphoton ionization. The mean rotational energy was varied from 3.4 to 46.8 meV for HBr{sup +}({sup 2}{Pi}{sub 1/2}) and from 1.8 to 40.9 meV for DBr{sup +}({sup 2}{Pi}{sub 1/2}). Both reactions studied are inhibited by collision energy, as expected for exothermic reactions. For all collision energies considered, the cross section decreases with increasing rotational energy of the ion, but the degree of the rotational dependence differs depending on the collision energy. For E{sub c.m.}= 0.31 eV, the cross sections of the deuteron transfer are significantly larger than those of the proton transfer. For higher E{sub c.m.} they differ very little. The current results for the exothermic proton transfer are systematically compared to previously published data for the endothermic proton transfer starting from HBr{sup +}({sup 2}{Pi}{sub 3/2}) [L. Paetow et al., J. Chem. Phys. 132, 174305 (2010)]. Additional new data regarding the latter reaction are presented to further confirm the conclusions. The dependences on rotational excitation found cannot be explained by the corresponding change in the total energy of the system. For both the endothermic and the exothermic reaction, the cross section is maximized for the smallest rotational energy, at least well above the threshold.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2015

Limitations to laser machining of silicon using femtosecond micro-Bessel beams in the infrared

We produce and characterize high-angle femtosecond Bessel beams at 1300-nm wavelength leading to nonlinearly ionized plasma micro-channels in both glass and silicon. With microjoule pulse energy, we demonstrate controlled through-modifications in 150-μm glass substrates. In silicon, strong two-photon absorption leads to larger damages at the front surface but also a clamping of the intensity inside the bulk at a level of ≈4 × 10{sup 11 }W cm{sup −2} which is below the threshold for volume and rear surface modification. We show that the intensity clamping is associated with a strong degradation of the Bessel-like profile. The observations highlight that the inherent limitation to ultrafast energy deposition inside semiconductors with Gaussian focusing [Mouskeftaras et al., Appl. Phys. Lett. 105, 191103 (2014)] applies also for high-angle Bessel beams.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2017

Contrasting behavior of covalent and molecular carbon allotropes exposed to extreme ultraviolet and soft x-ray free-electron laser radiation

All carbon materials, e.g., amorphous carbon (a-C) coatings and C 60 fullerene thin films, play an important role in short-wavelength free-electron laser (FEL) research motivated by FEL optics development and prospective nanotechnology applications. We investigate responses of a-C and C 60 layers to the extreme ultraviolet (SPring-8 Compact SASE Source in Japan) and soft x-ray (free-electron laser in Hamburg) free-electron laser radiation by Raman spectroscopy, differential interference contrast, and atomic force microscopy. A remarkable difference in the behavior of covalent (a-C) and molecular ( C 60 ) carbonaceous solids is demonstrated under these irradiation conditions. Low thresholds for ablation of a fullerene crystal (estimated to be around 0.15 eV/atom for C 60 vs 0.9 eV/atom for a-C in terms of the absorbed dose) are caused by a low cohesive energy of fullerene crystals. An efficient mechanism of the removal of intact C 60 molecules from the irradiated crystal due to Coulomb repulsion of fullerene-cage cation radicals formed by the ionizing radiation is revealed by a detailed modeling.

36 MATERIALS SCIENCE↗
DOE OSTI2013

Low-Dose Radiation Cataract and Genetic Determinants of Radiosensitivity

The lens of the eye is one of the most radiosensitive tissues in the body. Ocular ionizing radiation exposure results in characteristic, dose related, progressive lens changes leading to cataract formation. While initial, early stages of lens opacification may not cause visual disability, the severity of such changes progressively increases with dose until vision is impaired and cataract extraction surgery may be required. Because of the transparency of the eye, radiation induced lens changes can easily be followed non-invasively over time. Thus, the lens provides a unique model system in which to study the effects of low dose ionizing radiation exposure in a complex, highly organized tissue. Despite this observation, considerable uncertainties remain surrounding the relationship between dose and risk of developing radiation cataract. For example, a growing number of human epidemiological findings suggest significant risk among various groups of occupationally and accidentally exposed individuals and confidence intervals that include zero dose. Nevertheless, questions remain concerning the relationship between lens opacities, visual disability, clinical cataract, threshold dose and/or the role of genetics in determining radiosensitivity. Experimentally, the response of the rodent eye to radiation is quite similar to that in humans and thus animal studies are well suited to examine the relationship between radiation exposure, genetic determinants of radiosensitivity and cataractogenesis. The current work has expanded our knowledge of the low-dose effects of X-irradiation or high-LET heavy ion exposure on timing and progression of radiation cataract and has provided new information on the genetic, molecular, biochemical and cell biological features which contribute to this pathology. Furthermore, findings have indicated that single and/or multiple haploinsufficiency for various genes involved in DNA repair and cell cycle checkpoint control, such as Atm, Brca1 or Rad9, influence cataract development and thus radiosensitivity. These observations have direct applicability to various human populations including accidentally exposed individuals, interventional medical workers, astronauts and nuclear plant workers.

59 BASIC BIOLOGICAL SCIENCES↗
DOE OSTI2018

Magnetic-bottle and velocity-map imaging photoelectron spectroscopy of APS- (A = C14H10 or anthracene): electron structure, spin-orbit coupling of APS•, and dipole-bound state of APS-

Gaseous dibenzo-7-phosphanorbornadiene P-sulfide anions APS- (A = C14H10 or anthracene) were generated via electrospray ionization, and characterized by magnetic-bottle photoelectron spectroscopy, velocity-map imaging (VMI) photoelectron spectroscopy, and quantum chemical calculations. The electron affinity (EA) and spin-orbit splitting (SO) of the APS• radical are determined from the photoelectron spectra and Franck-Condon factor simulations to be EA = 2.62 ± 0.05 eV and SO splitting = 43 ± 7 meV. VMI photoelectron images show strong and sharp peaks near detachment threshold with an identical electron kinetic energy (eKE) of 17.9 meV at three different detachment wavelengths, which are therefore assigned due to autodetachment from dipole-bound anion states. The B3LYP/6-31++g(d,p) calculations indicate APS• has a dipole moment of 3.31 Debye, large enough to support a dipole-bound electron.

Dibenzo-7-phosphanorbornadiene P-sulfide, electron↗
DOE OSTI2020

Test GammaPix™ Radiation Detection Software with Smartphones

GammaPix™ is a smartphone application that uses smartphone cameras to detect ionizing radiation. Brookhaven National Laboratory (BNL) evaluated the performance of the software in detecting radioactive materials. For this purpose, a series of tests were conducted at the Radiation Calibration Facility Annex at BNL. The experiments included dose measurements with three types of NIST-traceable calibration sources, 60Co, 241Am, and 137Cs. The recorded results by GammaPix™ were compared with the values measured by calibrated dosimeters to determine the detection thresholds. Several selected models of iPhones and Android cell phones with different pixel sizes and resolution were tested. In this paper, we present the test procedures and discuss the test results.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Spectra and Kinetics of YAG:0.5%Er{sup 3+} Radiation Under Pulsed Laser Thermal Excitation

The dependences of single-crystal YAG:0.5%Er{sup 3+} spectra in the range 200–1700 nm and the kinetics of the integrated emission on the excitation-energy density W of a single CO{sub 2}-laser pulse of ~100 ns FWHM duration at λ{sub ex} = 10.6 μm were investigated experimentally. The spectra changed qualitatively when W exceeded the generation threshold W{sub t} of laser plasma near the single-crystal surface. The YAG:0.5%Er{sup 3+} spectra at W < Wt were represented by peaks of selective emission (SE) of Er{sup 3+} multiplets on the continuous spectrum background. New emission peaks and additional background corresponding to emission spectra in a laser-induced air plasma with intensities much higher than the SE peaks appeared due to air ionization near the crystal surface at W > W{sub t}. Oscillograms of the integral emission in the range 600–1700 nm were characterized by a pulse-front duration of τ{sub f} = 1.0–1.6 μs and a decay time τ{sub d} ≈ 2.5 μs if W changed by one order of magnitude. The kinetics of the integrated emission intensity were explained by calculating the single-crystal temperature and the populations of Er{sup 3+} energy levels during conversion of thermal energy into SE during unsteady energy transfer by internal radiation and thermal conductivity.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

A sub-5 ps jitter time-to-digital converter ASIC with back-gate delay tuning in 22 nm CMOS

We present the design of a Time-to-Digital Converter (TDC) ASIC together with performance characterization results at cryogenic temperature (6-8 K), and at room temperature using emulated Low-Gain Avalanche Detector (LGAD) signals. The TDC design uses a two-step architecture with a ring-oscillator based counter and a Vernier delay line fine TDC. The TDC is implemented in an FD-SOI process, and back-gate tuning is used not only to correct threshold variation due to cryogenic operation, but also as a novel way to tune TDC delay elements with very little overhead. Using this technique, we demonstrate a design with very low power (0.5 mW) and area (0.003 mm 2 ). We present test results using the Fermilab Constant Fraction Discriminator (FCFD) ASIC to produce discriminated signals from an internal charge injection mechanism that mimics the waveform and signal amplitude of minimum ionizing particles impinging on LGAD sensors. We characterize the time precision of the full system and verify that the TDC ASIC contributes a negligible amount to the total system time precision, fully consistent with the expected jitter contribution of less than 5 ps. In conclusion, the results presented here demonstrate the utility of our TDC for applications in physics and quantum communications.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Tonopah Test Range Air Monitoring: CY2017 Meteorological, Radiological, and Wind Transported Particulate Observations

In 1963, the U.S. Department of Energy (DOE) (formerly the Atomic Energy Commission [AEC]), implemented Operation Roller Coaster on the Tonopah Test Range (TTR) and an adjacent area of the Nevada Test and Training Range (NTTR) (formerly the Nellis Air Force Range). This operation resulted in radionuclide-contaminated soils at the Double Tracks site and Clean Slate I, II, and III sites. This report documents observations made during ongoing monitoring of radiological, meteorological, and dust conditions at stations installed adjacent to the Clean Slate sites and at the TTR Sandia National Laboratories (SNL) Range Operations Center (ROC). The primary objective of the monitoring effort is to support the DOE Environmental Management Nevada Program (EM NV) in the safe cleanup of the environmental legacy of nuclear device development and testing by determining if wind blowing across the Clean Slate sites is transporting particles of radionuclide-contaminated soil beyond the physical and administrative boundaries of the sites. The monitoring program underwent a significant change during 2017 with the decommissioning of one monitoring station and the establishment of three new stations. Station 400, located within TTR Area 3 and near the ROC, monitors conditions near the local workforce center and was in operation the full calendar year. Stations 401 and 403 are located on the northwest and southeast perimeter fence lines, respectively, of the Clean Slate III site. Station 401 operated throughout 2017, whereas Station 403 began operation at the end of April 2017. Stations 404 and 405 are along the northern and eastern boundary fence, respectively, at Clean Slate II and both began data collection at the end of April 2017. Also at the end of April, the Clean Slate I monitoring site, Station 402, was decommissioned. The stations are located to be generally downwind of the contaminated areas during either north-northwesterly or south-southeasterly winds, which are the predominant wind directions. The stations—which are similar in design to the Community Environmental Monitoring Program (CEMP) stations operating at locations surrounding the Nevada National Security Site and TTR—include meteorological instruments and continuous-flow, low-volume air samplers. Three pressurized ionization chambers for measuring gamma energy are in use at Stations 400, 401, and 403 (formerly at 402). Saltation sensors and saltation traps are deployed at the stations adjacent to the Clean Slate sites. Detailed meteorological data are recorded on data loggers, with periodic uploads via a satellite system to the Western Regional Climate Center (WRCC) at Desert Research Institute (DRI), to monitor instrument and site conditions. Air filter samples are collected every two weeks and the deposits in the saltation traps are collected when a sufficient sample mass for analysis has accumulated (generally a six- to eight-month interval). Dust transport by suspension and saltation is strongly dependent on wind speed. Concentrations of PM10 (particulate matter of aerodynamic diameter ≤10 micrometers [μm], a size fraction of small particles that are suspended in the air and can be easily inhaled) remain low until winds exceed approximately 32 km/hr (20 mph). Saltation particle counts also increase above the same general threshold wind speed. Wind speeds in excess of 32 km/hr (20 mph) occur less than three percent of the time. High winds are associated with two predominant directions: north-northwest and south. In 2017, the very highest winds were from the north, but all winds above 40 km/hr (25 mph) were approximately evenly split between south and northwest directions. The low-volume air samplers collect total suspended dust, and saltating particles are captured by the passive saltation traps, both for radiological analysis. Radionuclide monitoring at the ROC in TTR Area 3 (Station 400) found natural background levels of gross alpha and gross beta radiation. Similar background levels were found on filter samples analyzed using gamma and alpha spectroscopy. The gamma exposure rate data from pressurized ionization chambers (PIC) are comparable to those from the regional CEMP stations. Plutonium concentrations above background values were measured during 2017 from soil samples collected in passive saltation traps and on select air filters from the monitoring stations adjacent to the Clean Slate sites. The background for soils in the region is assumed to be 0.014 pCi/g plutonium-239+240 ( 239+240 Pu) as measured by Turner et al. (2003), whereas the background concentration of suspended 239+240Pu is assumed to be 9.5 x 10 -19 μCi/ml, which was determined by continuous air monitoring at the TTR airport in 1996 and 1997 (SNL, 1998). Background concentrations are exceeded by one to four orders of magnitude by the majority of samples from Clean Slate I, II, and III. The gross alpha and gross beta measurements of the air filters are also generally higher than those measured at the regional CEMP stations, although the gamma exposure rates determined by the PICs located at Clean Slate I and III are similar to CEMP measurements. The highest radionuclide concentrations of suspended dust are associated with individual filter samples from Clean Slate II Station 404 and Clean Slate III Station 401. Both of the stations are downwind of their respective sites during southerly winds, but they are also geographically closer to the highly contaminated detonation areas than the other monitoring stations. Considering all the analyzed samples, the 239+240Pu concentrations are generally higher for the Clean Slate II samples compared with those from Clean Slate III. The highest gross alpha and gross beta results are also observed for the Clean Slate II stations. The highest radionuclide concentrations are measured on the smaller (≤63 μm) saltation-sized particles and particulate matter collected downwind of each site. Nonetheless, traps oriented to collect dust moving toward the contamination areas also had plutonium concentrations significantly above background values, which is consistent with observations of low-level contamination dispersed beyond the fenced area. All the observed 239+240 Pu concentrations are below the risk-based action level (25 millirem per year, equivalent to a 239+240 Pu concentration of 4,120 pCi/g for an industrial worker scenario; U.S. DOE, 2014). The meteorological and particulate matter monitoring indicate that conditions for wind-borne contaminant movement exist at the Clean Slate sites, and that transport of radionuclide-contaminated soil by both suspension and saltation is occurring. The Corrective Action Unit (CAU) closure strategy uses a risk-based approach, whereby acceptable contaminant concentrations are determined as a function of anticipated human exposure. This strategy is consistent with the fence lines at the Clean Slate sites encircling areas of higher concentration and the observed presence of lower concentrations of contamination outside the fences.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2015

On the study of threshold intensity dependence on the gain and loss processes in laser induced spark ignition of molecular hydrogen

In the present work, a numerical analysis is performed to investigate the comparative contribution of the mechanisms responsible for electron gain and losses in laser spark ignition and plasma formation of H{sub 2}. The analysis considered H{sub 2} over pressure range 150 -3000 torr irradiated by a Nd:YAG laser radiation at wavelengths 1064 and 532 nm with pulse length 5.5 ns. The study based on a modified electron cascade model by one of the authors which solves numerically the time dependent Boltzmann equation as well as a set of rate equations that describe the rate of change of the excited states population. The model includes most of the physical processes that might take place during the interaction. Computations of The threshold intensity are performed for the combined and separate contribution of each of the gain and loss processes. Reasonable agreement with the measured values over the tested pressure range is obtained only for the case of the combined contribution. Basing on the calculation of the electron energy distribution function, the determined relations of the time evolution of the electrons density for selected values of the tested gas pressure region revealed that photo-ionization of the excited states could determine the time of electron generation and hence spark ignition. Collisional ionization contributes to this phenomenon only at the high pressure regime. Loss processes due to electron diffusion, vibrational excitation are found to have significant effect over examined pressure values for the two applied laser wavelengths.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2011

THE PITTSBURGH SLOAN DIGITAL SKY SURVEY Mg II QUASAR ABSORPTION-LINE SURVEY CATALOG

We present a catalog of intervening Mg II quasar absorption-line systems in the redshift interval 0.36 {<=} z {<=} 2.28. The catalog was built from Sloan Digital Sky Survey Data Release Four (SDSS DR4) quasar spectra. Currently, the catalog contains {approx}17, 000 measured Mg II doublets. We also present data on the {approx}44, 600 quasar spectra which were searched to construct the catalog, including redshift and magnitude information, continuum-normalized spectra, and corresponding arrays of redshift-dependent minimum rest equivalent widths detectable at our confidence threshold. The catalog is available online. A careful second search of 500 random spectra indicated that, for every 100 spectra searched, approximately one significant Mg II system was accidentally rejected. Current plans to expand the catalog beyond DR4 quasars are discussed. Many Mg II absorbers are known to be associated with galaxies. Therefore, the combination of large size and well understood statistics makes this catalog ideal for precision studies of the low-ionization and neutral gas regions associated with galaxies at low to moderate redshift. An analysis of the statistics of Mg II absorbers using this catalog will be presented in a subsequent paper.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2012

Shot-to-shot reproducibility in the emission of fast highly charged metal ions from a laser ion source

The generation of fast highly charged metal ions with the use of the sub-nanosecond Prague Asterix Laser System, operated at a fundamental wavelength of 1315 nm, is reported. Particular attention is paid to shot-to-shot reproducibility in the ion emission. Au and Pd targets were exposed to intensities up to 5 x 10{sup 16} W/cm{sup 2}. Above the laser intensity threshold of {approx}3 x 10{sup 14} W/cm{sup 2} the plasma is generated in a form of irregular bursts. The maximum energy of protons constituting the leading edge of the fastest burst reaches a value up to 1 MeV. The fast ions in the following bursts have energy gradually decreasing with the increasing burst number, namely, from a value of about 0.5 MeV/charge regardless of the atomic number and mass of the ionized species.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2011

K-SHELL PHOTOIONIZATION OF Na-LIKE TO Cl-LIKE IONS OF Mg, Si, S, Ar, AND Ca

We present R-matrix calculations of photoabsorption and photoionization cross sections across the K edge of Mg, Si, S, Ar, and Ca ions with more than 10 electrons. The calculations include the effects of radiative and Auger damping by means of an optical potential. The wave functions are constructed from single-electron orbital bases obtained using a Thomas-Fermi-Dirac statistical model potential. Configuration interaction is considered among all states up to n = 3. The damping processes affect the resonances converging to the K-thresholds causing them to display symmetric profiles of constant width that smear the otherwise sharp edge at the photoionization threshold. These data are important for the modeling of features found in photoionized plasmas.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2012

Effect of the Basic Residue on the Energetics and Dynamics of Dissociation of Phosphopeptides

Time- and collision-energy-resolved surface-induced dissociation (SID) of protonated peptides containing phosphoserine (s) was studied using a Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer configured for SID experiments. We examined fragmentation of three singly protonated peptides: GGGsGGG, KGGsGGG, and RGGsGGG. Fragmentation of GGGsGGG occurs under the mobile proton condition, while the ionizing proton is sequestered by the basic residue, resulting in the nonmobile proton condition in dissociation of the two basic peptides: KGGsGGG and RGGsGGG. RRKM modeling of the experimental data demonstrates that the energetics and dynamics of H3PO4 loss are different under mobile and nonmobile proton conditions. Specifically, fragmentation of GGGsGGG is characterized by a higher dissociation barrier, 1.68 eV, and higher activation entropy, 11 e.u. (e.u. = entropy unit), than fragmentation of the basic peptides. Similar threshold energies of 1.36 eV and 1.40 eV and activation entropies of -4.9 e.u. and 0.3 e.u. were obtained for KGGsGGG and RGGsGGG, respectively. We propose that the loss of H3PO4 from phosphoserine is a two-step process, in which the phosphate abstraction from the phosphorylated side chain is followed by dissociation of the ion-molecule complex.

Environmental Molecular Sciences Laboratory↗
DOE OSTI2016

Detection of Special Nuclear Material in Cargo using Continuous Neutron Interrogation and Tension Metastable Fluid Detectors

This paper presents results using a novel technique for detecting special nuclear materials (SNMs) based on interrogation with a continuous beam of 2.45 MeV neutrons coupled with high intrinsic efficiency tensioned metastable fluid detectors (TMFDs) operated in threshold rejection mode. While passive interrogation may be utilized for detecting SNMs such as {sup 239}Pu from their strong spontaneous fission neutron signatures, this is not so for highly-enriched uranium (HEU), the timely detection of which has been identified as a grand challenge by the U.S. Domestic Nuclear Detection Office (DNDO). Active (neutron and/or photon based) interrogation represents the only viable means for detecting HEU either shielded or unshielded within cargo containers. Active interrogation by neutrons or photons leads to unequivocal induced fission based signatures in terms of neutron energy and multiplicity. The main challenge under such circumstances pertains to being able to discern the relatively weak emission signatures from the intense interrogation pulses of neutrons and/or photons. Purdue University together with Sagamore Adams Laboratories, LLC (SAL) has been developing the TMFD sensor system that promises to provide high neutron detection efficiency for fast and thermal neutrons while remaining gamma-beta blind. As described in these references, the TMFD sensor system works on the principle of transient cavitation detection events (CDEs) caused by ionizing particles such as neutrons, alphas and fission fragments in fluids that have been placed in various states of tensioned (sub-zero) pressure states of fluid metastability. Such CDEs result in recordable signatures - both electronically as for conventional detectors, but also in the form of audio-visual signals. One key advantage that the TMFD holds over conventional neutron detectors is that it has proven gamma-beta 'blindness' and indeed, confirmed to possess GARRn = 1.0 to γ photons (tested in up to 10{sup 11} γ/s field from a 3 Ci {sup 137}Cs source). Such an enablement allows for detection without saturation from background, interrogating and fission created γ photons. Another key attribute is up to 60 % intrinsic fission spectrum neutron detection efficiency which, furthermore, is amenable to tailoring for threshold based rejection. That is, to be able to detect neutrons at or above a desired energy with good efficiency, while remaining relatively blind to neutrons below the chosen threshold. This research is the subject of our ongoing DNDO project at Purdue University, the results of which form the basis of this paper. (authors)

07 ISOTOPE AND RADIATION SOURCES↗
DOE OSTI2011

K-SHELL PHOTOIONIZATION OF NICKEL IONS USING R-MATRIX

We present R-matrix calculations of photoabsorption and photoionization cross sections across the K edge of the Li-like to Ca-like ion stages of Ni. Level-resolved, Breit-Pauli calculations were performed for the Li-like to Na-like stages. Term-resolved calculations, which include the mass-velocity and Darwin relativistic corrections, were performed for the Mg-like to Ca-like ion stages. This data set is extended up to Fe-like Ni using the distorted wave approximation as implemented by AUTOSTRUCTURE. The R-matrix calculations include the effects of radiative and Auger dampings by means of an optical potential. The damping processes affect the absorption resonances converging to the K thresholds causing them to display symmetric profiles of constant width that smear the otherwise sharp edge at the K-shell photoionization threshold. These data are important for the modeling of features found in photoionized plasmas.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2023

Scintillation light detection performance for the DUNE ND-LAr 2 × 2 modules

The Deep Underground Neutrino Experiment (DUNE) will be using a liquid argon time projection chamber (LAr TPC) with optically separated modules in the Near Detector (ND) complex. A prototype experiment, DUNE ND-LAr 2 × 2, is composed of four test modules. They detect ionization charge through a pixel-based readout and scintillation light through fibers in light collection modules and light traps called ArCLights. The light detection performance for two modules of DUNE ND-LAr 2 × 2 that took cosmic ray data at the University of Bern is shown. We present further the role of the 2 × 2 prototype in DUNE and how it is used to demonstrate the reconstruction capabilities of its light detectors in terms of energy thresholds and timing resolution.

47 OTHER INSTRUMENTATION↗
DOE OSTI2014

Sci—Fri PM: Dosimetry—06: Commissioning of a 3D patient specific QA system for hypofractionated prostate treatments

The objective of this work is to commission the 6MV-SRS beam model in COMPASS (v2.1, IBA-Dosimetry) and validate its use for patient specific QA of hypofractionated prostate treatments. The COMPASS system consists of a 2D ion chamber array (MatriXX{sup Evolution}), an independent gantry angle sensor and associated software. The system can either directly calculate or reconstruct (using measured detector responses) a 3D dose distribution on the patient CT dataset for plan verification. Beam models are developed and commissioned in the same manner as a beam model is commissioned in a standard treatment planning system. Model validation was initially performed by comparing both COMPASS calculations and reconstructions to measured open field beam data. Next, 10 hypofractionated prostate RapidArc plans were delivered to both the COMPASS system and a phantom with ion chamber and film inserted. COMPASS dose distributions calculated and reconstructed on the phantom CT dataset were compared to the chamber and film measurements. The mean (± standard deviation) difference between COMPASS reconstructed dose and ion chamber measurement was 1.4 ± 1.0%. The maximum discrepancy was 2.6%. Corresponding values for COMPASS calculation were 0.9 ± 0.9% and 2.6%, respectively. The average gamma agreement index (3%/3mm) for COMPAS reconstruction and film was 96.7% and 95.3% when using 70% and 20% dose thresholds, respectively. The corresponding values for COMPASS calculation were 97.1% and 97.1%, respectively. Based on our results, COMPASS can be used for the patient specific QA of hypofractionated prostate treatments delivered with the 6MV-SRS beam.

62 RADIOLOGY AND NUCLEAR MEDICINE↗