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At least 559 records · Page 31

SAGE III/ISS Data Product Improvements

In 2024 the Stratospheric Aerosol and Gas Experiment on the International Space Station (SAGE III/ISS) entered its eighth year of operations. Using a CCD spectrometer to observe solar and lunar occultations through Earth’s limb, the mission has retrieved tens of thousands of vertical profiles for ozone, aerosol, water vapor, and nitrogen dioxide. Retrieval algorithms are constantly under development to enhance these products. The next product version will improve upon previous versions by addressing problems with the aerosol extinction spectrum and recovering hundreds of profiles impeded by the recent proliferation of sunspots. Users of SAGE III/ISS data can also expect improvements to uncertainty estimates and a continued expansion of ancillary products.

Robert Manion↗

Humidified single-scattering albedometer (H-CAPS-PM SSA ): Design, data analysis, and validation

In this work, we report the development and validation of a new humidified aerosol single-scattering albedometer to quantify the effects of water uptake on submicrometer particle optical properties. The instrument simultaneously measures in situ aerosol light extinction ( σ ep ) and scattering ( σ sp ) using a cavity-attenuated phase shift-single scattering albedo particulate matter (PM) monitor (CAPS-PM SSA , Aerodyne Research, Inc., Billerica, MA, USA). It retrieves by difference aerosol light absorption ( σ ap ) and directly quantifies aerosol single-scattering albedo (SSA), the aerosol “brightness.” We custom built a relative humidity (RH) control system using a water vapor-permeable membrane humidifier and coupled it to the CAPS-PM SSA to enable humidified aerosol observations. Our humidified instrument (H-CAPS-PM SSA ) overcomes problems with noise caused by mirror purge-flow humidification, heating, and characterizing cell RH. Careful angular truncation corrections in scattering, particularly for larger particles, were combined with empirical observations. Results show that the optimal operational size to be D p < 400 nm. The H-CAPS-PM SSA was evaluated with several pure single-component aerosols including ammonium sulfate ((NH 4 ) 2 SO 4 ), absorbing nigrosin, and levoglucosan, an organic biomass smoke tracer. The measured σ ep , σ sp , and the derived optical hygroscopicity parameter ( κ ) for size-selected ammonium sulfate are in good agreement with literature values. For dry size-selected nigrosin in the 100 < D p < 400 nm range, SSA values increased from ~0.3 to 0.65 with increasing D p . The enhancement in nigrosin σ ap at RH = 80% was a factor of 1.05–1.20 relative to dry conditions, with the larger particles showing greater enhancement. SSA increased with RH with the largest fractional enhancement measured for the smallest particles. For polydisperse levoglucosan, we measured an optical κ of 0.26 for both light extinction and scattering and negligible absorption. Our new instrument enables reliable observations of the effects of ambient humidity on mixed aerosol optical properties, particularly for light-absorbing aerosols whose climate forcing is uncertain due to measurement gaps.

54 ENVIRONMENTAL SCIENCES↗

RingIR AG-4000 Testing

The AG-4000 detector can identify gas phase species using molecular fingerprinting and has potential application for SARS-CoV-2 detection in near real time. As part of the development process Sandia will utilize the biological aerosol test bed deployed at the Aerosol Complex to evaluate the penetration of MS2 bacteriophage aerosol through the Ring IR system. The objective of this project is to provide experimentally derived measurements of the RingIR AG-4000 penetration efficiency, including external exhaust filter for mitigation of exhaust aerosol and operation using MS2 bacteriophage as a biological surrogate to the SARS-CoV-2 virus.

60 APPLIED LIFE SCIENCES↗

Shallow- and deep-convection characteristics in the greater Houston, Texas, area using cell tracking methodology

The convective lifecycle, from initiation to maturity and dissipation, is driven by a combination of kinematic, thermodynamic, microphysical, and radiative processes that are strongly coupled and variable in time and space. Weather radars have been traditionally used to provide various convective-cloud characteristics. Here, we analyzed climatological convective-cell radar characteristics to obtain and assess the diurnal cycles of three convective-cell types – shallow, modest deep, and vigorous deep convective cells – that formed in the greater Houston area, using the National Weather Service radar from Houston, Texas, and a multi-cell identification and tracking algorithm. The examined dataset spans 4 years (2018–2021) and covers the warm-season months (June to September) in those years. The analysis showed clear diurnal cycles in cell initiation (CI) consistent with the sea breeze circulation and showed diurnal and normalized lifetime relationships in cell evolution parameters (e.g., maximum reflectivity, echo-top height, Geostationary Operational Environmental Satellite-16 (GOES-16) channel 13 brightness temperature, and the height of maximum reflectivity). The cell evolution is well represented by relationships between (1) the height and value of the maximum radar reflectivity, (2) the minimum GOES-16 channel 13 brightness temperature and the maximum vertically integrated liquid, (3) the maximum reflectivity and columnar-average reflectivity, and (4) the echo-top ascent rate and cell lifetime. The relationships presented herein help to identify the cell lifecycle stages such as early shallow convection, vigorous vertical development, anvil development, and convective core dissipation. GOES-16 Aerosol Optical Depth values are also used as a proxy for cell initiation aerosol concentrations to investigate any potential relationships between initiation location and aerosol concentration. Overall, no significant relationships between initiation location and aerosol concentration were found for the three cell types investigated, but there are some minor differences in the pre-CI aerosol optical depth for vigorous deep convective cells.

54 ENVIRONMENTAL SCIENCES↗

Long-term measurements of ice nucleating particles at Atmospheric Radiation Measurement (ARM) sites worldwide

Ice nucleating particles (INPs) play a critical role in cloud microphysics and precipitation formation, yet long-term, spatially extensive observational datasets remain limited. Here, we present one of the most comprehensive publicly available datasets of immersion-mode INP concentrations using a single analytical method, generated through the U.S. Department of Energy's (DOE) Atmospheric Radiation Measurement (ARM) user facility. INP filter samples have been collected across a broad range of environments – including agricultural plains, Arctic coastlines, high-elevation mountain sites, marine regions, and urban areas – via fixed observatories, mobile facility deployments, and vertically-resolved tethered balloon system operations. We describe the standardized processing and quality assurance pipeline, from filter collection and processing using the Ice Nucleation Spectrometer to final data products archived on the ARM Data Discovery portal. The dataset includes both total INP concentrations and selectively treated samples, allowing for classification of biological, organic, and inorganic INP types. It features a continuous 5-year record of INP measurements from a central U.S. site, with data collection still ongoing. Seasonal and site-specific differences in INP concentrations are illustrated through intercomparisons at −10 and −20 °C, revealing distinct regional sources and atmospheric drivers. We also outline mechanisms for researchers to access existing data, request additional sample analyses, and propose future field campaigns involving ARM INP measurements. This dataset supports a wide range of scientific applications, from observational and mechanistic studies to model development, and provides critical constraints on aerosol-cloud interactions across diverse atmospheric regimes (Creamean et al., 2024, 2020b; https://doi.org/10.5439/1770816).

Creamean, Jessie M. [Colorado State Univ., Fort Co↗

The E3SM version 1 single-column model

Abstract. The single-column model (SCM) functionality of the Energy Exascale Earth System Model version 1 (E3SMv1) is described in this paper. The E3SM SCM was adopted from the SCM used in the Community Atmosphere Model (CAM) but has evolved significantly since then. We describe changes made to the aerosol specification in the SCM, idealizations, and developments made so that the SCM uses the same dynamical core as the full general circulation model (GCM) component. Based on these changes, we describe and demonstrate the seamless capability to “replay” a GCM column using the SCM. We give an overview of the E3SM case library and briefly describe which cases may serve as useful proxies for replicating and investigate some long-standing biases in the full GCM runs while demonstrating that the E3SM SCM is an efficient tool for both model development and evaluation.

54 ENVIRONMENTAL SCIENCES↗

Design of an airborne lidar for stratospheric aerosol measurements

A modular, multiple-telescope receiving concept is developed to gain a relatively large receiver collection aperture without requiring extensive modifications to the aircraft. This concept, together with the choice of a specific photodetector, signal processing, and data recording system capable of maintaining approximately 1% precision over the required large signal amplitude range, is found to be common to all of the options. It is recommended that development of the lidar begin by more detailed definition of solutions to these important common signal detection and recording problems.

Evans, W. E.↗

A lidar instrument to measure H2O and aerosol profiles from the NASA ER-2 aircraft

Plans to develop the Lidar Atmospheric Sensing Experiment (LASE) instrument to conduct scientific experiments aboard a NASA U-2 (ER-2) aircraft are described. The LASE measurement objectives are listed, and the design of the LASE instrument is discussed, including performance criteria for the laser transmitter, wavemeter, telescope, optical receiver, and associated electronics. The instrument function is depicted with a block diagram, and layouts of various components are presented.

Vaughan, W. R.↗

On the growth of nitric and sulfuric acid aerosol particles under stratospheric conditions

A theory for the formation of frozen aerosol particles in the Antarctic stratosphere was developed and applied to the formation of polar stratospheric clouds. The theory suggests that the condensed ice particles are composed primarily of nitric acid and water, with small admixtures of sulfuric and hydrochloric acids in solid solution. The proposed particle formation mechanism is in agreement with the magnitude and seasonal behavior of the optical extinction observed in the winter polar stratosphere.

Hamill, Patrick↗

Theoretical simulation of a 2 micron airborne solid state laser anemometer

In the near future, military aircraft will need to know precisely their true airspeed in order to optimize flight conditions. In comparison with classical anemometer probes, an airborne Doppler lidar allows measurement of the air velocity without influence from aircraft aerodynamic disturbance. While several demonstration systems of heterodyne detection using a CO2 laser have been reported, improvements in the technology of solid state lasers have recently opened up the possibility that these devices can be used as an alternative to CO2 laser systems. In particular, a diode pumped Tm:Ho:YAG laser allows a reliable compact airborne system with an eye safe wavelength (lambda = 2.09 microns) to be achieved. The theoretical study of performances of a coherent lidar using a solid state diode pumped Tm:Ho:YAG laser, caled SALSA, for measuring aircraft airspeed relative to atmospheric aerosols is described. A computer simulation was developed in order to modelize the Doppler anemometer in the function of atmospheric propagation and optical design. A clever analysis of the power budget on the detector area allows optical characteristic parameters of the system to be calculated, and then it can be used to predict performances of the Doppler system. Estimating signal to noise ratios (SNR) and heterodyne efficiency provides the available energy of speed measurement as well as a useful measurement of the alignment of the backscattered and reference fields on the detector.

Imbert, Beatrice↗

AVIRIS user's guide

This paper serves as a brief overview of the AVIRIS instrument (Airborne Visible/Infrared Imaging Spectrometer). The AVIRIS sensor collects data that will be used for quantitative characterization of the Earth's surface and atmosphere from geometrically coherent spectroradiometric measurements. This data can be applied to studies in the fields of oceanography, environmental science, snow hydrology, geology, volcanology, soil and land management, atmospheric and aerosol studies, agriculture, and limnology. Applications under development include the assessment and monitoring of environmental hazards such as toxic waste, oil spills, and land/air/water pollution. Mission planning and flight operations are discussed, and recommendations are given regarding the deployment of ground truth experiments.

Johnson, Howell K.↗

Status of the Geostationary Spectrograph (GeoSpec) for Earth and Atmospheric Science Applications

GeoSpec will support future satellite mission concepts in the Atmospheric Sciences and in Land and Ocean Sciences by providing time-resolved measurements of both chemically linked atmospheric trace gas concentrations of important molecules such as O3, NO2, CH2O and SO2 and at the same time coastal and ocean pollution events, tidal effects, and the origin and evolution of aerosol plumes. The instrument design concept in development is a dual spectrograph covering the WMS wavelength region of 310-500 nm and the VIS/NIR wavelength region of 480-900 nm coupled to all reflective telescope and high sensitivity PIN/CMOS area detector. The goal of the project is to demonstrate a system capable of making moderate spatial resolution (750 meters at nadir) hyperspectral measurements (0.6 to 1.2 nm resolution) from a geostationary orbit. This would enable studies of time-varying pollution and coastal change processes with a temporal resolution of 5 minutes on a regional scale to 1 hour on a continental scale. Other spatial resolutions can be supported by varying the focal length of the input telescope. Scientific rationale and instrument design and status will be presented.

Janz, Scott↗

WIND MEASUREMENTS WITH HIGH-ENERGY DOPPLER LIDAR

Coherent lidars at 2-micron wavelengths from holmium or thulium solid-state lasers have been in use to measure wind for applications in meteorology, aircraft wake vortex tracking, and turbulence detection [1,2,3] These field-deployed lidars, however, have generally been of a pulse energy of a few millijoules, limiting their range capability or restricting operation to regions of high aerosol concentration such as the atmospheric boundary layer. Technology improvements in the form of high-energy pulsed lasers, low noise detectors, and high optical quality telescopes are being evaluated to make wind measurements to long ranges or low aerosol concentrations. This research is aimed at developing lidar technology for satellite-based observation of wind on a global scale. The VALIDAR project was initiated to demonstrate a high pulse energy coherent Doppler lidar. VALIDAR gets its name from the concept of validation lidar, in that it can serve as a calibration and validation source for future airborne and spaceborne lidar missions. VALIDAR is housed within a mobile trailer for field measurements.

Koch, Grady J.↗

A Machine Learning Approach for the Remote Sensing Retrieval of Oil Spills from Polarimetric Measurements

The Fresnel laws of specular reflection directly connect remote sensing observations of light polarization within the sunglint region to the ocean surface refractive index. This parameter is instrumental to identify areas affected by oil, or any other floating substance capable of modifying the refractive index of pure seawater. In preparation for the NASA Plankton, Aerosol, ocean Ecosystem (PACE) mission, we are developing an advanced retrieval scheme that exploits such measurements to deliver the refractive index as an operational product. The original method was developed based on observations of the airborne Research Scanning Polarimeter. Here we present several aspects related to the extension of this technique to the PACE HARP-2 sensor (especially regarding the projected accuracy), and discuss preliminary results obtained by applying neural-network trainings to look-up tables produced with the forward radiative transfer code, with the goal of improving the computational performance. Success in the final implementation will guarantee a version of the retrieval algorithm suitable to fast-response needs and disaster management.

machine learning↗

Durable Anti-Reflective and Anti-Fog Coatings Produced by Aerosol Impact Driven Assembly

The Exploration Extravehicular Mobility Unit’s (xEMU) helmet is a complex assembly designed to accomplish several tasks to protect and enable astronauts. In addition to maintaining a suitable environment for the wearer, it must also allow for appropriate mobility and provide a wide and undistorted view of the surroundings. A critical component of the helmet’s optical system is the anti-fog coating. While previous versions of the anti-fog coating have provided suitable anti-fog performance, they have been difficult to apply, lacked mechanical or chemical durability, or resulted in unanticipated failures (e.g., outgassing of eye-irritating materials during use). This work describes the use of a new coating technology, aerosol impact-driven assembly (AIDA), to develop a next-generation permanent anti-fog coating for the xEMU helmet. AIDA’s unique ability to tune both the refractive index and surface roughness of films was used to deposit a thin, transparent (>85% transmittance of visible light), and hydrophilic (contact angle <10°) anti-fog coating. The coating’s abrasion resistance and chemical resistance was evaluated and it was found that the coating maintained both its anti-fog and anti-reflective functionally. Finally, the scalability of the process was demonstrated by successfully coating the polycarbonate blanks used to form the helmet’s bubble.

Spacesuit↗

Extensive Characterization of Aerosol Optical Properties and Chemical Component Concentrations: Application of the GRASP/Component Approach to Long-term AERONET Measurements

A recently developed GRASP/Component approach (GRASP: Generalized Retrieval of Atmosphere and Surface Properties) was applied to AERONET (Aeronet Robotic Network) sun photometer measurements in this study. Unlike traditional aerosol component retrieval, this approach allows the inference of some information about aerosol composition directly from measured radiance, rather than indirectly through the inversion of optical parameters, and has been integrated into the GRASP algorithm. The newly developed GRASP/Component approach was applied to 13 AERONET sites for different aerosol types under the assumption of aerosol internal mixing rules to analyze the characteristics of aerosol components and their distribution patterns. The results indicate that the retrievals can characterize well the spatial and temporal variability of the component concentration for different aerosol types. A reasonable agreement between GRASP BC retrievals and MERRA-2 BC products is found for all different aerosol types. In addition, the relationships between aerosol component content and aerosol optical parameters such as aerosol optical depth (AOD), fine-mode fraction (FMF), absorption Ångström exponent (AAE), scattering Ångström exponent (SAE), and single scattering albedo (SSA) are also analyzed for indirect verifying the reliability of the component retrieval. It was demonstrated the GRASP/Component optical retrievals are in good agreement with AERONET standard products [e.g., correlation coefficient (R) of 0.93–1.0 for AOD, fine-mode AOD (AODF), coarse-mode AOD (AODC) and Ångström exponent (AE); R = ~ 0.8 for absorption AOD (AAOD) and SSA; RMSE (root mean square error) < 0.03 for AOD, AODF, AODC, AAOD and SSA]. Thus, it is demonstrated the GRASP/Component approach can provide aerosol optical products with comparable accuracy as the AERONET standard products from the ground-based sun photometer measurements as well as some additional important inside on aerosol composition.

Xindan Zhang↗

Visualization of Atmospheric Water Vapor Data for SAGE

The goal of this project was to develop visualization tools to study the water vapor dynamics using the Stratospheric Aerosol and Gas Experiment 11 (SAGE 11) water vapor data. During the past years, we completed the development of a visualization tool called EZSAGE, and various Gridded Water Vapor plots, tools deployed on the web to provide users with new insight into the water vapor dynamics. Results and experiences from this project, including papers, tutorials and reviews were published on the main Web page. Additional publishing effort has been initiated to package EZSAGE software for CD production and distribution. There have been some major personnel changes since Fall, 1998. Dr. Mou-Liang Kung, a Professor of Computer Science assumed the PI position vacated by Dr. Waldo Rodriguez who was on leave. However, former PI, Dr. Rodriguez continued to serve as a research adviser to this project to assure smooth transition and project completion. Typically in each semester, five student research assistants were hired and trained. Weekly group meetings were held to discuss problems, progress, new research direction, and activity planning. Other small group meetings were also held regularly for different objectives of this project. All student research assistants were required to submit reports for conference submission.

Kung, Mou-Liang↗

Emulating aerosol optics with randomly generated neural networks

Abstract. Atmospheric aerosols have a substantial impact on climate and remain one of the largest sources of uncertainty in climate prediction. Accurate representation of their direct radiative effects is a crucial component of modern climate models. However, direct computation of the radiative properties of aerosol populations is far too computationally expensive to perform in a climate model, so optical properties are typically approximated using a parameterization. This work develops artificial neural networks (ANNs) capable of replacing the current aerosol optics parameterization used in the Energy Exascale Earth System Model (E3SM). A large training dataset is generated by using Mie code to directly compute the optical properties of a range of atmospheric aerosol populations given a large variety of particle sizes, wavelengths, and refractive indices. Optimal neural architectures for shortwave and longwave bands are identified by evaluating ANNs with randomly generated wirings. Randomly generated deep ANNs are able to outperform conventional multilayer-perceptron-style architectures with comparable parameter counts. Finally, the ANN-based parameterization produces significantly more accurate bulk aerosol optical properties than the current parameterization when compared with direct Mie calculations using mean absolute error. The success of this approach makes possible the future inclusion of much more sophisticated representations of aerosol optics in climate models that cannot be captured by extension of the existing parameterization scheme and also demonstrates the potential of random-wiring-based neural architecture search in future applications in the Earth sciences.

54 ENVIRONMENTAL SCIENCES↗