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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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DOE OSTI2016

Interactive Correlation Analysis and Visualization of Climate Data

The relationship between our ability to analyze and extract insights from visualization of climate model output and the capability of the available resources to make those visualizations has reached a crisis point. The large volume of data currently produced by climate models is overwhelming the current, decades-old visualization workflow. The traditional methods for visualizing climate output also have not kept pace with changes in the types of grids used, the number of variables involved, and the number of different simulations performed with a climate model or the feature-richness of high-resolution simulations. This project has developed new and faster methods for visualization in order to get the most knowledge out of the new generation of high-resolution climate models. While traditional climate images will continue to be useful, there is need for new approaches to visualization and analysis of climate data if we are to gain all the insights available in ultra-large data sets produced by high-resolution model output and ensemble integrations of climate models such as those produced for the Coupled Model Intercomparison Project. Towards that end, we have developed new visualization techniques for performing correlation analysis. We have also introduced highly scalable, parallel rendering methods for visualizing large-scale 3D data. This project was done jointly with climate scientists and visualization researchers at Argonne National Laboratory and NCAR.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2014

A spectral transform dynamical core option within the Community Atmosphere Model (CAM4)

A spectral transform dynamical core with an 85 spectral truncation resolution (T85) within the Community Atmosphere Model (CAM), version 4, is evaluated within the recently released Community Earth System Model, version 1.0 (CESM) global climate model. The spectral dynamical core option provides a well-known base within the climate model community from which to assess climate behavior and statistics, and its relative computational efficiency for smaller computing platforms allows it to be extended to perform climate length simulations using high-resolution configurations in the near term. To establish the characteristics of the CAM4 T85, an ensemble of simulations covering the present day observational period using forced sea surface temperatures and prescribed sea-ice extent are evaluated. Overall, the T85 ensemble attributes and biases are similar to a companion ensemble of simulations using the one degree finite volume (FV1) dynamical core, relative to observed and model derived datasets. Notable improvements with T85 compared to FV1 include the representation of wintertime Arctic sea level pressure and summer precipitation over the Western Indian subcontinent. The mean and spatial patterns of the land surface temperature trends over the AMIP period are generally well simulated with the T85 ensemble relative to observations, however the model is not able to capture the extent nor magnitude of changes in temperature extremes over the boreal summer, where the changes are most dramatic. Biases in the wintertime Arctic surface temperature and annual mean surface stress fields persist with T85 as with the CAM3 version of T85.

atmosphere model analysis↗
DOE OSTI2023

Fusing time-varying mosquito data and continuous mosquito population dynamics models

Climate change is arguably one of the most pressing issues affecting the world today and requires the fusion of disparate data streams to accurately model its impacts. Mosquito populations respond to temperature and precipitation in a nonlinear way, making predicting climate impacts on mosquito-borne diseases an ongoing challenge. Data-driven approaches for accurately modeling mosquito populations are needed for predicting mosquito-borne disease risk under climate change scenarios. Many current models for disease transmission are continuous and autonomous, while mosquito data is discrete and varies both within and between seasons. This study uses an optimization framework to fit a non-autonomous logistic model with periodic net growth rate and carrying capacity parameters for 15 years of daily mosquito time-series data from the Greater Toronto Area of Canada. The resulting parameters accurately capture the inter-annual and intra-seasonal variability of mosquito populations within a single geographic region, and a variance-based sensitivity analysis highlights the influence each parameter has on the peak magnitude and timing of the mosquito season. This method can easily extend to other geographic regions and be integrated into a larger disease transmission model. This method addresses the ongoing challenges of data and model fusion by serving as a link between discrete time-series data and continuous differential equations for mosquito-borne epidemiology models.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2023

Important ice processes are missed by the Community Earth System Model (CESM) in Southern Ocean mixed–phase clouds: Bridging SOCRATES observations to model developments

Global climate models (GCMs) are challenged by difficulties in simulating cloud phase and cloud radiative effect over the Southern Ocean (SO). Some of the new generation GCMs predict too much liquid and too little ice in mixed-phase clouds. This misrepresentation of cloud phase in GCMs results in weaker negative cloud feedback over the SO and a higher climate sensitivity. Based on a model comparison with observational data obtained during the Southern Ocean Cloud Radiation and Aerosol Transport Experimental Study (SOCRATES), this study addresses a key uncertainty in the Community Earth System Model version 2 (CESM2) related to cloud phase, namely ice formation in pristine remote SO clouds. It is found that sea spray organic aerosols (SSOA) are the most important type of ice nucleating particles (INPs) over the SO with concentrations one order of magnitude higher than those of dust INPs based on measurements and CESM2 simulations. Secondary ice production (SIP) which includes riming splintering, rain droplet shattering, and ice-ice collisional fragmentation as implemented in CESM2 is the dominant ice production process in moderately cold clouds with cloud temperatures greater than –20°C. SIP enhances the in-cloud ice number concentrations (Ni) by 1-3 orders of magnitude and predicts more mixed-phase (with percentage occurrence increased from 15% to 21%), in better agreement with the observations. Finally, this study highlights the importance of accurately representing cloud phase over the pristine remote SO by considering the ice nucleation of SSOA and SIP processes, which are currently missing in most GCM cloud microphysics parameterizations.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2015

A unified parameterization of clouds and turbulence using CLUBB and subcolumns in the Community Atmosphere Model

Most global climate models parameterize separate cloud types using separate parameterizations. This approach has several disadvantages, including obscure interactions between parameterizations and inaccurate triggering of cumulus parameterizations. Alternatively, a unified cloud parameterization uses one equation set to represent all cloud types. Such cloud types include stratiform liquid and ice cloud, shallow convective cloud, and deep convective cloud. Vital to the success of a unified parameterization is a general interface between clouds and microphysics. One such interface involves drawing Monte Carlo samples of subgrid variability of temperature, water vapor, cloud liquid, and cloud ice, and feeding the sample points into a microphysics scheme.This study evaluates a unified cloud parameterization and a Monte Carlo microphysics interface that has been implemented in the Community Atmosphere Model (CAM) version 5.3. Results describing the mean climate and tropical variability from global simulations are presented. The new model shows a degradation in precipitation skill but improvements in short-wave cloud forcing, liquid water path, long-wave cloud forcing, precipitable water, and tropical wave simulation. Also presented are estimations of computational expense and investigation of sensitivity to number of subcolumns.

58 GEOSCIENCES↗
DOE OSTI2020

Pacific decadal oscillation remotely forced by the equatorial Pacific and the Atlantic Oceans

Abstract The Pacific Decadal Oscillation (PDO), the leading mode of Pacific decadal sea surface temperature variability, arises mainly from combinations of regional air-sea interaction within the North Pacific Ocean and remote forcing, such as from the tropical Pacific and the Atlantic. Because of such a combination of mechanisms, a question remains as to how much PDO variability originates from these regions. To better understand PDO variability, the equatorial Pacific and the Atlantic impacts on the PDO are examined using several 3-dimensional partial ocean data assimilation experiments conducted with two global climate models: the CESM1.0 and MIROC3.2m. In these partial assimilation experiments, the climate models are constrained by observed temperature and salinity anomalies, one solely in the Atlantic basin and the other solely in the equatorial Pacific basin, but are allowed to evolve freely in other regions. These experiments demonstrate that, in addition to the tropical Pacific’s role in driving PDO variability, the Atlantic can affect PDO variability by modulating the tropical Pacific climate through two proposed processes. One is the equatorial pathway, in which tropical Atlantic sea surface temperature (SST) variability causes an El Niño-like SST response in the equatorial Pacific through the reorganization of the global Walker circulation. The other is the north tropical pathway, where low-frequency SST variability associated with the Atlantic Multidecadal Oscillation induces a Matsuno-Gill type atmospheric response in the tropical Atlantic-Pacific sectors north of the equator. These results provide a quantitative assessment suggesting that 12–29% of PDO variance originates from the Atlantic Ocean and 40–44% from the tropical Pacific. The remaining 27–48% of the variance is inferred to arise from other processes such as regional ocean-atmosphere interactions in the North Pacific and possibly teleconnections from the Indian Ocean.

Meteorology & Atmospheric Sciences↗
DOE OSTI2013

Collaborative Research: Towards Advanced Understanding and Predictive Capability of Climate Change in the Arctic Using a High-Resolution Regional Arctic Climate System Model

The motivation for this project was to advance the science of climate change and prediction in the Arctic region. Its primary goals were to (i) develop a state-of-the-art Regional Arctic Climate system Model (RACM) including high-resolution atmosphere, land, ocean, sea ice and land hydrology components and (ii) to perform extended numerical experiments using high performance computers to minimize uncertainties and fundamentally improve current predictions of climate change in the northern polar regions. These goals were realized first through evaluation studies of climate system components via one-way coupling experiments. Simulations were then used to examine the effects of advancements in climate component systems on their representation of main physics, time-mean fields and to understand variability signals at scales over many years. As such this research directly addressed some of the major science objectives of the BER Climate Change Research Division (CCRD) regarding the advancement of long-term climate prediction.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Multifidelity Monte Carlo estimation for efficient uncertainty quantification in climate-related modeling

Abstract. Uncertainties in an output of interest that depends on the solution of a complex system (e.g., of partial differential equations with random inputs) are often, if not nearly ubiquitously, determined in practice using Monte Carlo (MC) estimation. While simple to implement, MC estimation fails to provide reliable information about statistical quantities (such as the expected value of the output of interest) in application settings such as climate modeling, for which obtaining a single realization of the output of interest is a costly endeavor. Specifically, the dilemma encountered is that many samples of the output of interest have to be collected in order to obtain an MC estimator that has sufficient accuracy – so many, in fact, that the available computational budget is not large enough to effect the number of samples needed. To circumvent this dilemma, we consider using multifidelity Monte Carlo (MFMC) estimation which leverages the use of less costly and less accurate surrogate models (such as coarser grids, reduced-order models, simplified physics, and/or interpolants) to achieve, for the same computational budget, higher accuracy compared to that obtained by an MC estimator – or, looking at it another way, an MFMC estimator obtains the same accuracy as the MC estimator at lower computational cost. The key to the efficacy of MFMC estimation is the fact that most of the required computational budget is loaded onto the less costly surrogate models so that very few samples are taken of the more expensive model of interest. We first provide a more detailed discussion about the need to consider an alternative to MC estimation for uncertainty quantification. Subsequently, we present a review, in an abstract setting, of the MFMC approach along with its application to three climate-related benchmark problems as a proof-of-concept exercise.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

The effect of temperature on photosystem II efficiency across plant functional types and climate

Modeling terrestrial gross primary productivity (GPP) is central to predicting the global carbon cycle. Much interest has been focused on the environmentally induced dynamics of photosystem energy partitioning and how improvements in the description of such dynamics assist the prediction of light reactions of photosynthesis and therefore GPP. The maximum quantum yield of photosystem II (Φ PSIImax ) is a key parameter of the light reactions that influence the electron transport rate needed for supporting the biochemical reactions of photosynthesis. Φ PSIImax is generally treated as a constant in biochemical photosynthetic models even though a constant Φ PSIImax is expected only for non-stressed plants. We synthesized reported Φ PSIImax values from pulse-amplitude-modulated fluorometry measurements in response to variable temperatures across the globe. We found that Φ PSIImax is strongly affected by prevailing temperature regimes with declined values in both hot and cold conditions. To understand the spatiotemporal variability in Φ PSIImax , we analyzed the temperature effect on Φ PSIImax across plant functional type (PFT) and habitat climatology. The analysis showed that temperature's impact on Φ PSIImax is shaped more by climate than by PFT for plants with broad latitudinal distributions or in regions with extreme temperature variability. There is a trade-off between the temperature range within which Φ PSIImax remains maximal and the overall rate of decline of Φ PSIImax outside the temperature range such that species cannot be simultaneously tolerant and resilient to extreme temperatures. Our study points to a quantitative approach for improving electron transport and photosynthetic productivity modeling under changing climates at regional and global scales.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

Conceptual Model of Climate Change Impacts at LANL

Goal 9 of the LANL FY15 Site Sustainability Plan (LANL 2014a) addresses Climate Change Adaptation. As part of Goal 9, the plan reviews many of the individual programs the Laboratory has initiated over the past 20 years to address climate change impacts to LANL (e.g. Wildland Fire Management Plan, Forest Management Plan, etc.). However, at that time, LANL did not yet have a comprehensive approach to climate change adaptation. To fill this gap, the FY15 Work Plan for the LANL Long Term Strategy for Environmental Stewardship and Sustainability (LANL 2015) included a goal of (1) establishing a comprehensive conceptual model of climate change impacts at LANL and (2) establishing specific climate change indices to measure climate change and impacts at Los Alamos. Establishing a conceptual model of climate change impacts will demonstrate that the Laboratory is addressing climate change impacts in a comprehensive manner. This paper fulfills the requirement of goal 1. The establishment of specific indices of climate change at Los Alamos (goal 2), will improve our ability to determine climate change vulnerabilities and assess risk. Future work will include prioritizing risks, evaluating options/technologies/costs, and where appropriate, taking actions. To develop a comprehensive conceptual model of climate change impacts, we selected the framework provided in the National Oceanic and Atmospheric Administration (NOAA) Climate Resilience Toolkit (http://toolkit.climate.gov/).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Global tropical cyclone precipitation scaling with sea surface temperature

Understanding the relationship between tropical cyclone (TC) precipitation and sea surface temperature (SST) is essential for both TC hazard forecasting and projecting how these hazards will change in the future due to climate change. This work untangles how global TC precipitation is impacted by present-day SST variability (known as apparent scaling) and by long-term changes in SST caused by climate change (known as climate scaling). A variety of datasets are used including precipitation and SST observations, realistic climate model simulations, and idealized climate model simulations. The apparent scaling rates depend on precipitation metric; examples shown here have ranges of 6.1 to 9.5% per K versus 5.9 to 9.8% per K for two different metrics. The climate scaling is estimated at about 5% per K, which is slightly less than the atmospheric moisture scaling based on thermodynamic principles of about 7% per K (i.e., the Clausius–Clapeyron scaling). The apparent scaling is greater than the climate scaling, which implies that the relationship between TC precipitation and present-day SST variability should not be used to project the long-term response of TC precipitation to climate change.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

Characterizing half‐a‐degree difference: a review of methods for identifying regional climate responses to global warming targets

The Paris Agreement long‐term global temperature goal refers to two global warming levels: well below 2°C and 1.5°C above preindustrial. Regional climate signals at specific global warming levels, and especially the differences between 1.5°C and 2°C, are not well constrained, however. In particular, methodological challenges related to the assessment of such differences have received limited attention. This article reviews alternative approaches for identifying regional climate signals associated with global temperature limits, and evaluates the extent to which they constitute a sound basis for impacts analysis. Four methods are outlined, including comparing data from different greenhouse gas scenarios, sub‐selecting climate models based on global temperature response, pattern scaling, and extracting anomalies at the time of each global temperature increment. These methods have rarely been applied to compare 2°C with 1.5°C, but some demonstrate potential avenues for useful research. Nevertheless, there are methodological challenges associated with the use of existing climate model experiments, which are generally designed to model responses to different levels of greenhouse gas forcing, rather than to model climate responses to a specific level of forcing that targets a given level of global temperature change. Novel approaches may be required to address policy questions, in particular: to differentiate between half degree warming increments while accounting for different sources of uncertainty; to examine mechanisms of regional climate change including the potential for nonlinear responses; and to explore the relevance of time‐lagged processes in the climate system and declining emissions, and the resulting sensitivity to alternative mitigation pathways. WIREs Clim Change 2017, 8:e457. doi: 10.1002/wcc.457 This article is categorized under: Assessing Impacts of Climate Change > Scenario Development and Application

James, Rachel↗
DOE OSTI2013

Greenland Surface Mass Balance as Simulated by the Community Earth System Model. Part I: Model Evaluation and 1850–2005 Results

The modeling of the surface mass balance (SMB) of the Greenland Ice Sheet (GIS) requires high-resolution models in order to capture the observed large gradients in the steep marginal areas. Until now, global climate models have not been considered suitable to model ice sheet SMB owing to model biases and insufficient resolution. This study analyzes the GIS SMB simulated for the period 1850–2005 by the Community Earth System Model (CESM), which includes a new ice sheet component with multiple elevation classes for SMB calculations. The model is evaluated against observational data and output from the regional model Regional Atmospheric Climate Model version 2 (RACMO2). Because of a lack of major climate biases, a sophisticated calculation of snow processes (including surface albedo evolution) and an adequate downscaling technique, CESM is able to realistically simulate GIS surface climate and SMB. CESM SMB agrees reasonably well with in situ data from 475 locations ($r$ = 0.80) and output from RACMO2 ($r$ = 0.79). The simulated mean SMB for 1960–2005 is 359 ± 120 Gt yr -1 in the range of estimates from regional climate models. The simulated seasonal mass variability is comparable with mass observations from the Gravity Recovery and Climate Experiment (GRACE), with synchronous annual maximum (May) and minimum (August–September) and similar amplitudes of the seasonal cycle. CESM is able to simulate the bands of precipitation maxima along the southeast and northwest margins, but absolute precipitation rates are underestimated along the southeastern margin and overestimated in the high interior. The model correctly simulates the major ablation areas. Total refreezing represents 35% of the available liquid water (the sum of rain and melt).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Analysis of secondary organic aerosol simulation bias in the Community Earth System Model (CESM2.1)

Organic aerosol (OA) has been considered as one of the most important uncertainties in climate modeling due to the complexity in presenting its chemical production and depletion mechanisms. To better understand the capability of climate models and probe into the associated uncertainties in simulating OA, we evaluate the Community Earth System Model version 2.1 (CESM2.1) configured with the Community Atmosphere Model version 6 (CAM6) with comprehensive tropospheric and stratospheric chemistry representation (CAM6-Chem) through a long-term simulation (1988–2019) with observations collected from multiple datasets in the United States. We find that CESM generally reproduces the interannual variation and seasonal cycle of OA mass concentration at surface layer with a correlation of 0.40 compared to ground observations and systematically overestimates (69%) in summer and underestimates (-19%) in winter. Through a series of sensitivity simulations, we reveal that modeling bias is primarily related to the dominant fraction of monoterpene-formed secondary organic aerosol (SOA), and a strong positive correlation of 0.67 is found between monoterpene emission and modeling bias in the eastern US during summer. In terms of vertical profile, the model prominently underestimates OA and monoterpene concentrations by 37%–99% and 82%–99%, respectively, in the upper air (>500 m) as validated against aircraft observations. Our study suggests that the current volatility basis set (VBS) scheme applied in CESM might be parameterized with monoterpene SOA yields that are too high, which subsequently results in strong SOA production near the emission source area. We also find that the model has difficulty in reproducing the decreasing trend of surface OA in the southeastern US probably because of employing pure gas VBS to represent isoprene SOA which is in reality mainly formed through multiphase chemistry; thus, the influence of aerosol acidity and sulfate particle change on isoprene SOA formation has not been fully considered in the model. This study reveals the urgent need to improve the SOA modeling in climate models.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Non-stationary Return Levels of CMIP5 Multi-model Temperature Extremes

The objective of this study is to evaluate to what extent the CMIP5 climate model simulations of the climate of the twentieth century can represent observed warm monthly temperature extremes under a changing environment. The biases and spatial patterns of 2-, 10-, 25-, 50- and 100-year return levels of the annual maxima of monthly mean temperature (hereafter, annual temperature maxima) from CMIP5 simulations are compared with those of Climatic Research Unit (CRU) observational data considered under a non-stationary assumption. The results show that CMIP5 climate models collectively underestimate the mean annual maxima over arid and semi-arid regions that are most subject to severe heat waves and droughts. Furthermore, the results indicate that most climate models tend to underestimate the historical annual temperature maxima over the United States and Greenland, while generally disagreeing in their simulations over cold regions. Return level analysis shows that with respect to the spatial patterns of the annual temperature maxima, there are good agreements between the CRU observations and most CMIP5 simulations. However, the magnitudes of the simulated annual temperature maxima differ substantially across individual models. Discrepancies are generally larger over higher latitudes and cold regions.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Tropical Cyclone Wind Shear-Relative Asymmetry in Reanalyses

Abstract While tropical cyclones (TCs) are axisymmetric vortices to the first order, they often exhibit noteworthy structural asymmetries. These often result from environmental vertical wind shear, which tilts the vortex and induces a wavenumber 1 pattern in the circulation and precipitation fields. Reanalyses and climate models have improved in representing the TC structure and climatology, but their relatively coarse resolution and dependence on parameterized physics cast doubt on their ability to capture the asymmetric TC structure. We perform the most comprehensive process-oriented assessment of TC asymmetry to date in reanalyses. Specifically, we analyze the composite shear-relative TC structure in ERA5 and Climate Forecast System Reanalysis (CFSR), which vary in their resolutions, physical parameterization suites, and data assimilation techniques. These structures are compared with aircraft reconnaissance radar observations. In agreement with the observations, the strongest tangential winds are usually found left-of-shear, while inner core rainfall, ascent, vortex tilt, and low-level inflow are favored directly downshear or in the downshear-left quadrant. Outer rainband convection generally peaks in the downshear-right quadrant. Thermodynamic asymmetries are also apparent, with anomalous low-level moisture right-of-shear, midlevel warmth in the upshear-right quadrant (uptilt), and cloud properties suggestive of a realistic precipitation life cycle from growth to fallout. We also decompose rainfall contributions from the convective parameterization and large-scale cloud schemes and highlight the roles of vorticity advection, buoyancy advection, and diabatic processes in driving asymmetric vertical motions in the inner core and outer rainband regions. Our results suggest that process-level studies of TC asymmetry and TC–wind shear interaction under future warming are viable using climate models. Significance Statement Asymmetries are common in tropical cyclones (TCs), influencing their intensity, track, and hazards. Vertical wind shear often plays a leading-order role in causing these asymmetries. It is uncertain how well asymmetric structures and processes are captured in reanalyses and global climate models (GCMs) with grid spacings of 0.25° and coarser. In this study, we first evaluate TC asymmetry in reanalyses, which have the benefit of being forced by observations. This helps to assess whether the resolutions associated with GCMs sufficiently capture asymmetric structures and processes and motivates upcoming work with free-running GCMs to study how TC asymmetry may change in a warming climate.

Carstens, Jacob D.↗
DOE OSTI2022

Small field campaign: aerosol – ice formation closure pilot study. Final Report

Prediction of atmospheric ice formation from aerosol particles by heterogeneous nucleation represents one of the grand challenges in atmospheric science. Our insufficient predictive understanding of primary ice formation is the reason that climate models typically do not include heterogeneous ice nucleation with subsequent effects on climate uncertainty. Mixed-phase clouds, where supercooled water droplets and ice crystals coexist play globally an important role regulating climate. This is especially the case for the Arctic region that experiences the greatest warming due to climate change compared to other regions in the world. Immersion freezing initiated by ice-nucleating particles (INPs) in supercooled water droplets is recognized as the dominant primary ice formation pathway in mixed-phase cloud regimes. For this reason, it is crucial to evaluate our capability to predict immersion freezing for a given ambient aerosol population. The goal of this project is conducting a field-based pilot study at the U.S. DOE Atmospheric Radiation Measurement (ARM) user facility at Southern Great Plains (SGP) to evaluate our capability to predict the number concentration of aerosol particles that serve as INPs in the immersion freezing mode. Successful prediction of INP number concentrations is also termed “closure”. This field-observational approach represents a first-of-its kind attempt of an aerosol–ice formation closure study (AEROICESTUDY). Very few closure studies related to INPs have been conducted, and to our knowledge, none using robust size-resolved ambient aerosol composition measurements as a starting point. Achievement of aerosol–ice formation closure relies on our ability to characterize the ambient aerosol population with respect to particles size and composition and to determine INP number concentrations for specified freezing temperatures. This requires numerous online and offline instrumentation resulting in this pilot field campaign being a multi-institutional and community-collaborative effort. We chose the ARM SGP megasite for this first aerosol-ice formation closure pilot study due to its significant measurement capabilities available to obtain detailed physical characterization of the local aerosol population including size distribution, mass loading, and chemical composition of non-refractory aerosol particles. The overall objective of this project is to identify ice nucleation parameterizations that produce the most robust predictions of INP numbers and thus are best suited to be included in cloud and climate models. This objective includes the following goals for this field and laboratory-based project: i) What are the crucial aerosol physicochemical property measurements needed to accurately guide ice nucleation representations in models and long-term INP measurements? ii) What level of parameter details needs to be known to achieve aerosol–ice formation closure? iii) What are the leading causes for climate model bias in INP predictions? We found that the advances in our understanding of immersion freezing garnered over the last 20 years allowed us to yield partial and full closures of atmospheric immersion freezing from ambient aerosol particles. When the aerosol population is physicochemically complex and parameterizations for representative INP types are not yet available, we still struggle to accurately predict INP number concentrations. This project clearly demonstrates that with more laboratory and field measurements that are accompanied by particle composition analysis, the necessary datasets to achieve aerosol–ice formation closure for various locations will emerge, thus providing a robust foundation for guiding the representation of INPs in cloud and climate models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

Collaborative Research: Understanding air‐sea feedbacks to the MJO through process evaluation of observations and E3SM experiments (Final Technical Report)

This project explored the role of tropical oceans in regulating cloud populations within the Madden-Julian oscillation (MJO)–a large-scale tropical weather disturbance that influences extreme weather events across the globe by affecting the position of the jet stream and patterns of moisture transport. Our project sought to 1) document ocean feedback strength to the MJO in climate models, 2) understand how air-sea interactions affect the intensity, organization, and propagation of MJO convection, 3) utilize existing observations to identify sources of model bias for tropical air-sea interactions, and 4) better understand the effects of slow and fast ocean variability on MJO cloudiness. We found that transfers of heat and moisture across the air-sea interface (i.e., surface fluxes) in most climate models are over-supportive in maintaining MJO convection and under-supportive in propagating MJO convection. This can lead to misrepresentations in the frequency of extreme weather events across the globe through erroneous MJO feedbacks to jet stream position and moisture transport. Furthermore, using observations collected by ocean moorings across the tropical oceans, we showed that most models greatly overestimate surface evaporation in the subtropics, and that this bias is likely one contributor to a pervasive bias among climate models in their ability to simulate the mean state of rainfall over the tropical oceans (i.e., the “double ITCZ bias”). Replacing the default surface flux algorithm in two climate models with a state-of-the-art surface flux algorithm modestly reduced the double ITCZ bias in those models. Our work produced two model diagnostics packages that are now publicly available through DOE and NOAA model diagnostics archives. The first, the Analysis of Scales of Precipitation (ASoP) diagnoses scales of precipitation variability across space and time, with temporal resolution as fine as the model integration timestep. The second, the air-sea flux diagnostic diagnoses model surface fluxes and allows direct comparison of model fluxes to observations without having to recompute fluxes using model output and a state-of-the-art flux algorithm. These diagnostics, which were developed using climate models, can be readily applied to regional and global forecast model output to improve forecasts for the benefit of society.

54 ENVIRONMENTAL SCIENCES↗