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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 559 records · Page 31
All sourcesNASA NTRSDOE OSTI
NASA NTRS1993

Excitation of positive ions by low-energy electrons - Relevance to the Io Torus

The importance of measuring electron-ion excitation cross sections in singly and multiply charged positive ions is outlined, and recent results for Mg II and O II ions are given using the JPL's electron energy-loss merged-beams apparatus. Theoretical comparisons are given with two five-state close-coupling calculations. The energy variation of the collision strength is fitted with a semiempirical analytic function which includes approximations to polarization, resonance, and exchange contributions. In O II, first spectra anywhere of electron excitation of the optically allowed transitions are presented. In addition, excitations of two low lying, optically forbidden transitions are detected for the first time.

Smith, Steven J.↗
DOE OSTI2024

Observation of bound valence excited electronic states of deprotonated 2-hydroxytriphenylene using photoelectron, photodetachment, and resonant two-photon detachment spectroscopy of cryogenically cooled anions

Polycyclic aromatic hydrocarbons (PAHs) are common atmospheric pollutants, and they are also ubiquitous in the interstellar medium. Here, we report the study of a complex O-containing PAH anion, the deprotonated 2-hydroxytriphenylene (2-OtPh–), using high-resolution photoelectron imaging and photodetachment spectroscopy of cryogenically cooled anions. Vibrationally resolved photoelectron spectra yield the electron affinity of the 2-OtPh radical as 2.629(1) eV and several vibrational frequencies for its ground electronic state. Photodetachment spectroscopy reveals bound valence excited electronic states for the 2-OtPh– anion, with unprecedentedly rich vibronic features. Evidence is presented for a low-lying triplet state (T1) and two singlet states (S1 and S2) below the detachment threshold. Single-color resonant two-photon photoelectron spectroscopy uncovers rich photophysics for the 2-OtPh– anion, including vibrational relaxation in S1, internal conversion to the ground state of 2-OtPh–, intersystem crossing from S2 to T1, and a long-lived autodetaching shape resonance about 1.3 eV above the detachment threshold. The rich electronic structure and photophysics afforded by the current study suggest that 2-OtPh– would be an interesting system for pump–probe experiments to unravel the dynamics of the excited states of this complex PAH anion.

Chemistry↗
DOE OSTI2024

Test of light-lepton universality in τ decays with the Belle II experiment

We present a measurement of the ratio R µ = $\mathcal{B}$($τ^- → µ^-\overline{ν}_µν_τ$)/$\mathcal{B}(τ^- → e^-\overline{ν}_eν_τ$) of branching fractions B of the τ lepton decaying to muons or electrons using data collected with the Belle II detector at the SuperKEKB e + e - collider. The sample has an integrated luminosity of 362 ± 2 fb -1 at a centre-of-mass energy of 10.58 GeV. Using an optimised event selection, a binned maximum likelihood ft is performed using the momentum spectra of the electron and muon candidates. The result, R µ = 0.9675 ± 0.0007 ± 0.0036, where the first uncertainty is statistical and the second is systematic, is the most precise to date. It provides a stringent test of the light-lepton universality, translating to a ratio of the couplings of the muon and electron to the W boson in τ decays of 0.9974 ± 0.0019, in agreement with the standard model expectation of unity.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS1977

Studies of Ar and N2 using threshold photoelectron spectroscopy by electron attachment /TPSA/

Threshold photoelectron spectra of Ar and N2 are studied by a technique called threshold photoelectron spectroscopy by electron attachment, which involves the attachment of the threshold electron to SF6 followed by the detection of SF6(-). Studies on Ar provide a measure of the rejection ratio for nonthreshold electrons of this technique. A rotational propensity rule is given which states that an autoionizing N2 state prefers to decay to N2(+) states with a minimum change in rotational angular momentum.

Chutjian, A.↗
DOE OSTI2025

Test of lepton flavour universality in W-boson decays into electrons and τ-leptons using pp collisions at s = 13 TeV with the ATLAS detector

A measurement of the ratio of the branching fractions, Rτ/e = B(W → τν)/B(W → eν), is performed using a sample of W bosons originating from top-quark decays to final states containing τ-leptons or electrons. This measurement uses pp collisions at s$$ \sqrt{s} $$ = 13 TeV, collected by the ATLAS experiment at the Large Hadron Collider during Run 2, corresponding to an integrated luminosity of 140 fb−1. The W → τντ (with τ → eνeντ) and W → eνe decays are distinguished using the differences in the impact parameter distributions and transverse momentum spectra of the electrons. The measured ratio of branching fractions Rτ/e = 0.975 ± 0.012 (stat.) ± 0.020 (syst.), is consistent with the Standard Model assumption of lepton flavour universality in W-boson decays.

Aad, G↗
NASA NTRS2010

Fisk-Gloeckler Suprathermal Proton Spectrum in the Heliosheath and the Local Interstellar Medium

Convergence of suprathermal keV-MeV proton and ion spectra approximately to the Fisk-Gloeckler (F-G) form j(E) = j(sub 0) E(sup -1.5) in Voyager land 2 heliosheath measurements is suggestive of distributed acceleration in Kolmogorov turbulence which may extend well beyond the heliopause into the local interstellar medium (LISM). Turbulence of this type is already indicated by interstellar radio scintillation measurements of electron density power spectra. Previously published extrapolations (Cooper et al., 2003, 2006) of the LISM proton spectrum from eV to GeV energies are highly consistent with the F-G power-law and further indicative of such turbulence and LISM effectiveness of the F-G cascade acceleration process. The LISM pressure computed from this spectrum well exceeds that from current estimates for the LISM magnetic field, so exchange of energy between the protons and the magnetic field would likely have a strong role in evolution of the turbulence as per the F-G theory and as long ago proposed for cosmic ray energies by Parker and others. Pressure-dependent estimates of the LISM field strength should not ignore this potentially strong and even dominant contribution from the plasma. Presence of high-beta suprathermal plasma on LISM field lines could significantly affect interactions with the heliospheric outer boundary region and might potentially account for distributed and more discrete features in ongoing measurements of energetic neutral emission from the Interstellar Boundary Explorer (IBEX) mission.

Cooper, John F.↗
NASA NTRS1988

A cosmic and solar X-ray and gamma-ray instrument for a scout launch

An overview is presented for a set of simple and robust X-ray and gamma ray instruments which have both cosmic and solar objectives. The primary solar scientific objective is the study of the beaming of energetic electrons and ions in solar flares. The instrument will measure spectra and polarization of flare emissions up to 10 MeV. At X-ray energies both the directly emitted flux and the reflected albedo flux will be measured with a complement of six X-ray sensors. Each of these detectors will have a different high Z filter selected to optimize both the energy resolution and high rate capabilities in the energy band 10 to 300 keV. At energies greater than 100 keV seven 7.6 x 7.6 cm NaI and a set of 30 concentric plastic scattering detectors will record the spectra and polarization of electron bremsstrahlung and nuclear gamma rays. All of the components of the instrument are in existence and have passed flight tests for earlier space missions. The instrument will use a spinning solar oriented Scout spacecraft. The NaI detectors will act as a self-modulating gamma ray detector for cosmic sources in a broad angular band which lies at 90 degrees to the Sun-Earth vector and hence will scan the entire sky in 6 months.

Forrest, D. J.↗
NASA NTRS1999

Secondary Electron Emission Spectroscopy of Diamond Surfaces

This report presents the results of the secondary electron emission spectroscopy study of hydrogenated diamond surfaces for single crystals and chemical vapor-deposited polycrystalline films. One-electron calculations of Auger spectra of diamond surfaces having various hydrogen coverages are presented, the major features of the experimental spectra are explained, and a theoretical model for Auger spectra of hydrogenated diamond surfaces is proposed. An energy shift and a change in the line shape of the carbon core-valence-valence (KVV) Auger spectra were observed for diamond surfaces after exposure to an electron beam or by annealing at temperatures higher than 950 C. This change is related to the redistribution of the valence-band local density of states caused by hydrogen desorption from the surface. A strong negative electron affinity (NEA) effect, which appeared as a large, narrow peak in the low-energy portion of the spectrum of the secondary electron energy distribution, was also observed on the diamond surfaces. A fine structure in this peak, which was found for the first time, reflected the energy structure of the bottom of the conduction band. Further, the breakup of the bulk excitons at the surface during secondary electron emission was attributed to one of the features of this structure. The study demonstrated that the NEA type depends on the extent of hydrogen coverage of the diamond surface, changing from the true type for the completely hydrogenated surface to the effective type for the partially hydrogenated surface.

Krainsky, Isay L.↗
NASA NTRS1984

Angular distributions for electron impact excitation of ions from energy-loss spectra measurements

Energy-loss spectra for excitation of the 2S to 2PO transitions in ZNII and CdII by electrons have been observed for the first time. Differential scattering cross sections are reported at 75 eV electron energy. Comparisons are made to close-coupling theory for the 4,2S to 4,2P transition in ZnII. In CdII comparisons are made to the 5,2S(1/2) to 5,2S(3/2) integral cross section from absolute emission measurements, to theoretical results for the analogous 2S to 2P transition in ZnII, and to Gaunt-factor calculations. A description of the crossed beam apparatus is given, and conversion of scattering intensity to absolute cross section discussed.

Chutjian, A.↗
NASA NTRS1982

Theory of electron-positron showers in double radio sources

A black hole of mass of about 300 million solar masses is assumed to be present in the nucleus of an active galaxy or quasar. With an axial magnetic field near 1000 gauss, a potential drop 10 to the 19th volts is generated by the unipolar induction of a rotating accretion disk surrounding the black hole. The possibility that the acceleration of electrons or positrons in the unipolar fields initiates an electromagnetic cascade shower at distances at least 10 to the 16th cm from the black hole is investigated. The scattering medium for the shower is considered to be the spectrum of low energy photons originating from the inner region of the disk. It is found that at completion of the cascade, power-law energy spectra of relativistic electrons and positrons and of gamma-rays emerge under appropriate conditions. If the cascade-initiating particles are collimated, the electrons and positrons emerge in a collimated beam. Such beams may power extragalactic double radio sources.

Burns, M. L.↗
NASA NTRS1975

Echo 2 - Observations at Fort Churchill of a 4-keV peak in low-level electron precipitation

The Echo 2 rocket flight launched from Fort Churchill, Manitoba, offered the opportunity to observe high-latitude low-level electron precipitation during quiet magnetic conditions. Although no visual aurora was evident at the time of the flight, an auroral spectrum sharply peaked at a few keV was observed to have intensities from 1 to 2 orders of magnitude lower than peaked spectra typically associated with bright auroral forms. There is a growing body of evidence that relates peaked electron spectra to discrete aurora. The Echo 2 observations show that whatever the mechanism for peaking the electron spectrum in and above discrete forms, it operates over a range of precipitation intensities covering nearly 3 orders of magnitude down to subvisual or near subvisual events.

Arnoldy, R. L.↗
NASA NTRS1987

Separating Peaks in X-Ray Spectra

Deconvolution algorithm assists in analysis of x-ray spectra from scanning electron microscopes, electron microprobe analyzers, x-ray fluorescence spectrometers, and like. New algorithm automatically deconvolves x-ray spectrum, identifies locations of spectral peaks, and selects chemical elements most likely producing peaks. Technique based on similarities between zero- and second-order terms of Taylor-series expansions of Gaussian distribution and of damped sinusoid. Principal advantage of algorithm: no requirement to adjust weighting factors or other parameters when analyzing general x-ray spectra.

Nicolas, David↗
NASA NTRS2013

Insights into Collisional between Small Bodies: Comparison of Impacted Magnesium-rich Minerals

Impacts are sustained by comets and asteroids throughout their lives, especially early in the Solar system's history, as described by the Nice model. Identifying observable properties that may be altered due to impacts can lead to a better understanding their collisional histories. Here, we investigate spectral effects and physical shock features observed in infrared spectra and Transmission Electron Microscope (TEM) images, respectively, of magnesium-rich minerals subjected to shock through impact experiments. Samples of magnesium-rich forsterite (Mg2SiO4, olivine), orthoenstatite (Mg2SiO3, pyroxene), diopside (MgCaSi2O6, monoclinic pyroxene), and magnesite (MgCO3, carbonate) were impacted at speeds of 2.4 km/s, 2.6 km/s and 2.8 km/s. Impact experiments were conducted in the Johnson Space Center Experimental Impact Laboratory using the vertical gun. Clear signatures are observed in both the mid-IR spectra (shift in wavelengths of the spectral peaks and relative amplitude changes) of all minerals except magnesite, and in TEM images (planar dislocations) of both the forsterite and orthoenstatite samples. Further discussion on forsterite and enstatite analyses can be found in Jensen et al., this meeting.

Lederer, Susan M.↗
NASA NTRS1978

Measurements of material properties for solar cells

Measurements on two candidate materials for space flight are reported. The observed optical transmittance of aluminum films vapor deposited on fused quartz showed anomalously high transmittance thru 400 A and 600 A and showed an effective skin depth of 110 A in the latter part of the 1000 A thickness. KAPTON films are shown by their optical transmission spectra to have an energy gap for electron excitation of approximately 2.5 eV, which value depends on the thickness as manufactured. The resistance of KAPTON film to ionizing radiation is described by their optical spectra and their electron spin resonance spectra.

Castle, J. G., Jr.↗
NASA NTRS2005

Differential Cross Sections for the Electron Impact Excitation of the A(sup 3)(Sigma)(sub u)(sup +), B(sup 3)Pi(sub g), W(sup 3)(Delta)(sub u), B'(sup 3)(Sigma)(sub u)(sup -), a'(sup 1)Sigma(sub u)(sup -), a(sup 1)Pi(sub g), w(sup 1)Delta(sub u), and C(sup 3)Pi(sub u) States of N(sub 2)

Measurements of differential cross sections for the electron-impact excitation of molecular nitrogen from the ground X(sup 1)(Sigma)(sub g)(sup +)(v''=0)level to the A(sup 3)(Sigma)(sub u)(sup +)(v'), B(sup 3)Pi(sub g)(v'), W(sup 3)(Delta)(sub u)(v'),B'(sup 3)(Sigma)(sub u)(sup -)(v'), a(sup 1)(Pi)(sub g)(v'), w(sup 1)(Delta)(sub u)(v'), and C(sup 3)(Pi)(sub u)(v') levels are presented. The data are obtained at the incident energies of 10, 12.5, 15, 17.5, 20, 30, 50, and 100 eV over the angular range of 5(deg)-130(deg) in 5(deg) intervals. The individual electronic state excitation differential cross sections are obtained by unfolding electron energy-loss spectra of molecular nitrogen using available semiempirical Frank-Condon factors. The data are compared to previous measurements and to available theory. We also make several important suggestions regarding future work that, like the present, relies on the unfolding of electron energy-loss spectra for obtaining differential cross sections.

electron impact↗
DOE OSTI2020

Initial-state preparation effects in time-resolved electron paramagnetic resonance experiments

In this paper, we explain a recent experimental observation that the time-resolved electron paramagnetic resonance spectra of an organic molecule for optical excitation within a highly absorbing region of the molecule has similar intensities to the spectra for optical excitation in a nonabsorbing region [D. L. Meyer et al., J. Phys. Chem. Lett. 8, 1677 (2017)]. We demonstrate that this phenomenon is due to an initial-state preparation effect of photoexcitation that leads to similar initial populations of triplet states for both optical excitation regions. Due to the low intersystem crossing rates, the initial triplet populations are not perturbed on the time scale of the experiment, so they determine the relative intensities of the paramagnetic resonance spectra. The effect is surprising given the weak spin-orbit interactions of organic molecules. Such initial-state preparation effects are likely to occur in systems where the intersystem crossing time scales are long compared to the time scale of the experiment.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗