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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 559 records · Page 31
All sourcesNASA NTRSDOE OSTI
NASA NTRS1994

Evolution of the 1991-1992 Arctic vortex and comparison with the Geophysical Fluid Dynamics Laboratory SKYHI general circulation model

Nitrous oxide (N2O) measured on board the ER-2 aircraft during the Airborne Arctic Stratospheric Expedition 2 (AASE 2) has been used to monitor descent of air inside the Arctic vortex between October 1991 and March 1992. Monthly mean N2O fields are calculated from the flight data and then compared with mean fields calculated from the high-resolution Geophysical Fluid Dynamics Laboratory general circulation model SKYHI in order to evaluate the model's simulation of the polar vortex. From late fall through winter the model vortex evolves in much the same way as the 1991-1992 vortex, with N2O gradients at the edge becoming progressively steeper. The October to March trends in N2O profiles inside the vortex are used to verify daily net heating rates in the vortex that were computed from clear sky radiative heating rates and National Meteorological Center temperature observations. The computed heating rates successfully estimate the descent of vortex air from December through February but suggest that before December, air at high latitudes may not be isolated from the midlatitudes. SKYHI heating rates are in good agreement with the computed rates but tend to be slightly higher (i.e., less cooling) due to meteorological differences between SKYHI and the 1991-1992 winter. Three ER-2 flights measured N2O just north of the subtropical jet. These low-midlatitude profiles show only slight differences from the high-midlatitude profiles (45 deg - 60 deg N), indicating strong meridional mixing in the midlatitude 'surf zone.' Mean midwinter N2O profiles inside and outside the vortex calculated from AASE 2 data are shown to be nearly identical to 1989 AASE profiles, pointing to the N2O/potential temperature relationship as an excellent marker for vortex air.

Strahan, S. E.↗
NASA NTRS2002

MPL-Net Measurements of Aerosol and Cloud Vertical Distributions at Co-Located AERONET Sites

In the early 1990s, the first small, eye-safe, and autonomous lidar system was developed, the Micropulse Lidar (MPL). The MPL acquires signal profiles of backscattered laser light from aerosols and clouds. The signals are analyzed to yield multiple layer heights, optical depths of each layer, average extinction-to-backscatter ratios for each layer, and profiles of extinction in each layer. In 2000, several MPL sites were organized into a coordinated network, called MPL-Net, by the Cloud and Aerosol Lidar Group at NASA Goddard Space Flight Center (GSFC) using funding provided by the NASA Earth Observing System. tn addition to the funding provided by NASA EOS, the NASA CERES Ground Validation Group supplied four MPL systems to the project, and the NASA TOMS group contributed their MPL for work at GSFC. The Atmospheric Radiation Measurement Program (ARM) also agreed to make their data available to the MPL-Net project for processing. In addition to the initial NASA and ARM operated sites, several other independent research groups have also expressed interest in joining the network using their own instruments. Finally, a limited amount of EOS funding was set aside to participate in various field experiments each year. The NASA Sensor Intercomparison and Merger for Biological and Interdisciplinary Oceanic Studies (SIMBIOS) project also provides funds to deploy their MPL during ocean research cruises. All together, the MPL-Net project has participated in four major field experiments since 2000. Most MPL-Net sites and field experiment locations are also co-located with sunphotometers in the NASA Aerosol Robotic Network. (AERONET). Therefore, at these locations data is collected on both aerosol and cloud vertical structure as well as column optical depth and sky radiance. Real-time data products are now available from most MPL-Net sites. Our real-time products are generated at times of AERONET aerosol optical depth (AOD) measurements. The AERONET AOD is used as input to our processing routines, which calculate the aerosol layer top height and extinction profile, and our MPL calibration value. A variety of other data products are available or under development. We present an overview of the MPL-Net project and discuss data products useful to the AERONET community. Results from several sites and field experiments will be presented.

Welton, Ellsworth J.↗
NASA NTRS2007

Spectral Absorption Properties of Atmospheric Aerosols

We have determined the solar spectral absorption optical depth of atmospheric aerosols for specific case studies during several field programs (three cases have been reported previously; two are new results). We combined airborne measurements of the solar net radiant flux density and the aerosol optical depth with a detailed radiative transfer model for all but one of the cases. The field programs (SAFARI 2000, ACE Asia, PRIDE, TARFOX, INTEX-A) contained aerosols representing the major absorbing aerosol types: pollution, biomass burning, desert dust and mixtures. In all cases the spectral absorption optical depth decreases with wavelength and can be approximated with a power-law wavelength dependence (Absorption Angstrom Exponent or AAE). We compare our results with other recent spectral absorption measurements and attempt to briefly summarize the state of knowledge of aerosol absorption spectra in the atmosphere. We discuss the limitations in using the AAE for calculating the solar absorption. We also discuss the resulting spectral single scattering albedo for these cases.

Bergstrom, R. W.↗
NASA NTRS2013

The Thermal Expansion of Ring Particles and the Secular Orbital Evolution of Rings Around Planets and Asteroids

The thermal expansion and contraction of ring particles orbiting a planet or asteroid can cause secular orbit evolution. This effect, called here the thermal expansion effect, depends on ring particles entering and exiting the shadow of the body they orbit. A particle cools off in the shadow and heats up again in the sunshine, suffering thermal contraction and expansion. The changing cross-section it presents to solar radiation pressure plus time lags due to thermal inertia lead to a net along-track force. The effect causes outward drift for rocky particles. For the equatorial orbits considered here, the thermal expansion effect is larger than Poynting-Robertson drag in the inner solar system for particles in the size range approx. 0.001 - 0.02 m. This leads to a net increase in the semimajor axis from the two opposing effects at rates ranging from approx. 0.1 R per million years for Mars to approx. 1 R per million years for Mercury, for distances approx. 2R from the body, where R is the body's radius. Asteroid 243 Ida has approx. 10 R per million years, while a hypothetical Near-Earth Asteroid (NEA) can have faster rates of approx. 0.5 R per thousand years, due chiefly to its small radius compared to the planets. The thermal expansion effect weakens greatly at Jupiter and is overwhelmed by Poynting-Robertson for icy particles orbiting Saturn. Meteoroids in eccentric orbits about the Sun also suffer the thermal expansion effect, but with only approx. 0.0003e2 AU change in semimajor axis over a million years for a 2 m meteoroid orbiting between Mercury and Earth.

Ring particles↗
NASA NTRS1999

Remote Sensing of smoke and its Direct Radiative Forcing in South America

Smoke aerosol, organic and black carbon particles suspended in the air, can absorb and reflect solar radiation to space, i.e., direct radiative forcing. Depending on the ratio of scattering to absorption, and the surface spectral properties, the net smoke effect can be warming or cooling of the climate system. Data from the Airborne Visible/Infrared Imaging Spectrometer (AVIRIS) flown on the ER-2 at altitude of 20km, and of the AERONET ground based sun/sky radiometers are used to assess the smoke aerosol optical thickness over the land and the direct radiative forcing at the top of the atmosphere and at ground level, respectively. The data are collected during the Smoke, Clouds, and Radiation - Brazil (SCAR-B) experiment. In contrast to model results of the smoke effect, we show using the AVIRIS data, that even though the surface albedo is high (0.17 - average on the solar spectrum) and the smoke single scattering albedo is low (0.88), smoke does increase the instantaneous reflectance of sunlight to space by 30-40 W/m2 for an increase in the smoke optical thickness of 0.5. The AERONET data are used to derive, simultaneously, the effect of smoke on the downward radiation. Models using spectrally averaged smoke optical properties and averaged surface reflectance, predicted very small smoke forcing. The reason is that smoke is mainly opaque in short wavelengths (e.g.<0.7 micron) while the surface is mainly bright in longer wavelengths (>0.7 micron). Modeling the effect of smoke on climate forcing cannot be done using the spectrally average properties. It requires the knowledge of the smoke and surface spectral properties.

Kaufman, Yoram J.↗
NASA NTRS2015

Using the Shuttle In Situ Window and Radiator Data for Meteoroid Measurements

Every time NASA's Space Shuttle flew in orbit, it was exposed to the natural meteoroid and artificial debris environment. NASA Johnson Space Center maintains a database of impact cratering data of 60 Shuttle missions flown since the mid‐1990's that were inspected after flight. These represent a total net exposure time to the space environment of 2 years. Impact damage was recorded on the windows and radiators, and in many cases information on the impactor material was determined by later analysis of the crater residue. This information was used to segregate damage caused by natural meteoroids and artificial space debris. The windows represent a total area of 3.565 sq m, and were capable of resolving craters down to about 10 micrometers in size. The radiators represent a total area of 119.26 sq m, and saw damage from objects up to approximately 1 mm in diameter. These data were used extensively in the development of NASA's ORDEM 3.0 Orbital Debris Environment Model, and gives a continuous picture of the orbital debris environment in material type and size ranging from about 10 micrometers to 1 mm. However, the meteoroid data from the Shuttles have never been fully analyzed. For the orbital debris work, special "as flown" files were created that tracked the pointing of the surface elements and their shadowing by structure (such as the ISS during docking). Unfortunately, such files for the meteoroid environment have not yet been created. This talk will introduce these unique impact data and describe how they were used for orbital debris measurements. We will then discuss some simple first‐order analyses of the meteoroid data, and point the way for future analyses.

Matney, Mark↗
NASA NTRS1980

Outer atmospheres of cool stars. IV - A discussion of cool stellar wind models

Possible wind models for late-type stars which appear not to have hot coronae and transition regions are investigated; taking Arcturus and the prototypical star, models with T less than approximately 20,000 K are considered, and solutions with mass loss rates of 10 to the -9th solar masses per year are sought. The radiation pressure of L-alpha resonance scattering can exceed the force of gravity in the chromosphere and initiate a net outflow, but is insufficient to sustain a wind, except perhaps in the presence of an additional momentum input term such as Alfven wave pressure. It is concluded that L-alpha radiation-pressure-initiated winds can occur in stars to the right of the Linsky-Haisch dividing line in the H-R diagram between stars with and without transition regions and presumably hot coronae, and that the existence of these winds may explain energetically the absence of hot coronae in these stars.

Haisch, B. M.↗
NASA NTRS1981

Earth radiation budgets

The annual and seasonal averaged earth atmosphere radiation budgets, derived from the most complete set of satellite observations available in late 1979, are presented. The budgets are derived using a composite of 48 monthly mean radiation budget maps. The annual, global average emitted infrared flux is 234 W/sq m, the planetary albedo is 0.30, and the net flux is zero within measurement uncertainty. In addition, the annual cycle of net flux is studied in detail, and the observed globally averaged net flux is found to display an annual cycle that is of similar magnitude and phase to the annual cycle imposed by the influence of sun-earth distance variations on solar radiation input into the atmosphere.

Stephens, G. L.↗
NASA NTRS1999

Remote Sensing of Smoke and its Direct Radiative Forcing in South-America

Smoke aerosol, organic and black carbon particles suspended in the air, are capable to absorb and reflect solar radiation to space - direct radiative forcing. Depending on the ratio of scattering to absorption, and on the surface spectral properties, the net smoke effect can be warming or cooling of the climate system. Data from the AVIRIS spectrometer flown on the ER-2 at altitude of 20 km, and of the AERONET ground based sun/sky radiometers are used to assess the smoke aerosol optical thickness over the land and the direct radiative forcing at the top of the atmosphere and at ground level, respectively. The data are collected during the SCAR-B experiment in Brazil. In contrast to model results of the smoke effect, we show using the AVIRIS data, that even though the surface albedo is high (0.17 - average on the solar spectrum) and the smoke single scattering albedo is low (0.88), smoke does increase the instantaneous reflectance of sunlight to space by 30-40 W/m(exp 2) for an increase in the smoke optical thickness of 0.5. The AERONET data are used to derive, simultaneously, the effect of smoke on the downward radiation. Models using spectrally averaged smoke optical properties and averaged surface reflectance, predicted very small smoke forcing. The reason is that smoke is mainly opaque in short wavelengths (e.g.< 0.7 micron) while the surface is mainly bright in longer wavelengths (> 0.7 micron). Modeling the effect of smoke on climate forcing cannot be done using the spectrally average properties. It requires the knowledge of the smoke and surface spectral properties.

Kaufman, Yoram↗
NASA NTRS2011

Coupled Aerosol-Chemistry-Climate Twentieth-Century Transient Model Investigation: Trends in Short-Lived Species and Climate Responses

The authors simulate transient twentieth-century climate in the Goddard Institute for Space Studies (GISS) GCM, with aerosol and ozone chemistry fully coupled to one another and to climate including a full dynamic ocean. Aerosols include sulfate, black carbon (BC), organic carbon, nitrate, sea salt, and dust. Direct and BC snow-albedo radiative effects are included. Model BC and sulfur trends agree fairly well with records from Greenland and European ice cores and with sulfur deposition in North America; however, the model underestimates the sulfur decline at the end of the century in Greenland. Global BC effects peak early in the century (1940s); afterward the BC effects decrease at high latitudes of the Northern Hemisphere but continue to increase at lower latitudes. The largest increase in aerosol optical depth occurs in the middle of the century (1940s-80s) when sulfate forcing peaks and causes global dimming. After this, aerosols decrease in eastern North America and northern Eurasia leading to regional positive forcing changes and brightening. These surface forcing changes have the correct trend but are too weak. Over the century, the net aerosol direct effect is -0.41 Watts per square meter, the BC-albedo effect is -0.02 Watts per square meter, and the net ozone forcing is +0.24 Watts per square meter. The model polar stratospheric ozone depletion develops, beginning in the 1970s. Concurrently, the sea salt load and negative radiative flux increase over the oceans around Antarctica. Net warming over the century is modeled fairly well; however, the model fails to capture the dynamics of the observedmidcentury cooling followed by the late century warming.Over the century, 20% of Arctic warming and snow ice cover loss is attributed to the BC albedo effect. However, the decrease in this effect at the end of the century contributes to Arctic cooling. To test the climate responses to sulfate and BC pollution, two experiments were branched from 1970 that removed all pollution sulfate or BC. Averaged over 1970-2000, the respective radiative forcings relative to the full experiment were +0.3 and -0.3 Watts per square meter; the average surface air temperature changes were +0.2 degrees and -0.03 C. The small impact of BC reduction on surface temperature resulted from reduced stability and loss of low-level clouds.

Koch, Dorothy↗
NASA NTRS1988

Sensitivity of satellite-derived net shortwave irradiance at the Earth's surface to radiometric calibration

The effect of radiometric calibration uncertainties on satellite-derived net shortwave irradiance at the Earth's surface was examined. Net shortwave irradiance sensitivity to calibration is expressed as a function of two basic components that depend on surface and cloud albedo sensitivities, respectively. The analysis of these sensitivities for a wide range of atmospheric and surface conditions, as well as radiation geometries, shows that a 10 percent uncertainty in the calibration induces up to 40 W/sqm errors in instantaneous net shortwave irradiance (negative when the calibration uncertainty is positive). The maximum relative errors are obtained in overcast conditions when cloud albedos are high. On a monthly time scale, the induced error becomes typically 13 W/sqm in the tropics and 16 W/sqm in higher latitude regions during summer. The error almost vanishes at high latitudes during winter. A 10 percent positive uncertainty in the calibration gives a net shortwave irradiance error similar to that induced by the 3 hr sampling of the ISCCP Project.

Gautier, C.↗
NASA NTRS2003

Interannual Variability of the Tropical Water Cycle: Capabilities in the TRMM Era and Challenges for GPM

Considerable uncertainty surrounds the issue of whether precipitation over the tropical oceans (30" NE) systematically changes with interannual sea-surface temperature (SST) anomalies that accompany El Nino (warm) and La Nina (cold) events. Although it is well documented that El Nino-Southern Oscillation (ENSO) events with marked SST changes over the tropical oceans, produce significant regional changes in precipitation, water vapor, and radiative fluxes in the tropics, we still cannot yet adequately quantify the associated net integrated changes to water and heat balance over the entire tropical oceanic or land sectors. Robertson et al., [2001 GRL] for example, showed that substantial disagreement exists among contemporary satellite estimates of interannual variations in tropical rainfall that are associated with SST changes. Berg et al., [2002 J. Climate] have documented the distinct differences between precipitation structure over the eastern and western Pacific ITCZ and noted how various satellite precipitation algorithms may respond quite differently to ENSO modulations of these precipitation regimes. Resolving this uncertainty is important since precipitation and latent heat release variations over land and ocean sectors are key components of the tropical heat balance in its most aggregated form. Rainfall estimates from the Tropical Rainfall Measuring Mission (TRMM) Precipitation Radar (PR) averaged over the tropical oceans have not solved this issue and, in fact, show marked differences with estimates from two TRMM Microwave Imager (TMI) passive microwave algorithms. In this paper we will focus on findings that uncertainties in microphysical assumptions necessitated by the single-frequency PR measurement pose difficulties for detecting climate-related precipitation signals. Recent work has shown that path-integrated attenuation derived from the effects of precipitation on the radar return from the ocean surface exhibits interannual variability that agrees closely with the TMI time series, yet the PR rainfall interannual variability (and attenuation derived predominantly from reflectivity) differs even in sign. We will explore these apparent inconsistencies and detail their impact on estimates of how ENSO events perturb the tropical rainfall. We will place these results in perspective by considering requirements for precipitation accuracy for global climate variability and change studies involving ENSO, monsoon dynamics and variations, and climate model improvement and validation. The discussion will conclude with an assessment of the implications of these findings for Global Precipitation Mission (GPM) requirements.

Robertson, Franklin R.↗
NASA NTRS2005

Interannual Variability of Tropical Rainfall as Seen From TRMM

Considerable uncertainty surrounds the issue of whether precipitation over the tropical oceans (30deg N/S) systematically changes with interannual sea-surface temperature (SST) anomalies that accompany El Nino (warm) and La Nina (cold) events. Although it is well documented that El Nino-Southern Oscillation (ENSO) events with marked SST changes over the tropical oceans produce significant regional changes in precipitation, water vapor, and radiative fluxes in the tropics, we still cannot yet adequately quantify the associated net integrated changes to water and heat balance over the entire tropical oceanic or land sectors. Resolving this uncertainty is important since precipitation and latent heat release variations over land and ocean sectors are key components of the tropical heat balance in its most aggregated form. Rainfall estimates from the Version 5 Tropical Rainfall Measuring Mission (TRMM) Precipitation Radar (PR) averaged over the tropical oceans have not solved this issue and, in fact, show marked differences with estimates from two TRMM Microwave Imager (TMI) passive microwave algorithms. In this paper we will focus on findings that uncertainties in microphysical assumptions necessitated by the single-frequency PR measurement pose difficulties for detecting climate-related precipitation signals. Recent work has shown that path-integrated attenuation derived from the effects of precipitation on the radar return from the ocean surface exhibits interannual variability that agrees closely with the TMI time series, yet the PR rainfall interannual variability (and attenuation derived predominantly from reflectivity) differs even in sign. We will explore these apparent inconsistencies and examine changes in new TRMM Version 6 retrievals. To place these results in a tropical water balance perspective we also examine interannual variations in evaporation over the tropical oceans made from TRMM and SSM/I (Special Sensor Microwave Imager) measurements of surface winds and humidity. Evaporation estimates from reanalysis and several global model experiments will also be compared to the TRMM findings and evaluated for consistency. The ability to detect regional shifts in freshwater flux over the oceans (equivalently, integrated moisture convergence) and moisture transport will be discussed.

Robertson, Franklin R.↗
NASA NTRS2007

Charges on Strange Quark Nuggets in Space

Since Witten's seminal 1984 paper on the subject, searches for evidence of strange quark nuggets (SQNs) have proven unsuccessful. In the absence of experimental evidence ruling out SQNs, the validity of theories introducing mechanisms that increase their stability should continue to be tested. To stimulate electromagnetic SQN searches, particularly space searches, we estimate the net charge that would develop on an SQN in space exposed to various radiation baths (and showers) capable of liberating their less strongly bound electrons, taking into account recombination with ambient electrons. We consider, in particular, the cosmic background radiation, radiation from the sun, and diffuse galactic and extragalactic gamma-ray backgrounds. A possible dramatic signal of SQNs in explosive astrophysical events is noted.

Abers, E. S.↗
NASA NTRS2009

NanoSail-D: A Solar Sail Demonstration Mission

During the past decade, within the United States, NASA Marshall Space Flight Center (MSFC) was heavily engaged in the development of revolutionary new technologies for in-space propulsion. One of the major in-space propulsion technologies developed was a solar sail propulsion system. Solar sail propulsion uses the solar radiation pressure exerted by the momentum transfer of reflected photons to generate a net force on a spacecraft. To date, solar sail propulsion systems have been designed for large spacecraft in the tens to hundreds of kilograms mass range. Recently, however, MSFC has been investigating the application of solar sails for small satellite propulsion. Likewise, NASA Ames Research Center (ARC) has been developing small spacecraft missions that have a need for amass-efficient means of satisfying deorbit requirements. Hence, a synergistic collaboration was established between these two NASA field Centers with the objective of conducting a flight demonstration of solar sail technologies for small satellites. The NanoSail-D mission flew onboard the ill-fated Falcon Rocket launched August 2, 2008, and, due to the failure of that rocket, never achieved orbit. The NanoSail-D flight spare is ready for flight and a suitable launch arrangement is being actively pursued. Both the original sailcraft and the flight spare are hereafter referred to as NanoSail-D. The sailcraft consists of a sail subsystem stowed in a three-element CubeSat. Shortly after deployment of the NanoSail-D, the solar sail will deploy and mission operations will commence. This demonstration flight has two primary technical objectives: (1) to successfully stow and deploy the sail and (2) to demonstrate deorbit functionality. Given a near-term opportunity for launch on Falcon, the project was given the challenge of delivering the flight hardware in 6 mo, which required a significant constraint on flight system functionality. As a consequence, passive attitude stabilization of the spacecraft will be achieved using permanent magnets to detumble and orient the body with the magnetic field lines and then rely on atmospheric drag to passively stabilize the sailcraft in an essentially maximum drag attitude. This paper will present an introduction to solar sail propulsion systems and an overview of the NanoSail-D spacecraft.

Johnson, Les↗
NASA NTRS2019

Inter-relationship Between Subtropical Pacific Sea Surface Temperature, Arctic Sea Ice Concentration, and North Atlantic Oscillation in Recent Summers

The inter-relationship between subtropical western–central Pacific sea surface temperatures (STWCPSST), sea ice concentrations in the Beaufort Sea (SICBS), and the North Atlantic Oscillation (NAO) in summer are investigated over the period 1980–2016. It is shown that the Arctic response to the remote impact of the Pacific SST is more dominant in recent summers, leading to a frequent occurrence of the negative phase of the NAO following the STWCPSST increase. Lag–correlations of STWCPSST positive (negative) anomalies in spring with the negative (positive) NAO and SICBS loss (recovery) in summer have increased over the last two decades, reaching r = 0.4–0.5 with significance at the 5 percent level. Both observations and the atmospheric general circulation model experiments suggest that the positive STWCPSST anomaly and subsequent planetary-scale wave propagation act to increase the Arctic upper-level geopotential heights and temperatures in the following season. This response extends to Greenland, providing favorable conditions for developing the negative phase of the NAO. Connected with this atmospheric response, SIC and surface albedo decrease with an increase in the surface net shortwave flux over the Beaufort Sea. Examination of the surface energy balance (radiative and turbulent fluxes) reveals that surplus energy that can heat the surface increases over the Arctic, enhancing the SIC reduction.

SST↗
NASA NTRS1994

Computations of diabatic descent in the stratospheric polar vortex

A radiation model, together with National Meteorological Center temperature observations, was used to compute daily net heating rates in the northern hemisphere (NH) for the Arctic late fall and winter periods of both 1988-1989 and 1991-1992 and in the southern hemisphere (SH) for the Antarctic fall and winters of 1987 and 1992. The heating rates were interpolated to potential temperature (theta) surfaces between 400 K and 2000 K and averaged within the polar vortex, the boundary of which was determined by the maximum gradient in potential vorticity. The averaged heating rates were used in a one-dimensional vortex interior descent model to compute the change in potential temperature with time of air parcels initialized at various theta values, as well as to compute the descent in log pressure coodinates. In the NH vortex, air parcels which were initialized at 18 km on November 1, descended about 6 km by March 21, while air initially at 25 km descended 9 km in the same time period. this represents an average descent rate in the lower stratosphere of 1.3 to 2 km per month. Air initialized at 50 km descended 27 km between November 1 and March 21. In the SH vortex, parcels initialized at 18 km on March 1, descended 3 km, while air at 25 km descended 5-7 km by the end of October. This is equivalent to an average descent in the lower stratosphere of 0.4 to 0.9 km per month during this 8-month period. Air initialized at 52 km descended 26-29 km between March 1 and October 31. In both the NH and the SH, computed descent rates increased markedly with height. The descent for the NH winter of 1992-1993 and the SH winter of 1992 computed with a three-dimensional trajectory model using the same radiation code was within 1 to 2 km of that calculated by the one-dimensional model, thus validating the vortex averaging procedure. The computed descent rates generally agree well with observations of long-lived tracers, thus validating the radiative transfer model.

Rosenfield, Joan E.↗
NASA NTRS1994

Effects of the Mount Pinatubo eruption on the radiative and chemical processes in the troposphere and stratosphere

The Lawrence Livermore National Laboratory two-dimensional zonally-averaged chemical-radiative-transport model of the global atmosphere was used to study the effects of the 15 June 1991 eruption of the Mt. Pinatubo volcano on stratospheric processes. SAGE 2 time-dependent aerosol surface area density and optical extinction data were used as input into the model. By 22 December 1991, a maximum equatorial change of -1.8 percent in column ozone was derived from heterogeneous chemical processes that convert NO(x) into HNO3 on sulfuric acid aerosols. Radiative feedbacks from increased aerosol optical thickness independently changes column ozone by approximately -3.5 percent for the same period. This occurs from increasing the net heating of the lower stratosphere, which indirectly increases chemical reaction rates via their temperature dependence and from changes in actinic fluxes, which directly modify photodissociation rates. Including both heterogeneous and radiative effects changes column ozone by -5.5 percent. The model-derived change overestimates the decrease in column ozone relative to the TOMS instrument on the Nimbus 7 satellite. Maximum local ozone decreases of 12 percent were derived in the equatorial region, at 25 km. Model-derived column NO2 peaked (-14 percent) at 30 deg S in October 1991. The timing of the NO2 peak is consistent with observation, but the model underestimates the magnitude of the decrease. Local concentrations of NO(x) (NO + NO2), ClO(x) (Cl + ClO), and HO(x) (OH + HO2), in the lower stratosphere between 30 deg S and 30 deg N, were calculated to have changed by -40 percent, +100 to +160 percent, and +120 to +140 percent respectively.

Kinnison, Douglas E.↗