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At least 577 records · Page 32

Using coherent phonons for ultrafast control of the Dirac node of SrMnSb 2

SrMnSb 2 is a candidate Dirac semimetal whose electrons near the Y point have the linear dispersion and low mass of a Dirac cone. Here we demonstrate that ultrafast, 800-nm optical pulses can launch coherent phonon oscillations in Sr 0.94 Mn 0.92 Sb 2 , particularly an A g mode at 4.4 THz. Through first-principles calculations of the electronic and phononic structure of SrMnSb 2 , we show that high-amplitude oscillations of this mode would displace the atoms in a way that transiently opens and closes a gap at the node of the Dirac cone. Furthermore, the ability to control the nodal gap on a subpicosecond timescale could create opportunities for the design and manipulation of Dirac fermions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic Field Modulated Photoreflectance Study of the Electron Effective Mass in Dilute Nitride Semiconductors

Magnetic field modulated photoreflectance measurements are performed on the dilute nitride semiconductor Ga(AsN) in quantizing magnetic fields. From the measured cyclotron energies, the conduction band effective mass and its dependence on the nitrogen content are determined. The effective mass is found to become significantly heavier in samples with high nitrogen composition (>0.1%).

36 MATERIALS SCIENCE↗

Electron and Hole Spin Relaxation in InAs Quantum Dots and Quasi-2D Structure

Temperature dependence of hole and electron spin relaxation times in both InAs quantum dots (QDs) and quasi-two-dimensional (2D) monolayers has been investigated experimentally using time-resolved photoluminescence (TRPL). The results show that hole spin relaxation time is long enough to be comparable with that of electrons in the quasi-2D InAs structure, but is one order of magnitude smaller than the electron spin relaxation time in QDs structure. It is shown that both hole and electron spin relaxation times decrease monotonically with increasing temperature for InAs QDs, but show non-monotonic temperature-dependent behavior for the quasi-2D structure. Different spin relaxation mechanisms responsible for spin relaxation in the two structures have been discussed.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Superconductivity in a system of interacting spinful semions

Noninteracting particles obeying certain fractional statistics have been predicted to exhibit superconductivity. We discuss the issue in an attractively interacting system of spinful semions on a lattice by numerically investigating the presence of off-diagonal long-range order at zero temperature. For this purpose we construct a Hubbard model wherein two semions with opposite spin can virtually coincide while maintaining consistency with the fractional braiding statistics. Clear off-diagonal long-range order is seen in the strong coupling limit, consistent with the expectation that a pair of semions obeys Bose statistics. We find that the semion system behaves similarly to a system of fermions with the same attractive Hubbard U interaction for a wide range of U, suggesting that semions also undergo a BCS to BEC crossover as a function of U.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Quantum critical point revisited by dynamical mean-field theory

Dynamical mean-field theory is used to study the quantum critical point (QCP) in the doped Hubbard model on a square lattice. We characterize the QCP by a universal scaling form of the self-energy and a spin density wave instability at an incommensurate wave vector. The scaling form unifies the low-energy kink and the high-energy waterfall feature in the spectral function, while the spin dynamics includes both the critical incommensurate and high-energy antiferromagnetic paramagnons. Here, we use the frequency-dependent four-point correlation function of spin operators to calculate the momentum-dependent correction to the electron self-energy. Furthermore, by comparing with the calculations based on the spin-fermion model, our results indicate the frequency dependence of the quasiparticle-paramagnon vertices is an important factor to capture the momentum dependence in quasiparticle scattering.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Vacancy Spectroscopy of Non-Abelian Kitaev Spin Liquids

Spin vacancies in the non-Abelian Kitaev spin liquid are known to harbor Majorana zero modes, potentially enabling topological quantum computing at elevated temperatures. Here, we study the spectroscopic signatures of such Majorana zero modes in a scanning tunneling setup where a non-Abelian Kitaev spin liquid with a finite density of spin vacancies forms a tunneling barrier between a tip and a substrate. In this study, our key result is a well-defined peak close to zero bias voltage in the derivative of the tunneling conductance whose voltage and intensity both increase with the density of vacancies. This “quasi-zero-voltage peak” is identified as the closest analog of the zero-voltage peak observed in topological superconductors that additionally reflects the fractionalized nature of spin-liquid-based Majorana zero modes. We further highlight a single-fermion Van Hove singularity at a higher voltage that reveals the energy scale of the emergent Majorana fermions in the Kitaev spin liquid. Our proposed signatures are within reach of current experiments on the candidate material α-RuCl 3 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Concurrence of superconductivity and structure transition in Weyl semimetal TaP under pressure

Weyl semimetal defines a material with three-dimensional Dirac cones, which appear in pair due to the breaking of spatial inversion or time reversal symmetry. Superconductivity is the state of quantum condensation of paired electrons. Turning a Weyl semimetal into superconducting state is very important in having some unprecedented discoveries. In this work, by doing resistive measurements on a recently recognized Weyl semimetal TaP under pressures up to about 100 GPa, we show the concurrence of superconductivity and a structure transition at about 70 GPa. It is found that the superconductivity becomes more pronounced when decreasing pressure and retains when the pressure is completely released. High-pressure x-ray diffraction measurements also confirm the structure phase transition from I41md to P-6m2 at about 70 GPa. More importantly, ab-initial calculations reveal that the P-6m2 phase is a new Weyl semimetal phase and has only one set of Weyl points at the same energy level. Our discovery of superconductivity in TaP by high pressure will stimulate investigations on superconductivity and Majorana fermions in Weyl semimetals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Classical and quantum simulations of 1+1-dimensional ${\mathbb{Z}}_{2}$ gauge theory at finite temperature and density

Simulating strongly coupled gauge theories at finite temperature and density is a longstanding challenge in nuclear and high-energy physics with fundamental implications for condensed matter physics. Here, we simulate such systems using minimally entangled typical thermal state (METTS) approaches, which combine classical random sampling with imaginary-time evolution, implementable on either classical or quantum computers, to estimate thermal averages of observables. We study 1+1-dimensional ${\mathbb{Z}}_{2}$ gauge theory coupled to spinless fermionic matter, which maps onto a local quantum spin chain. We benchmark both a classical matrix-product-state implementation of METTS and a recently proposed adaptive variational approach for near-term quantum devices, focusing on the equation of state and measures of fermion confinement. Of particular importance is the choice of basis for METTS sampling, which impacts both the sampling overhead and quantum circuit complexity. Our work sets the stage for future studies of strongly coupled gauge theories using classical and quantum hardware.

Chen, I-Chi [Iowa State Univ., Ames, IA (United St↗

Free Carrier Absorption due to Dislocation Scattering in GaN Quantum Wells

Free carrier absorption (FCA) is studied in quantum well structures assuming electrons to be scattered by dislocations via strain field. Expression for FCA coefficient, {alpha} is obtained assuming radiation field to be polarized along the plane of quantum well. Numerical results of {alpha}, as function of photon frequency, {Omega} and well width, d are presented. Calculations show, FCA to decrease with increase in {Omega} with a kink observed at {Omega} = 7.79x10{sup 13} s{sup -1} indicating onset of inter subband transitions. {alpha} is found to be proportional to d{sup -3} and to increase with increase in dislocation density.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Universal spin wave damping in magnetic Weyl semimetals

We analyze the decay of spin waves into Stoner excitations in magnetic Weyl semimetals. The lifetime of a mode is found to have a universal dependence on its frequency and momentum, and on a few parameters that characterize the relativistic Weyl spectrum. At the same time, uniform Gilbert damping by Weyl electrons is absent. Here, the decay rate of spin waves is calculated perturbatively using the s-d model of itinerant Weyl or Dirac electrons coupled to local moments. We show that many details of the Weyl spectrum, such as the momentum-space locations, dispersions, and sizes of the Weyl Fermi pockets, can be deduced indirectly by probing the spin waves of local moments using inelastic neutron scattering.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Doping as a tuning mechanism for magnetothermoelectric effects to improve z T in polycrystalline NbP

Weyl semimetals combine topological and semimetallic effects, making them candidates for interesting and effective thermoelectric transport properties. Here, we present experimental results on polycrystalline NbP, demonstrating the simultaneous existence of a large Nernst effect and a large magneto-Seebeck effect, which is typically not observed in a single material at the same temperature. We compare transport results from two polycrystalline samples of NbP with previously published work, observing a shift in the temperature at which the maximum Nernst and magneto-Seebeck thermopowers occur, while still maintaining thermopowers of similar magnitude. Theoretical modeling shows how doping strongly alters both the Seebeck and Nernst magneto-thermopowers by shifting the temperature-dependent chemical potential, and the corresponding calculations provide a consistent interpretation of our results. Thus, we offer doping as a tuning mechanism for shifting magneto-thermoelectric effects to temperatures appropriate for device applications, improving zT at desirable operating temperatures. Furthermore, the simultaneous presence of both a large Nernst and magneto-Seebeck thermopower is uncommon and offers unique device advantages if the thermopowers are used additively. Finally, we also propose a unique thermoelectric device which would collectively harness the large Nernst and magneto-Seebeck thermopowers to greatly enhance the output and zT of conventional thermoelectric devices.

30 DIRECT ENERGY CONVERSION↗

Disentanglement of electron dynamics and space-charge effects in time-resolved photoemission from h-BN/Ni(111)

We observe time-resolved and polarization dependent two-, three-, and four-photon transitions from a Ni(111) surface covered with a monolayer of hexagonal boron nitride. The spectra show features due to transitions involving two unoccupied intermediate states: the n=1 image potential state of Ni(111) and a boron nitride-related interface state. We use these transitions in order to track the effects of space-charge on the spectra in view of pump-probe experiments, at high excitations densities. A simple model is presented, which reproduces the measured energy shifts and broadenings in great detail, allowing the ultrafast dynamics and the space-charge effects to be disentangled. Moreover, owing to the high excitation densities an additional particular three-photon transition via both the interface state and a virtual intermediate state could be measured and identified. The polarization-dependent transient of this transition has successfully been simulated, allowing the lifetime of the involved intermediate state to be extracted from the data.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Superconductivity in a topological lattice model with strong repulsion

The highly tunable nature of synthetic quantum materials-both in the solid-state and cold atom contexts-invites examining which microscopic ingredients aid in the realization of correlated phases of matter such as superconductors. Recent experimental advances in moiré materials suggest that unifying the features of the Fermi-Hubbard model and quantum Hall systems creates a fertile ground for the emergence of such phases. Here, we introduce the "double Hofstadter"model, a minimal 2D lattice model that incorporates exactly these features: Time-reversal symmetry, band topology, and strong repulsive interactions. By using infinite cylinder density matrix renormalization group methods (cylinder iDMRG), we investigate the ground state phase diagram of this model. We find that it hosts an interaction-induced quantum spin Hall insulator and demonstrate that weakly hole-doping this state gives rise to a superconductor at a finite circumference, with indications that this behavior persists on larger cylinders. Further, at the aforementioned circumference, the superconducting phase is surprisingly robust to perturbations including additional repulsive interactions in the pairing channel. By developing a technique to probe the superconducting gap function in iDMRG, we phenomenologically characterize the superconductor. Namely, we demonstrate that it is formed from the weak pairing of holes atop the quantum spin Hall insulator. Furthermore, we determine the pairing symmetry of the superconductor, finding it to be p-wave-reminiscent of the unconventional superconductivity reported in experiments on twisted bilayer graphene (TBG). Motivated by this, we elucidate structural similarities and differences between our model and those of TBG in its chiral limit. Finally, to provide a more direct experimental realization, we detail an implementation of our Hamiltonian in a system of cold fermionic alkaline-earth atoms in an optical lattice.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Vortexlike excitations in the heavy-fermion superconductor CeIrIn 5

Here, we report a systematic study of temperature- and field-dependent charge (ρ) and entropy (S) transport in the heavy-fermion superconductor CeIrIn 5 . Its large positive thermopower S xx is typical of Ce-based Kondo lattice systems, and strong electronic correlations play an important role in enhancing the Nernst signal S xy . By separating the off-diagonal Peltier coefficient α xy from S xy , we find that αxy becomes positive and greatly enhanced at temperatures well above the bulk T c . Compared with the nonmagnetic analog LaIrIn 5 , these results suggest vortexlike excitations in a precursor state to unconventional superconductivity in CeIrIn 5 . This study sheds light on the similarity of heavy-fermion and cuprate superconductors and on the possibility of states not characterized by the amplitude of an order parameter.

36 MATERIALS SCIENCE↗

Two-dimensional conductors with interactions and disorder from particle-vortex duality

Here, we study Dirac fermions in two spatial dimensions (2D) coupled to strongly fluctuating U (1) gauge fields in the presence of quenched disorder. Such systems are dual to theories of free Dirac fermions, which are vortices of the original theory. In analogy to superconductivity, when these fermionic vortices localize, the original system becomes a perfect conductor, and when the vortices possess a finite conductivity, the original fermions do as well. We provide several realizations of this principle and thereby introduce examples of strongly interacting 2D metals that evade Anderson localization.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Two-dimensional spin liquid behaviour in the triangular-honeycomb antiferromagnet TbInO 3

Spin liquid ground states are predicted to arise within several distinct scenarios in condensed matter physics. The observation of these disordered magnetic states is particularly pervasive among a class of materials known as frustrated magnets, in which the competition between various magnetic exchange interactions prevents the system from adopting long-range magnetic order at low temperatures. Spin liquids continue to be of great interest due to their exotic nature and the possibility that they may support fractionalized excitations, such as Majorana fermions. Systems that allow for such phenomena are not only fascinating from a fundamental perspective but may also be practically significant in future technologies based on quantum computation. Here we show that the underlying antiferromagnetic sublattice in TbInO 3 can undergo a crystal field-induced distortion of its buckled triangular arrangement to one based on a honeycomb. The absence of a conventional magnetic ordering transition at the lowest measurable temperatures indicates that another critical mechanism must govern in the ground-state selection of TbInO 3 . Here, we suggest that anisotropic exchange interactions—mediated through strong spin–orbit coupling on the emergent honeycomb lattice of TbInO 3 —give rise to a highly frustrated spin liquid.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Edge-Channel Photo-Effect In Asymmetric Two-Dimensional Systems

We report on the photo-effect in an asymmetric two dimensional electron system where edge currents are induced by homogeneous terahertz (THz) radiation in tilted magnetic field without any external bias. We discuss the features of the observed effect and its mechanism taking into account properties of edge states in magnetic fields. The process is understood as the quantum Hall effect associated with electron-hole pairs generated in Landau levels by THz radiation under CR conditions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Optical electron spin orientation in Ga-doped and undoped ZnO films

We have studied the optical orientation and polarization relaxation dynamics of electron spins in Ga-doped and undoped ZnO films by time-resolved Kerr rotation (TRKR). In the Ga-doped film, we have observed a long-lived spin signal more than 10 ns when the pump-probe energy is resonant to the neutral donor-bound excitons (D deg. X). It is not observed in the undoped film. Meanwhile, when the energy is resonant to free excitons, faster spin relaxation of about 2 ns is observed for itinerant electrons in both the films. The optical spin orientation is always parallel to the c-axis in the ZnO films, and independent of the pump incidence angle. This contrasts with the observation in crystals with the zincblende structure.

36 MATERIALS SCIENCE↗