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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 577 records · Page 32
All sourcesNASA NTRSDOE OSTI
NASA NTRS2009

Radiative Effects of African Dust and Smoke Observed from CERES and CALIOP Data

Cloud and aerosol effects have a significant impact on the atmospheric radiation budget in the Tropical Atlantic because of the spatial and temporal extent of desert dust and smoke from biomass burning in the atmosphere. The influences of African dust and smoke aerosols on cloud radiative properties over the Tropical Atlantic Ocean were analyzed for the month of July for three years (2006-2008) using collocated data collected by the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and Clouds and the Earth s Radiant Energy System (CERES) instruments on the CALIPSO and Aqua satellites. Aerosol layer height and type can be more accurately determined using CALIOP data, through parameters such as cloud and aerosol layer height, optical depth and depolarization ratio, than data from atmospheric imagers used in previous cloud-aerosol interaction studies. On average, clouds below 5 km had a daytime instantaneous shortwave (SW) radiative flux of 270.2 +/- 16.9 W/sq m and thin cirrus clouds had a SW radiative flux of 208.0 +/- 12.7 W/sq m. When dust aerosols interacted with clouds below 5 km, as determined from CALIPSO, the SW radiative flux decreased to 205.4 +/- 13.0 W/sq m. Similarly, smoke aerosols decreased the SW radiative flux of low clouds to a value of 240.0 +/- 16.6 W/sq m. These decreases in SW radiative flux were likely attributed to the aerosol layer height and changes in cloud microphysics. CALIOP lidar observations, which more accurately identify aerosol layer height than passive instruments, appear essential for better understanding of cloud-aerosol interactions, a major uncertainty in predicting the climate system.

Yorks, John E.↗
NASA NTRS2020

First Results From an Uncooled LWIR Polarimeter for Cubesat Deployment

A compact long-wave infrared (LWIR) channeled spectro-polarimeter (IRCSP) has been developed for integration into the NASA Earth Science Technology Office (ESTO) funded submm-wave and LWIR polarimeters project to measure the microphysical properties of cloud ice. Once deployed, the IRCSP will produce the first linear Stokes measurements ( S0 , S1 , S2 ) of upper-tropospheric cirrus clouds from 8.5 to 12.5 μm. For the first time, a compact, light-weight, and uncooled LWIR polarimeter with off-the-shelf thermal optical components is demonstrated. We report narrowband calibration measurements which quantify metrics of polarimetric system performance. The response of the system to linearly polarized light is shown to agree with both a Mueller matrix model and modulation function for narrowband calibration measurements with an R2 > 0.98 from 8 to 11 μm. The polarimetric efficiency is >0.8 from 8 to 11 μm for narrowband measurements indicating satisfactory performance of the polarization optics. Beyond 11 μm, the agreement is significantly reduced as thermal noise compounds with reduced detector response. Ultimately, the observed system performance is limited by the spectral response of the detector past 11 μm in addition to the thermal noise inherent for the measurements at room temperature.

LWIR↗
NASA NTRS2006

Electromagnetic Properties of Filled, Pixellated Arrays

Filled arrays of bolometers are currently being employed for use in astronomy from the far-infrared through millimeter parts of the electromagnetic spectrum. Because of the large range of wavelengths for which this is applicable, the number of modes supported by a bolometric pixel will vary according to specific application. Withington et al. (2003) have built a formalism for treating the electromagnetic properties of such bolometers by propagating the second order statistical properties of the radiation through a canonical optical system. In this work, we use this formalism to construct beam pattern images of square pixels for various ratios of p/lambda where p is the pixel size and lambda is the wavelength. In the low mode limit, the diffraction effects cause the beam pattern to be circular with a quadrupole dependence of Stokes Q and U. High mode cases approach the geometric limit. The polarization in these cases can be seen to trace the pixel edges. The effective size of the beam has a direct impact on the inter-pixel coupling and sets the number of independent detectors in an astronomical focal plane. This technique illustrates and quantifies the relationship between pixel size and angular resolution limits for a given wavelength and telescope. This is especially true in the limit of low p/lambda. In this case, the diffraction due to pixelization is non-negligible for the calculation of the overall angular resolution of the telescope. In addition, for instruments that are polarization sensitive, this method also provides a quantitative method for determining the contribution of the instrument to the measured polarization.

Chuss, David T.↗
NASA NTRS2018

Toward a Satellite-Derived Climatology of Blowing Snow Over Antarctica

Satellite lidar remote sensing of the atmosphere has been ongoing for more than a decade providing the opportunity to study atmospheric processes in great detail. Here we use 12 years of Cloud‐Aerosol Lidar with Orthogonal Polarization measurements to derive a climatology of blowing snow layer height, optical depth, and frequency over Antarctica for the period 2006–2017. Limited to the vertical resolution of the Cloud‐Aerosol Lidar with Orthogonal Polarization data, our climatology includes all blowing snow layers greater than about 30 m in thickness for clear or optically thin cloud regions. Our results show that blowing snow occurs over 50% of the time over large regions with frequencies often exceeding 70%. The overall pattern of blowing snow frequency is fairly consistent from year to year, but there are regional differences. We examined the data for temporal trends in blowing snow properties and found significant trends only in blowing snow frequency. A small area of East Antarctica with generally low blowing snow frequency shows a statistically significant increase in blowing snow frequency ranging from 10% to 100% per decade. No significant trends in frequency were found in regions of high (>50%) blowing snow frequency, and only isolated small areas exhibited a decrease in frequency through the study period.

Palm, Stephen P.↗
DOE OSTI2024

minimpl (b1)

The micropulse lidar (MPL) is a ground-based, optical, remote-sensing system designed primarily to determine the altitude of clouds; however, it is also used for detection of atmospheric aerosols. The physical principle is the same as for radar. Pulses of energy are transmitted into the atmosphere; the energy scattered back to the transceiver is collected and measured as a time-resolved signal, thereby detecting clouds and aerosols in real time. From the time delay between each outgoing pulse and the backscattered signal, the distance to the scatterer is inferred. Post-processing of the lidar return characterizes the extent and properties of aerosols or other particles in a region.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1977

Suits reflectance models for wheat and cotton - Theoretical and experimental tests

Plant canopy reflectance models developed by Suits are tested for cotton and Penjamo winter wheat. Properties of the models are discussed, and the concept of model depth is developed. The models' predicted exchange symmetry for specular irradiance with respect to sun polar angle and observer polar angle agreed with field data for cotton and wheat. Model calculations and experimental data for wheat reflectance vs sun angle disagreed. Specular reflectance from 0.50 to 1.10 micron shows fair agreement between the model and wheat measurements. An Appendix includes the physical and optical parameters for wheat necessary to apply Suits' models.

Chance, J. E.↗
NASA NTRS1991

Coupled bipolarons and optical phonons as a model for high-Tc superconductors

The coherence length of the new high-temperature superconductors reaches a small value which is comparable to the dimensions of the unit cell of the compound. This means that a pair consists of two holes occupying the same site or two adjacent sites. Such a situation is described by a model of the local-pairs (bipolarons). The origin of local-pairs may come not only from strong enough electron or hole-phonon interaction but also from other interactions. Independent of the specific nature of such local-pairs, they can undergo a Bose-like condensation to the superconducting state at a critical temperature which is usually much lower than the temperature of the pair formation. An interplay of ferroelectric and superconducting properties is considered within the model of hole-like local-pairs interacting with optical phonons. Therefore, researchers extend the usual local-pair Hamiltonian by including a direct interaction between the local-pairs and the optical phonons. These optical phonons are known to play an important role in the ferroelectric transition and they transform into an additional pseudo-acoustic branch at the ferroelectric critical temperature. (This is associated with nonzero electric polarization due to the existence of two separate lattices composed of negative and positive ions, respectively.)

Kasperczyk, J.↗
NASA NTRS1994

Robotic vision techniques for space operations

Automation and robotics for space applications are being pursued for increased productivity, enhanced reliability, increased flexibility, higher safety, and for the automation of time-consuming tasks and those activities which are beyond the capacity of the crew. One of the key functional elements of an automated robotic system is sensing and perception. As the robotics era dawns in space, vision systems will be required to provide the key sensory data needed for multifaceted intelligent operations. In general, the three-dimensional scene/object description, along with location, orientation, and motion parameters will be needed. In space, the absence of diffused lighting due to a lack of atmosphere gives rise to: (a) high dynamic range (10(exp 8)) of scattered sunlight intensities, resulting in very high contrast between shadowed and specular portions of the scene; (b) intense specular reflections causing target/scene bloom; and (c) loss of portions of the image due to shadowing and presence of stars, Earth, Moon, and other space objects in the scene. In this work, developments for combating the adverse effects described earlier and for enhancing scene definition are discussed. Both active and passive sensors are used. The algorithm for selecting appropriate wavelength, polarization, look angle of vision sensors is based on environmental factors as well as the properties of the target/scene which are to be perceived. The environment is characterized on the basis of sunlight and other illumination incident on the target/scene and the temperature profiles estimated on the basis of the incident illumination. The unknown geometrical and physical parameters are then derived from the fusion of the active and passive microwave, infrared, laser, and optical data.

Krishen, Kumar↗
DOE OSTI2025

Interplay between Chiro-Optical and Spin Transport Properties in Chiral CdSe Quantum Dots

The chiral-induced spin selectivity (CISS) effect offers compelling approaches for manipulating spin-dependent processes in both chemistry and physics, yet the physical mechanism(s) underpinning CISS are still debated. Here we present a study of structure-property relationships in chiral quantum dot assemblies to identify attributes of CISS-based phenomena. Our results show that the circular dichroism (CD) strength of chiral CdSe quantum dots’ primary exciton transition correlates with two CISS properties, the propensity to transmit pure spin currents and to produce spin-polarized charge currents. While the spin-polarized charge current reverses its sign with a change in the polarity of the CD signal, the pure spin current transport does not. The trends in both transport types can be rationalized in terms of chirality-induced splitting of spin sub-bands, which are modulated by chiral symmetry breaking under charge transport through the CdSe quantum dots.

cadmium selenide↗
DOE OSTI2024

Mechanochromic Palettes Based on Optical Rotation in Cholesteric Liquid Crystal Elastomers for Visual Signalling

Mechanochromic photonic materials present promising prospects for enhancing diverse facets of human life. Cholesteric liquid crystal elastomers (CLCEs) present immediate mechanochromic properties, allowing their utility in various fields, including camouflages, textiles, and anticounterfeiting. Nonetheless, it is essential to provide differentiated color information corresponding to diverse types and degrees of deformation for practical use in real life. Herein, the mechanochromic responses of CLCEs are investigated using their optical rotation under compression and uniaxial stretching. The CLCEs exhibit the same reflection colors indistinguishable for compression and uniaxial stretching due to their contracted pitches. In contrast, the linearly polarized light passing through deformed CLCEs can be modulated by optical rotation, resulting in distinct transmission colors that can be discerned through mechanical deformations. A visual signaling system with color information derived from optical rotation is demonstrated. By comprehending and manipulating the mechanoresponsive behavior of CLCEs, these materials can be advanced into innovative solutions with enhanced functionality and performance, thereby broadening their applications for human life enhancement.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Single-particle scattering spectroscopy: fundamentals and applications

Metallic nanoparticles supporting a localized surface plasmon resonance have emerged as promising platforms for nanoscopic labels, sensors, and (photo-) catalysts. To use nanoparticles in these capacities, and to gain mechanistic insight into the reactivity of inherently heterogeneous nanoparticles, single-particle characterization approaches are needed. Single-particle scattering spectroscopy has become an important, highly sensitive tool for localizing single plasmonic nanoparticles and studying their optical properties, local environment, and reactivity. In this review, we discuss approaches taken for collecting the scattered light from single particles, their advantages and disadvantages, and present some recent applications. We introduce techniques for the excitation and detection of single-particle scattering such as high-angle dark-field excitation, total internal reflection dark-field excitation, scanning near-field microscopy, and interferometric scattering. We also describe methods to achieve polarization-resolved excitation and detection. We then discuss different approaches for scanning, ratiometric, snapshot, and interferometric hyperspectral imaging techniques used to extract spectral information. Finally, we provide a brief overview of specialized setups for in situ measurements of nanoparticles in liquid systems and setups coupled to scanning tip microscopes.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

Mechanochromic Palettes of Cholesteric Liquid Crystal Elastomers for Visual Signaling

Mechanochromic photonic materials present promising prospects for enhancing diverse facets of human life. Cholesteric liquid crystal elastomers (CLCEs) present immediate mechanochromic properties, allowing their utility in various fields, including camouflages, textiles, and anticounterfeiting. Nonetheless, it is essential to provide differentiated color information corresponding to diverse types and degrees of deformation for practical use in real life. Herein, we investigate the mechanochromic responses of CLCEs using their optical rotation under compression and uniaxial stretching. The CLCEs exhibit the same reflection colors indistinguishable for compression and uniaxial stretching due to their contracted pitches. In contrast, the linearly polarized light passing through deformed CLCEs can be modulated by optical rotation, resulting in distinct transmission colors that can be discerned through mechanical deformations. We demonstrate a visual signaling system with color information derived from optical rotation. By comprehending and manipulating the mechanoresponsive behavior of CLCEs, we can advance these materials into innovative solutions with enhanced functionality and performance, thereby broadening their applications for human life enhancement.

36 MATERIALS SCIENCE↗
NASA NTRS2002

MODIS Observations of Smoke and Fires

The MODIS (Moderate Resolution Imaging Spectroradiometer) instruments collect daily measurements of our planet since early 2000 from the Terra spaceborne polar platform. It has unique channels to observe smoke over land and ocean and to observe fires. Using unsaturated channels at 3.9 micron MODIS detects the fires and estimates the fire radiative energy. Using solar channels in the visible (0.47 and 0.66 micron) and in the mid IR (2.1 micron) MODIS measures the smoke optical thickness distribution and evolution over the land. Seven Channels in the solar spectrum are used to detect the smoke properties and distribution over the oceans. Data from the Aerosol Robotic Network, are used to validate the MODIS observations. The MODIS aerosol data presented in a movie form is used to observe the generation of smoke plumes and their dispersion around the globe. For example a key conclusion is that smoke in particular from Southern Africa can pollute significantly the 'pristine' Southern Hemisphere zonal range of 45'S-60'S, and the Northern Pacific.

Kaufman, Yoram↗
NASA NTRS2006

Spatial and Temporal Distribution of Clouds as Observed by MODIS Onboard the Terra and Aqua Satellites

The Moderate Resolution Imaging Spectroradiometer (MODIS) was developed by NASA and launched onboard the Terra spacecraft on December 18,1999 and Aqua spacecraft on May 4, 2002. It achieved its final orbit and began Earth observations on February 24,2000 for Terra and June 24,2002 for Aqua. A comprehensive set of remote sensing algorithms for cloud masking and the retrieval of cloud physical and optical properties has been developed by members of the MODIS atmosphere science team. The archived products from these algorithms have applications in climate change studies, climate modeling, numerical weather prediction, and fundamental atmospheric research. In addition to an extensive cloud mask, products include cloud-top properties (temperature, pressure, effective emissivity), cloud thermodynamic phase, cloud optical and microphysical parameters (optical thickness, effective particle radius, water path), as well as derived statistics. Over the last year, extensive improvements and enhancements in the global cloud products have been implemented, and reprocessing of all MODIS data on Terra has commenced since first light in February 2000. In the cloud mask algorithm, the most extensive improvements were in distinguishing clouds at nighttime, including the challenging polar darkness regions of the world. Additional improvements have been made to properly distinguish sunglint from clouds in the tropical ocean regions, and to improve the identification of clouds from snow during daytime in Polar Regions. We will show global monthly mean cloud fraction for both Terra and Aqua, and show how similar the global daytime cloud fraction is from these morning and afternoon orbits, respectively. We will also show the zonal distribution of cloud fraction over land and ocean regions for both Terra and Aqua, and show the time series of global cloud fraction from July 2002 through June 2006.

King, Michael D.↗
NASA NTRS1998

Ladder-structured photonic variable delay device

An ladder-structured variable delay device for providing variable true time delay to multiple optical beams simultaneously. The device comprises multiple basic units stacked on top of each other resembling a ladder. Each basic unit comprises a polarization sensitive corner reflector formed by two polarization beamsplitters and a polarization rotator array placed parallel to the hypotenuse of the corner reflector. Controlling an array element of the polarization rotator array causes an optical beam passing through the array element to either go up to a basic unit above it or reflect back towards output. The beams going higher on the ladder experience longer optical path delay. Finally, the ladder-structured variable device can be cascaded with another multi-channel delay device to form a new device which combines the advantages of the two individual devices. This programmable optic device has the properties of high packing density, low loss, easy fabrication, and virtually infinite bandwidth. In addition, the delay is reversible so that the same delay device can be used for both antenna transmitting and receiving.

Yao, X. Steve↗
NASA NTRSDate not supplied

Satellite-Assisted Particulate Matter (SAPM) for the Models, In situ, and Remote sensing of Aerosols (MIRA) Working Group

Models, In situ, and Remote sensing of Aerosols (MIRA) is an international working group that aims to foster collaborations amongst these three major aerosol specialties. It consists of a collection of interdisciplinary and independently funded projects/topics with clearly-defined goals. Currently there are four MIRA topic areas, including Satellite-Assisted Particulate Matter (SAPM), which is focused specifically on fine particulate matter (PM2.5). The study of PM2.5 is important due to its significant contribution to air pollution and resultant, adverse human health effects. The goal of the SAPM topic group is to conduct and provide intercomparisons of various methods and techniques to obtain surface PM2.5 estimates assisted by satellite remote sensors, global aerosol models, and in situ aerosol measurements. Some benefits of space-based/model-assisted PM2.5 retrievals include providing PM2.5 approximations in regions with poor in situ ground station coverage and a means for assessing spatial/temporal PM2.5 variations on regional and/or global scales. Furthermore, benefits of spaceborne lidar/model-assisted PM2.5 retrievals include providing nighttime PM2.5 estimates and characterization of near-surface aerosol vertical structure. SAPM is seeking international datasets of mass scattering/absorption coefficient and aerosol hygroscopic properties for different aerosol species, as well as ground-based in situ PM2.5 measurements. In this poster presentation, we give an overview of SAPM, and show results from three recent/ongoing PM2.5 studies. These efforts involve deriving surface PM2.5 concentrations from two spaceborne lidars, the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and Cloud-Aerosol Transport System (CATS), and investigating key variables that impact the estimation of PM2.5 from model simulated aerosol optical depth (AOD) using the Goddard Earth Observing System (GEOS) model.

Travis D. Toth↗
NASA NTRS2003

Scanning Tunneling Optical Resonance Microscopy

Scanning tunneling optical resonance microscopy (STORM) is a method, now undergoing development, for measuring optoelectronic properties of materials and devices on the nanoscale by means of a combination of (1) traditional scanning tunneling microscopy (STM) with (2) tunable laser spectroscopy. In STORM, an STM tip probing a semiconductor is illuminated with modulated light at a wavelength in the visible-to-near-infrared range and the resulting photoenhancement of the tunneling current is measured as a function of the illuminating wavelength. The photoenhancement of tunneling current occurs when the laser photon energy is sufficient to excite charge carriers into the conduction band of the semiconductor. Figure 1 schematically depicts a proposed STORM apparatus. The light for illuminating the semiconductor specimen at the STM would be generated by a ring laser that would be tunable across the wavelength range of interest. The laser beam would be chopped by an achromatic liquid-crystal modulator. A polarization-maintaining optical fiber would couple the light to the tip/sample junction of a commercial STM. An STM can be operated in one of two modes: constant height or constant current. A STORM apparatus would be operated in the constant-current mode, in which the height of the tip relative to the specimen would be varied in order to keep the tunneling current constant. In this mode, a feedback control circuit adjusts the voltage applied to a piezoelectric actuator in the STM that adjusts the height of the STM tip to keep the tunneling current constant. The exponential relationship between the tunneling current and tip-to-sample distance makes it relatively easy to implement this mode of operation. The choice of method by which the photoenhanced portion of the tunneling current would be measured depends on choice of the frequency at which the input illumination would be modulated (chopped). If the frequency of modulation were low enough (typically < 10 Hz) that the feedback circuit could respond, then the voltage applied to the piezoelectric tip-height actuator could be measured by use of a lock-in amplifier locked to the modulation (chopping) signal. However, at a high modulation frequency (typically in the kilohertz range or higher), the feedback circuit would be unable to respond. In this case, the photoenhanced portion of the tunneling current could be measured directly. For this purpose, the tunneling current would be passed through a precise resistor and the voltage drop would be measured by use of the lock-in amplifier.

Bailey, Sheila↗
NASA NTRS2016

Reducing Multisensor Satellite Monthly Mean Aerosol Optical Depth Uncertainty: 1. Objective Assessment of Current AERONET Locations

Various space-based sensors have been designed and corresponding algorithms developed to retrieve aerosol optical depth (AOD), the very basic aerosol optical property, yet considerable disagreement still exists across these different satellite data sets. Surface-based observations aim to provide ground truth for validating satellite data; hence, their deployment locations should preferably contain as much spatial information as possible, i.e., high spatial representativeness. Using a novel Ensemble Kalman Filter (EnKF)- based approach, we objectively evaluate the spatial representativeness of current Aerosol Robotic Network (AERONET) sites. Multisensor monthly mean AOD data sets from Moderate Resolution Imaging Spectroradiometer, Multiangle Imaging Spectroradiometer, Sea-viewing Wide Field-of-view Sensor, Ozone Monitoring Instrument, and Polarization and Anisotropy of Reflectances for Atmospheric Sciences coupled with Observations from a Lidar are combined into a 605-member ensemble, and AERONET data are considered as the observations to be assimilated into this ensemble using the EnKF. The assessment is made by comparing the analysis error variance (that has been constrained by ground-based measurements), with the background error variance (based on satellite data alone). Results show that the total uncertainty is reduced by approximately 27% on average and could reach above 50% over certain places. The uncertainty reduction pattern also has distinct seasonal patterns, corresponding to the spatial distribution of seasonally varying aerosol types, such as dust in the spring for Northern Hemisphere and biomass burning in the fall for Southern Hemisphere. Dust and biomass burning sites have the highest spatial representativeness, rural and oceanic sites can also represent moderate spatial information, whereas the representativeness of urban sites is relatively localized. A spatial score ranging from 1 to 3 is assigned to each AERONET site based on the uncertainty reduction, indicating its representativeness level.

aerosol optical depth↗