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At least 577 records · Page 32

Soil moisture-atmosphere feedbacks mitigate declining water availability in drylands

Global warming alters surface water availability (precipitation minus evapotranspiration, P–E) and hence freshwater resources. However, the influence of land–atmosphere feedbacks on future P–E changes and the underlying mechanisms remain unclear. Here we demonstrate that soil moisture (SM) strongly impacts future P–E changes, especially in drylands, by regulating evapotranspiration and atmospheric moisture inflow. Using modelling and empirical approaches, we find a consistent negative SM feedback on P–E, which may offset ~60% of the decline in dryland P–E otherwise expected in the absence of SM feedbacks. The negative feedback is not caused by atmospheric thermodynamic responses to declining SM; rather, reduced SM, in addition to limiting evapotranspiration, regulates atmospheric circulation and vertical ascent to enhance moisture transport into drylands. This SM effect is a large source of uncertainty in projected dryland P–E changes, underscoring the need to better constrain future SM changes and improve the representation of SM–atmosphere processes in models.

precipitation↗

Response Versus Scan-Angle Assessment of MODIS Reflective Solar Bands in Collection 6.1 Calibration

The Moderate Resolution Imaging Spectroradiometer (MODIS) instruments onboard the Aqua and Terra satellites have been operated for nearly two decades, producing high-quality earth observation data sets suitable for a broad range of scientific studies regarding the earth’s land, ocean, and atmospheric processes. The high radiometric accuracy of MODIS reflective solar band (RSB) calibration has also served as benchmark measurements for on-orbit cross-calibration studies. As the two MODIS instruments have operated well beyond their design lifespan of six years, the measurements from the onboard calibrators alone become inadequate to characterize the sensor’s response at all scan angles, as evinced by long-term drifts observed at certain scan positions of the Aqua-MODIS 0.64- and 0.86-μm bands in Collection 6 (C6) data set. The latest MODIS Level 1B C6.1 data set incorporates earth-view response trending from invariant desert sites as supplemental inputs to characterize the scan-angle calibration dependencies for all RSB. This article presents a deep convective cloud (DCC)-based calibration approach for an independent evaluation of the MODIS RSB response versus scan-angle (RVS) performance in C6.1. The long-term calibration stability and RVS differences in C6.1 have been significantly improved for Aqua-MODIS RSB. The observed RVS differences of more than 2% in Aqua-MODIS C6 bands 1 and 2 have been reduced to within 1% in C6.1. Some RSBs of Terra-MODIS have suffered temporal drifts up to ~2% and calibration shifts up to 3%, particularly around 2016 when the Terra satellite entered into safe mode. The DCC approach has been found very effective in tracking the on-orbit RVS changes over time.

Clouds and the Earth’s Radiant Energy System (CERE↗

Drought Relief and Reversal Over North America from 1500 to 2016

Season-to-season persistence of soil moisture drought varies across North America. Such inter-seasonal autocorrelation can have modest skill in forecasting future conditions several months in advance. Because robust instrumental observations of precipitation span less than 100 years, the temporal stability of the relationship between seasonal moisture anomalies is uncertain. The North American Seasonal Precipitation Atlas (NASPA) is a gridded network of separately reconstructed cool (December-April) and warm (May-July) season precipitation series and offers new insights on the intra-annual changes in drought for up to 2,000 years. Here, the NASPA precipitation reconstructions are rescaled to represent the long-term soil moisture balance during the cool season and three-month long atmospheric moisture during the warm season. These rescaled seasonal reconstructions are then used to quantify the frequency, magnitude, and spatial extent of cool season drought that was relieved or reversed during the following summer months. The adjusted seasonal reconstructions reproduce the general patterns of large-scale drought amelioration and termination in the instrumental record during the 20th century and are used to estimate relief and reversals for the most skillfully reconstructed past 500-years. Sub-continental to continental scale reversals of cool season drought in the following warm season have been rare, but the reconstructions display periods prior to the instrumental data of increased reversal probabilities for the Mid-Atlantic region and the US Southwest. Drought relief at the continental scale may arise in part from macroscale ocean-atmosphere processes, while the smaller scale regional reversals may reflect land-surface feedbacks and stochastic variability.

Drought↗

Relating Lightning Activity to the Convective Evolution of Pre-Genesis Tropical Disturbances

Lightning and environmental characteristics are analyzed for National Hurricane Center (NHC) invest disturbances. For 2019-2021, Atlantic NHC invest tracks are grouped into disturbances that eventually developed into tropical cyclones (TCs) and ones that did not. Data from the NASA/NOAA Geostationary Lightning Mapper (GLM) is used to quantify potential differences in total optical energy, flash extent density, and flash area between the groups. To provide environmental context to the lightning results, vertical profiles from the NOAA Unique Combined Atmospheric Processing System (NUCAPS) dataset will be investigated. Specifically, the profiles will provide insight into the temperature and moisture structure of the invests. In addition to the composite analysis, interesting cases of tropical cyclogenesis will be examined in further detail. Overall, this work seeks to further our understanding of lightning properties and convective environments in tropical cyclogenesis.

Justin W Whitaker↗

The Project “Analogs for VENus’s GEologically Recent Surfaces” (AVENGERS): Unveiling Active Volcanism on Venus

The recently selected missions to Venus opened a new era for the exploration of the Earth’s hellish twin sister. One of the key questions that the selected missions to Venus will address is whether the planet is volcanically active. The identification of ongoing volcanic activity on Venus can indeed unveil important clues on the geologic evolution of the planet, also helping us to better understand how volcanic and atmospheric processes work on Earth, especially those related to the climate change produced by greenhouse gases. To fully contextualize the higher resolution datasets to be provided by the future missions to Venus, we need to be able to exploit the wealth of data to be produced in the best possible way. Different types of instruments will indeed perform unprecedent orbiting and in-situ investigations of the surface and subsurface of Venus. To this regard, the Project “Analogs for VENus’s GEologically Recent Surfaces” (AVENGERS) aims to build a comprehensive database of Terrestrial active volcanoes which may act as suitable analogs for identifying ongoing volcanic activity on Venus. To do this, the project AVENGERS will combine the implementation of terrestrial orbiter radar data analysis techniques (i.e., radar interferometry) with infrared and laboratory analyses of lava flow samples from Terrestrial active volcanoes. As a first suitable analog of the Project AVENGERS, we selected Mount Etna in Sicily for a direct comparison with potentially active volcanic structures of Venus, and with Idunn Mons, one of the most promising possibly active volcanoes of Venus. Given its composite nature, Mount Etna offers the opportunity to identify and study multiple types of eruptive products (both effusive and explosive) from the analysis of high-resolution radar images. The frequent eruptions characterizing this volcano will also allow to test techniques of radar interferometry. Moreover, its ease of access facilitates geologic field trips and in-situ investigations with related sample retrieving. Ongoing infrared laboratory analysis on several altered and unaltered samples retrieved by Mount Etna will help to distinguish spectral signatures of fresh vs weathered volcanic deposits.

P. D’Incecco↗

A Nowcasting Approach for Low Earth Orbit Hyperspectral Infrared Soundings Within the Convective Environment

Low Earth orbit (LEO) hyper-spectral infrared (IR) sounders have significant yet untapped potential for characterizing thermodynamic environments of convective initiation and ongoing convection. While LEO soundings are of value to weather forecasters, the temporal resolution needed to resolve the rapidly evolving thermodynamics of the convective environment is limited. We have developed a novel nowcasting methodology to extend snapshots of LEO soundings forward in time up to six hours to create a product available within National Weather Service systems for user assessment. Our methodology is based on parcel forward-trajectory calculations from the satellite observing time to generate future soundings of temperature (T) and specific humidity (q) at regularly gridded intervals in space and time. The soundings are based on NOAA-Unique Combined Atmospheric Processing System (NUCAPS) retrievals from the Suomi NPP and NOAA-20 satellite platforms. The tendencies of derived convective available potential energy (CAPE) and convective inhibition (CIN) are evaluated against gridded, hourly accumulated rainfall obtained from the Multi-Radar Multi-Sensor (MRMS) observations for 24 hand-selected cases over the Contiguous United States. Areas with forecast increases in CAPE (reduced CIN) are shown to be associated with areas of precipitation. The increases in CAPE and decreases in CIN are largest for areas that have the heaviest precipitation and are statistically significant compared to areas without precipitation. These results imply that adiabatic parcel advection of LEO satellite sounding snapshots forward in time are capable of identifying convective initiation over an expanded temporal scale compared to soundings used only during the LEO satellite overpass time.

North America↗

Pyroscopegridding: Geo-Leo Aerosol Data Fusion (an Open-Source Package)

The retrieval of aerosol optical depths (AODs) from sun-synchronous polar orbiting satellites, such as MODISs, VIIRSs, OMI, TROPOMI, etc., has been widely adopted as a method for obtaining information regarding particulate matter (PM) and related atmospheric processes. However, the advent of recently launched geostationary satellites, such as GOES-16/17/18, Himawari-8/9, and Meteosat Third Generation (MTG), has led to an increased temporal resolution of AOD observations (order of 10 minutes), resulting in typically one or more images per hour during daylight hours, compared to the once-per-day observations obtained from LEO satellites. By integrating these observations, the diurnal cycle of global AOD can be characterized at local, regional, and global scales. The scientific community is still examining the novel data from geostationary satellite observations and evaluating methods for effectively merging these observations with differing spatial and temporal resolutions. This presents a significant ""Big Data"" challenge, encompassing not only data storage, but also data discoverability, accessibility, and migration within cloud computing environments. This study presents our attempts at fusing Level 2 aerosol data from six satellites, three of which are geostationary (GOES-16/17 and Himawari-8) and three of which are polar orbiting (TERRA/MODIS, AQUA/MODIS, and SNPP-VIIRS), using the Dark Target aerosol retrieval algorithm. The ability to fuse remote sensing products on demand into desired temporal and spatial domains empowers researchers and practitioners to more efficiently work with satellite and sensor data. It is our hope that through making our open-source package and accompanying functionality available, the scientific community will have improved access to aerosol data processing resources.

Jennifer Wei↗

Improving Simulation of Irrigation in a Global Land Surface Model

Studies have shown that irrigated agriculture has substantial effects on local to regional hydrologic and atmospheric processes. These effects include increased evapotranspiration and near surface humidity, decreased air and ground temperature, augmented downwind precipitation, enhanced recharge, depletion of source water stocks, and overall changes to the regional water budget. However, developers of global offline and coupled modeling systems have been slow to incorporate irrigation. This presentation will describe progress towards simulating irrigation worldwide in the Land Information System (LIS) and Global Land Data Assimilation System (GLDAS). We have developed and refined the ability to simulate sprinkler irrigation, furrow irrigation, paddy irrigation, and drip irrigation. We have reconciled multiple global and national irrigation, land cover, and crop type databases in an effort to (1) distinguish irrigated and rainfed agriculture, (2) simulate the proper distribution of crops (as sub-grid tiles) in each model grid pixel, and (3) apply the most likely irrigation method in each tile based on the crop type and country or state level information on the relative usage of sprinkler, flood, and drip irrigation. Using agricultural water withdrawal data, as available, for calibration and evaluation, we show that the implemented approach is promising but that much fine tuning remains to be done. In particular, irrigation model parameters that produce good results in one location often produce less satisfying results in others.

Matthew Rodell↗

CALIGOLA: A New Multidisciplinary Spaceborne Lidar Mission (Cloud Aerosol Lidar for Global scale Observations of the ocean-Land-Atmosphere system)

Spaceborne lidars provide unique and valuable insight into the vertical structure of clouds and aerosols over the globe as well as insight into their microphysical and optical properties. Over the past two decades, lidar observations from CALIPSO, ICESAT-2 and CATS fundamentally advanced our understanding of the roles of clouds and aerosols play in weather, climate and air quality. The measurement records further served as important references for validating and improving retrieval algorithms of cloud/aerosol properties from operational weather satellites. A more recent development is the emerging awareness on how spaceborne lidar profile observations can also enhance knowledge of Earth’s coupled atmosphere-ocean-land system. Here we report on a new and powerful spaceborne lidar mission concept known as CALIGOLA (Cloud Aerosol Lidar for Global Scale Observations of the Ocean-Land Atmosphere System). The mission is multidisciplinary and will provide new insights into atmospheric processes with advance measurement capabilities beyond CALIPSO and the recently launched EarthCARE mission. CALIGOLA will further provide the first profiling of the world’s oceans to reveal unprecedented observations on the health and productivity of marine biology (phytoplankton and zooplankton) as well as provide unique observations of surface vegetation, ice, and snow. The mission will feature an innovative three-wavelength lidar, that will simultaneously acquire elastic backscatter, Raman, and fluorescence measurements, with polarization sensitivity on the elastic channels. The instrument is further designed with greater sensitivity than CALIOP and with vertical resolution on the order of a few meters near the surface. The mission is planned for launch early next decade and is baselined to fly in a polar orbit that is compatible with the previous A-Train constellation to extend the long-term measurement record. CALIGOLA is being developed through a partnership between Agenzia Spaziale Italiana (ASI) and National Aeronautics and Space Administration (NASA).

Lidar Aerosols Clouds Ocean Biology↗

Improved Air Quality Forecasts using NASA’s Pandora and GEOS CF at International and Domestic Sites for SNWG Stakeholders

Air pollution prediction is complex due to the dynamic nature of atmospheric processes and the variability in data resolutions and availability. This project addresses these challenges by integrating and analyzing high-resolution ground-based measurements with global air quality models. Through this integration, we have gained a deeper understanding of how these processes interact under various conditions, which we then use to model and enhance the accuracy of forecasts.

Noussair Lazrak↗

Initiation of the Madden-Julian Oscillation

Many storms around the world have roots in the Indian Ocean, where they are churned up by the atmospheric process called the Madden-Julian Oscillation (MJO). PNNL is working to unlock the secrets of the MJO, particularly how it initiates in the Indian Ocean every 30-60 days. Better prediction of the MJO will help resource managers, weather forecasters and people worldwide better prepare for its effects.

54 ENVIRONMENTAL SCIENCES↗

ARM Radiosondes for National Polar-Orbiting Operational Environmental Satellite System Preparatory Project Validation Field Campaign Report

This IOP has been a coordinated effort involving the U.S. Department of Energy (DOE) Atmospheric Radiation (ARM) Climate Research Facility, the University of Wisconsin (UW)-Madison, and the JPSS project to validate SNPP NOAA Unique Combined Atmospheric Processing System (NUCAPS) temperature and moisture sounding products from the Cross-track Infrared Sounder (CrIS) and the Advanced Technology Microwave Sounder (ATMS). In this arrangement, funding for radiosondes was provided by the JPSS project to ARM. These radiosondes were launched coincident with the SNPP satellite overpasses (OP) at four of the ARM field sites beginning in July 2012 and running through September 2017. Combined with other ARM data, an assessment of the radiosonde data quality was performed and post-processing corrections applied producing an ARM site Best Estimate (BE) product. The SNPP targeted radiosondes were integrated into the NOAA Products Validation System (NPROVS+) system, which collocated the radiosondes with satellite products (NOAA, National Aeronautics and Space Administration [NASA], European Organisation for the Exploitation of Meteorological Satellites [EUMETSAT], Geostationary Operational Environmental Satellite [GOES], Constellation Observing System for Meteorology, Ionosphere, and Climate [COSMIC]) and Numerical Weather Prediction (NWP forecasts for use in product assessment and algorithm development. This work was a fundamental, integral, and cost-effective part of the SNPP validation effort and provided critical accuracy assessments of the SNPP temperature and water vapor soundings.

54 ENVIRONMENTAL SCIENCES↗

Atmospheric Radiation Measurement Climate Research Facility Operations Quarterly Report July 1-September 30, 2015

For this reporting period the TARGET uptimes for the fixed ARM research sites were: North Slope of Alaska (NSA) locale is 1988 hours (0.90 x ACTUAL) Southern Great Plains (SGP) locale is 2098 hours (0.95 x ACTUAL) Eastern North Atlantic (ENA) locale is 1877 hours (0.85 x ACTUAL). Beginning in FY2014, and continuing through the next two fiscal years, the ARM Facility is being reconfigured to focus on the improvement of high-resolution atmospheric process models. This strategy includes the formation of two megasites: the first will be located at the SGP for continental U.S. process measurements; the second is at NSA for arctic process measurements. Supporting this reconfiguration, the tropical facilities have been shut down and their systems and components are being redeployed to the continental U.S. megasite. Most of the equipment from the tropical sites is now in the SGP site inventory to support the reconfiguration

Southern Great Plains, Eastern North Atlantic, Nor↗

Oxygen Isotope Fractionation in U 3 O 8 during Thermal Processing in Humid Atmospheres

The incorporation of oxygen isotopes from water into uranium oxides during industrial processing presents a pathway for determining a material’s geographical origin. This study is founded on the hypothesis that oxygen isotopes from atmospheric water vapor will exchange with isotopes of oxygen in solid uranium oxides during thermal processing or calcination. Using a commonly encountered oxide, U 3 O 8 , the exchange kinetics and equilibrium fractionation with water vapor (in a concentration range of 50–55% relative humidity) were investigated using processing temperatures of 400, 600, and 800 °C. In an atmosphere containing only water vapor diluted in N 2 , oxygen isotope equilibration in U 3 O 8 occurred within 12 h at 400 °C and within 2 h at 600 and 800 °C. Fractionation factors (1000lnα, U 3 O 8 –H 2 O) between the water and oxide were –12.1, –11.0, and –8.0 at 400, 600, and 800 °C, respectively. With both humidity and O 2 present in the calcining atmosphere, isotopic equilibration is attained within 2 h at and above 400 °C. In this mixed atmosphere, which was designed to emulate Earth’s troposphere, isotopes are incorporated preferentially from water vapor at 400 °C and from O 2 at 600 and 800 °C. Rapid and temperature/species-dependent isotope exchange also elucidated the impact of retrograde exchange in humid air, showing a shift from O 2 -dependent to H 2 O-dependent fractionation as U 3 O 8 cooled from 800 °C. These results confirm that uranium oxides inherit oxygen isotopes from humidity during thermal processing, illuminating an important mechanism in the formation of this forensic signature.

07 ISOTOPE AND RADIATION SOURCES↗

Laboratory Studies of Processing of Carbonaceous Aerosols by Atmospheric Oxidants/Hygroscopicity and CCN Activity of Secondary & Processed Primary Organic Aerosols

The atmosphere is composed of a complex mixture of gases and suspended microscopic aerosol particles. The ability of these particles to take up water (hygroscopicity) and to act as nuclei for cloud droplet formation significantly impacts aerosol light scattering and absorption, and cloud formation, thereby influencing air quality, visibility, and climate in important ways. A substantial, yet poorly characterized component of the atmospheric aerosol is organic matter. Its major sources are direct emissions from combustion processes, which are referred to as primary organic aerosol (POA), or in situ processes in which volatile organic compounds (VOCs) are oxidized in the atmosphere to low volatility reaction products that subsequent condense to form particles that are referred to as secondary organic aerosol (SOA). POA and VOCs are emitted to the atmosphere from both anthropogenic and natural (biogenic) sources. The overall goal of this experimental research project was to conduct laboratory studies under simulated atmospheric conditions to investigate the effects of the chemical composition of organic aerosol particles on their hygroscopicity and cloud condensation nucleation (CCN) activity, in order to develop quantitative relationships that could be used to more accurately incorporate aerosol-cloud interactions into regional and global atmospheric models. More specifically, the project aimed to determine the products, mechanisms, and rates of chemical reactions involved in the processing of organic aerosol particles by atmospheric oxidants and to investigate the relationships between the chemical composition of organic particles (as represented by molecule sizes and the specific functional groups that are present) and the hygroscopicity and CCN activity of oxidized POA and SOA formed from the oxidation of the major classes of anthropogenic and biogenic VOCs that are emitted to the atmosphere, as well as model hydrocarbons. The general approach for this project was to carry out reactions of representative anthropogenic and biogenic VOCs and organic particles with ozone (O 3 ), and hydroxyl (OH), nitrate (NO 3 ), and chlorine (Cl) radicals, which are the major atmospheric oxidants, under simulated atmospheric conditions in large-volume environmental chambers. A combination of on-line and off-line analytical techniques were used to monitor the chemical and physical properties of the particles including their hygroscopicity and CCN activity. The results of the studies were used to (1) improve scientific understanding of the relationships between the chemical composition of organic particles and their hygroscopicity and CCN activity, (2) develop an improved molecular level theoretical framework for describing these relationships, and (3) establish a large database that is being used to develop parameterizations relating organic aerosol chemical properties and SOA sources to particle hygroscopicity and CCN activity for use in regional and global atmospheric air quality and climate models.

54 ENVIRONMENTAL SCIENCES↗

Broadband Outdoor Radiometer Calibration (BORCAL) Process for the Atmospheric Radiation Measurement (ARM) Program: Second Edition

The Atmospheric Radiation Measurement program (ARM) maintains a fleet of monitoring stations to aid in the improved scientific understanding of the basic physics related to radiative feedback processes in the atmosphere, particularly the interactions among clouds and aerosols. ARM obtains continuous measurements and conducts field campaigns to provide data products that aid in the improvement and further development of climate models. All of the measurement campaigns include a suite of solar measurements. The Solar Radiation Research Laboratory at the National Renewable Energy Laboratory supports ARM's full suite of stations in a number of ways, including troubleshooting issues that arise as part of the data-quality reviews; managing engineering changes to the standard setup; and providing calibration services and assistance to the full fleet of solar-related instruments, including pyranometers, pyrgeometers, pyrheliometers, as well as the temperature/relative humidity probes, multimeters, and data acquisition systems that are used in the calibrations performed at the Southern Great Plains Radiometer Calibration Facility. This paper discusses all aspects related to the support provided to the calibration of the instruments in the solar monitoring fleet.

14 SOLAR ENERGY↗

Oxidation of the Martian surface - Constraints due to chemical processes in the atmosphere

Dissociation of water in the Martian atmosphere may supply oxygen to the surface and may result in the formation of minerals such as goethite, as proposed by Huguenin. The supply rate is limited by chemical processes in the atmosphere which regulate the abundance of O2. The net surface sink for atmospheric oxygen can be as large as 33 million atoms per sq cm per sec which compares to the escape rate of 60 million atoms per sq cm per sec.

Mcelroy, M. B.↗

The Long-Term Evolution of the Atmosphere of Venus: Processes and Feedback Mechanisms

This work reviews the long-term evolution of the atmosphere of Venus, and modulation of its composition by interior/exterior cycling. The formation and evolution of Venus’s atmosphere, leading to contemporary surface conditions, remain hotly debated topics, and involve questions that tie into many disciplines. We explore these various inter-related mechanisms which shaped the evolution of the atmosphere, starting with the volatile sources and sinks. Going from the deep interior to the top of the atmosphere, we describe volcanic out-gassing, surface-atmosphere interactions, and atmosphere escape. Furthermore, we address more complex aspects of the history of Venus, including the role of Late Accretion impacts, how magnetic field generation is tied into long-term evolution, and the implications of geochemical and geodynamical feedback cycles for atmospheric evolution. We highlight plausible end-member evolutionary pathways that Venus could have followed, from accretion to its present-day state, based on modeling and observations. In a first scenario, the planet was desiccated by atmospheric escape during the magma ocean phase. In a second scenario, Venus could have harbored surface liquid water for long periods of time, until its temperate climate was destabilized and it entered a runaway greenhouse phase. In a third scenario, Venus’s inefficient outgassing could have kept water inside the planet, where hy- drogen was trapped in the core and the mantle was oxidized. We discuss existing evidence and future observations/missions required to refine our understanding of the planet’s history and of the complex feedback cycles between the interior, surface, and atmosphere that have been operating in the past, present or future of Venus.

Venus↗