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DOE OSTI2020

Little influence of Arctic amplification on mid-latitude climate

Observations and model simulations show enhanced warming in the Arctic under increasing greenhouse gases, a phenomenon known as the Arctic amplification (AA), that is likely caused by sea-ice loss. AA reduces meridional temperature gradients linked to circulation, thus mid-latitude weather and climate changes have been attributed to AA, often on the basis of regression analysis and atmospheric simulations. However, other modelling studies show only a weak link. This inconsistency may result from deficiencies in separating the effects of AA from those of natural variability or background warming. In this work, using coupled model simulations with and without AA, we show that cold-season precipitation, snowfall and circulation changes over northern mid-latitudes come mostly from background warming. AA and sea-ice loss increase precipitation and snowfall above ~60° N and reduce meridional temperature gradients above ~45° N in the lower–mid troposphere. However, minimal impact on the mean climate is seen below ~60° N, with weak reduction in zonal wind over 50°–70° N and 150–700 hPa, mainly over the North Atlantic and northern central Asia. These results suggest that the climatic impacts of AA are probably small outside the high latitudes, thus caution is needed in attributing mid-latitude changes to AA and sea-ice loss on the basis of statistical analyses that cannot distinguish the impact of AA from other correlated changes.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2015

Reaction studies of neutral atomic C with H{sub 3}{sup +} using a merged-beams apparatus

We have investigated the chemistry of C+H{sub 3}{sup +} forming CH{sup +}, CH{sub 2}{sup +}, and CH{sub 3}{sup +}. These reactions are believed to be some of the key gas-phase astrochemical processes initiating the formation of organic molecules in molecular clouds. For this work, we have constructed a novel merged fast-beams apparatus which overlaps a beam of molecular ions onto a beam of ground-term neutral atoms. Here, we describe the apparatus in detail and present cross section data for forming CH{sup +} and CH{sub 2}{sup +} at relative energies from ≈9 meV to ≈20 and 3 eV, respectively. Measurements were performed for statistically populated C ({sup 3}P{sub J}) in the ground term reacting with hot H{sub 3}{sup +} (at an internal temperature of ∼2550 K). Using these data, we have derived rate coefficients for translational temperatures from ≈72 K to ∼2.3×10{sup 5} and 3.4×10{sup 4} K, respectively. For the formation of CH{sub 3}{sup +}, we are only able to place an upper limit on the rate coefficient. Our results for CH{sup +} and CH{sub 2}{sup +} are in good agreement with the mass-scaled results from a previous ion trap study of C + D{sub 3}{sup +}, at a translational temperature of ∼1000 K. That work also used statistically populated C ({sup 3}P{sub J}) but internally cold D{sub 3}{sup +} (∼77 K). The good agreement between the two experiments implies that the internal excitation of the H{sub 3}{sup +} is not significant so long as the reaction proceeds adiabatically. At 300 K, the C fine-structure levels are predicted to be essentially statistically populated, enabling us to compare our translational temperature results to thermal equilibrium calculations. At this temperature, our rate coefficient for forming CH{sup +} lies a factor of ≈2.9 below the Langevin rate coefficient currently given in astrochemical databases, and a factor of ∼1.8−3.3 below the published classical trajectory studies using quantum mechanical potential energy surfaces. Our results for CH{sub 2}{sup +} formation at 300 K are a factor of ≈26.7 above these semi-classical results. Astrochemical databases do not currently include this channel. We also present a method for converting our translational temperature results to thermal rate coefficients for temperatures below ∼300 K. The results indicated that CH{sub 2}{sup +} formation dominates over that of CH{sup +} at temperatures ≲50 K.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2016

Effects of chemistry and microstructure on corrosion performance of Zircaloy-2-based BWR cladding - 2016-0066

In boiling water reactors (BWRs), Zircaloy-2 is typically the material of choice for fuel cladding. With increased focus on fuel performance and reliability, consistent cladding corrosion performance under varying BWR conditions has become an acknowledged requirement for modern BWR fuel. To support optimization of corrosion performance, modifications to alloy chemistry and manufacture conditions can be made, supported by ex-reactor corrosion testing and demonstrated through in-reactor operation. In this work, the combined effects of alloy chemistry and fabrication process were investigated. The effect of alloy chemistry is often complicated by variation within a production ingot. In this work, additional measurements were intentionally taken at the tube-shell stage (before cold pilgering) so that chemistry more representative of the final cladding could be obtained and the effect of iron, nickel, and tin could be examined more closely. Although chemistry range of Zircaloy-2 was the primary focus, the effect of iron above the ASTM limit in a new alloy was also explored. Three types of cladding fabrication processes were considered. Two types included a heat treatment applied after the first cold pilgering and annealing, and the treatment was limited to the outer portion of the cladding and differed in the temperature of the heat treatment; the third type had no special heat treatments after the first cold pilgering and annealing. The weight gain of the three types of cladding with varying compositions under two corrosion test conditions (400 deg. C steam and 410/520 deg. C two-stage steam) are discussed in terms of the initial second-phase particle sizes obtained from transmission electron microscopy examinations. Based on poolside inspections and hot-cell examinations, the in-reactor corrosion performance of the two cladding types up to typical discharge exposures are discussed in the terms of corrosion margin, microstructure evolution, and correlation with ex-reactor corrosion test data. (authors)

36 MATERIALS SCIENCE↗

DOE OSTI2023

Field Testing of Self-Healing Metallic Coatings for Internal Corrosion Protection of Natural Gas Pipelines

Internal corrosion occurs in natural gas pipelines primarily due to the presence of water, carbon dioxide, and hydrogen sulfide. Internal corrosion can eventually result in leakage, cracks, and rupture of the pipeline. The objective of this work is to mitigate internal corrosion in steel pipelines transporting natural gas using cold spray coatings. The corrosion behavior of carbon steel coated with self-healing zinc chromium (ZnCr) and zinc niobium (ZnNb) cold spray coatings was investigated in a natural gas environment. For comparison purposes, hot-dip galvanized steel (HDGS) was tested under the same conditions as cold spray coatings. The field test was performed at the NW Natural gas storage facility in Mist, Oregon. The field test was conducted in a 6-inch diameter pipe transporting wet natural gas out of an underground storage well at 500 psi and 4.4 °C. The coupons were tested for 15 and 32 days under stagnant and flow conditions, respectively. Weight loss method was used to measure the corrosion rate of metallic coatings. Post-corrosion surface characterization was performed on the specimen using a scanning electron microscopy (SEM) equipped with energy dispersive X-ray spectroscopy (EDS). Crystalline phases were determined by X-ray diffraction (XRD). The field-test results confirmed that the metallic coatings provided corrosion protection of carbon steel exposed to wet natural gas under stagnant and flow conditions. The formation of the ZnCO 3 layer on top of ZnNb and ZnCr coatings led to passivation of the coatings which helps to reduce the self-corrosion. These layers form a barrier for diffusion of corrosive species to the surface.

03 NATURAL GAS↗

DOE OSTI2023

Tracking Aerosol Convection Interactions Experiment (TRACER) Field Campaign Report

Convective clouds serve a critical role in the Earth’s energy and water cycles through their transport of heat, moisture, momentum, and chemical species through the troposphere driving the global circulation (e.g., Hartmann et al. 1984, Del Genio et al. 2012, Su et al. 2014). On more local scales, convective clouds impact the atmospheric heating profile through diabatic heating effects, removal of water from the atmospheric column through precipitation, and conditioning of the local environment impacting further development of clouds (e.g., Sullivan and Voigt 2021). These critical roles underscore the importance of realistic representation of convective processes across scales of models from large-eddy simulation (LES), to convection-permitting models (CPM; e.g., Kendon et al. 2020, Marinescu et al. 2021), to numerical weather prediction (NWP) models used for operational weather forecasting, to Earth system models used to predict climate sensitivity (Sanderson et al. 2011, Sherwood et al. 2014, Tomassini et al. 2014, Zhao et al. 2016, Cronin et al. 2017). A key component of improving model representation of convective clouds is better quantification and parameterization of updraft microphysics and dynamics, including their interactions with the surrounding environment and storm organization (Bony et al. 2015, Hagos and Houze 2016, Donner et al. 2016, Morrison et al. 2020). Aerosol is an important environmental factor that could affect convective clouds and precipitation since cloud droplet and ice formation processes are initiated by it. Andrae et al. (2004) hypothesized that aerosols associated with increased biomass burning particles acting as cloud condensation nuclei (CCN) result in smaller and more monodisperse cloud droplets leading to suppression of warm rain formation, ultimately leading to more cloud water being lofted above the freezing level based on observations in the Amazon region. The subsequent increase in latent heat release increases the buoyancy of rising convective parcels invigorating the deep convection. This work was followed by a description of the theoretical basis for this “cold-phase invigoration” by Rosenfeld et al. (2008), who argued that it could have a significant effect for deep convective clouds with warm cloud-bases. Several modeling studies (e.g., Khain et al. 2005, 2009, van den Heever et al. 2006, Fan et al. 2007, 2009, 2012, Lee et al. 2008, Storer et al. 2010, Lebo et al. 2012, Storer and van den Heever 2013, Chen et al. 2020, Dagan et al. 2022) have investigated these aerosol-convection interactions and the environmental factors that influence their relative importance and magnitude. More recently, several studies have indicated that “warm-phase invigoration”, the enhancement of convection through condensational heating, also appears to play a role in enhancing both shallow cumuli (Seiki and Nakajima 2014, Saleeby et al 2015) and deeper tropical convection (Lebo and Seinfeld 2011, Khain et al. 2012, Sheffield et al 2015, Fan et al. 2018, Igel and van den Heever 2021), as well as Houston thunderstorms (Fan et al. 2007, 2020). However, still other studies have provided additional evidence of systematic biases in simulated convective outflow ice size distribution properties, which are consistent with a lack of poorly understood secondary ice production within convective updrafts (e.g., Fridlind et al. 2017). To help address these critical gaps in our understanding of cloud processes, aerosol processes and aerosol-cloud interactions, the Tracking Aerosol Convection Interactions Experiment was designed building upon efforts by the Aerosol, Cloud, Precipitation and Climate (ACPC) Initiative (http://acpcintiative.org/), a joint effort of the International Geosphere-Biosphere Programme (IGBP) and the World Climate Research Program (WCRP) that focused on resolving uncertainties in the interactions between aerosol and clouds towards better understanding the role that these interactions play in the climate system. The TRACER campaign was motivated by recommendations from a number of pilot studies undertaken by ACPC (van den Heever et al. 2017, Fridlind et al. 2019, Hu et al. 2019, Fan et al. 2020, Marinescu et al. 2021, Hernandez-Deckers et al. 2022) that pointed towards the southeastern Texas region as a locale where aerosol-convection interactions could be studied owing to the copious occurrence of isolated convection during the summer months accompanied by diverse and significant sources of aerosols from both anthropogenic and natural sources. The TRACER campaign began on 01 October 2021 and extended through 30 September 2022 with an intensive operational period (IOP) during June-September 2022. Three main sites (Table 1) were managed by the U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1994

Building on the foundation for an engineering career

A predictable and preventable hurdle stops a majority of young women from entering the scientific and technical fields. This cuts down the individual's career possibilities and cuts in half the pool of potential U.S. engineers later available to industry. The waste of talent does not advance our country's competitive position. The typical American adolescent girl has acquired all the basic mathematical skills needed to pursue science and math, but, from adolescence on, she does not build the foundation of science and math courses that she would need later in life to work in engineering. Several questions are addressed: Why are some young women stopped cold in their mathematical tracks during adolescence? What is the influence of psychology, including discussion of the personality traits quantifiably shared by women in technical fields? and How should the school system adapt to keep their female charges learning math and science?

White, Susan↗

NASA NTRS2000

Failure Engineering Study and Accelerated Stress Test Results for the Mars Global Surveyor Spacecraft's Power Shunt Assemblies

An Engineering-of-Failure approach to designing and executing an accelerated product qualification test was performed to support a risk assessment of a "work-around" necessitated by an on-orbit failure of another piece of hardware on the Mars Global Surveyor spacecraft. The proposed work-around involved exceeding the previous qualification experience both in terms of extreme cold exposure level and in terms of demonstrated low cycle fatigue life for the power shunt assemblies. An analysis was performed to identify potential failure sites, modes and associated failure mechanisms consistent with the new use conditions. A test was then designed and executed which accelerated the failure mechanisms identified by analysis. Verification of the resulting failure mechanism concluded the effort.

Gibbel, Mark↗

NASA NTRS2004

Analysis of Electrical Characteristics of Thin Film Photovoltaic Cells

Solar energy is the most abundant form of energy in many terrestrial and extraterrestrial environments. Often in extraterrestrial environments sunlight is the only readily available form of energy. Thus the ability to efficiently harness solar energy is one of the ultimate goals in the design of space power systems. The essential component that converts solar energy into electrical energy in a solar energy based power system is the photovoltaic cell. Traditionally, photovoltaic cells are based on a single crystal silicon absorber. While silicon is a well understood technology and yields high efficiency, there are inherent disadvantages to using single crystal materials. The requirements of weight, large planar surfaces, and high manufacturing costs make large silicon cells prohibitively expensive for use in certain applications. Because of silicon s disadvantages, there is considerable ongoing research into alternative photovoltaic technologies. In particular, thin film photovoltaic technologies exhibit a promising future in space power systems. While they are less mature than silicon, the better radiation hardness, reduced weight, ease of manufacturing, low material cost, and the ability to use virtually any exposed surface as a substrate makes thin film technologies very attractive for space applications. The research group lead by Dr. Hepp has spent several years researching copper indium disulfide as an absorber material for use in thin film photovoltaic cells. While the group has succeeded in developing a single source precursor for CuInS2 as well as a unique method of aerosol assisted chemical vapor deposition, the resulting cells have not achieved adequate efficiencies. While efficiencies of 11 % have been demonstrated with CuInS2 based cells, the cells produced by this group have shown efficiencies of approximately 1 %. Thus, current research efforts are turning towards the analysis of the individual layers of these cells, as well as the junctions between them, to determine the cause of the poor yields. As a student of electrical engineering with some material science background, my role in this research is to develop techniques for analyzing the electrical characteristics of the CuInS2 cells. My first task was to design a shadow mask to be used to place molybdenum contacts under a layer of CuInS;! in order to analyze the contact resistance between the materials. In addition, I have also analyzed evaporated aluminum top contacts and have tested various methods of increasing their thicknesses in order to decrease series resistance. More recently I have worked with other members of the research group in reviving a vertical cold-wall reactor for experimentation with CuInS2 quantum dots. As part of that project, I have improved the design for a variable frequency and pulse width square wave generator to be used in driving the precursor injection process. My task throughout the remainder of my tenure is to continue to analyze and develop tools for the analysis of electrical properties of the CuInS2 cells with the ultimate goal of discovering ways to improve the efficiency of our photovoltaic cells. Traditionally, photovoltaic cells are based on a single crystal silicon absorber. While The research group lead by Dr. Hepp has spent several years researching copper indium

Kasick, Michael P.↗

DOE OSTI2025

Closeout Report of BNL LDRD 23-050 A Second EIC Detector: Physics Case and Conceptual Design

This document is the closeout report for LDRD 23-050, a type-A LDRD project awarded in FY2022 under the title “ A Second EIC Detector: Physics Case and Conceptual Design ”. The project was motivated by the strong interest within the EIC community in a second general-purpose detector and interaction region, and by the recognition that such a detector is essential to fully exploit the scientific potential of the EIC over its multi-decade lifetime. The key goals of the LDRD were to (i) strengthen the case for a second EIC detector, building on the arguments already articulated in the community Yellow Report, (ii) provide a realistic detector concept that is complementary to the current project detector, ePIC, in terms of physics reach, precision, and control of systematics, and (iii) broaden the overall physics program of the EIC facility. Since a possible second detector is expected to be realized with a delay of several years relative to the first detector, the project explicitly aimed at identifying technologies that are not yet sufficiently mature for ePIC but could be deployed on the later timescale of a second detector, thereby providing genuine complementarity and room for innovation. LDRD 23-050 provided support for two postdoctoral researchers and partial support for several BNL staff members, and the effort ramped up in mid-2023. Work was carried out in close collaboration with colleagues from the EIC project, the Cold QCD and STAR groups at BNL, and with substantial input from members of the EIC User Group and the ePIC Collaboration as reflected in the author list. Over the period from October 2022 through September 2025, this team developed and refined a physics program tailored to a second detector, translated the resulting physics requirements into detector-level performance targets, and explored multiple conceptual detector layouts capable of meeting these targets within the constraints of the second interaction region. The expected outcome, as stated in the original proposal, was a document detailing the physics potential and requirements of a second EIC detector, accompanied by a comprehensive conceptual detector design and an outline of the remaining R&D needed to bring the relevant technologies to maturity. The present report summarizes the progress that has been achieved toward these goals. It consolidates the physics studies, detector concepts, and technology assessments developed under this LDRD and places them in the broader context of worldwide detector R&D. While the evolving priorities of the EIC project and the substantial community effort required to design and construct ePIC naturally limited the scope of EIC-wide activities toward a second detector during this period, the work documented here is intended to provide a foundation and a point of reference for future efforts. Whatever form a second EIC detector may ultimately take, we hope that this report will serve as a useful guide for colleagues who continue to advance this program in the near- and mid-term future.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2018

Small Fatigue Crack Growth Mechanisms and Interfacial Stability in Cold-Spray 6061 Aluminum Alloys and Coatings

Cold-spray-processed aluminum alloys have static mechanical properties superior to those of aerospace cast alloys, and similar to those of their wrought counterparts, making them good candidates for structural applications. However, their broad and confident use relies upon systematic fatigue crack growth studies to investigate and demonstrate the materials' performance in critical high-integrity components. In this work, the fatigue crack growth behavior in early stages (small crack growth regime) was investigated for cold-spray processed 6061 aluminum alloys and coatings, at stress ratio R = 0.1, in room temperature laboratory air. The effects of the characteristic microstructure and initial flaw size on the fatigue crack growth response were systematically examined, and the crack growth mechanisms at the microstructural scale were established and compared to those of long cracks. The mechanical interfacial stability of coatings was examined in cold-spray 6061-rolled 6061-T6 couples. An original method of quantifying the deposition-substrate interfacial strength, and correlating it to the response under cyclic loading via crack-interface stability maps, was developed. The proposed methodology is based on combined scratch testing and fracture mechanics formulations, and failure at the coating-substrate interface can be predicted for any crack growth scenario under cyclic loading. The method can be broadly used for the design and optimization of cold-spray and other coatings, as well as in structural repair.

36 MATERIALS SCIENCE↗

DOE OSTI2011

Electrical time resolved metrology of dust particles growing in low pressure cold plasmas

The electrical parameters of a capacitively coupled radiofrequency (CCRF) discharge change significantly when dust arises in the discharge. This work demonstrates the ability to follow in real time the evolution of the size and of the concentration of dust particles forming in a CCRF discharge from the variation of the electron density and of the self-bias voltage of the active electrode. According to experimental findings, it appears that the variation of this self-bias voltage depends on the surface of the dust particles. This trend is confirmed by an analytical modelling considering the low frequency behaviour of the phenomenon.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

Multimodal 3D quantification of particle stimulated nucleation in industrially manufactured aluminium AA5182 sheet

Particle stimulated nucleation is a dominant recrystallisation mechanism observed in many industrially relevant aluminium alloys during thermomechanical processing. Here, in this work, we quantify particle stimulated nucleation in 3D in an aluminium AA5182 alloy sheet cold-rolled to 75% thickness reduction. Second phase particles and nuclei are mapped in the same sample volume by conventional laboratory absorption X-ray tomography and synchrotron X-ray Laue micro-diffraction. The large second phase particles are classified as Fe- and Mg-rich phases. It is found that 84% of the nuclei are particle stimulated and 40% of the particles stimulate nucleation. The critical particle diameter is found to be 4 μm. Deviatoric elastic strains are derived from micro-diffraction data and it is found that elastic strains are present in the recrystallised nuclei. The effects of the different particle types, particle clustering, particle size and aspect ratio as well as strain inheritance are discussed. This work provides a full 3D quantification of particle stimulated nucleation behaviour in AA5182 alloy sheet deformed to high strain.

Deviatoric strain↗

DOE OSTI2019

Novel Radiometry for In-Pipe Robotic Inspection of Holdup Deposits in Gaseous Diffusion Piping - 19503

This paper details the first complete, DOE approved, deployed and operational radiometry for robotic nondestructive assay (NDA) of holdup deposits in gaseous diffusion piping. Some features, like peak-finding, Compton correction, detector efficiency, and material properties are characteristic of typical manual methods. Most features are specific to in-pipe robotic deployment. These include in-motion radiometry, self-determined location, geometric modeling of thick deposits, bounding of self-attenuation thickness and auto-checking of replicate measurements. Significant are the means for determining all the properties, equations, and constants for automatically computing and displaying all the quantities, uncertainties and information needed for NDA reporting, analysis, and review. Earlier work by this team demonstrated rudimentary but convincing robotic in-pipe NDA of holdup deposits in pipes. Cold testing with high-enrichment mat sources and hot tests with low U-235 loadings together succeeded to exhibit convincing proof-of-principle. This research-grade radiometry implementation lacked accurate odometry, efficiency calibration, high-fidelity detector modeling, attenuation modeling, forward geometric modeling, auto-segmenting, uncertainty modeling, replicate checking, deconvolution and much more. This work explains the technical basis behind robotic in-pipe NDA. It includes discussion of a new method for modeling of self-attenuation using in-pipe deposit geometry information, detail of the method's total measurement uncertainty, and explanation of calibration methods and results. Beyond development of automation-specific radiometric elements, the paper highlights analyses, testing, and technical bases specific to and supportive of the methodology. Examples include collimation characterization, detector efficiency determination, auto-calibration methodology, and odometric replicate-checking. Results of this methodology are formalized in a DOE EM Technical Basis Document, implemented in software, formally verified in review and acceptance testing and proceduralized as a means for D and D NDA at the Portsmouth enrichment facility. Measurement of U-235 quantity is a well-known cost and schedule driver in D and D of every defunct gaseous diffusion enrichment facility in the world. The radiometry methodologies and results detailed in this paper were the high hurdles. Having established the technical basis for this automated NDA, the opportunity is to apply this to many sizes and robot forms for addressing holdup deposit NDA throughout the D and D community. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

NASA NTRSDate not supplied

A Cold Wet Mars: A Testable Hypothesis for Ancient Mars Ocean Freezing Point Depression Via Low Molecular Weight Organics

Mars exhibits widespread evidence of surface water in the distant past, but global modeling has had difficulty producing climatological conditions conducive to a wet surface. The hypothesis discussed here examines a different way of approaching the problem rather than focusing on climate, instead an examination of the nature of the surface liquid itself. Previous work has largely assumed that martian surface water was a brine analogous to terrestrial ocean water, but recent discoveries suggest that significant amounts of light organic compounds may have been present via abiogenic native production of light organics on Mars [1]. Light organics such as methanol and formaldehyde have an approximate order-of-magnitude greater freezing point depression than brine, potentially lowering the freezing point of martian surface fluids sufficiently to remain liquid even if the mean surface temperature is below zero Centigrade. As Mars evolved and the surface transitioned to the strongly oxidized conditions seen today, the light organics would have oxidized to carbon dioxide and may be a constituent of the atmosphere today. Considerable work must be done to constrain the freezing points of Mars-relevant organic/water and organic/salt/water mixtures, but this investigation might explain the presence of surface fluid on a cold early Mars – a cold, wet Mars as opposed to a warm, wet Mars. Additionally, this approach may work in conjunction with climatological modeling to better describe early conditions conducive which adequately explain observations. This hypothesis can be tested by examination of ancient fluid inclusions (either in situ or via Mars Sample Return) such as those commonly found in halite, preserving samples of ancient martian surface fluid.

M D Fries↗

DOE OSTI2026

Overview of MARS: The Multimodal Advanced Radiography Station at the High-Flux Isotope Reactor

Neutron imaging is a powerful tool used for inspecting internal structures and studying macroscale particle dynamics. This work is performed at the Multimodal Advanced Radiography Station (MARS), which is the cold-neutron imaging beamline at the High-Flux Isotope Reactor at Oak Ridge National Laboratory. Herein is a summary of recent upgrades to instrumentation, software, and methods, driven by needs from the user community. Planned upgrades within the next decade are included that will significantly enhance instrument capability and performance.

Torres, James [ORNL] (ORCID:0000000289407610)↗

DOE OSTI2016

Modulation of electron-acoustic waves in a plasma with kappa distribution

In the present work, employing a one dimensional model of an unmagnetized collisionless plasma consisting of a cold electron fluid, hot electrons obeying κ velocity distribution, and stationary ions, we study the amplitude modulation of an electron-acoustic waves by use of the conventional reductive perturbation method. Employing the field equations of such a plasma, we obtained the nonlinear Schrödinger equation as the evolution equation. Seeking a harmonic wave solution with progressive wave amplitude to the evolution equation, as opposed to the plasma with vortex distribution, the amplitude wave assumes a shock wave type of solution. Finally, the modulational stability of the wave is studied and it is observed that the wave is modulationally stable for all admissible wave numbers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2015

FINGERING CONVECTION AND CLOUDLESS MODELS FOR COOL BROWN DWARF ATMOSPHERES

This work aims to improve the current understanding of the atmospheres of brown dwarfs, especially cold ones with spectral types T and Y, whose modeling is a current challenge. Silicate and iron clouds are believed to disappear at the photosphere at the L/T transition, but cloudless models fail to reproduce correctly the spectra of T dwarfs, advocating for the addition of more physics, e.g., other types of clouds or internal energy transport mechanisms. We use a one-dimensional radiative/convective equilibrium code ATMO to investigate this issue. This code includes both equilibrium and out-of-equilibrium chemistry and solves consistently the PT structure. Included opacity sources are H{sub 2}-H{sub 2}, H{sub 2}-He, H{sub 2}O, CO, CO{sub 2}, CH{sub 4}, NH{sub 3}, K, Na, and TiO, VO if they are present in the atmosphere. We show that the spectra of Y dwarfs can be accurately reproduced with a cloudless model if vertical mixing and NH{sub 3} quenching are taken into account. T dwarf spectra still have some reddening in, e.g., J–H, compared to cloudless models. This reddening can be reproduced by slightly reducing the temperature gradient in the atmosphere. We propose that this reduction of the stabilizing temperature gradient in these layers, leading to cooler structures, is due to the onset of fingering convection, triggered by the destabilizing impact of condensation of very thin dust.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2011

Rovibrational analysis of the XUV photodissociation of HeH{sup +} ions

We investigate the dynamics of the photodissociation of the helium hydride ion HeH{sup +} by XUV radiation with the aim to establish a detailed comparison with a recent experimental work carried out at the FLASH free electron laser using both vibrationally hot and cold ions. We determine the corresponding rovibrational distributions using a dissociative charge transfer setup and the same source conditions as in the FLASH experiment. Using a nonadiabatic time-dependent wave-packet method, we calculate the partial photodissociation cross sections for the n=1-3 coupled electronic states of HeH{sup +}. We find good agreement with the experiment for the cross section into the He + H{sup +} dissociative channel. On the other hand, we show that the experimental observation of the importance of the electronic states with n>3 cannot be well explained theoretically, especially for cold (v=0) ions. We find a good agreement with the experiment on the relative contribution of the {Sigma} and {Pi} states to the cross section for the He{sup +} + H channel, but only a qualitative one for the He + H{sup +} channel. We discuss the factors that could explain the remaining discrepancies between theory and experiment.

74 ATOMIC AND MOLECULAR PHYSICS↗