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At least 595 records · Page 33

Studies of Spinons, Majoranas, and Monopoles in Spin Liquid and Quantum Critical Magnets with Neutrons

Quantum and frustrated materials have eminent potential for the future with the promise of transformative properties in energy storage, conversion, and transmission as well as for new types of computing. Many of the new materials being explored are introduced to have highly unusual ground states that show quantum critical behavior or exotic disorder such as spin liquids. Intense interest is focused on the unusual types of fractionalized quasiparticles that these phases can support such as spin-1/2 spinons, Majorana fermions, and magnetic monopoles. Neutron scattering provides a remarkable tool for probing quantum and frustrated states of real magnetic system by measuring the structure and dynamics of atomic spins on the important energy scales involved. Here I review the signatures of these unusual quasiparticles and the evidence for them starting with quasi-1D magnets covering fractionalization of magnons into spinons, confinement effects, and three classes of quantum critical behavior. In 2D I report on the status of quantum spin liquids in triangular and Kagome magnets before considering the current evidence for exotic Majorana fermions in materials that approximate the Kitaev model. Following this I outline the current status of research into magnetic monopoles in 3D spin ice and the potential for emergent electrodynamics in quantum spin ice. Finally, I consider where new developments in materials, experiment, and theory and modeling could lead to new discoveries.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Hybrid magnonics in hybrid perovskite antiferromagnets

Abstract Hybrid magnonic systems are a newcomer for pursuing coherent information processing owing to their rich quantum engineering functionalities. One prototypical example is hybrid magnonics in antiferromagnets with an easy-plane anisotropy that resembles a quantum-mechanically mixed two-level spin system through the coupling of acoustic and optical magnons. Generally, the coupling between these orthogonal modes is forbidden due to their opposite parity. Here we show that the Dzyaloshinskii–Moriya-Interaction (DMI), a chiral antisymmetric interaction that occurs in magnetic systems with low symmetry, can lift this restriction. We report that layered hybrid perovskite antiferromagnets with an interlayer DMI can lead to a strong intrinsic magnon-magnon coupling strength up to 0.24 GHz, which is four times greater than the dissipation rates of the acoustic/optical modes. Our work shows that the DMI in these hybrid antiferromagnets holds promise for leveraging magnon-magnon coupling by harnessing symmetry breaking in a highly tunable, solution-processable layered magnetic platform.

14 SOLAR ENERGY↗

Direct detection system for full-field nanoscale X-ray diffraction-contrast imaging

Recent developments in X-ray science provide methods to probe deeply embedded mesoscale grain structures and spatially resolve them using dark field X-ray microscopy (DFXM). Extending this technique to investigate weak diffraction signals such as magnetic systems, quantum materials and thin films prove challenging due to available detection methods and incident X-ray flux at the sample. We present a direct detection method developed in conjunction with KAImaging which focuses on DFXM studies in the hard X-ray range of 10s of keV and above capable of approaching nanoscale resolution. Additionally, we compare this direct detection scheme with routinely used scintillator-based optical detection and achieve an order of magnitude improvement in exposure times allowing for imaging of weakly diffracting ordered systems.

47 OTHER INSTRUMENTATION↗

Plasma system of the GOL-3T facility

The plasma system and diagnostics of the new facility GOL-3T are described. This facility is the final result of the first stage in the deep upgrade of the GOL-3 multiple-mirror system, which has operated at the Budker Institute of Nuclear Physics since 1988. The upgrade project supposes creation of two new independent facilities at the site of GOL-3. The GOL-3T facility is intended to study the physics of beam—plasma interaction and generation of subterahertz electromagnetic radiation during the collective relaxation of a high-power relativistic electron beam with a duration of 5–10 μs. Studies on the physics of multiple-mirror plasma confinement in axisymmetric magnetic systems will be continued in a new range of experiment parameters at the second facility, named GOL-NB.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

THE SHOENBERG EFFECT IN A RELATIVISTIC DEGENERATE ELECTRON GAS AND OBSERVATIONAL EVIDENCE IN MAGNETARS

The electron gas inside a neutron star is highly degenerate and relativistic. Due to electron-electron magnetic interactions, the differential susceptibility can equal or exceed one, which causes the magnetic system of the neutron star to become metastable or unstable. The Fermi liquid of nucleons under the crust can be in a metastable state, while the crust is unstable to the formation of layers of alternating magnetization. The change of the magnetic stress acting on adjacent domains can result in a series of shifts or fractures in the crust. The release of magnetic free energy and elastic energy in the crust can cause the bursts observed in magnetars. Simultaneously, a series of shifts or fractures in the deep crust that is close to the Fermi liquid of nucleons can trigger a phase transition of the Fermi liquid of nucleons from a metastable state to a stable state. The magnetic free energy released in the Fermi liquid of nucleons corresponds to the giant flares observed in some magnetars.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Features of the Development of Electron-Optical Systems for Pulsed Terahertz Traveling-Wave Tubes (Review)

We present an analysis of the current state and development of pulsed amplifying traveling-wave tubes for terahertz radiation operation at frequencies of at least 200 GHz, as well as the development prospects of the principles of creating electron-optical and magnetic systems. The possibility of using field emission cathodes based on carbon nanotubes for constructing an electron-optical system with the compression of a sheet beam is discussed. A numerical simulation of a field emission electron gun forming a sheet electron beam for traveling-wave tubes of the terahertz range is carried out.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Ferromagnetic ordering of Cr and Fe doped p-type diamond: An ab initio study

Ferromagnetic ordering of transition metal dopants in semiconductors holds the prospect of combining the capabilities of semiconductors and magnetic systems in single hybrid devices for spintronic applications. Various semiconductors have so far been considered for spintronic applications, but low Curie temperatures have hindered room temperature applications. We report ab initio DFT calculations on the stability and magnetic properties of Fe and Cr impurities in diamond, and show that their ground state magnetic ordering and stabilization energies depend strongly on the charge state and type of co-doping. We predict that divacancy Cr{sup +2} and substitutional Fe{sup +1} order ferromagnetically in p-type diamond, with magnetic stabilization energies (and magnetic moment per impurity ion) of 16.9 meV (2.5 μ{sub B}) and 33.3 meV (1.0 μ{sub B}), respectively. These magnetic stabilization energies are much larger than what has been achieved in other semiconductors at comparable impurity concentrations, including the archetypal dilute magnetic semiconductor GaAs:Mn. In addition, substitutional Fe{sup +1} exhibits a strong half-metallic character, with the Fermi level crossing bands in only the spin down channel. These results, combined with diamond’s extreme properties, demonstrate that Cr or Fe dopedp-type diamond may successfully be considered in the search for room temperature spintronic materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Theory of the spin-Seebeck effect at a topological-insulator/ferromagnetic-insulator interface

The spin-Seebeck effect refers to voltage signals induced in metals by thermally driven spin currents in adjacent magnetic systems. We present a theory of the spin-Seebeck signal in the case where the conductor that supports the voltage signal is the topologically protected two-dimensional surface-state system at the interface between a ferromagnetic insulator (FI) and a topological insulator (TI). Our theory uses a Dirac model for the TI surface states and assumes Heisenberg exchange coupling between the TI quasiparticles and the FI magnetization. The spin-Seebeck voltage is induced by the TI surface states scattering off the nonequilibrium magnon population at the surface of the semi-infinite thermally driven FI. Our theory is readily generalized to spin-Seebeck voltages in any two-dimensional conductor that is exchange-coupled to the surface of a FI. Surface-state carrier-density-dependent signal strengths calculated using Bi 2 Te 3 and yttrium iron garnet material parameters are consistent with recent experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Ice sculpting: An artificial spin ice Tutorial on controlling microstate and geometry for magnonics and neuromorphic computing

Artificial spin ice, arrays of strongly interacting nanomagnets, are complex magnetic systems with many emergent properties, rich microstate spaces, intrinsic physical memory, high-frequency dynamics in the GHz range, and compatibility with a broad range of measurement approaches. This Tutorial article aims to provide the foundational knowledge needed to understand, design, develop, and improve the dynamic properties of artificial spin ice. Special emphasis is placed on introducing the theory of micromagnetics, which describes the complex dynamics within these systems, along with their design, fabrication methods, and standard measurement and control techniques. The article begins with a review of the historical background, introducing the underlying physical phenomena and interactions that govern artificial spin ice. We then explore the standard experimental techniques used to prepare the microstate space of the nanomagnetic array and to characterize magnetization dynamics, both in artificial spin ice and more broadly in ferromagnetic materials. Finally, we introduce the basics of neuromorphic computing applied to the case of artificial spin ice systems with a goal to help researchers new to the field grasp these exciting new developments.

Sultana, Rawnak [Univ. of Delaware, Newark, DE (Un↗

Neutron diffraction studies and magnetism in Ti doped SrFeO{sub 3−δ} systems

The magnetic ground state of single phase tetragonal crystal structure with I4/mmm space group SrFe{sub 1−x}Ti{sub x}O{sub 3−δ} (x = 0.2 and 0.3) is investigated from 2 K to 300 K. Strong irreversibility is observed in zero-field-cooled (ZFC) and field-cooled DC magnetization curves. Arrott plots show the absence of spontaneous magnetization (M{sub S}) down to 2 K, ruling out the possibility of long range ferromagnetic order. Neutron diffraction measurements carried out at H = 0, 7 T (field cooled) at several temperatures above and below the T* (temperature at which M{sub ZFC}(T) is maximum) do not show any additional peaks and also no difference in intensity rules out, both the long range antiferromagnetic and ferromagnetic orders. Hence, the combined study of dc magnetization and neutron diffraction results reveals cluster spin glass behavior in SrFe{sub 1−x}Ti{sub x}O{sub 3−δ} (x = 0.2 and 0.3)

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

FORMATION AND RECONNECTION OF THREE-DIMENSIONAL CURRENT SHEETS IN THE SOLAR CORONA

Current-sheet formation and magnetic reconnection are believed to be the basic physical processes responsible for much of the activity observed in astrophysical plasmas, such as the Sun's corona. We investigate these processes for a magnetic configuration consisting of a uniform background field and an embedded line dipole, a topology that is expected to be ubiquitous in the corona. This magnetic system is driven by a uniform horizontal flow applied at the line-tied photosphere. Although both the initial field and the driver are translationally symmetric, the resulting evolution is calculated using a fully three-dimensional (3D) magnetohydrodynamic simulation with adaptive mesh refinement that resolves the current sheet and reconnection dynamics in detail. The advantage of our approach is that it allows us to directly apply the vast body of knowledge gained from the many studies of two-dimensional (2D) reconnection to the fully 3D case. We find that a current sheet forms in close analogy to the classic Syrovatskii 2D mechanism, but the resulting evolution is different than expected. The current sheet is globally stable, showing no evidence for a disruption or a secondary instability even for aspect ratios as high as 80:1. The global evolution generally follows the standard Sweet-Parker 2D reconnection model except for an accelerated reconnection rate at a very thin current sheet, due to the tearing instability and the formation of magnetic islands. An interesting conclusion is that despite the formation of fully 3D structures at small scales, the system remains close to 2D at global scales. We discuss the implications of our results for observations of the solar corona.

79 ASTRONOMY AND ASTROPHYSICS↗

Strong Photon‐Magnon Coupling Using a Lithographically Defined Organic Ferrimagnet

Abstract A cavity‐magnonic system composed of a superconducting microwave resonator coupled to a magnon mode hosted by the organic‐based ferrimagnet vanadium tetracyanoethylene (V[TCNE] x ) is demonstrated. This work is motivated by the challenge of scalably integrating a low‐damping magnetic system with planar superconducting circuits. V[TCNE] x has ultra‐low intrinsic damping, can be grown at low processing temperatures on arbitrary substrates, and can be patterned via electron beam lithography. The devices operate in the strong coupling regime, with a cooperativity exceeding 1000 for coupling between the Kittel mode and the resonator mode at T≈0.4 K, suitable for scalable quantum circuit integration. Higher‐order magnon modes are also observed with much narrower linewidths than the Kittel mode. This work paves the way for high‐cooperativity hybrid quantum devices in which magnonic circuits can be designed and fabricated as easily as electrical wires.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Chemically-Controlled Stacking of Inorganic Subnets in Coordination Networks: Metal–Organic Magnetic Multilayers

Coordination networks (CNs), such as, for instance, metal–organic frameworks (MOFs), can turn into remarkable magnets, with various topologies of spin carriers and unique opportunities of cross-coupling to other functionalities. Alternatively, distinct inorganic subnetworks that are spatially segregated by organic ligands can lead to coexisting magnetic systems in a single bulk material. Here, we present a system of two CNs of general formula Mn(H 2 O) x (OOC-(C 6 H 4 ) y -COO). The compound with two water molecules and one aromatic ring (x = 2; y = 1) has a single two-dimensional magnetic subnet, while the material with x = 1.5 and y = 2 shows, additionally, another type of magnetic layer. In analogy to magnetic multilayers that are deposited by physical methods, these materials can be regarded as metal–organic magnetic multilayers (MOMMs), where the stacking of different types of magnetic layers is controlled by the choice of an organic ligand during the chemical synthesis. Lastly, this work further paves the way toward organic–inorganic nanostructures with functional magnetic properties.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Quantum wake dynamics in Heisenberg antiferromagnetic chains

Traditional spectroscopy, by its very nature, characterizes physical system properties in the momentum and frequency domains. However, the most interesting and potentially practically useful quantum many-body effects emerge from local, short-time correlations. Here, using inelastic neutron scattering and methods of integrability, we experimentally observe and theoretically describe a local, coherent, long-lived, quasiperiodically oscillating magnetic state emerging out of the distillation of propagating excitations following a local quantum quench in a Heisenberg antiferromagnetic chain. This “quantum wake” displays similarities to Floquet states, discrete time crystals and nonlinear Luttinger liquids. We also show how this technique reveals the non-commutativity of spin operators, and is thus a model-agnostic measure of a magnetic system’s “quantumness.”

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

The exceedingly strong two-dimensional ferromagnetism in bi-atomic layer SrRuO 3 with a critical conduction transition

In recent years, few-layer or even monolayer ferromagnetic materials have drawn a great deal of attention due to the promising integration of two-dimensional (2D) magnets into next-generation spintronic devices. The SrRuO 3 monolayer is a rare example of stable 2D magnetism under ambient conditions, but only weak ferromagnetism or antiferromagnetism has been found. The bi-atomic layer SrRuO3 as another environmentally inert 2D magnetic system has been paid less attention heretofore. Here we study both the bi-atomic layer and monolayer SrRuO 3 in (SrRuO 3 ) n /(SrTiO 3 ) m (n = 1, 2) superlattices in which the SrTiO 3 serves as a non-magnetic and insulating space layer. Although the monolayer exhibits arguably weak ferromagnetism, we find that the bi-atomic layer exhibits exceedingly strong ferromagnetism with a T c of 125 K and a saturation magnetization of 1.2 μ B /Ru, demonstrated by both superconducting quantum interference device (SQUID) magnetometry and element-specific X-ray circular dichroism. Moreover, in the bi-atomic layer SrRuO 3 , we demonstrate that random fluctuations and orbital reconstructions inevitably occurring in the 2D limit are critical to the electrical transport, but are much less critical to the ferromagnetism. Our study demonstrates that the bi-atomic layer SrRuO 3 is an exceedingly strong 2D ferromagnetic oxide which has great potentials for applications of ultracompact spintronic devices.

36 MATERIALS SCIENCE↗

Nonlinear Modeling of Macroscopic Plasma Dynamics Final Scientific Report May 1, 2006 – April 30, 2018

The project entitled, "Nonlinear Modeling of Macroscopic Plasma Dynamics," applied numerical computation to solve mathematical models of plasma behavior in laboratory systems. Plasma is the state of matter with sufficiently large internal energy density such that electrons dissociate from atoms to form gas of electrically charged particles. It occurs naturally in stars, planetary magnetospheres, and interstellar and intergalactic media. It is also used for industrial purposes and in lighting. Fusion energy science seeks to create and sustain plasma conditions where atomic nuclei fuse to create energy that can be captured for power production. Many laboratory experiments for this effort use magnetic field to contain plasma and to thermally insulate it from its surroundings. Possible plasma dynamics in magnetized systems include collective behavior over spatial scales that are comparable to the configuration size, and these dynamics often include evolution of the magnetic field that is used for confinement. Solving the mathematical models that describe these dynamics in specific experiments often requires computer simulations, as done in this project. This project analyzed plasma magnetic relaxation dynamics in the laboratory configurations known as the reversed-field pinch (RFP), the spheromak, and the spherical torus (ST). It also developed capabilities for modeling disruptive plasma dynamics in the tokamak, which has achieved the highest performance for magnetized plasma and is the design of the large international ITER experiment (https://www.iter.org) that is under construction and is expected to be the first to achieve self-heating conditions. Dynamic evolution to states of low energy, the aforementioned magnetic relaxation, is known to be important for generating the RFP and spheromak configurations. Nonlinear computational modeling with the Non-Ideal Magnetohydrodynamics with Rotation, Open Discussion code (NIMROD, https://nimrodteam.org) was applied to understand specific aspects of magnetic relaxation in RFPs, spheromaks, and STs. The RFP study considered how the nonlinear transfer of power among different fluctuation harmonics is altered due to the application of pulses of electric field, as done experimentally in the Madison Symmetric Torus RFP device at the University of Wisconsin-Madison. It also investigated the separation of electron and ion dynamics, known as two-fluid effects, including effects on the evolution of the plasma flow profile. The spheromak study considered the influence of these two-fluid effects in conditions relevant to the Sustained Spheromak Experiment (SSPX), formerly at Lawrence Livermore National Laboratory. Our study found that two-fluid effects enhance stability with respect to interchange in SSPX-relevant conditions, but having a complete model with two-fluid effects in separate electron and ion temperature equations is important. The study for STs focused on plasma startup in the Pegasus Toroidal Experiment at UW-Madison, which uses DC voltage applied through a small plasma gun. The simulations show how the resulting helical current stream relaxes through repetitive merging, forming current rings that accumulate into a tokamak-like configuration. Analytical theory was also developed to help explain behavior that was observed in the RFP and spheromak computations. Although the tokamak configuration has outperformed other magnetic confinement configurations, it has a tendency to undergo discharge-terminating dynamics that release energy onto plasma-facing surfaces and exert electromechanical forces on magnetic coils and structures. Our efforts have improved NIMROD's capabilities to model tokamak disruption by incorporating a resistive wall model that can be applied to axisymmetric, as well as asymmetric, distortions of the magnetic field configuration. Computations addressed whether mathematical conditions applied to plasma flow at the wall influence disruptive dynamics.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Behavior of thermally quenched topological defects in quasicrystal artificial spin ices

We report that understanding the formation of topological defects in connected magnetic nanowires such as in artificial spin ices (ASIs) is critical to controlling their behavior. Moreover, emergent frustration behavior of these defects can be expected due to complex underlying lattice geometry of the ASIs. We have explored in situ thermalization and quenching of quasicrystalline ASIs, which exhibit additional frustration due to aperiodicity from near the Curie temperature, and we observe the formation of two sets of topological vortex defects: within the magnetic bars and within the vertices at which the bars meet. By varying the laser fluence, we show that the number of defects in the vertices varies as the quenching rate changes following a power law relation, which we interpret as being related to the ferromagnetic-to-paramagnetic phase transition. Conversely, the defects formed within the bars are metastable states related to the spontaneous magnetization reversal of the magnetic bars and are therefore strongly dependent on underlying lattice geometry. These results provide insight into the emergence and control of topological defects in confined frustrated magnetic systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Accretion Flows in Magnetic White Dwarf Systems

We received Type A and B funding under the NASA Astrophysics Data Program for the analysis and interpretation of hard x-ray data obtained by the Rossi X-ray Timing Explorer and other NASA sponsored missions for Intermediate Polars (IPS) and Polars. For some targets, optical data was available. We reduced and analyzed the X-ray spectra and the X-ray and optical (obtained at the Cerro Tololo Inter-American Observatory) timing data using detailed shock models (which we constructed) to place constraints on the properties of the accreting white dwarfs, the high energy emission mechanisms of white dwarfs, and the large-scale accretion flows of Polars and IPS. IPS and Polars are white dwarf mass-transfer binaries, members of the larger class of cata,clysmic variables. They differ from the bulk of the cataclysmic variables in that they contain strongly magnetic white dwarfs; the white dwarfs in Polars have B, = 7 to 230 MG and those in IPS have B, less than 10 MG. The IPS and Polars are both examples of funneled accretion flows in strong magnetic field systems. The IPS are similar to x-ray pulsars in that accretion disks form in the systems which are disrupted by the strong stellar magnetic fields of the white dwarfs near the stellar surface from where the plasma is funneled to the surface of the white dwarf. The localized hot spots formed at the footpoints of the funnels coupled with the rotation of the white dwarf leads to coherent pulsed x-ray emission. The Polars offer an example of a different accretion topology; the magnetic field of the white dwarf controls the accretion flow from near the inner Lagrangian point of the system directly to the stellar surface. Accretion disks do not form. The strong magnetic coupling generally leads to synchronous orbital/rotational motion in the Polars. The physical system in this sense resembles the Io/Jupiter system. In both IPS and Polars, pulsed emission from the infrared to x-rays is produced as the funneled flows merge onto the white dwarfs through the formation of strong radiating shock waves. A comparative study of the IPS and Polars can elucidate the primary effects of the magnetic fields on the dynamics and thermodynamics in accreting white dwarf systems.

Imamura, James N.↗