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DOE OSTI2016

COSMIC-RAY SMALL-SCALE ANISOTROPIES AND LOCAL TURBULENT MAGNETIC FIELDS

Cosmic-ray anisotropy has been observed in a wide energy range and at different angular scales by a variety of experiments over the past decade. However, no comprehensive or satisfactory explanation has been put forth to date. The arrival distribution of cosmic rays at Earth is the convolution of the distribution of their sources and of the effects of geometry and properties of the magnetic field through which particles propagate. It is generally believed that the anisotropy topology at the largest angular scale is adiabatically shaped by diffusion in the structured interstellar magnetic field. On the contrary, the medium- and small-scale angular structure could be an effect of nondiffusive propagation of cosmic rays in perturbed magnetic fields. In particular, a possible explanation for the observed small-scale anisotropy observed at the TeV energy scale may be the effect of particle propagation in turbulent magnetized plasmas. We perform numerical integration of test particle trajectories in low- β compressible magnetohydrodynamic turbulence to study how the cosmic rays’ arrival direction distribution is perturbed when they stream along the local turbulent magnetic field. We utilize Liouville’s theorem for obtaining the anisotropy at Earth and provide the theoretical framework for the application of the theorem in the specific case of cosmic-ray arrival distribution. In this work, we discuss the effects on the anisotropy arising from propagation in this inhomogeneous and turbulent interstellar magnetic field.

79 ASTRONOMY AND ASTROPHYSICS↗

NASA NTRS1987

Magnetic flux tubes as sources of wave generation

The structure of solar, and very likely stellar, surface magnetic fields is highly inhomogeneous: at the photospheric level, the fields are locally strong, and show concentration into a flux tube structure. In this case, the wave energy generated in stellar convection zones may be largely carried away by flux tube waves, which can then become important sources for the heating of the outer atmospheric layers. Such flux tube wave generation may help to explain the UV and X-ray fluxes observed by the IUE and Einstein observatories. The generation of longitudinal tube waves in magnetic flux tubes embedded in an otherwise magnetic field-free, turbulent, and stratified medium was considered. It is shown that compressible tube waves are generated by dipole emission and that the generation efficiency is a strong function of the magnetic field strength. Energy flux calculations are presented for different magnetic flux tubes, and show how the results depend on the magnetic field strength and the characteristics of the convective turbulence.

Musielak, Z. E.↗

DOE OSTI2024

The Role of Interfacial Interactions and Oxygen Vacancies in Tuning Magnetic Anisotropy in LaCrO 3 /LaMnO 3 Heterostructures

The interplay of lattice, electronic, and spin degrees of freedom at epitaxial complex oxide interfaces provides a route to tune their magnetic ground states. Unraveling the competing contributions is critical for tuning their functional properties. The relationship between magnetic ordering and magnetic anisotropy and the lattice symmetry, oxygen content, and film thickness in compressively strained LaMnO 3 (LMO)/LaCrO 3 (LCO) superlattices is investigated. Mn–O–Cr antiferromagnetic superexchange interactions across the heterointerface result in a net ferrimagnetic magnetic structure. Bulk magnetometry measurements reveal isotropic in-plane magnetism for as-grown oxygen-deficient thin samples due to equal fractions of orthorhombic a+a-c-, and a-a+c- twin domains. As the superlattice thickness is increased, in-plane magnetic anisotropy emerges as the fraction of the a+a-c- domain increases. On annealing in oxygen, the suppression of oxygen vacancies results in a contraction of the lattice volume, and an orthorhombic to rhombohedral transition leads to isotropic magnetism independent of the film thickness. The complex interactions are investigated using high-resolution synchrotron diffraction and X-ray absorption spectroscopy. These results highlight the role of the evolution of structural domains with film thickness, interfacial spin interactions, and oxygen-vacancy-induced structural phase transitions in tuning the magnetic properties of complex oxide heterostructures.

36 MATERIALS SCIENCE↗

NASA NTRS1984

Stellar fibril magnetic systems. I - Reduced energy state

The remarkable fibril structure of the magnetic fields at the surface of the sun (with fibrils compressed to 1,000-2,000 gauss) lies outside existing statistical theories of magnetohydrodynamic turbulence. The total energy of the fibril field is enhanced by a factor of more than 100 above the energy for the mean field in a continuum state. The magnetic energy density within a fibril is of the order of 100 times the local kinetic energy density, so that no simple application of equipartition principles is possible. It is pointed out that the total energy of the atmosphere (thermal + gravitational + magnetic) is reduced by the fibril state of the field by avoiding the magnetic inhibition of the convective overturning, suggesting that the formation of the observed intense fibril state may be in response to the associated energy reduction. Calculation of the minimum total energy of a polytropic atmosphere permeated by magnetic fibrils yields theoretical fibril fields of the order of 1-5 kilogauss when characteristics appropriate to the solar convective zone are introduced, in rough agreement with the actual fields of 1-2 kilogauss. The polytrope model, although crude, establishes that a large reduction in total energy is made possible by the fibril state.

Parker, E. N.↗

DOE OSTI2019

Inferring fuel areal density from secondary neutron yields in laser-driven magnetized liner inertial fusion

A technique to infer the areal density ρR of compressed deuterium (D) in cylindrical implosions from the ratio of secondary D–T (deuterium–tritium) neutrons to primary D–D neutrons is described and evaluated. For ρR to be proportional to the ratio of D–T to D–D yield, the increase in the D–T fusion cross section with collisional slowing of the tritium must be small, requiring where TkeV is the electron temperature in keV. The technique is applied to results from laser-driven magnetized liner inertial fusion (MagLIF) targets on OMEGA, where ρR is certainly less than 4 mg/cm 2 . OMEGA MagLIF targets do not achieve a sufficiently high, radially integrated, axial magnetic field BR to confine the tritium, as occurs in Z MagLIF targets, because they are ~10× smaller in radius. The inferred areal densities show that fuel convergence is reduced by preheating, by an applied axial magnetic field, and by increasing the initial fuel density, which are key features of the MagLIF scheme. The results are compared with 1-D and 2-D magnetohydrodynamic simulations for nominal laser and target parameters, which predict areal densities 2× to 3× higher than the measurements.

Davies, J. R.↗

DOE OSTI2016

Reproducible and controllable induction voltage adder for scaled beam experiments

A reproducible and controllable induction adder was developed using solid-state switching devices and Finemet cores for scaled beam compression experiments. A gate controlled MOSFET circuit was developed for the controllable voltage driver. The MOSFET circuit drove the induction adder at low magnetization levels of the cores which enabled us to form reproducible modulation voltages with jitter less than 0.3 ns. Preliminary beam compression experiments indicated that the induction adder can improve the reproducibility of modulation voltages and advance the beam physics experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2020

Machine-learning-assisted insight into spin ice Dy 2 Ti 2 O 7

Complex behavior poses challenges in extracting models from experiment. An example is spin liquid formation in frustrated magnets like Dy 2 Ti 2 O 7 . Understanding has been hindered by issues including disorder, glass formation, and interpretation of scattering data. Here, we use an automated capability to extract model Hamiltonians from data, and to identify different magnetic regimes. This involves training an autoencoder to learn a compressed representation of three-dimensional diffuse scattering, over a wide range of spin Hamiltonians. The autoencoder finds optimal matches according to scattering and heat capacity data and provides confidence intervals. Validation tests indicate that our optimal Hamiltonian accurately predicts temperature and field dependence of both magnetic structure and magnetization, as well as glass formation and irreversibility in Dy 2 Ti 2 O 7 . The autoencoder can also categorize different magnetic behaviors and eliminate background noise and artifacts in raw data. Our methodology is readily applicable to other materials and types of scattering problems.

36 MATERIALS SCIENCE↗

DOE OSTI2022

An overview of magneto-inertial fusion on the Z Machine at Sandia National Laboratories

We present an overview of the magneto-inertial fusion (MIF) concept MagLIF (Magnetized Liner Inertial Fusion) pursued at Sandia National Laboratories and review some of the most prominent results since the initial experiments in 2013. In MagLIF, a centimeter-scale beryllium tube or "liner" is filled with a fusion fuel, axially pre-magnetized, laser pre-heated, and finally imploded using up to 20 MA from the Z machine. All of these elements are necessary to generate a thermonuclear plasma: laser preheating raises the initial temperature of the fuel, the electrical current implodes the liner and quasi-adiabatically compresses the fuel via the Lorentz force, and the axial magnetic field limits thermal conduction from the hot plasma to the cold liner walls during the implosion. MagLIF is the first MIF concept to demonstrate fusion relevant temperatures, significant fusion production (>10^13 primary DD neutron yield), and magnetic trapping of charged fusion particles. On a 60 MA next-generation pulsed-power machine, two-dimensional simulations suggest that MagLIF has the potential to generate multi-MJ yields with significant self-heating, a long-term goal of the US Stockpile Stewardship Program. At currents exceeding 65 MA, the high gains required for fusion energy could be achievable.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2020

Fast electron transport dynamics and energy deposition in magnetized, imploded cylindrical plasma

Inertial confinement fusion approaches involve the creation of high-energy-density states through compression. High gain scenarios may be enabled by the beneficial heating from fast electrons produced with an intense laser and by energy containment with a high-strength magnetic field. Here, we report experimental measurements from a configuration integrating a magnetized, imploded cylindrical plasma and intense laser-driven electrons as well as multi-stage simulations that show fast electrons transport pathways at different times during the implosion and quantify their energy deposition contribution. The experiment consisted of a CH foam cylinder, inside an external coaxial magnetic field of 5 T, that was imploded using 36 OMEGA laser beams. Two-dimensional (2D) hydrodynamic modelling predicts the CH density reaches 9.0 g cm − 3 , the temperature reaches 920 eV and the external B-field is amplified at maximum compression to 580 T. At pre-determined times during the compression, the intense OMEGA EP laser irradiated one end of the cylinder to accelerate relativistic electrons into the dense imploded plasma providing additional heating. The relativistic electron beam generation was simulated using a 2D particle-in-cell (PIC) code. Finally, three-dimensional hybrid-PIC simulations calculated the electron propagation and energy deposition inside the target and revealed the roles the compressed and self-generated B-fields play in transport. During a time window before the maximum compression time, the self-generated B-field on the compression front confines the injected electrons inside the target, increasing the temperature through Joule heating. For a stronger B-field seed of 20 T, the electrons are predicted to be guided into the compressed target and provide additional collisional heating. This article is part of a discussion meeting issue ‘Prospects for high gain inertial fusion energy (part 2)’.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2017

Synthesis and characterization of two novel chiral-type formate frameworks templated by protonated diethylamine and ammonium cations

Two novel formate frameworks templated by ammonium and diethylammonium (DEtA{sup +}) cations have been synthesized. Chemical analysis as well as optical, Raman and IR studies showed partial substitution of nickel ions by Cr(III) or Fe(III). X-ray diffraction revealed that these compounds crystallize in the chiral-type structure of P6{sub 3}22 symmetry. The oxygen atoms from formate ligands form octahedral coordination around the metal centers and the octahedra are bridged by the formate groups in the anti-anti mode configuration forming the hexagonal structure with large channels expanding along the c direction. The channels are filled with disordered DEtA{sup +} and NH{sub 4}{sup +} ions and they show unusual compression with the c/a ratio of only 0.862 and 0.852 for the iron- and chromium-containing compound, respectively. Magnetic studies revealed that the both compounds order magnetically at low temperatures but the ordering temperature is significantly higher for the iron compound (37 K) compared to the chromium analogue (26 K). - Graphical abstract: Temperature dependence of magnetization M of DEtAFeNi showing magnetic order at 37 K. - Highlights: • Two novel chiral formates of P6{sub 3}22 symmetry were synthesized. • The structures contain strongly compressed hexagonal channels filled with disordered cations. • The obtained compounds exhibit magnetic order at low temperatures. • Raman, IR and absorption spectra prove incorporation of Cr(III) and Fe(III) in the frameworks.

36 MATERIALS SCIENCE↗

DOE OSTI2020

Local strain-dependent electronic structure and perpendicular magnetic anisotropy of a MnGaN 2D magnetic monolayer

Local strain-dependent spin-polarized electronic structure of a two-dimensional (2D) magnetic layer is an exciting property for practical applications. For example, it holds the promise for advanced ultrathin spintronic nanodevices with customized electronic and magnetic properties by local strain engineering. Here, we demonstrate that the spin-polarized electronic structure of a 2D manganese gallium nitride (MnGaN-2D) magnetic monolayer is sensitive to intrinsic local lattice strain, as proven by first-principles calculations and indicated by scanning tunneling spectroscopy measurements. Atomic resolution images reveal a highly non-Gaussian lattice spacing/strain distribution, while the spectroscopy reveals variations in the electronic density of states. Simulations of the MnGaN-2D monolayer based on first-principles calculations, including both isotropic and anisotropic strains, confirm a highly strain-dependent manganese partial density of states. Spin-orbit coupling is included which indicates either out-of-plane perpendicular magnetic anisotropy (PMA) or in-plane magnetic anisotropy, dependent on the type of strain whether compressive or tensile, suggesting that MnGaN-2D is magnetoelastic. The MnGaN-2D PMA is further supported by superconducting quantum interference device magnetometry measurements which reveal a high spin polarization of ~ 79 % at room temperature.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2023

Designing Magnetic Properties in CrSBr through Hydrostatic Pressure and Ligand Substitution

Abstract Magnetic van der Waals (vdW) materials are a promising platform for producing atomically thin spintronic and optoelectronic devices. The A‐type antiferromagnet CrSBr has emerged as a particularly exciting material due to its high magnetic ordering temperature, semiconducting electrical properties, and enhanced chemical stability compared to other vdW magnets. Exploring mechanisms to tune its magnetic properties will facilitate the development of nanoscale devices based on vdW materials with designer magnetic properties. Here it is investigated how the magnetic properties of CrSBr change under pressure and ligand substitution. Pressure compresses the unit cell, increasing the interlayer exchange energy while lowering the Néel temperature. Ligand substitution, realized synthetically through Cl alloying, anisotropically compresses the unit cell and suppresses the Cr‐halogen covalency, reducing the magnetocrystalline anisotropy energy and decreasing the Néel temperature. A detailed structural analysis combined with first‐principles calculations reveals that alterations in the magnetic properties are intricately related to changes in direct Cr–Cr exchange interactions and the Cr–anion superexchange pathways. Further, it is demonstrated that Cl alloying enables chemical tuning of the interlayer coupling from antiferromagnetic to ferromagnetic, which is unique among known two‐dimensional magnets.

Telford, Evan J.↗

DOE OSTI2024

Anomalous Landau Level Gaps Near Magnetic Transitions in Monolayer WSe 2

First-order phase transitions produce abrupt changes to the character of both ground and excited electronic states. Here we conduct electronic compressibility measurements to map the spin phase diagram and Landau level (LL) energies of monolayer WSe 2 in a magnetic field. We resolve a sequence of first-order phase transitions between completely spin-polarized LLs and states with LLs of both spins. Unexpectedly, the LL gaps are roughly constant over a wide range of magnetic fields below the transitions, which we show reflects spin-polarized ground states with opposite spin excitations. These transitions also extend into compressible regimes, with a sawtooth boundary between full and partial spin polarization. We link these observations to the important influence of LL filling on the exchange energy beyond a smooth density-dependent contribution. Our results show that WSe 2 realizes a unique hierarchy of energy scales where such effects induce reentrant magnetic phase transitions tuned by density and magnetic field. Published by the American Physical Society 2024

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2021

Abrupt orthorhombic relaxation in compressively strained ultrathin SrRuO 3 films

Lattice structure can dictate electronic and magnetic properties of a material. Especially, reconstruction at a surface or heterointerface can create properties that are fundamentally different from those of the corresponding bulk material. In this work, we have investigated the lattice structure on the surface and in the thin films of epitaxial SrRuO 3 with the film thickness up to 22 pseudo-cubic unit cells (u.c.), using the combination of surface sensitive low energy electron diffraction and bulk sensitive scanning transmission electron microscopy. Our analysis indicates that, in contrast to many perovskite oxides, the RuO6 tilt and rotational distortions appear even in single unit cell SrRuO 3 thin films on cubic SrTiO 3 , while the full relaxation to the bulk-like orthorhombic structures takes 3-4 u.c. from the interface for thicker films. Yet the TiO 6 octahedra of the substrate near the interface with SrRuO 3 films show no sign of distortion, unlike those near the interface with CaRuO 3 films. Two orthogonal in-plane rotated structural domains are identified. These octahedral distortions are essential for the understanding of the thickness dependent transport and magnetism in ultrathin films.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

NASA NTRS1990

A compressed marine data set for geomagnetic field modeling

Some 13 million scalar magnetic field data points that have been collected from the world's ocean areas reside in the collection of the National Geophysical Data Center. In order to derive a suitable data set for modeling the geomagnetic field of the earth, each ship track is divided into 220 km segments. The distribution of the reduced data in position, time and local time is discussed. The along-track filtering process described has proved to be an effective method of condensing large numbers of shipborne magnetic data into a manageable and meaningful data set for field modeling. This process also provides the benefits of smoothing short-wavelength crystal anomalies, discarding data recorded during magnetically noisy periods, and assigning reasonable error estimates to be utilized in the least squares modeling.

Langel, R. A.↗

NASA NTRS2011

Effect of Inductive Coil Geometry and Current Sheet Trajectory of a Conical Theta Pinch Pulsed Inductive Plasma Accelerator

Results are presented demonstrating the e ect of inductive coil geometry and current sheet trajectory on the exhaust velocity of propellant in conical theta pinch pulsed induc- tive plasma accelerators. The electromagnetic coupling between the inductive coil of the accelerator and a plasma current sheet is simulated, substituting a conical copper frustum for the plasma. The variation of system inductance as a function of plasma position is obtained by displacing the simulated current sheet from the coil while measuring the total inductance of the coil. Four coils of differing geometries were employed, and the total inductance of each coil was measured as a function of the axial displacement of two sep- arate copper frusta both having the same cone angle and length as the coil but with one compressed to a smaller size relative to the coil. The measured relationship between total coil inductance and current sheet position closes a dynamical circuit model that is used to calculate the resulting current sheet velocity for various coil and current sheet con gura- tions. The results of this model, which neglects the pinching contribution to thrust, radial propellant con nement, and plume divergence, indicate that in a conical theta pinch ge- ometry current sheet pinching is detrimental to thruster performance, reducing the kinetic energy of the exhausting propellant by up to 50% (at the upper bound for the parameter range of the study). The decrease in exhaust velocity was larger for coils and simulated current sheets of smaller half cone angles. An upper bound for the pinching contribution to thrust is estimated for typical operating parameters. Measurements of coil inductance for three di erent current sheet pinching conditions are used to estimate the magnetic pressure as a function of current sheet radial compression. The gas-dynamic contribution to axial acceleration is also estimated and shown to not compensate for the decrease in axial electromagnetic acceleration that accompanies the radial compression of the plasma in conical theta pinches.

Hallock, Ashley K.↗

NASA NTRS1991

Different FTE signatures generated by the bursty single X line reconnection and the multiple X line reconnection at the dayside magnetopause

This paper examines magnetic signatures associated with the time-dependent magnetic reconnection processes at the dayside magnetopause, using two-dimensional compressible MHD simulations. Emphasis is placed on the different flux-transfer-event (FTE) signatures generated by the bursty single X-line reconnection (BSXR) and the multiple X-line reconnection processes. It is shown that the FTE magnetic signatures are not exhibited on the magnetospheric side if the FTEs are due to the BSXR process and the ratio between the magnetic field strength in the magnetosheath to that in the magnetosphere is not less than 1.7. The simulation results are compared with satellite observations.

Ding, D. Q.↗

NASA NTRS1988

Magnetohydrodynamic (MHD) modelling of solar active phenomena via numerical methods

Numerical ideal MHD models for the study of solar active phenomena are summarized. Particular attention is given to the following physical phenomena: (1) local heating of a coronal loop in an isothermal and stratified atmosphere, and (2) the coronal dynamic responses due to magnetic field movement. The results suggest that local heating of a magnetic loop will lead to the enhancement of the density of the neighboring loops through MHD wave compression. It is noted that field lines can be pinched off and may form a self-contained magnetized plasma blob that may move outward into interplanetary space.

Wu, S. T.↗