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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Iron nitride permanent magnet and technique for forming iron nitride permanent magnet

A permanent magnet may include a Fe 16 N 2 phase constitution. In some examples, the permanent magnet may be formed by a technique that includes straining an iron wire or sheet comprising at least one iron crystal in a direction substantially parallel to a <001> crystal axis of the iron crystal; nitridizing the iron wire or sheet to form a nitridized iron wire or sheet; annealing the nitridized iron wire or sheet to form a Fe 16 N 2 phase constitution in at least a portion of the nitridized iron wire or sheet; and pressing the nitridized iron wires and sheets to form bulk permanent magnet.

Wang, Jian-Ping↗
DOE OSTI2024

Magnetic Field Sensing via Optically Detected Magnetic Resonance and Spin Relaxometry Using Nitrogen Vacancies in Nanodiamonds

Quantum sensing is broadly defined as the use of quantum materials, quantum coherence, and/or quantum entanglement to measure physical quantities and/or to enhance the sensitivity of classical analytical measurements. Certain materials exhibit interesting quantum properties that have the potential to be utilized in quantum sensing applications. One such quantum property is electronic spin, which is utilized in this work. Here, we built a custom apparatus capable of conducting both optically detected magnetic resonance (ODMR) and spin relaxometry. The quantum material investigated was an ensemble of nitrogen vacancies (NV) in nanodiamonds. We have characterized the system and measured ODMR spectra for different strengths of the applied DC magnetic field and clearly observed the expected splitting of the resonances due to Zeeman splitting. We also have measured the spin relaxation times for two different powers of the applied AC magnetic field. The lower power dataset exhibited expected exponential temporal dependence of the relaxation of a modified spin state, whereas the higher power dataset exhibited stretched exponential dependence of the modified spin state, indicating the presence of high-power phenomena that emerge that retard the relaxation of the spin state.

Lander, Gary↗
DOE OSTI2018

Effects of Fe and Co Co-doping on Structural, Magnetic, and Optical Properties of Ti{sub 0.9}Fe{sub 0.1−x}Co{sub x}O{sub 2} Magnetic Semiconductors

A series of six samples with a general formula Ti{sub 0.9}Fe{sub 0.1−x}Co{sub x}O{sub 2} (x = 0.0, 0.02, 0.04, 0.06, 0.08, and 0.1) has been synthesized by solid-state reaction method at annealing temperature of 1150 {sup ∘}C for 2 hours. The synthesized samples have been characterized by X-ray diffractometer, Raman spectroscopy, scanning electron microscopy, EDX, vibrating sample magnetometer, and ultraviolet-visible spectroscopy to investigate structural, defective, morphological, elemental, magnetic, and optical properties. Structural analysis revealed dominant structure of rutile with a minor peak of hematite and anatase. An intensity loss and peak broadening of TiO{sub 2} (rutile) vibration lines has been observed from Raman analysis. Magnetic characterization showed ferromagnetic behavior at room temperature. Optical characterization revealed blue shift in band gap energy with increasing amount of Co concentration.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Wave-Vector Filtering Effect in a Novel Magnetic Nanostructure with Zero Average Magnetic Field

We report a theoretical investigation on wave-vector filtering (WVF) effect in a magnetic nanostructure, which can be experimentally realized by depositing ferromagnetic (FM) stripes on the surface of GaAs/Al{sub x}Ga{sub 1-x}As heterostructure. An appreciable WVF effect appears in this nanosystem. The WVF efficiency is associated with structural parameters of magnetic nanostructure. Therefore, such a device can be employed as a momentum filter for nanoelectronics device applications.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Synthesis and Characterization of Hydrophobic Fe{sub 3}O{sub 4} Magnetic Nanoparticles with High Saturation Magnetization

A simple one-step solvothermal method is proposed to prepare hydrophobic Fe{sub 3}O{sub 4} nanoparticles (MNPs) using iron acetylacetonate (Fe(acac){sub 3}), oleylamine (OAm), and ethylene glycol (EG). X-ray powder diffraction, scanning electron microscope, infrared spectroscopy, transmission electron microscopy, X-ray photoelectron spectrometry, and vibrating sample magnetometer are used to characterize the structure, morphology, and properties of products. The testing results indicate that the as-synthesized products are spherical-like hydrophobic MNPs, superparamagnetic at room temperature, with a saturation magnetization up to 76.8 emu/g. The good hydrophobic property of MNPs is attributed to the coverage of oleylamine, without causing a remarkable loss of magnetic property. In addition, the influences of material ratio, aging time, oleic acid, and stearic acid used as additives are studied in our research.

77 NANOSCIENCE AND NANOTECHNOLOGY↗
DOE OSTI2025

Magnetized ICF implosions: non-axial magnetic field topologies

This paper explores four different magnetic field topologies for application to spherical inertial confinement fusion implosions: axial, mirror, cusp and closed field lines. A mirror field is found to enhance the impact of magnetization over an axial field; this is because the mirror field more closely follows the hot-spot surface. A cusp field, while simple to generate, is not found to have any benefits over the tried-and-tested axial field. Closed field lines are found to be of the greatest benefit to hot-spot performance, with the simulated design undergoing a 2× increase in ion temperature before α-heating is considered. The plasma properties of the simulation with closed field lines are radically different from the unmagnetized counterpart, with electron temperatures in excess of 100 keV, suggesting that a fundamental redesign of the capsule implosion is possible if this method is pursued.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2019

Effect of Thermoelectric Magnetic Convection on Shrinkage Porosity at the Final Stage of Solidification of GCr18Mo Steel Under Axial Static Magnetic Field

Adopting effective strategies to eliminate the shrinkage porosity at the final stage of steel solidification is one of the most attractive research subjects for metallurgists. Despite the progress in understanding the thermoelectric magnetic convection (TEMC) in the solidification process, utilization of TEMC for modifying the solidification feeding of steel has been ignored. The effects of TEMC on the shrinkage porosity at the final stage of solidification of GCr18Mo steel were investigated under an axial static magnetic field (ASMF). The morphology and porosity of GCr18Mo steel were investigated quantitatively by X-ray microtomography. We found that the amount of porosity first decreases and then increases with increasing intensity of the ASMF. Meanwhile, the shape of the porosity changed from tortuous to elliptic under the ASMF. On the basis of both the experimental and simulated results, the decrease in porosity is attributed to an adequate development of the TEMC leading to sufficient feeding. This study sheds light on an alternative technique for eliminating the shrinkage porosity at the final stage of steel solidification in industrial applications.

36 MATERIALS SCIENCE↗
DOE OSTI2025

Single-Layer Magnet Phase in Intrinsic Magnetic Topological Insulators, [MnTe][Bi 2 Te 3 ] n , Far beyond the Thermodynamic Limit

The intrinsic magnetic topological insulator (IMTI) family [MnTe][Bi 2 Te 3 ]n has demonstrated magneto-topological properties dependent on n, making it a promising platform for advanced electronics and spintronics. However, due to technical barriers in sample synthesis, their properties in the large n limit remain unknown. To overcome this, we utilized the atomic layer-by-layer molecular beam epitaxy (ALL-MBE) technique and achieved IMTIs with n as large as 15, far beyond that previously reported in bulk crystals or thin films. Then, we discover that the “single-layer magnet (SLM)” phase, primarily determined by intralayer ferromagnetic coupling, emerges for n > ∼4 and remains little affected up to n = 15. Nonetheless, still, nonzero, interlayer ferromagnetic coupling is necessary to stabilize the SLM phase, suggesting that the SLM phase eventually disappears in the n → ∞ limit. This study uncovers the secrets of IMTIs beyond the thermodynamic limit and opens a door to diverse magneto-topological applications.

2D ferromagnets↗
DOE OSTI2018

Structure and Magnetism Evolution from FeCo Nanoparticles to Hollow Nanostructure Conversion for Magnetic Applications

Hollow nanostructures have witnessed an increasing interest in emerging fields, including energy storage electrodes, nanocatalysis, photonics, and biomedical carriers, etc. The fundamental mechanisms for hollowing conversion chemistry of complex nanoalloys is indispensable to grow such nanostructures with controlled compositions and functionalities. In this contribution, the Kirkendall effect on magnetic Fe-Co bimetallic alloys with the formation of hollow nanostructures for exchange interactions was studied. The rich diffusion kinetics of binary Fe-Co alloys accompanied with its conversion from solid, core-shell to hollow nanostructures were been captured through X-ray spectroscopy and electron microscopy. We further report the cation exchange improved magnetic performance of hollow nanostructures with increasing the crystallinity.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Static magnetic order with strong quantum fluctuations in spin-1/2 honeycomb magnet Na 2 Co 2 TeO 6

Kitaev interactions, arising from the interplay of frustration and bond anisotropy, can lead to strong quantum fluctuations and, in an ideal case, to a quantum-spin-liquid state. However, in many nonideal materials, spurious non-Kitaev interactions typically promote a zigzag antiferromagnetic order in the d-orbital transition-metal compounds. Here, by combining neutron scattering with muon-spin rotation and relaxation techniques, we provide mechanism insights into the exotic properties of Na 2 Co 2 TeO 6 , a candidate material of the Kitaev model. Below T N , the zero-field muon-spin relaxation rate becomes almost constant (~0.45 μs –1 ). We attribute this temperature-independent relaxation rate to the strong quantum fluctuations, as well as to the frustrated Kitaev interactions. As the magnetic field increases, neutron scattering data indicate a broader spin-wave excitation at the K-point. Therefore, quantum fluctuations seem not only robust but are even enhanced by the applied magnetic field. Our findings provide valuable hints for understanding the onset of the quantum-spin-liquid state in Kitaev materials.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Transient magnetic field diffusion considerations relevant to magnetically assisted indirect drive inertial confinement fusion

We report application of a magnetic field to an indirect drive inertial confinement fusion target requires diffusion of the field through the high-Z and electrically conducting Hohlraum. The onset of the external field generates eddy currents in the Hohlraum wall that result in (1) a reduction of the peak field at the capsule, (2) heating of the Hohlraum wall through Ohmic dissipation, and (3) wall movement due to the inward force from the eddy current interacting with the field. Heating of the wall causes an increase in blackbody radiation which can preheat the capsule and frozen deuterium–tritium fuel, while wall motion leads to potential misalignment of the lasers at the Hohlraum wall. Limiting these detrimental effects sets requirements on the tolerable magnitude of each effect. We present a nonlinear model for B-field diffusion through an infinitely long thin-walled cylinder with a temperature dependent resistivity, to show that a 15 μm thick wall of pure gold fails to meet these requirements. A new Hohlraum material made from an alloy of Au and Ta has a measured resistivity of ≥60 times that of Au and is shown with the nonlinear model to meet the requirements for magnetization. We compare the nonlinear model to simulations of the actual Hohlraum target using a finite element code which includes temperature-dependent Hohlraum resistivity.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Accelerating the magnetic island by the modulated resonant magnetic perturbation for the disruption avoidance on J-TEXT

We report the acceleration of the magnetic island rotation by the modulated resonant magnetic perturbation (MRMP) has been studied in J-TEXT tokamak experiments. After applying the MRMP, the phase difference between the tearing mode (TM) and MRMP, Δξ, oscillated near the effective phase difference, Δξ eff , which was defined as the time averaged value of Δξ. When the Δξ eff was closed to the—π/2, the MRMP only contributed an accelerating torque on the TM. As the result, the TM rotation frequency was increased by a few kilohertz for the optimized relative phase by small RMPs of the order of 10 -5 of the toroidal field and the locked mode induced disruption was avoided. It is found that the TM rotation could be increased to a higher frequency by applying a stronger MRMP. There is a negative sinusoidal relationship between TM frequency and Δξ eff .

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Spatial decomposition of magnetic anisotropy in magnets: Application to doped Fe 16 N 2

We propose a scheme of decomposition of the total relativistic energy in solids to intra- and interatomic contributions. The method is based on a site variation of such fundamental constant as the speed of light. As a practical illustration of the method, we tested such decomposition in the case of a spin-orbit interaction variation for the decomposition of the magnetic anisotropy energy (MAE) in CoPt. We further studied the α" - Fe 16 N 2 magnet doped by Bi, Sb, Co, and Pt atoms. It was found that the addition of Pt atoms can enhance the MAE by as much as five times while Bi and Sb substitutions double the total MAE. Using the proposed technique, we demonstrate the spatial distribution of these enhancements. Our studies also suggest that Sb, Pt, and Co substitutions could be synthesized by experiments.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗