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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 595 records · Page 33
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Temporal dynamics of large-scale structures for turbulent Rayleigh–Bénard convection in a moderate aspect-ratio cylinder

We investigate the spatial organization and temporal dynamics of large-scale, coherent structures in turbulent Rayleigh–Bénard convection via direct numerical simulation of a 6.3 aspect-ratio cylinder with Rayleigh and Prandtl numbers of 9.6×10 7 and 6.7, respectively. Fourier modal decomposition is performed to investigate the structural organization of the coherent turbulent motions by analysing the length scales, time scales and the underlying dynamical processes that are ultimately responsible for the large-scale structure formation and evolution. We observe a high level of rotational symmetry in the large-scale structure in this study and that the structure is well described by the first four azimuthal Fourier modes. Two different large-scale organizations are observed during the duration of the simulation and these patterns are dominated spatially and energetically by azimuthal Fourier modes with frequencies of 2 and 3. Studies of the transition between these two large-scale patterns, radial and vertical variations in the azimuthal energy spectra, as well as the spatial and modal variations in the system's correlation time are conducted. Rotational dynamics are observed for individual Fourier modes and the global structure with strong similarities to the dynamics that have been reported for unit aspect-ratio domains in prior works. It is shown that the large-scale structures have very long correlation time scales, on the order of hundreds to thousands of free-fall time units, and that they are the primary source for a horizontal inhomogeneity within the system that can be observed during a finite, but a very long-time simulation or experiment.

42 ENGINEERING↗
DOE OSTI2026

Multi-diagnostic characterization of laser-produced tin plasmas for EUV lithography

We present a comprehensive characterization of laser-produced tin (Sn) plasmas relevant to extreme ultraviolet (EUV) lithography using a multi-diagnostic suite integrated into the new experimental platform, “SparkLight.” Tin plasmas are generated by irradiating a continuously moving tin-coated wire with laser pulses (1064 nm, 10 ns, up to 5.7 × 10 10 W/cm 2 ) and probed via coherent Thomson scattering, laser interferometry, and EUV emission spectroscopy. Thomson scattering measurements reveal electron temperatures and densities that decay with distance from the target. Densities derived from Thomson scattering are cross-validated against laser interferometry, showing excellent agreement. Correlating the results of these laser diagnostics with spatially resolved EUV spectroscopy suggests that the bulk of useful EUV emission originates within 150 μm of the target and is generated under suboptimal plasma conditions. This work demonstrates a practical integrated approach for plasma characterization in EUV source development.

Musikhin, S. [Princeton Plasma Physics Laboratory ↗
DOE OSTI2024

Alpha particle loss measurements and analysis in JET DT plasmas

Abstract Burning reactor plasmas will be self-heated by fusion born alpha particles from deuterium-tritium reactions. Consequently, a thorough understanding of the confinement and transport of DT-born alpha particles is necessary to maintain the plasma self-heating. Measurements of fast ion losses provide a direct means to monitor alpha particle confinement. JET’s 2021–2022 second experimental DT-campaign offers burning plasma scenarios with advanced fast ion loss diagnostics for the first time in nearly 25 years. Coherent and non-coherent alpha losses were observed due to a variety of low frequency MHD activity. This manuscript will present the loss mechanisms, spatial and pitch dependencies, scalings with plasma parameters, correlations with wall impurities, and magnitude of DT-alpha born losses.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

On-shot, high-intensity laser aberration measurements via ponderomotive electron ejection

We present a technique to assess the spatial aberration content of a focused multi-terawatt laser when fired at full power. This method leverages the direct detection of electrons ponderomotively accelerated from the focal volume formed in a low-pressure gaseous back-fill. Furthermore, our results show that the spatial distribution of emitted electrons exhibits distinct features correlated to the laser aberration type and magnitude. This work represents progress toward the complete and accurate in-situ spatiotemporal characterization of focused high-intensity lasers.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2022

Fast External Quantum Efficiency Measurements of Photovoltaic Modules

The external quantum efficiency (EQE) or associated spectral response is widely used to evaluate the performance of photovoltaics, light emitting diodes, photodetectors, photodiodes, semiconductor lasers, laser-induced refrigeration of solids etc. For photovoltaic (PV) devices, The EQE is used to determine the spectral mismatch correction that is used to convert a performance measurement from a non-ideal simulator spectrum to a standard spectrum in PV device calibrations. Moreover, EQE can provide important insight into the physics of a PV device. For instance, the EQE shape can be used to infer mechanisms limiting the performance of the device. However, EQE measurements of full-size PV modules remain a challenge in the PV community due to rare availability of reliable module QE measurement tools worldwide and the size and complexity of module architecture that comprises several cells connected in strings (series or/and parallel). Here, we use a customized nondestructive tool made of high-power light emitting diodes to perform high-throughput EQE measurements on PV modules. Circuit simulations show that the measurement system can safely be used to measure both crystalline silicon and thin film-based PV modules with series connected cells without the risk of damage through reverse bias. In addition, EQE mapping combined with electroluminescence show a strong correlation and provide a way to determine both spatial non-uniformity of the spectral response and defects/degradation effects across the module.

PV module↗
DOE OSTI2017

Galactos: computing the anisotropic 3-point correlation function for 2 billion galaxies

The nature of dark energy and the complete theory of gravity are two central questions currently facing cosmology. A vital tool for addressing them is the 3-point correlation function (3PCF), which probes deviations from a spatially random distribution of galaxies. However, the 3PCF's formidable computational expense has prevented its application to astronomical surveys comprising millions to billions of galaxies. We present Galactos, a high-performance implementation of a novel, O( N 2 ) algorithm that uses a load-balanced k-d tree and spherical harmonic expansions to compute the anisotropic 3PCF. Our implementation is optimized for the Intel Xeon Phi architecture, exploiting SIMD parallelism, instruction and thread concurrency, and significant L1 and L2 cache reuse, reaching 39% of peak performance on a single node. Galactos scales to the full Cori system, achieving 9.8 PF (peak) and 5.06 PF (sustained) across 9636 nodes, making the 3PCF easily computable for all galaxies in the observable universe.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2024

Imaging Enhanced Simulation Validation for Directed Energy Deposition Additive Manufacturing (Final CRADA Report – NFE-22-09107)

Directed Energy Deposition (DED) is a welding-based metal Additive Manufacturing (AM) process that relies on the programmed rastering of an electric arc or laser induced weld pool to construct a component in a layerwise fashion. The induced complex thermal field and uneven thermal contraction depends on the printed geometry and scan pattern, and as such, accumulated residual stresses and distortions are complex and difficult to predict. Several prior works have resulted in tools to combat this issue; ANSYS has developed a thermoplastic simulation package targeting DED AM, and ORNL has developed an in-situ imaging sensor package ‘Stereo Correlated Optical and Pyrometric System’ (SCOPS) that can spatially monitor temperature and full field strain. In this CRADA, these tools are compared in order to validate the results and complimentarily address the weaknesses in each other.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Agglomerate Sizing in Aluminized Propellants Using Digital Inline Holography and Traditional Diagnostics

Aluminized ammonium perchlorate composite propellants can form large molten agglomerated particles that may result in poor combustion performance, slag accumulation, and increased two-phase flow losses. Quantifying agglomerate size distributions are needed to gain an understanding of agglomeration dynamics and ultimately design new propellants for improved performance. Due to complexities of the reacting multiphase environment, agglomerate size diagnostics are difficult and measurement accuracies are poorly understood. To address this, the current paper compares three agglomerate sizing techniques applied to two propellant formulations. Particle collection on a quench plate and backlit videography are two relatively common techniques, whereas digital inline holography is an emerging alternative for three-dimensional measurements. Atmospheric pressure combustion results show that all three techniques are able to capture the qualitative trends; however, significant differences exist in the quantitative size distributions and mean diameters. For digital inline holography, methods are proposed that combine temporally resolved high-speed recording with lower-speed but higher spatial resolution measurements to correct for size–velocity correlation biases while extending the measurable size dynamic range. Finally, the results from this work provide new guidance for improved agglomerate size measurements along with statistically resolved datasets for validation of agglomerate models.

42 ENGINEERING↗
DOE OSTI2022

Description of historical and future projection simulations by the global coupled E3SMv1.0 model as used in CMIP6

Abstract. This paper documents the experimental setup and general features of the coupled historical and future climate simulations with the first version of the US Department of Energy (DOE) Energy Exascale Earth System Model (E3SMv1.0). The future projected climate characteristics of E3SMv1.0 at the highest emission scenario (SSP5-8.5) designed in the Scenario Model Intercomparison Project (ScenarioMIP) and the SSP5-8.5 greenhouse gas (GHG) only forcing experiment are analyzed with a focus on regional responses of atmosphere, ocean, sea ice, and land. Due to its high equilibrium climate sensitivity (ECS of 5.3 K), E3SMv1.0 is one of the Coupled Model Intercomparison Project phase 6 (CMIP6) models with the largest surface warming by the end of the 21st century under the high-emission SSP5-8.5 scenario. The global mean precipitation change is highly correlated with the global temperature change, while the spatial pattern of the change in runoff is consistent with the precipitation changes. The oceanic mixed layer generally shoals throughout the global ocean. The annual mean Atlantic meridional overturning circulation (AMOC) is overly weak with a slower change from ∼ 11 to ∼ 6 Sv (Sverdrup) relative to other CMIP6 models. The sea ice, especially in the Northern Hemisphere, decreases rapidly with large seasonal variability. We detect a significant polar amplification in E3SMv1.0 from the atmosphere, ocean, and sea ice. Comparing the SSP5-8.5 all-forcing experiment with the GHG-only experiment, we find that the unmasking of the aerosol effects due to the decline of the aerosol loading in the future projection period causes transient accelerated warming in the all-forcing experiment in the first half of the 21st century. While the oceanic climate response is mainly controlled by the GHG forcing, the land runoff response is impacted primarily by forcings other than GHG over certain regions, e.g., southern North America, southern Africa, central Africa, and eastern Asia. However, the importance of the GHG forcing on the land runoff changes grows in the future climate projection period compared to the historical period.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2019

Comparison of fluence-rate determination techniques for the Advanced Test Reactor-Critical Facility

The Advanced Test Reactor (ATR) at the Idaho National Laboratory (INL) is a unique, water-cooled, high-flux test reactor capable of performing tests prototypical of PWR operating conditions. The design and safe operation of experiments in ATR is aided by the operation of the ATR-Critical Facility (ATR-C), a lower-power reactor with the same size and geometry of the ATR. Short, low-power irradiations at the ATR-C are used to study the effects of control devices and test assemblies on the overall power distribution of various core loadings and to compare calculated data for reactor models. A technique was developed at INL to measure fission rates in fuel plate assembly reactors utilizing small, enriched uranium-aluminum (U-Al) alloy monitors, and to support ATR-C irradiations for forty years. Several hundred monitor wires placed throughout the reactor provide fine spatial resolution of the fission rates. A direct correlation exists between the fission rates of the U-Al monitors and the immediately adjacent reactor region. Extensive calibration was previously performed to determine the conversion factor for beta-particle activity of the irradiated U-Al monitors. The fission rate in the U-Al monitors can thus be determined by measuring the beta-particle decay of fission-products following irradiation of the monitors. The American Society for Testing and Materials (ASTM International) has established a standard practice for determining neutron fluence rate by radioactivation of depleted uranium. The ASTM standard practice also measures the concentration of fission-products in the uranium monitors. Rather than measuring the beta-particle decay from fission-products, the decay rate of fission-products is determined by gamma-ray spectroscopy. The feasibility of the ASTM standard practice was investigated for ATR-C irradiations and compared to the present method. The need to analyze hundreds of samples for each irradiation posed several challenges. Therefore, practical considerations such as expected fluence-rates, sample activity, and counting-time were compared between the two methods and the expected sources of error for each method were investigated.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2019

Uncovering the Materials Paradigm for Solar Absorbers Through Insitu Imaging and Characterization

The behavior of solar cells is very often limited by inhomogeneously distributed nanoscale defects. This is the case throughout the entire lifecycle of the solar cell, from the distribution of elements and defects during solar cell growth as well as the charge-collection and recombination during operation, to degradation and failure mechanisms due to impurity diffusion, crack formation, and irradiation- and heat-induced cell damage This has been known for a while in the field of crystalline silicon, but inhomogeneities are far more abundant in polycrystalline materials, and are the limiting factor in thin-film solar cells where grain sizes are often on the order of the diffusion length. We will show that the high penetration of hard X-rays combined with the high sensitivity to elemental distribution, structure, and spatial resolution offers a unique avenue for highly correlative studies at the nanoscale. We will present results on CdTe and Cu(In,Ga)Se2 where carrier collection is directly correlated to the compositional and structural properties of the material under a large variety of synthesis and operating conditions. The segregation of copper at the grain boundaries of both solar absorbers will be discussed in detail as well as the defects impact to carrier collection efficiency. Furthermore, the kinetics of copper segregation during growth and processing will be presented.

Bertoni, Mariana↗
DOE OSTI2019

Uncovering the Materials Paradigm at the Nanoscale: The Role of Next Generation Imaging and Characterization

The behavior of many energy materials and devices is very often limited by inhomogeneously distributed nanoscale defects. This is the case throughout the entire lifecycle of the solar cell, from the distribution of elements and defects during solar cell growth as well as the charge-collection and recombination during operation, to degradation and failure mechanisms due to impurity diffusion, crack formation, and irradiation- and heat-induced cell damage. This has been known for a while in the field of crystalline silicon, but inhomogeneities are far more abundant and smaller in scale for the case of polycrystalline materials. We showed that the high penetration of hard X-rays combined with the high sensitivity to elemental distribution, structure, and spatial resolution offers a unique avenue for highly correlative studies at the nanoscale. We presented results on CdTe and Cu(In,Ga)Se2 where carrier collection is directly correlated to the compositional and structural properties of the material under a large variety of synthesis and operating conditions. The segregation of copper at the grain boundaries of both solar absorbers was discussed in detail as well as the defects impact to carrier collection efficiency. Furthermore, the kinetics of copper segregation during growth and processing was presented and discussed.

Bertoni, Mariana↗
DOE OSTI2021

Multimodal X-ray Microscopy: The Kinetics of Cu in CdTe Absorbers

The behavior of solar cells is very often limited by inhomogeneously distributed nanoscale defects. This is the case throughout the entire lifecycle of the solar cell, from the distribution of elements and defects during solar cell growth as well as the charge-collection and recombination during operation, to degradation and failure mechanisms due to impurity diffusion, crack formation, and irradiation- and heat-induced cell damage This has been known for a while in the field of crystalline silicon, but inhomogeneities are far more abundant in polycrystalline materials, and are the limiting factor in thin-film solar cells where grain sizes are often on the order of the diffusion length. We showed that the high penetration of hard X-rays combined with the high sensitivity to elemental distribution, structure, and spatial resolution offers a unique avenue for highly correlative studies at the nanoscale. We presented results on Cu-doped CdTe, where carrier collection is directly correlated to the kinetics of Cu inside the absorber and the particular Cu-phases at the ZnTe/CdTe interface. We complemented the results with modeling using PVRD-FASP and PyCDTS, where the X-ray beam induced profile can be reproduced by the equilibrium defect concentrations proposed by the solvers.

Bertoni, Mariana↗
DOE OSTI2022

An influence of manufacturing tolerances on Pin-Cell k-infinity of MOX fuel using data from the FUBILA experiment program

An influence of manufacturing tolerances (MTs) was evaluated on the pin-cell k-infinity of MOX fuel through the random sampling of CASMO5 calculations. The data from the FUBILA experiment program was used as the manufacturing parameters. For the uncertainties of element/isotope mass fractions, their covariance matrices were calculated by the generalized least square method. The total k-infinity uncertainty was 120-250 pcm (percent mille). From the breakdown of k-infinity uncertainty per materials, the MTs of fuel pellet had a dominant influence. The individual influences were also evaluated for element/isotope mass fractions, an inner/outer diameter, and a density. Those of element/isotope mass fractions were less than a few dozen pcm. Since the perturbations of fuel pellet diameter and density caused large variations to the total amount of heavy metals and effect of spatial self-shielding, they had a negative correlation with the k-infinity perturbation. On the AG3 (Al-Mg alloy) over-cladding, the inner/outer diameter perturbations had both negative and positive correlations. The negative one was due to decrease in amount of light water and the positive one was due to increase in amount of AG3. Since the effect of neutron slowing-down by light water had a dominant influence, the influence of the former negative correlation was larger than that of the latter positive correlation. It is, therefore, concluded that the consideration of the MTs that had a large influence on the effect of neutron slowing-down is important for precise quantification of the pin-cell k-infinity uncertainty of MOX fuel. (author)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗
DOE OSTI2026

EXCLUSIVE NEUTRAL PION ELECTROPRODUCTION CROSS SECTION MEASUREMENTSWITHANEUTRALPARTICLE SPECTROMETER

Deep Virtual Compton Scattering (DVCS), the exclusive electron-proton scattering process ep ¿e'p'¿, provides access to generalized parton distributions (GPDs), which correlate information about the longitudinal momentum and transverse spatial structure of quarks inside the nucleon. Experiment E12-13-010 in Hall C at Jefferson Lab was designed to take high-precision measurements of the DVCS cross section over an extended kinematic range using the newly commissioned Neutral Particle Spectrometer (NPS). The NPS features a high-resolution electromagnetic calorimeter and a streaming data acquisition system optimized for operation at high luminosities. This thesis presents the detector and analysis work carried out to support the NPS DVCS program. In particular, it focuses on the hardware design, calibration, and performance of the calorimeter. A development of a waveform reconstruction analysis of the calorimeter signals enabled improved extraction of pulse amplitudes and times. The waveform analysis was also extended to operate in a multithreaded environment, substantially reducing processing time for large datasets. Analysis of exclusive neutral pion electroproduction events in the calorimeter gives a strong validation of the calorimeter’s performance and resolution. Together these developments establish a foundation for future analyses and extraction of the DVCS cross section and its use in constraining the GPDs.

Kerver, Mitchell [Old Dominion Univ., Norfolk, VA ↗
DOE OSTI2018

A Modeling Study of Direct and Indirect N 2 O Emissions From a Representative Catchment in the U.S. Corn Belt

Indirect nitrous oxide (N 2 O) emissions from drainage ditches and headwater streams are poorly constrained. Few studies have monitored stream N 2 O emissions and fewer modeling studies have been conducted to simulate stream N 2 O emissions. Here, we determined direct and indirect N 2 O emission modules and a corresponding calibration module for use in the Soil and Water Assessment Tool (SWAT) model, and implemented the expanded SWAT model (termed SWAT-N 2 O) to a representative fourth-stream-order catchment (210 km 2 ) and six first-order stream catchments (0.22–1.83 km 2 ) in southeastern Minnesota. We simulated the spatial and temporal fluctuations of the indirect emissions from streams, identified emission “hot spots” and “hot moments,” and diagnosed the correlations between direct and indirect emissions. We demonstrated that zero-order streams and first-order streams could contribute 0.034–0.066 and 0.011 nmol N 2 O m –2 s –1 (expressed on the basis of unit catchment area) to the total surface emissions, respectively. Emissions from zero-order and first-order streams equal 24–41% of direct emissions from soil, which may explain the emission gap between calculations using top-down and bottom-up methods. Clear spatial patterns were identified for both direct and indirect emissions and their spatial variations were negatively correlated. Our results indicate that the IPCC N 2 O emission factor for streams in the Corn Belt should be increased by 3.2–5.7 times. Increasing precipitation and streamflow in the Corn Belt may potentially increase frequencies of soil anoxic conditions and nitrate leaching to streams, and subsequently increase N 2 O emissions from both soils and streams.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Implications of increased spatial and trophic overlap between juvenile Pacific salmon and Sablefish in the northern California Current

Abstract Objective The study was designed to assess long-term variability in the distribution of juvenile Pacific salmon Oncorhynchus spp. and Sablefish Anoplopoma fimbria. The study also evaluated whether Sablefish and Pacific salmon shared food resources and looked to characterize Sablefish during an understudied period of their life cycle. Methods To meet the objectives, the study used data from 26 years of surface trawls conducted in Oregon and Washington coastal waters (1998–2023). Spatial–temporal models were used to measure changes in abundance and distribution of Pacific salmon and Sablefish along with covariates of ocean temperature. The study evaluated trophic characteristics of Pacific salmon and Sablefish from 2020 for differences. The temporal variation in size and diets of Sablefish were also analyzed, along with energy density of fish caught in 2020. Result The spatial–temporal model demonstrated that there has been a nearshore expansion of juvenile Sablefish over the past 26 years that was correlated with increased ocean temperature. The nearshore expansion of Sablefish resulted in increased spatial and trophic overlap with juvenile Pacific salmon. While feeding in nearshore waters, juvenile Sablefish demonstrated competitive feeding advantages over juvenile Pacific salmon during a critical phase of salmonid early marine life history. Juvenile Sablefish exhibited significant ontogenetic diet and energetic shifts, and even the smallest (68–80 mm fork length) were piscivorous. Conclusions If juvenile Sablefish numbers continue to increase relative to Pacific salmon, they could exert more competitive pressure, especially if food resources become limited. Pacific salmon may experience adverse effects from competition, regardless of whether or not juvenile Sablefish, which have recently expanded into nearshore waters, successfully recruit to the adult population.

Daly, Elizabeth A. (ORCID:0000000195334457)↗
DOE OSTI2020

Correlation Function Approach for Diffusion in Confined Geometries

This paper describes a formalism for extracting spatially varying transport coefficients from simulations of a molecular fluid in a nano channel. This approach is applied to self-diffusion of a Lennard-Jones fluid confined between two parallel surfaces. A numerical grid is laid over the domain confining the fluid, and fluid properties are projected onto the grid cells. The time correlation functions between properties in different grid cells are calculated and can be used as the basis for a fitting procedure for extracting spatially varying diffusion coefficients from the simulation. Results for the Lennard-Jones system show that transport behavior varies sharply near the liquid-solid boundary and that the changes depend on the details of the liquid-solid interaction. A quantitative difference between the reduced and detailed models is discussed. It is found that the difference could be associated with assumptions about the form of the transport equations at molecular scales in lieu of problems with the method itself. The study suggests that this approach to fitting molecular simulations to continuum equations may guide the development of appropriate coarse-grained equations to model transport phenomena at nanometer scales.

Nanoscale flow, Transport, molecular simulation↗