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NASA NTRS1985

Spectroscopic measurements of atmospheric HCN at northern and southern latitudes

A number of lines belonging to the nu(3) fundamental vibration-rotation band of hydrogen cyanide (HCN) have been identified in atmospheric infrared absorption spectra obtained on high-altitude balloon flights at 32 deg N in 1976 and at 30 deg S in 1977. Quantitative analysis of these spectral features has resulted in the first determination of atmospheric HCN concentrations in the Southern Hemisphere, as well as an independent estimate of stratospheric HCN abundance in the Northern Hemisphere. Within the uncertainties of the present and previous measurements, the Northern Hemisphere result is consistent with those of other investigators, and Southern Hemisphere HCN concentrations appear to be similar to those in the Northern Hemisphere.

Smith, M. A. H.↗

NASA NTRS1978

Feasibility of an orbital simulator of stratospheric photochemistry

It is proposed that a stratospheric photochemistry simulator could be created in sun-synchronous orbit, so that diffusion and photochemistry could be decoupled and uncertainties in photochemical reaction rates could be substantially reduced. The proposed test chamber is described, and it is suggested that the technology of superpressure balloons seems to be the best short-term solution to the construction of the proposed facility. Both unreinforced polyester films and gelatin films are considered as candidate chamber coatings. It is noted that the experiments can be performed early in the space-manufacturing era and that at least three dedicated Shuttle launches will be required to establish the proposed facility.

Matloff, G. L.↗

NASA NTRS1991

On the wave forcing of the semi-annual zonal wind oscillation

Observational evidence of rather large period waves (23-60 d) in the troposphere/stratosphere, particularly during the winter months, is presented. Wind data collected on a regular basis employing high-altitude balloons and meteorological rockets over the past few years are used. Maximum entropy methods applied to the time series of zonal wind data indicate the presence of 23-60-waves more prominently than shorter-period waves. The waves have substantial amplitudes in the stratosphere and lower mesosphere, often larger than those noted in the troposphere. The mean zonal wind in the troposphere (5-15 km altitude) during December, January, and February exhibits the presence of strong westerlies at latitudes between 8 and 21 deg N.

Nagpal, O. P.↗

NASA NTRSDate not supplied

Analog Environments for Venus Aerosol Instrument and Mission Concept Testing

The most common hypothesis discussed for life on Venus is a habitat in the dense, persistent clouds, which are primarily sulfuric acid with a secondary water component. Although Earth lacks a complete Venus analog environment, several partial analogs exist which can inform our understanding of the requirements for cloud habitability as well as serving as potential testbeds for future Venus instruments or missions. Earth’s tropospheric clouds have larger particles, more water, and shorter lifetimes than Venus’s; however, they have a partial overlap in pressure and temperature, and are our only example of an airborne habitat.They can inform how particle residence time and microbial generation time constrain habitable atmospheric regions. On the biological side, this includes available nutrients and energy, environmental stressors such as radiation, osmotic potential and acidity, and time spent in protective but inactive forms (endospores, cysts, akinetes); on the physical side, gravity, air density and viscosity, thermal lofting, gravity waves, scavenging due to precipitation, and other airflow dynamics, as well as effective particle radius and electrical charge. They can also enable sampling strategy tests for airborne life detection, ranging from10 2 to10 8 viable cells/mL (10 -3 to 10 -9 cells/particle). Conversely, Earth's stratospheric sulfate layer lacks an active microbial presence, and is at a colder and less dense altitude but has partially analogous values in terms of H2SO4 and water concentration, particle size, and number density. These aerosols are accessible to aircraft and high-altitude balloons. Even more accessible potential analogs include sea spray, which overlaps with the smaller (haze) particle sizes and densities at Venus and contains trace organic constituents; marine fog, which at higher densities can match Venus’s larger (Mode 2) particle properties and contains a range of trace compounds including ammonia, phosphates, sulfates, and nitrates; and spray from acidic hydrothermal systems, which can cover a wide variety of sizes, densities, and chemical compositions. These analogs could improve the development of Venus cloud sampling instruments or sondes, including field tests of material compatibility, particle capture efficiency, and analysis sensitivity.

Analog↗

NASA NTRSDate not supplied

Formation of Tropopause Cirrus clouds by Typhoon-induced gravity waves during the Asian Summer Monsoon: A Case Study from the BATAL 2017 Campaign

Cirrus clouds in the Tropical Tropopause Layer (TTL) have a net warming impact on Earth’s climate and they regulate the amount of water vapor entering the lower stratosphere through dehydration process near the cold-point tropopause. During the Boreal summer, Asian Summer Monsoon (ASM) is an important source of cirrus clouds and humidity in the TTL owing to frequent deep convection. However, better representation of convection and TTL cirrus clouds in global climate models is needed for accurate assessment of their response to changing climate. In this study, we investigate the mechanisms involved in the formation of a tropopause cirrus cloud layer observed during the Balloon measurement campaigns of the Asian Tropopause Aerosol Layer (BATAL) over Hyderabad (17.47 °N, 78.58 °E), India on 23 August 2017. A subvisible cirrus cloud layer (optical thickness ~0.025) was detected by a backscatter sonde (COBALD) onboard a balloon near the cold-point tropopause (CPT, temperature~ -86.4 ° C, altitude~17.9 km) which was later confirmed by the CATS lidar on the ISS. Simultaneous measurements from an optical particle counter (Boulder Counter) revealed the presence of ice crystals smaller than 50 microns in this layer. The formation mechanism responsible for this tropopause cirrus is investigated using a technique combining three-dimensional back-trajectories, satellite observations, and ERA5 reanalysis data. Satellite observations revealed that the overshooting convection associated with a category-3 typhoon Hato, which hit Macau and Hong Kong on 23 August 2017 injected ice into the lower stratosphere. This caused a hydration patch that followed the ASM anticyclone subsequently moving towards Hyderabad. The presence of tropopause cirrus cloud layers in the cold temperature anomalies and updrafts along the back-trajectories indicated towards the role of typhoon-induced gravity waves in their formation. This case study highlights the role of typhoons in influencing the formation of tropopause cirrus clouds through stratospheric hydration and gravity waves in the ASM anticyclone.

Amit Kumar Pandit↗

NASA NTRS2001

Tunable Far Infrared Studies in Support of Stratospheric Measurements

This report summarizes research done under NASA Grant NAG5-4653. The research performed under this grant has been a collaboration between institutions including the Smithsonian Astrophysical Observatory, the National Institute of Standards and Technology, the University of Oregon, and the NASA Langley Research Center. The program has included fully line-resolved measurements of submillimeter and far infrared spectroscopic line parameters (pressure broadening coefficients and their temperature dependences, and line positions) for the analysis of field measurements of stratospheric constituents, far infrared database improvements, and studies for improved satellite measurements of the Earth's atmosphere. This research program is designed to enable the full utilization of spectra obtained in far infrared/submillimeter field measurements, such as FIRS-2, FILOS, IBEX, SLS, EosMLS, and proposed European Space Agency measurements of OH (e.g., PIRAMHYD and SFINX) for the retrieval of accurate stratospheric altitude profiles of key trace gases involved in ozone layer photochemistry. For the analysis of the spectra obtained in the stratosphere from far infrared measurements it is necessary to have accurate values of the molecular parameters (line positions, strengths, and pressure broadening coefficients) for the measured molecules and for possible interfering species. Knowledge of line positions is in increasingly good shape, with some notable exceptions. The increase in position information includes research that has been performed in the present program of research on HO2, H2O, H2O2, O3, HCl, HF, HBr, HI, CO, OH, and ClO. Examples where further line position studies are necessary include hot band and minor isotopomer lines of some of the major trace species (H2O, O3) and normal lines of some triatomic and larger molecules (NO2). Knowledge of strengths is in generally good shape, since most of the lines are from electric dipole transitions whose intensities are well determined from Stark effect measurements; exceptions include some molecules with large vibration-rotation interactions (NO2) and internal motions (H2O2 above the lowest torsional state). The line parameters that are still the least well determined are pressure broadening coefficients, and their temperature coefficients, These are strongly dependent on the quantum states involved in the transitions, in a way that is much more complex than the simple projection by directional cosine matrix elements involved in determination of rotational line strengths from static dipole moments. The following molecules have now been measured or detected in the atmosphere using far infrared and millimeter-wave emission spectroscopy from balloon- and satellite-borne spectrometers: OH, HO2, H2O (including minor isotopomers and hot band lines), H2O2, O3P, O2 (including minor isotopomers), O3 (including minor isotopomers and hot band lines), HOCl, HCl, HF, HBr, CIO, CO, CO2, N2O, NO2, N2O5, HNO3, ClNO3, and HCN. Many of these species have spectral lines that are saturated in stratospheric spectra. In these cases, the measured line equivalent widths are proportional to (line strength x Lorentz width) (exp 1/2) so that the pressure broadening coefficients are as important as the line intensities in determining concentration profiles. Interpretation of field measurements for these species have required ongoing measurement programs of pressure broadening measurements. Other species (HO2, HGCl, H2O2, HBr, and NO2, as examples) have required further line position studies in order to fully analyze the field measurements.

Chance, Kelly V.↗

NASA NTRS1981

Comparisons of global ozone trends inferred from the BUV experiment on Nimbus 4 and the ground-based network

Preliminary comparisons between global ozone burdens derived from the backscattered ultraviolet (BUV) experiment on Nimbus 4 and those inferred from an analysis of ground-based network data seem to indicate significant differences in the inter-annual variability of ozone. Some of the observed differences may be due to improper weighting of the ground-based network data, slowly changing planetary wave structure over the fixed station, of small inter-annual changes in meridional transport parameters. There is also some evidence which indicates that the polar stratosphere at high latitudes may represent an important ozone storage resevoir which tends to compensate for large scale changes observed in the regions outside of the polar stratosphere. Possible consequences of this are that the global trends derived from ground based ozone measurements may not be valid and furthermore that the current satellite techniques by themselves may be sufficient. An ozone monitoring system which includes observations from satellites, ground-based stations, balloons and rockets may be necessary.

Heath, D. F.↗

NASA NTRS1987

SAGE II aerosol extinction and scattering data from balloon-borne photography

Earth limb radiance and extinction near sunset have been observed from a balloon-borne gondola nearly simultaneously and on air masses close to those probed by the SAGE II instrumentation on April 22, 1985. The results show the importance of accuracy of the altitude determination on the aerosol measurements. They indicate an important altitude dependence of the stratospheric aerosol granulometry in agreement with SAGE II results.

Ackerman, M.↗

NASA NTRS1984

Estimation of vertical diffusion from observations of Atmospheric turbulence layers, part 4.4B

There have been numerous studies addressing the turbulent diffusion in the stratosphere and mesosphere during the last two decades. The motivation for such studies was the need for an understanding of the thermal and constituent structure of the middle atmosphere. Observational estimates of the horizontal and/or vertical diffusion were obtained using chemical release, rocket vapor trail, aircraft, balloon, and radar techniques. During the same period, a number of theoretical studies were performed to infer the level of vertical diffusion needed to account for observed constituent profiles. There appears to be a discrepancy between the level of vertical diffusion required for the dissipation of gravity wave and tidal motions on the one hand and for the maintenance of observed temperature and constituent profiles on the other. A possible explanation of this discrepancy is outlined. Measurements that may help verify this explanation are suggested.

Fritts, D. C.↗

NASA NTRS1984

Unusual structures of high-latitude stratospheric electric fields

A possible explanation is given for three unusual stratospheric electric field structures reported by Madsen et al. (1983). It is suggested that stratospheric vertical electric-current structures may arise as extensions into the stratosphere of tropospheric currents generated by convective charge transport. A convective tropospheric current generator is presented which is capable of producing, at altitudes of about 30 km, the vertical electric field intensities of several volts per meter that are sometimes (although very rarely) observed by balloon-borne sensors (Madsen et al., 1983).

Dangelo, N.↗

NASA NTRS2014

Total Volcanic Stratospheric Aerosol Optical Depths and Implications for Global Climate Change

Understanding the cooling effect of recent volcanoes is of particular interest in the context of the post-2000 slowing of the rate of global warming. Satellite observations of aerosol optical depth above 15 km have demonstrated that small-magnitude volcanic eruptions substantially perturb incoming solar radiation. Here we use lidar, Aerosol Robotic Network, and balloon-borne observations to provide evidence that currently available satellite databases neglect substantial amounts of volcanic aerosol between the tropopause and 15 km at middle to high latitudes and therefore underestimate total radiative forcing resulting from the recent eruptions. Incorporating these estimates into a simple climate model, we determine the global volcanic aerosol forcing since 2000 to be 0.19 +/- 0.09W/sq m. This translates into an estimated global cooling of 0.05 to 0.12 C. We conclude that recent volcanic events are responsible for more post-2000 cooling than is implied by satellite databases that neglect volcanic aerosol effects below 15 km.

aerosols↗

NASA NTRS1999

The Goddard Three Dimensional Chemistry and Transport Model-A Waystation on the Road to Predicting the Future of Stratospheric Ozone

The Goddard 3D Chemistry and Transport Model (CTM) is an off-line model which includes a full description of stratospheric photochemistry and calculates constituent transport using winds and temperatures from the Goddard Earth Observing System Data Assimilation System. The model can be used to understand and quantify the photochemical and transport processes which produce observed constituent evolution and variability. Data from any platform - ground based, aircraft, balloon, satellite - can play a role. Since any measurement systems has its own set of advantages and disadvantages (e.g., good temporal sampling but poor spatial sampling; good spatial and temporal sampling but poor vertical resolution; high vertical resolution and spatial sampling but poor temporal sampling), using data from disparate sources and a CTM can provide a more complete picture of atmospheric processes.

Douglass, Anne↗

NASA NTRS2007

Validation of the Aura Microwave Limb Sounder middle atmosphere water vapor and nitrous oxide measurements

The quality of the version 2.2 (v2.2) middle atmosphere water vapor and nitrous oxide measurements from the Microwave Limb Sounder (MLS) on the Earth Observing System (EOS) Aura satellite is assessed. The impacts of the various sources of systematic error are estimated by a comprehensive set of retrieval simulations. Comparisons with correlative data sets from ground-based, balloon and satellite platforms operating in the UV/visible, infrared and microwave regions of the spectrum are performed. Precision estimates are also validated, and recommendations are given on the data usage. The v2.2 H2O data have been improved over v1.5 by providing higher vertical resolution in the lower stratosphere and better precision above the stratopause. The single-profile precision is ~0.2–0.3 ppmv (4–9%), and the vertical resolution is ~3–4 km in the stratosphere. The precision and vertical resolution become worse with increasing height above the stratopause. Over the pressure range 0.1–0.01 hPa the precision degrades from 0.4 to 1.1 ppmv (6–34%), and the vertical resolution degrades to ~12–16 km. The accuracy is estimated to be 0.2–0.5 ppmv (4–11%) for the pressure range 68–0.01 hPa. The scientifically useful range of the H2O data is from 316 to 0.002 hPa, although only the 82–0.002 hPa pressure range is validated here. Substantial improvement has been achieved in the v2.2 N2O data over v1.5 by reducing a significant low bias in the stratosphere and eliminating unrealistically high biased mixing ratios in the polar regions. The single-profile precision is ~13–25 ppbv (7–38%), the vertical resolution is ~4–6 km and the accuracy is estimated to be 3–70 ppbv (9–25%) for the pressure range 100–4.6 hPa. The scientifically useful range of the N2O data is from 100 to 1 hPa.

Atlas, E.↗

NASA NTRS2014

10 meter Sub-Orbital Large Balloon Reflector (LBR)

The realization of a large, space-based 10 meter class telescope for far-infrared/THz studies has long been a goal of NASA. Such a telescope could study the origins of stars, planets, molecular clouds, and galaxies; providing a much needed means of following-up on tantalizing results from recent successful missions such as Spitzer, Herschel, and SOFIA. Indeed, Herschel began its life in the US space program as the Large Deployable Reflector (LDR) to be assembled in low Earth orbit by shuttle astronauts. Escalating costs and smaller federal budget allocations resulted in a downsizing of the mission. However, by combining successful suborbital balloon and ground-based telescope technologies, the dream of a 10 meter class telescope free of ~99% of the Earth's atmospheric absorption in the far-infrared can be realized. The same telescope can also be used to perform sensitive, high spectral and spatial resolution limb sounding studies of the Earth's atmosphere in greenhouse gases such as CO, ClO, O3, and water, as well as serve as a high flying hub for any number of telecommunications and surveillance activities. Flight times of 100+ days will be possible, with instruments having mass and power requirements in excess of ~500 kg and ~1 kW.Here we present the results of our NIAC Step 1, Phase B design study where each key aspect of the LBR concept is discussed and recommendations made for further study in Phase II.These aspects include realization of a large spherical reflecting surface, spherical corrector, pointing system, instrument module, and service module/gondola. Once each hardware component is introduced, a typical LBR Mission profile is described that enables the realization of a stratospheric 10 meter THz observatory and limb sounder. Verification of the design approach was achieved by using a combination of analytical modelling, lab testing of materials and techniques, and building a 3 meter rooftop LBR prototype.

Telescope↗

NASA NTRS1984

Validation of nitrogen dioxide results measured by the limb infrared monitor of the stratosphere (LIMS) experiment on NIMBUS 7

The validation of results from the nitrogen dioxide channel and the quality of the data are examined in connection with the LIMS experiment which ran from late October 1978 to late May 1979. Factors studied include: channel characteristics, experiment errors due to instrument and spacecraft effects, predicted and measured precision, predicted accuracy, and comparisons with correlative measurements made in a series of balloon underflights. Features such as profile shape and slope of the mixing ratio altitude distribution are in good agreement. The LIMS data also fall within the range of previous mixing ratio measurements and are consistent with model estimates. The calculated on-orbit precision is about 0.3 ppbv and the estimated accuracy from simulations is about 2 ppbv over the 3-10-mbar range. Accuracy is less at higher and lower pressure levels. These results provide the first day-night set of nitrogen dioxide measurements from space.

Russell, J. M., III↗

NASA NTRS2001

Inorganic Chlorine Partitioning in the Summer Lower Stratosphere: Modeled and Measured [ClONO2/HCl] During POLARIS

We examine inorganic chlorine (Cly) partitioning in the summer lower stratosphere using in situ ER-2 aircraft observations made during the Photochemistry of Ozone Loss in the Arctic Region in Summer (POLARIS) campaign. New steady state and numerical models estimate [ClONO2]/[HCl] using currently accepted photochemistry. These models are tightly constrained by observations with OH (parameterized as a function of solar zenith angle) substituting for modeled HO2 chemistry. We find that inorganic chlorine photochemistry alone overestimates observed [ClONO2]/[HCl] by approximately 55-60% at mid and high latitudes. On the basis of POLARIS studies of the inorganic chlorine budget, [ClO]/[ClONO2], and an intercomparison with balloon observations, the most direct explanation for the model-measurement discrepancy in Cly partitioning is an error in the reactions, rate constants, and measured species concentrations linking HCl and ClO (simulated [ClO]/[HCl] too high) in combination with a possible systematic error in the ER-2 ClONO2 measurement (too low). The high precision of our simulation (+/-15% 1-sigma for [ClONO2]/[HCl], which is compared with observations) increases confidence in the observations, photolysis calculations, and laboratory rate constants. These results, along with other findings, should lead to improvements in both the accuracy and precision of stratospheric photochemical models.

Voss, P. B.↗

NASA NTRS1978

Upper atmosphere research satellite program

A satellite program to conduct research on the chemistry, energetics, and dynamics of the upper atmosphere was developed. The scientific goals of the Upper Atmospheric Research Program, the program requirements, and the approach toward meeting those requirements are outlined. An initial series of two overlapping spacecraft missions is described. Both spacecraft are launched and recovered by the STS, one in the winter of 1983 at a 56 deg inclination, and the other a year later at a 70 deg inclination. The duration of each mission is 18 months, and each carries instruments to make global measurements of the temperature, winds, composition, irradation, and radiance in the stratosphere, mesosphere, and lower thermosphere between the tropopause and 120 km altitude. The program requires a dedicated ground-based data system and a science team organization that leads to a strong interaction between the experiments and theory. The program includes supportive observations from other platforms such as rockets, balloons, and the Spacelab.

Huntress, W. T., Jr.↗

NASA NTRS2004

Radicals and Reservoirs in the GMI Chemistry and Transport Model: Comparison to Measurements

The most important use of atmospheric chemistry and transport models is to predict the future composition of the atmosphere. The amounts of gases like chlorofluorcarbons, methyl bromide, nitrous oxide and methane are changing and the stratospheric ozone layer will change because these gases are changing. Methyl bromide, nitrous oxide and methane all have natural sources, and also change because of human activity. Chlorofluorcarbons are man-made gases; these are known to decrease stratospheric ozone and future production is banned. They are long-lived gases, and many decades will pass before they are insignificant in the atmosphere. The models are used to predict changes in ozone and other gases; this is a straightforward application. The models must be also tested using observations for the present day atmosphere. This is a challenging task, because the model contains more than 50 species and more than 150 chemical reactions. Data from satellites, ground stations, aircraft and balloons are used to evaluate the model. Different models that are used in international assessments produce different results; in the most recent assessment some predict that ozone will return to 1980 levels by 2025 and others predict that this will not happen until 2050. Since all the parts of the models are conceptually the same, there must be differences in implementation that produce these differences, This work takes a single model, two different sets of winds and temperatures, and repeats the same prediction for the future. Here we compare the results for these two simulations with many observations. The purpose is to identify differences in the model results for the present atmosphere that will lead to different predictions. This sort of controlled comparison will reduce uncertainty in the predictions for stratospheric ozone.

Douglas, Anne R.↗