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DOE OSTI2020

Covariant density functional theory input for r-process simulations in actinides and superheavy nuclei: The ground state and fission properties

A systematic investigation of the ground-state and fission properties of even-even actinides and superheavy nuclei with Z = 90–120 from the two-proton up to two-neutron drip lines with proper assessment of systematic theoretical uncertainties has been performed for the first time in the framework of covariant density functional theory (CDFT). Furthermore, these results provide a necessary theoretical input for the r-process modeling in heavy nuclei and, in particular, for the study of fission cycling. Four state-of-the-art globally tested covariant energy density functionals (CEDFs), namely, DD-PC1, DD-ME2, NL3*, and PC-PK1, representing the major classes of the CDFT models are employed in the present paper. Ground-state deformations, binding energies, two-neutron separation energies, α-decay Q α values and half-lives, and the heights of fission barriers have been calculated for all these nuclei. Theoretical uncertainties in these physical observables and their evolution as a function of proton and neutron numbers have been quantified and their major sources have been identified. Spherical shell closures at Z = 120, N = 184, and N = 258 and the structure of the single-particle (especially, high-j) states in their vicinities as well as nuclear matter properties of employed CEDFs are two major factors contributing to theoretical uncertainties. However, different physical observables are affected in a different way by these two factors. For example, theoretical uncertainties in calculated ground-state deformations are affected mostly by the former factor, while theoretical uncertainties in fission barriers depend on both of these factors.

190 ≤ A ≤ 219↗

DOE OSTI2017

New excitations in Ba 142 and Ce 144 : Evolution of γ bands in the N = 86 isotones

New excited states in 142 Ba and 144 Ce are investigated by means of prompt γ-ray spectroscopy of the radiation following spontaneous fission of 252 Cf. Measurements of angular correlations and the observed branchings allowed the assignment of spins and parities with confidence. The new measurements are reinforced by shell-model calculations where energy levels, electric transitions, and magnetic moments are consistent with experimental data. Lastly, the presence of collectivity in the N = 86 isotones is confirmed by clear signatures of soft triaxial γ bands in both nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2020

Vadose Zone Model for B Complex for Composite Analysis

The objectives of the vadose modeling for the updated Hanford Site composite analysis (CA) are to simulate the flow and transport of water and radionuclide releases from the surface to the water table and to provide radionuclide transfer rates for the plateau to river (P2R) model, version 8.3. Water additions include natural recharge and water discharged to the ground as a result of industrial processes associated with Hanford Site operations. Contaminant sources include radionuclides in water discharged to the ground during operations and radionuclides disposed “dry” in solid waste burial grounds or other means. The simulation time starts in 1943 and ends at 12070, which is 10,000 years after assumed Hanford Site closure in 2070. The scope of this ECF is to document the development and results of the B Complex vadose zone model. The B Complex model encompasses the region around single-shell tank farms 241-B, 241-BX, and 241-BY, and adjacent cribs, trenches, and burial grounds in the northwestern part of the 200 East Area. Sources of waste to this area were primarily from B Plant (221-B) and U Plant (221-U).

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2021

Coexisting normal and intruder configurations in 32 Mg

Situated in the so-called “island of inversion,” the nucleus 32 Mg is considered as an archetypal example of the disappearance of magicity at N = 20. We report on high statistics in-beam spectroscopy of 32 Mg with a unique approach, in that two direct reaction probes with different sensitivities to the underlying nuclear structure are employed at the same time. More specifically, states in 32 Mg were populated by knockout reactions starting from 33 Mg and 34 Si, lying inside and outside the island of inversion, respectively. The momentum distributions of the reaction residues and the cross sections leading to the individual final states were confronted with eikonal-based reaction calculations, yielding a significantly updated level scheme for 32 Mg and spin-parity assignments. By fully exploiting observables obtained in this measurement, a variety of structures coexisting in 32 Mg was unraveled. Comparisons with theoretical predictions based on shell-model overlaps allowed for clear discrimination between different structural models, revealing that the complete theoretical description of this key nucleus is yet to be achieved.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2016

Investigation of Fission Product Interaction with the SiC Containment Layer of High Turnup TRISO Fuel Particles

Tri-structural Isotropic (TRISO) encapsulated fuel particles are used in high-temperature gas-cooled nuclear reactors. Fuel performance is limited by the propensity of metallic fission products to be released under high temperature testing to simulate hypothesized accident scenarios. The current particle design consists of a 350 μm or 425 μm UO{sub 2} or UCO fuel kernel surrounded by a 100μm porous carbon buffer layer, a 40μm inner pyrolytic carbon (IPyC) layer, a 35μm high-density silicon carbide (SiC) layer, and a 40μm outer pyrolytic carbon (OPyC) layer. Of interest is the fission product interaction with the SiC layer, which provides the most structural support and is the main barrier to the diffusion of fission products. Previous laboratory examination studies have indicated the release of Ag through seemingly intact particles and the localized corrosion of the SiC due to Pd. Although a number of studies have been conducted, the specifics of both the Ag and Pd reaction mechanisms, in addition to U and Pu, through SiC are currently not well understood. This work aims to understand the pathways and kinetics of these interactions under normal operation as well as accident conditions. In order to improve our understanding of this, we have the unique opportunity to examine irradiated TRISO particles to study post-irradiation effects on these materials. Experimental data is necessary to constrain the current models used to predict the behavior of fission products in the SiC layer of TRISO fuels. This work aims to understand the interaction of fission products with the SiC containment layer in TRISO particles. We have systematically examined three SiC shells from irradiated TRISO particles using XAFS, TEM, and EDS. Results indicate the formation of palladium silicides, and uranium and plutonium carbides. Additionally, silver is seen to be metallic. Preliminary microscopy results indicate fission products throughout the SiC layer of the TRISO particles, and microstructural changes have been observed between the as-irradiated and safety tested particles. These results have provided key information on the fission product transport behavior through irradiated SiC at varying temperatures. Knowledge of these reaction pathways will allow for better simulation of the long-term behavior of TRISO fuels. They may also suggest ways to modify the SiC layer to improve fuel performance and mitigate fission product release, which is critical for safety strategies required to commercialize these nuclear fuel technologies. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

DOE OSTI2018

Validity of the distorted-wave impulse-approximation description of Ca 40 ( e , e ' p ) K 39 data using only ingredients from a nonlocal dispersive optical model

The nonlocal implementation of the dispersive optical model (DOM) provides all the ingredients for distorted-wave impulse-approximation (DWIA) calculations of the (e,e'p) reaction. It provides both the overlap function, including its normalization, and the outgoing proton distorted wave. This framework is applied to describe the knockout of a proton from the 0d3/2 and 1s1/2 orbitals in 40 Ca with fixed normalizations of 0.71 and 0.60, respectively. Data were obtained in parallel kinematics for three outgoing proton energies: 70, 100, and 135 MeV. Agreement with the data is as good as, or better than, previous descriptions employing local optical potentials and overlap functions from Woods-Saxon potentials—both with standard nonlocality corrections—whose normalization (spectroscopic factor) and radius were fitted to the data. The present analysis suggests that slightly larger spectroscopic factors are obtained when nonlocal optical potentials are employed than those generated with local potentials. The results further suggest that the chosen kinematical window around 100 MeV proton energy provides the best and cleanest method to employ the DWIA for the analysis of this reaction. The conclusion that substantial ground-state correlations cannot be ignored when describing a closed-shell atomic nucleus is therefore confirmed in detail. To reach these conclusions, it is essential to have a complete description of the nucleon single-particle propagator that accounts for all elastic nucleon-scattering observables in a wide energy domain up to 200 MeV. Lastly, the current nonlocal implementation of the DOM fulfills this requirement.

39 ≤ A ≤ 58↗

DOE OSTI2022

Proton decay spectroscopy of S 28 and Cl 30

States in 28 S and 30 Cl have been studied using one- and two-proton decay spectroscopy. In the first spectrometer setting, states in 28 S were populated following one-neutron knockout from a fast 29 S beam. Three new states are observed in 28 S from one- and two-proton decay. For the two-proton case the nature of the decay was investigated and found to proceed via sequential two-proton emission. For the second setting, states in 30 Cl were populated via one-proton knockout from a fast 31 Ar beam. The decay energy of the ground and first excited state were measured, with the ground-state decay energy found to be in disagreement with a previous measurement. Here, the spin and parity of these two 30 Cl states were inferred from shell-model calculations.

20 ≤ A ≤ 38↗

DOE OSTI2023

Semimicroscopic description of isoscalar giant multipole resonances in medium-mass closed-shell nuclei

Main properties of isoscalar giant multipole resonances (up to L=3), including L=0,and 2 overtones, in medium-mass closed-shell nuclei are described within the semimicroscopic particle-hole dispersive optical model. Further, main properties are characterized by the energy-averaged strength distribution, projected (one-body) transition density, and probabilities of direct one-nucleon decay. Calculation results obtained for characteristics of the mentioned resonances in the 48 Ca, 90 Zr, and 132 Sn nuclei are compared with available experimental data.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

NASA NTRS1994

The radio emission from the ultraluminous far-infrared galaxy NGC 6240

We present new radio observations of the 'prototypical' ultraluminous far-infrared galaxy NGC 6240, obtained using the Very Large Array (VLA) at lambda = 20 cm in B-configuration and at lambda = 3.6 cm in A-configuration. These data, along with those from four previous VLA observations, are used to perform a comprehensive study of the radio emission from NGC 6240. Approximately 70% (approximately 3 x 10(exp 23) W/Hz) of the total radio power at 20 cm originates from the nuclear region (approximately less than 1.5 kpc), of which half is emitted by two unresolved (R approximately less than 36 pc) cores and half by a diffuse component. The radio spectrum of the nuclear emission is relatively flat (alpha approximately equals 0.6; S(sub nu) proportional to nu(exp -alpha). The supernova rate required to power the diffuse component is consistent with that predicted by the stellar evolution models of Rieke et al. (1985). If the radio emission from the two compact cores is powered by supernova remnants, then either the remnants overlap and form hot bubbles in the cores, or they are very young (approximately less than 100 yr.) Nearly all of the remaining 30% of the total radio power comes from an 'armlike' region extending westward from the nuclear region. The western arm emission has a steep spectrum (alpha approximately equals 1.0), suggestive of aging effects from synchrotron or inverse-Compton losses, and is not correlated with starlight; we suggest that it is synchrotron emission from a shell of material driven by a galactic superwind. Inverse Compton scattering of far-infrared photons in the radio sources is expected to produce an X-ray flux of approximately 2 - 6 x 10(exp -14) ergs/s/sq cm in the 2 - 10 keV band. No significant radio emission is detected from or near the possible ultramassive 'dark core'.

Colbert, Edward J. M.↗

DOE OSTI2019

$β^-$ decay of $T_z$ = +$\frac{11}{2}$ isotopes $\mathrm{^{37}Al}$ and $\mathrm{^{39}Si}$: Understanding Gamow-Teller strength distribution in neutron-rich nuclei

$β^-$ decay of $T_z$ = +$\frac{11}{2}$ nuclei $\mathrm{^{37}Al}$ and $\mathrm{^{39}Si}$ was studied to obtain information about excited states in the daughter and granddaughter nuclei. New information on excited states has been obtained for $\mathrm{^{37,39}P}$ whereas level schemes for $\mathrm{^{37}Si}$ and $\mathrm{^{37,39}S}$ were confirmed and expanded on as compared to the most recent investigations. For the nuclei studied, the valence proton and neutron occupy different major shells with opposite parities, hence, the $β^-$ decay preferentially and primarily populates core-excited $1p1h$ intruder states with a parity opposite to the ground state of the daughter nucleus. These low-lying intruder states shed light on the $N = 20$ shell gap and its evolution with neutron number. The $β^-$ decay of very neutron-rich nuclei also illustrates how the Gamow-Teller (GT) strength distribution changes with neutron excess. Comparing $β^-$ decay of $\mathrm{^{37,39}Si}$ presented here with $\mathrm{^{38,40}Si}$ from a previous study, we clearly see an even-odd effect in the GT strength distribution with the decay from even-even nuclei showing strong low-lying strength whereas for the odd $A$ being very fragmented. Finally, configuration interaction shell-model calculations with the state-of-art SDPFSDG-MU effective interaction were performed to understand the structure of the $1p1h$ states and explore the GT strength distribution.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2017

Experimental study of the β decay of the very neutron-rich nucleus Ge 85

The β -decay properties of the very neutron-rich nucleus 85 Ge, produced in the proton-induced fission of 238 U, were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. The level scheme of 33 85 As 52 populated in 85 Geβ γ decay was reconstructed and compared to shell-model calculations. The investigation of the systematics of low-energy levels in N =52 isotones together with shell-model analysis allowed us to provide an estimate of the low-energy structure of the more exotic N =52 isotone 81 Cu.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

DOE OSTI2016

Allowance for the tunnel effect in the entrance channel of fusion–fission reactions

A two-stage model is developed in order to describe fusion–fission reactions. The process in the course of which colliding ions approach each other is simulated at the first stage, the deformations and relative orientations of the ions being taken into account. The first stage of the calculation is completed as soon as colliding nuclei touch each other. A continuous nuclear system (monosystem) is formed at this instant. The emerging distributions of the angular momenta of this system and of its potential and internal energies at the point of touching are used as input data that are necessary for triggering the second stage of the calculation. The evolution of collective coordinates that describe the shape of the monosystem is calculated at the second stage. The description of this evolution is terminated either at the instant of its fission or upon the release of a major part of its excess energy via particle and photon emission. In the latter case, the probability for the fission of the monosystem or a further decrease in its excitation energy becomes extremely small. The ion-collision process and the evolution of the monosystem formed after primary nuclei come into contact are simulated on the basis of stochastic Langevin equations. The quantities appearing in them (which include the potential energy and inertial and friction parameters) are determined with allowance for the shell structure of nuclei. The tunneling of colliding nuclei through the Coulomb barrier is taken into account, and the effect of this phenomenon on model predictions is studied.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2020

Revealing 3D Morphological and Chemical Evolution Mechanisms of Metals in Molten Salt by Multimodal Microscopy

Growing interest in molten salts as effective high-temperature heat-transfer fluids for sustainable energy systems drives a critical need to fundamentally understand the interactions between metals and molten salts. This work utilizes the multimodal microscopy methods of synchrotron X-ray nanotomography and electron microscopy to investigate the 3D morphological and chemical evolution of two-model systems, pure nickel metal and Ni-20Cr binary alloy, in a representative molten salt (KCl-MgCl2 50–50 mol %, 800 °C). In both systems, unexpected shell-like structures formed because of the presence of more noble tungsten, suggesting a potential route of using Ni–W alloys for enhanced molten-salt corrosion resistance. The binary alloy Ni-20Cr developed a bicontinuous porous structure, reassembling functional porous metals manufactured by dealloying. This work elucidates better mechanistic understanding of corrosion in molten salts, which can contribute to the design of more reliable alloys for molten salt applications including next-generation nuclear and solar power plants and opens the possibility of using molten salts to fabricate functional porous materials.

36 MATERIALS SCIENCE↗

DOE OSTI2024

Berkeley Lab Finite Element Framework (BELFEM) v0.1

The software program, referred to as BELFEM, is a specialized finite element code designed for the magnetodynamic modeling of high-temperature superconducting (HTS) tapes. It incorporates novel mixed finite element formulations, particularly the h-ϕ-formulation with thin-shell simplification, to efficiently simulate larger geometries. This methodology is extremely promising for predicting the electrodynamic performance of HTS tapes used in superconducting cables and magnets, offering the benefit of reduced computational cost. Compared to similar technologies like COMSOL Multiphysics and GetDP, BELFEM's performance benchmarking indicates superior efficiency in its thin-shell implementation. In the future, it will also support features like thermal coupling and inter-tape current sharing, enhancing its utility in research and development, particularly in nuclear fusion applications. The intent is to develop BELFEM as a robust and efficient tool for the HTS community, contributing to the analysis and design of superconducting cables and magnets.

Messe, Christian↗

DOE OSTI2024

Hydrodynamical Simulations of Proton Ingestion Flashes in Type I X-Ray Bursts

We perform the first multidimensional fluid simulations of thermonuclear helium ignition underneath a hydrogen-rich shell. This situation is relevant to Type I X-ray bursts on neutron stars that accrete from a hydrogen-rich companion. Using the low-Mach number fluid code MAESTROeX, we investigate the growth of the convection zone due to nuclear burning, and the evolution of the chemical abundances in the atmosphere of the star. We also examine the convective boundary mixing processes that cause the evolution to differ significantly from previous one-dimensional simulations that rely on mixing-length theory. We find that the convection zone grows outward as penetrating fluid elements cool the overlying radiative layer, rather than directly from the increasing entropy of the convection zone itself. Simultaneously, these flows efficiently mix composition, carrying carbon out of and protons into the convection zone even before contact with the hydrogen shell. We discuss the implications of these effects for future modeling of these events and observations.

astrophysical fluid dynamics↗

DOE OSTI2026

Collapse of Nuclear Collectivity along the 𝑁 = 𝑍 Line

The lifetime of the 𝐽 𝜋 = 2 + state in the self-conjugate 88 Ru nucleus has been determined in an experiment performed using rare-isotope beams provided by the new Facility for Rare Isotope Beams. This is the heaviest 𝑁 = 𝑍 nucleus for which such a measurement has been achieved. 88 Ru was populated by both one-neutron knockout and charge-exchange reactions, and the lifetime of 14.3$^{+2.5}_{−3.4}$ ps was determined using the triple-foil plunger technique. The extracted electromagnetic transition strength shows that the quadrupole collectivity has dropped significantly compared with the highly deformed 𝑁 = 𝑍 region around 𝐴 ∼ 80. These results are compared with state-of-the-art large-scale shell-model and discrete nonorthogonal shell-model calculations. The theoretical calculations indicate a moderate triaxial deformation and suggest that low-lying states in this nucleus are no longer dominated by strong many-particle many-hole excitations, unlike the lighter, highly deformed 𝑁 = 𝑍 nuclei nearby.

59 ≤ A ≤ 89↗

NASA NTRS1981

A model for dwarf novae as progenitors of Type I supernovae

It is suggested that a Type I supernova event can be produced as a result of accretion at low rates (less than 10 to the -10th solar mass/year) onto the white dwarf component of a dwarf-nova close binary. At these low rates, diffusion of the CNO nuclei out of the accreted hydrogen envelope can occur on the accretion time scale, and nuclear burning will occur mainly by the proton-proton chain. Studies of this process show that, when the CNO abundance in the envelope is less than 0.0025 of solar, no thermonuclear flash occurs and no mass is lost. The result of the evolution is a gradually increasing layer of helium beneath the hydrogen-burning shell.

Starrfield, S.↗

DOE OSTI2019

Possible evidence of nonstatistical properties in the Cl 35 ( n , p ) S 35 cross section

In this work, the Cl 35 ( n , p ) and Cl 35 ( n , α ) cross sections at incident neutron energies between 2.42 and 2.74 MeV were measured using the Berkeley High Flux Neutron Generator. The cross sections for Cl 35 ( n , p ) were more than a factor of 3 to 5 less than all of the values in the neutron absorption data libraries, while the Cl 35 ( n , α ) cross sections are in reasonable agreement with the data libraries. Furthermore, the measured energy-differential cross section is consistent with a single resonance with a width of 293(46) keV. This finding indicates that, despite the high incident neutron energy, any attempt to model ($n, x$) cross sections in the vicinity of the $N = Z$ = 20 shell gap requires a resolved resonance approach rather than a Hauser-Feshbach approach.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗