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At least 613 records · Page 34

Primary and secondary ice production: interactions and their relative importance

A discrepancy of up to 5 orders of magnitude between ice crystal and ice nucleating particle (INP) number concentrations was found in the measurements, indicating the potentially important role of secondary ice production (SIP) in the clouds. However, the interactions between primary and SIP processes and their relative importance remain unexplored. In this study, we implemented five different ice nucleation schemes as well as physical representations of SIP processes (i.e., droplet shattering during rain freezing, ice-ice collisional break-up, and rime splintering) in the Community Earth System Model version 2 (CESM2). We ran CESM2 in the single column mode for model comparisons with the DOE Atmospheric Radiation Measurement (ARM) Mixed-Phase Arctic Cloud Experiment (M-PACE) observations. We found that the model experiments with aerosol-aware ice nucleation schemes and SIP processes yield the best simulation results for the M-PACE single-layer mixed-phase clouds. We further investigated the relative importance of ice nucleation and SIP to ice number and cloud phase as well as interactions between ice nucleation and SIP in the M-PACE single-layer mixed-phase clouds. Our results show that SIP contributes 80 % to the total ice formation and transforms ~30 % of pure liquid-phase clouds simulated in the model experiments without considering SIP into mixed-phase clouds. The SIP is not only a result of ice crystals produced from ice nucleation, but also competes with the ice nucleation by reducing the number concentrations of cloud droplets and cloud-borne dust INPs. Conversely, strong ice nucleation also suppresses SIP by glaciating mixed-phase clouds and thereby reducing the amount of precipitation particles (rain and graupel).

54 ENVIRONMENTAL SCIENCES↗

Characterizing the Small-Scale Dynamical, Ice Microphysical, and Residual Aerosol Properties of Mid-Latitude Cold Clouds: A Pilot Study (Final Report)

Our understanding of cirrus clouds has been advancing rapidly due to improvements in measurements made inside clouds, computer cloud models, and laboratory experimentation. This advancement in knowledge has made it clear that cirrus are complicated systems where the intricate interactions among dynamic air motions, solar and terrestrial radiation, ice crystal growth, and water and air chemistry can substantially influence cirrus structure and evolution. Measurements made inside clouds have shown that cirrus crystals are often complex with shapes that are often unclassifiable, especially at small sizes. Laboratory measurements have revealed that the ice crystal surface is complex, even at small sizes. Recent laboratory and satellite studies show that this surface complexity modifies the radiative properties of cirrus clouds in important ways. Moreover, observations and computer cloud modeling work show that the larger and smaller scale properties of cirrus are sensitive to the interplay between small-scale air motions and the aerosol articles upon which cirrus ice crystals form. Taken together, these studies indicate that accurately accounting for the radiative properties of cirrus clouds requires knowing the air motions and aerosol properties that influence the number concentration and crystal size, along with an understanding of the surface properties of vapor grown ice. Although this prior work has been illuminating, there have been few studies that provide detailed shape and surface complexity measurements for the small ice crystals that often compose cirrus clouds.

54 ENVIRONMENTAL SCIENCES↗

Updates on Modeling the Water Cycle with the NASA Ames Mars Global Climate Model

Global Circulation Models (GCMs) have made steady progress in simulating the current Mars water cycle. It is now widely recognized that clouds are a critical component that can significantly affect the nature of the simulated water cycle. Two processes in particular are key to implementing clouds in a GCM: the microphysical processes of formation and dissipation, and their radiative effects on heating/ cooling rates. Together, these processes alter the thermal structure, change the dynamics, and regulate inter-hemispheric transport. We have made considerable progress representing these processes in the NASA Ames GCM, particularly in the presence of radiatively active water ice clouds. We present the current state of our group's water cycle modeling efforts, show results from selected simulations, highlight some of the issues, and discuss avenues for further investigation.­

Global Circulation Models (GCMs)↗

A Global Modeling Study on Carbonaceous Aerosol Microphysical Characteristics and Radiative Effects

Recently, attention has been drawn towards black carbon aerosols as a short-term climate warming mitigation candidate. However the global and regional impacts of the direct, indirect and semi-direct aerosol effects are highly uncertain, due to the complex nature of aerosol evolution and the way that mixed, aged aerosols interact with clouds and radiation. A detailed aerosol microphysical scheme, MATRIX, embedded within the GISS climate model is used in this study to present a quantitative assessment of the impact of microphysical processes involving black carbon, such as emission size distributions and optical properties on aerosol cloud activation and radiative effects. Our best estimate for net direct and indirect aerosol radiative flux change between 1750 and 2000 is -0.56 W/m2. However, the direct and indirect aerosol effects are quite sensitive to the black and organic carbon size distribution and consequential mixing state. The net radiative flux change can vary between -0.32 to -0.75 W/m2 depending on these carbonaceous particle properties at emission. Taking into account internally mixed black carbon particles let us simulate correct aerosol absorption. Absorption of black carbon aerosols is amplified by sulfate and nitrate coatings and, even more strongly, by organic coatings. Black carbon mitigation scenarios generally showed reduced radiative fluxeswhen sources with a large proportion of black carbon, such as diesel, are reduced; however reducing sources with a larger organic carbon component as well, such as bio-fuels, does not necessarily lead to a reduction in positive radiative flux.

Bauer, S. E.↗

High-resolution photography of clouds from the surface: Retrieval of optical depth of thin clouds down to centimeter scales: High-Resolution Photography of Clouds

This article describes the approach and presents initial results, for a period of several minutes in north central Oklahoma, of an examination of clouds by high resolution digital photography from the surface looking vertically upward. A commercially available camera having 35-mm equivalent focal length up to 1200 mm (nominal resolution as fine as 6 µrad, which corresponds to 9 mm for cloud height 1.5 km) is used to obtain a measure of zenith radiance of a 30 m × 30 m domain as a two-dimensional image consisting of 3456 × 3456 pixels (12 million pixels). Downwelling zenith radiance varies substantially within single images and between successive images obtained at 4-s intervals. Variation in zenith radiance found on scales down to about 10 cm is attributed to variation in cloud optical depth (COD). Attention here is directed primarily to optically thin clouds, COD less than about 2. A radiation transfer model used to relate downwelling zenith radiance to COD and to relate the counts in the camera image to zenith radiance, permits determination of COD on a pixel-by-pixel basis. COD for thin clouds determined in this way exhibits considerable variation, for example, an order of magnitude within 15 m, a factor of 2 within 4 m, and 25% (0.12 to 0.15) over 14 cm. In conclusion, this approach, which examines cloud structure on scales 3 to 5 orders of magnitude finer than satellite products, opens new avenues for examination of cloud structure and evolution.

54 ENVIRONMENTAL SCIENCES↗

A Two-Habit Ice Cloud Optical Property Parameterization for GCM Application

We present a novel ice cloud optical property parameterization based on a two-habit ice cloud model that has been proved to be optimal for remote sensing applications. The two-habit ice model is developed with state-of-the-art numerical methods for light scattering property calculations involving individual columns and column aggregates with the habit fractions constrained by in-situ measurements from various field campaigns. Band-averaged bulk ice cloud optical properties including the single-scattering albedo, the mass extinction/absorption coefficients, and the asymmetry factor are parameterized as functions of the effective particle diameter for the spectral bands involved in the broadband radiative transfer models. Compared with other parameterization schemes, the two-habit scheme generally has lower asymmetry factor values (around 0.75 at the visible wavelengths). The two-habit parameterization scheme was widely tested with the broadband radiative transfer models (i.e. Rapid Radiative Transfer Model, GCM version) and global circulation models (GCMs, i.e. Community Atmosphere Model, version 5). Global ice cloud radiative effects at the top of the atmosphere are also analyzed from the GCM simulation using the two-habit parameterization scheme in comparison with CERES satellite observations.

Yi, Bingqi↗

Data management and scientific integration within the Atmospheric Radiation Measurement Program

The Atmospheric Radiation Measurement (ARM) Program has been developed by the U.S. Department of Energy with the goal to improve the predictive capabilities of General Circulation Models (GCM's) in their treatment of clouds and radiative transfer effects. To achieve this goal, three experimental testbeds were designed for the deployment of instruments that will collect atmospheric data used to drive the GCM's. Each site, known as a Cloud and Radiation Testbed (CART), consists of a highly available, redundant data system for the collection of data from a variety of instrumentation. The first CART site was deployed in April 1992 in the Southern Great Plains (SGP), Lamont, Oklahoma, with the other two sites to follow in September 1995 in the Tropical Western Pacific and in 1997 on the North Slope of Alaska. Approximately 400 MB of data are transferred per day via the Internet from the SGP site to the ARM Experiment Center at Pacific Northwest Laboratory in Richland, Washington. The Experiment Center is central to the ARM data path and provides for the collection, processing, analysis, and delivery of ARM data. Data are received from the CART sites from a variety of instrumentation, observational systems, amd external data sources. The Experiment Center processes these data streams on a continuous basis to provide derived data products to the ARM Science Team in near real-time while providing a three-month running archive of data. A primary requirement of the ARM Program is to preserve and protect all data produced or acquired. This function is performed at Oak Ridge National Laboratory where leading edge technology is employed for the long-term storage of ARM data. The ARM Archive provides access to data for participation outside of the ARM Program. The ARM Program involves a collaborative effort by teams from various DOE National Laboratories, providing multi-disciplinary areas of expertise. This paper will discuss the collaborative methods in which the ARM teams translate the scientific goals of the Program into data products. By combining atmospheric scientists, systems engineers, and software engineers, the ARM Program has successfully designed and developed an environment where advances in understanding the parameterizations of GCM's can be made.

Gracio, Deborah K.↗

The Influence of the Photoionizing Radiation Spectrum on Metal-Line Ratios in Ly(alpha) Forest Clouds

Recent measurements of Si IV/C IV ratios in the high-redshift Ly(alpha) forest (Songaila & Cowie, AJ, 112, 335 (1996a); Savaglio et at., A&A (in press) (1997)) have opened a new window on chemical enrichment and the first generations of stars. However, the derivation of accurate Si/C abundances requires reliable ionization corrections, which are strongly dependent on the spectral shape of the metagalactic ionizing background and on the 'local effects' of hot stars in nearby galaxies. Recent models have assumed power-law quasar ionizing backgrounds plus a decrement at 4 Ryd to account for He II attenuation in intervening clouds. However, we show that realistic ionizing backgrounds based on cosmological radiative transfer models produce more complex ionizing spectra between 1-5 Ryd that are critical to interpreting ions of Si and C. We also make a preliminary investigation of the effects of He II ionization front nonoverlap. Because the attenuation and reemission by intervening clouds enhance Si IV relative to C the observed high Si IV/C IV ratios do not require an unrealistic Si overproduction (Si/C greater than or equal to 3 (Si/C)(solar mass)). If the ionizing spectrum is dominated by 'local effects' from massive stars, even larger Si IV/C IV ratios are possible. However, unless stellar radiation dominates quasars by more than a factor of 10, we confirm the evidence for some Si overproduction by massive stars; values Si/C approx. 2(Si/C)(solar mass) fit the measurements better than solar abundances. Ultimately, an adequate interpretation of the ratios of C IV, Si IV, and C II may require hot, collisionally ionized gas in a multiphase medium.

Giroux, Mark L.↗

Resolving Low Cloud Feedbacks Globally With E3SM High‐Res MMF: Agreement With LES but Stronger Shortwave Effects

This study investigates low cloud feedback in a warmer climate using global simulations from the High-Resolution Multi-scale Modeling Framework (HR-MMF), which explicitly simulates small-scale eddies globally. Two 5-year simulations—one with present-day sea surface temperatures (SSTs) and a second with SSTs warmed uniformly by 4 K—reveal a positive global shortwave cloud radiative effect (SWCRE = 0.3 W/m 2 /K), comparable to estimates from CMIP models. As the climate warms, significant reductions in low cloud cover occur over stratocumulus regions. This study is the first attempt to compare HR-MMF results with predictions from idealized large-eddy simulations from the CGILS intercomparison. Despite different underlying assumptions, we find qualitative agreement in SWCRE and inversion height changes between HR-MMF and CGILS predictions. This suggests reasonable credibility for the CGILS framework in predicting cloud responses under the out-of-sample conditions found in HR-MMF. However, the HR-MMF exhibits stronger SWCRE changes than predicted by CGILS. We explore potential causes for this discrepancy, examining variations in cloud-controlling factors (CCFs) and cloud conditions. Our results show a fairly homogeneous SWCRE response, with little systematic variation tied to the variations in CCFs. This reveals a dominant role for SST forcing in modulating SWCRE.

boundary-layer clouds↗

Using Microwave Limb Sounder Data to Validate Model Ice Fields

MLS IWC overall tends to be higher relative to ECMWF after considering MLS track sampling and sensitivity (cutoff application). Disagreement tends to be accentuated over Indian and Western Pacific Oceans and over tropical landmasses. Large disagreement occur at upper level at 147 hPa but small at lower levels at 215 and 316 hPa suggesting the need to investigate the strength of model large-scale circulation and physics associated with the IWC formation. Future work includes: Present MMF/ECMWF Comparisons at AGU/Baltimore Session on MMF/Cloud Resolving Modeling, GMAO/GSFC & at the WPac/Bejing/AGU in Tao's Cloud-Radiation Session. Write-up Results on ECMWF/MLS Comparisons for GRL. Continue with MLS vs ECMWF Water Vapor & Temperature comparisons - will seek more interaction with other MLS colleagues. Investigate the Development of Biases in ECMWF Forecasts - i.e. in the actual model. Work with GMAO-5 development team regarding their cloud microphysics performance. Integrate CloudSat into IWC Analyses.

cloud ice↗

Clouds enhance Greenland ice sheet meltwater runoff

The Greenland ice sheet has become one of the main contributors to global sea level rise, predominantly through increased meltwater runoff. The main drivers of Greenland ice sheet runoff, however, remain poorly understood. Here we show that clouds enhance meltwater runoff by about one-third relative to clear skies, using a unique combination of active satellite observations, climate model data and snow model simulations. This impact results from a cloud radiative effect of 29.5 (±5.2)Wm -2 . Contrary to conventional wisdom, however, the Greenland ice sheet responds to this energy through a new pathway by which clouds reduce meltwater refreezing as opposed to increasing surface melt directly, thereby accelerating bare-ice exposure and enhancing meltwater runoff. The high sensitivity of the Greenland ice sheet to both ice-only and liquid-bearing clouds highlights the need for accurate cloud representations in climate models, to better predict future contributions of the Greenland ice sheet to global sea level rise.

54 ENVIRONMENTAL SCIENCES↗

Drivers of the Low-Cloud Response to Poleward Jet Shifts in the North Pacific in Observations and Models

The long-standing expectation that poleward shifts of the midlatitude jet under global warming will lead to poleward shifts of clouds and a positive radiative feedback on the climate system has been shown to be misguided by several recent studies. On interannual time scales, free-tropospheric clouds are observed to shift along with the jet, but low clouds increase across a broad expanse of the North Pacific Ocean basin, resulting in negligible changes in total cloud fraction and top-of-atmosphere radiation. Here it is shown that this low-cloud response is consistent across eight independent satellite-derived cloud products. Using multiple linear regression, it is demonstrated that the spatial pattern and magnitude of the low-cloud-coverage response is primarily driven by anomalous surface temperature advection. In the eastern North Pacific, anomalous cold advection by anomalous northerly surface winds enhances sensible and latent heat fluxes from the ocean into the boundary layer, resulting in large increases in low-cloud coverage. Local increases in low-level stability make a smaller contribution to this low-cloud increase. Despite closely capturing the observed response of large-scale meteorology to jet shifts, global climate models largely fail to capture the observed response of clouds and radiation to interannual jet shifts because they systematically underestimate how sensitive low clouds are to surface temperature advection, and to a lesser extent, low-level stability. More realistic model simulations of cloud–radiation–jet interactions require that parameterizations more accurately capture the sensitivity of low clouds to surface temperature advection.

54 ENVIRONMENTAL SCIENCES↗

Spatial Distribution of Large Cloud Drops

By analyzing aircraft measurements of individual drop sizes in clouds, we have shown in a companion paper (Knyazikhin et al., 2004) that the probability of finding a drop of radius r at a linear scale l decreases as l(sup D(r)) where 0 less than or equal to D(r) less than or equal to 1. This paper shows striking examples of the spatial distribution of large cloud drops using models that simulate the observed power laws. In contrast to currently used models that assume homogeneity and therefore a Poisson distribution of cloud drops, these models show strong drop clustering, the more so the larger the drops. The degree of clustering is determined by the observed exponents D(r). The strong clustering of large drops arises naturally from the observed power-law statistics. This clustering has vital consequences for rain physics explaining how rain can form so fast. It also helps explain why remotely sensed cloud drop size is generally biased and why clouds absorb more sunlight than conventional radiative transfer models predict.

Marshak, A.↗

Radiative Heating Profiles over Ascension Island during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between cloud morphology and the environmental conditions in which marine boundary layer clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean, where it is likely that the absorbing and heating properties of these aerosols modify the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to observe thermodynamic, cloud and aerosol properties during two consecutive biomass burning seasons from July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). These observations in conjunction with radiation transfer modeling were used to assess the impact of biomass burning carbonaceous aerosol plumes as they passed over the site.Thermodynamic profiles were generated using a combination of radiosonde data and thermodynamic profilers to provide high temporal resolution profiles of quantities that are important for cloud development, such as CAPE and CIN. Coincident Ka-band radar and lidar profiles were used to characterize the cloud and sub-cloud structure. The resulting thermodynamic and cloud profiles are used as input forcing for the Rapid Radiative Transfer Model (RRTM) to compute radiative heating profiles over the observation site. Idealized experiments using RRTM, with and without aerosols present, are used to assess the impacts of the absorbing aerosol on the heating rate profiles.

Cumulus↗

The winter central Arctic surface energy budget: A model evaluation using observations from the MOSAiC campaign

This study evaluates the simulation of wintertime (15 October, 2019, to 15 March, 2020) statistics of the central Arctic near-surface atmosphere and surface energy budget observed during the MOSAiC campaign with short-term forecasts from 7 state-of-the-art operational and experimental forecast systems. Five of these systems are fully coupled ocean-sea ice-atmosphere models. Forecast systems need to simultaneously simulate the impact of radiative effects, turbulence, and precipitation processes on the surface energy budget and near-surface atmospheric conditions in order to produce useful forecasts of the Arctic system. This study focuses on processes unique to the Arctic, such as, the representation of liquid-bearing clouds at cold temperatures and the representation of a persistent stable boundary layer. It is found that contemporary models still struggle to maintain liquid water in clouds at cold temperatures. Given the simple balance between net longwave radiation, sensible heat flux, and conductive ground flux in the wintertime Arctic surface energy balance, a bias in one of these components manifests as a compensating bias in other terms. This study highlights the different manifestations of model bias and the potential implications on other terms. Three general types of challenges are found within the models evaluated: representing the radiative impact of clouds, representing the interaction of atmospheric heat fluxes with sub-surface fluxes (i.e., snow and ice properties), and representing the relationship between stability and turbulent heat fluxes.

54 ENVIRONMENTAL SCIENCES↗

How Well are Recent Climate Variability Signals Resolved by Satellite Radiative Flux Estimates?

One notable aspect of Earth s climate is that although the planet appears to be very close to radiative balance at top-of-atmosphere (TOA), the atmosphere itself and underlying surface are not. Profound exchanges of energy between the atmosphere and oceans, land and cryosphere occur over a range of time scales. Recent evidence from broadband satellite measurements suggests that even these TOA fluxes contain some detectable variations. Our ability to measure and reconstruct radiative fluxes at the surface and at the top of atmosphere is improving rapidly. Understanding the character of radiative flux estimates and relating them to variations in other energy fluxes and climate state variables is key to improving our understanding of climate. In this work we will evaluate several recently released estimates of radiative fluxes, focusing primarily on surface estimates. The International Satellite Cloud Climatology Project FD radiative flux profiles are available from rnid-1983 to near present and have been constructed by driving the radiative transfer physics from the Goddard Institute for Space Studies (GISS) global model with ISCCP clouds and HlRS operational soundings profiles. Full and clear sky SW and LW fluxes are produced. A similar product from the NASA/GEWEX Surface Radiation Budget Project using different radiative flux codes and thermodynamics from the NASA/Goddard Earth Observing System assimilation model makes a similar calculation of surface fluxes. However this data set currently extends only through 1995. Several estimates of downward LW flux at the surface inferred from microwave data are also examined. Since these products have been evaluated with Baseline Surface Radiation Network data over land we focus over ocean regions and use the DOE/NOAA/NASA Shipboard Ocean Atmospheric Radiation (SOAR) surface flux measurements to characterize performance of these data sets under both clear and cloudy conditions. Some aspects of performance are stratified according to SST and vertical motion regimes. Comparisons to the TRMM/CERES SRB data in 1998 are also interpreted. These radiative fluxes are then analyzed to determine how surface (and TOA) radiative exchanges respond to interannual signals of ENS0 warm and cold events. Our analysis includes regional changes as well as integrated signals over land, ocean and various latitude bands. Changes in water vapor and cloud forcing signatures are prominent on interannual time scales. Prominent signals are also found in the SW fluxes for the Pinatubo volcanic event. These systematic changes in fluxes are related to changes in large-scale circulations and energy transport in the atmosphere and ocean. Some estimates of signal-to-noise and reliability are discussed to place our results in context.

Robertson, Franklin R.↗

Can Biomass Burning Aerosol Induced Surface Cooling Be Amplified Through Sea Surface Temperature‐Cloud Feedback Over the Southeast Atlantic?

Biomass burning (BB) aerosols exert a strong surface cooling effect over the southeast Atlantic (SEA) via aerosol-radiation and aerosol-cloud interactions. The reduction of the sea surface temperature (SST) can trigger the SST-low cloud feedback. Whether this feedback can amplify the surface cooling effect is examined. The modeling results from the Community Earth System Model version 2 (CESM2) demonstrate that counterintuitively the cloud radiative effect (CRE) caused by the BB aerosols is weaker if SST-low cloud feedback is considered compared to fixed-SST simulation (-2.99 W m -2 vs. -4.79 W m -2 ). This is caused by (a) stronger sea breeze due to larger sea-land temperature contrast causing less smoke transport over SEA and (b) less moisture supply from surface due to colder SST. Changes in SST also lead to counterclockwise rotation of ocean circulation anomalies. Consequently, the excess heat transport from the equator reverses the direction of SST-cloud feedback in this region.

0305↗

Cloud/climate sensitivity experiments

A study of the relationships between large-scale cloud fields and large scale circulation patterns is presented. The basic tool is a multi-level numerical model comprising conservation equations for temperature, water vapor and cloud water and appropriate parameterizations for evaporation, condensation, precipitation and radiative feedbacks. Incorporating an equation for cloud water in a large-scale model is somewhat novel and allows the formation and advection of clouds to be treated explicitly. The model is run on a two-dimensional, vertical-horizontal grid with constant winds. It is shown that cloud cover increases with decreased eddy vertical velocity, decreased horizontal advection, decreased atmospheric temperature, increased surface temperature, and decreased precipitation efficiency. The cloud field is found to be well correlated with the relative humidity field except at the highest levels. When radiative feedbacks are incorporated and the temperature increased by increasing CO2 content, cloud amounts decrease at upper-levels or equivalently cloud top height falls. This reduces the temperature response, especially at upper levels, compared with an experiment in which cloud cover is fixed.

Roads, J. O.↗