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Electric field effect on lattice dynamics of a relaxor ferroelectric PMN-30PT measured on ARCS.

The combined inelastic neutron scattering data from ARCS for poled PMN-30PT single crystal is at 300K and for unpoled crystal the data were collected at 300K and at 488K. The incident neutron energy for both poled and unpoled crystals was 25 meV . To obtain a significant four-dimensional Q-E volume, the crystal was rotated with steps of 0.5 degree in the beam. All individual angles were combined using HORACE software package (https://pace-neutrons.github.io/Horace/unstable/user_guide/Getting_started.html) to generate these sqw files. The file labeled PMN_PT_poled_new.sqw is for poled crystal and files labeled PMN_PT_300K.sqw and PMN_PT_488K.sqw are for unpoled crystal at 300K and 488K respectively.

MATERIALS SCIENCE↗

Theoretical Studies of Polar Systems near Ferroelectrics Quantum Critical Points (Final Report)

The PI has studied emergent quantum phases near polar quantum critical points. A first challenge was to develop a theoretical description of the observation that many polar materials undergo classical first-order transitions while displaying quantum criticality. The possibility of novel metallic states near polar quantum critical points was then studied; identification and characterization of a non-Fermi liquid phase was made in a multiband system. In dilute quantum critical polar metals, electronic coupling to polar energy fluctuations was shown to result in attractive electron-electron interactions and to superconductivity. A spin-phonon resonance measurement in applied magnetic field was proposed to determine the magnitude of spin-orbit mediated electron-phonon coupling; furthermore in the polar phase new field-induced phonon collective modes were identified with specific signatures for experiment. In order to keep current, the PI has also worked on other types of strongly correlated problems. With experimental groups, she has developed phenomenologies to identify and explain observed dynamical critical behaviors. The PI has studied the interplay of topology, fractionalization and deconfinement in a minimalist spin model. An emergent phase transition in a 1 + 1 frustrated spin nanotube has also been identified and characterized. The PI has also begun exploring criticality out of equilibrium, characterizing rich dynamical phases associated with photoinduced polar transitions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗