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At least 613 records · Page 34

Topological and magnetic properties of a noncollinear spin state on a honeycomb lattice in a magnetic field

Here, this paper studies the topological and magnetic properties of a noncollinear spin state on a honeycomb lattice that evolves from coplanar to ferromagnetic with a magnetic field applied along the z axis. The coplanar state is stabilized by nearest-neighbor ferromagnetic interactions, single-ion anisotropy along z, and DzyaloshinskiiMoriya interactions between next-nearest-neighbor sites. Below the critical field H$_c$ that aligns the spins, the magnetic unit cell contains six sites and the spin dynamics contains six magnon modes. Although the classical energy is degenerate with respect to the twist angle φ between nearest-neighbor spins, the dependence of the free energy on φ at low temperatures is dominated by the magnon zero-point energy, which contains extremum at φ = πl/3 for integer l. The only unique ground states GS(φ) have l = 0 or 1. For H < H$'_c$, the zero-point energy has minima at even l and the ground state is GS(0); for H$'_c$ < H < H$'_c$, the zero-point energy has minima at odd l and the ground state is GS(π/3). In GS(0), the magnon density of states exhibits five distinct topological phases with increasing field associated with the opening and closing of energy gaps between two or three magnonic bands. While the Berry curvature vanishes for the coplanar φ = 0 phase in zero field, the Berry curvature and Chern numbers exhibit signatures of the five topological phases below H$'_c$. Whereas the Berry curvature and Chern number are sensitive to changes in the magnon density of states within GS(π/3), the inelastic spectrum S(k,ω) is sensitive to changes in the intensity of the magnon modes in the different magnetic phases GS(0) and GS(π/3) rather than the five topological phases within GS(π/3).

Fishman, Randy S. [Oak Ridge National Laboratory (↗

Magnetic glassiness in noncentrosymmetric Sm 7 Pd 3 : Interplay of magnetic frustration, long-range order, and frozen domains

Here, we present a comprehensive investigation of the intricate spin dynamics in the noncentrosymmetric compound Sm 7 ⁢Pd 3 , revealing the coexistence of spin-glass, domain-glass, and ferromagnetic (FM) behaviors. Magnetic field-dependent measurements indicate large coercivity, suggesting ferromagnetic domain formation below the Curie temperature (𝑇 C ≈ 173 K), while temperature-dependent magnetization data point to antiferromagnetic (AFM) coupling, highlighting the competition between FM and AFM interactions. Detailed ac susceptibility, isothermal remanent magnetization, and aging effect measurements demonstrate the presence of two distinct types of glassiness in the sample, and their possible origins are discussed extensively. Magnetization measurements reveal the mixing of the 𝐽 = 5/2 ground state of Sm 3+ with the excited 𝐽 = 7/2 multiplet, lying 965 K above. The specific heat data show further crystalline electric field splitting of the 𝐽 = 5/2 state into a ground-state doublet and a fourfold-degenerate excited state.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Detailed magnetic and structural analysis mapping a robust magnetic C 4 dome in Sr 1 - x Na x Fe 2 As 2

The recently discovered C 4 tetragonal magnetic phase in hole-doped members of the iron-based superconductors provides new insights into the origin of unconventional superconductivity. Previously observed in Ba 1-x Na x Fe 2 As 2 (with A = K, Na), the C 4 magnetic phase exists within the well studied C 2 spin-density wave (SDW) dome, arising just before the complete suppression of antiferromagnetic (AFM) order but after the onset of superconductivity. Here in this paper, we present detailed x-ray and neutron diffraction studies of Sr 1-x Na x Fe 2 As 2 (0.10 ≤ x ≤ 0.60) to determine their structural evolution and the extent of the C 4 phase. Spanning Δx ~ 0.14 in composition, the C 4 phase is found to extend over a larger range of compositions, and to exhibit a significantly higher transition temperature, T r ~ 65K, than in either of the other systems in which it has been observed. The onset of this phase is seen near a composition (x~0:30) where the bonding angles of the Fe 2 As 2 layers approach the perfect 109.46° tetrahedral angle. We discuss the possible role of this return to a higher symmetry environment for the magnetic iron site in triggering the magnetic reorientation and the coupled re-entrance to the tetragonal structure. Finally, we present a new phase diagram, complete with the C 4 phase, and use its observation in a third hole-doped 122 system to suggest the universality of this phase.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Tipping the magnetic instability in paramagnetic S r 3 R u 2 O 7 by Fe impurities [Tipping the magnetic instability in paramagnetic S r 3 R u 2 O 7 by modest Fe substitution]

We report the magnetic and electronic properties of the bilayer ruthenate Sr 3 Ru 2 O 7 upon Fe substitution for Ru. We find that Sr 3 (Ru 1-x Fe x ) 2 O 7 shows spin-glass-like phase below 4 K for x = 0.01 and commensurate E-type antiferromagnetically ordered insulating ground state characterized by the propagation vector q c = (0.25 0.25 0) for x ≥ 0.03, in contrast to the paramagnetic metallic state in the parent compound with strong spin fluctuations occurring at wave vectors q = (0.09 0 0) and (0.25 0 0). The observed antiferromagnetic ordering is quasitwo-dimensional with very short correlation length along the c axis, a feature similar to the Mndoped Sr 3 Ru 2 O 7 . Lastly, our results suggest that this ordered ground state is associated with the intrinsic magnetic instability in the pristine compound, which can be readily tipped by the local magnetic coupling between the 3d orbitals of the magnetic dopants and Ru 4d orbitals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic interactions in PdCrO 2 and their effects on its magnetic structure

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO 2 . Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains R$\bar{3}$m below T N . This implies that magnetic interactions consistent with the crystal symmetry do not stabilize the noncoplanar magnetic structure, which was one of two structures previously proposed on the basis of single crystal neutron diffraction measurements. Inelastic neutron scattering measurements find two gaps at low energies, which can be explained as arising from a dipolar-type exchange interaction. This symmetric anisotropic interaction also stabilizes a magnetic structure very similar to the coplanar magnetic structure, which was also suggested by the single crystal diffraction study. In conclusion, the higher-energy magnon dispersion can be modelled by linear spin-wave theory with exchange interactions up to sixth nearest neighbors, but discrepancies remain which hint at additional effects unexplained by the linear theory.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Pair Invariant Mass to Isolate Background in the Search for the Chiral Magnetic Effect in Au+Au Collisions at √sNN = 200 GeV

Quark interactions with topological gluon configurations can induce local chirality imbalance and parity violation in quantum chromodynamics, which can lead to the chiral magnetic effect (CME)-an electric charge separation along the strong magnetic field in relativistic heavy-ion collisions. The CME-sensitive azimuthal correlator observable (Delta gamma) is contaminated by background arising, in part, from resonance decays coupled with elliptic anisotropy (v(2)). We report here differential measurements of the correlator as a function of the pair invariant mass (m(inv)) in 20-50% centrality Au + Au collisions at root s(NN) = 200 GeV by the STAR experiment at the BNL Relativistic Heavy Ion Collider. Strong resonance background contributions to Delta gamma. are observed. At large m(inv) where this background is significantly reduced, the Delta gamma. value is found to be significantly smaller. An event-shape-engineering technique is deployed to determine the v(2) background shape as a function of m(inv). We extract a v(2)-independent and m(inv)-averaged signal Delta gamma(sig) = (0.03 +/- 0.06 +/- 0.08) x 10(-4), or (2 +/- 4 +/- 5)% of the inclusive Delta gamma (m(inv) > 0.4 GeV/c(2)) = (1.58 +/- 0.02 +/- 0.02) x 10(-4), within pion p(T) = 0.2-0.8 GeV/c and averaged over pseudorapidity ranges of -1 < eta < -0.05 and 0.05 < eta < 1. This represents an upper limit of 0.23 x 10(-4), or 15% of the inclusive result, at 95% confidence level for the m(inv)-integrated CME contribution.

Adam, J.↗

Tuning Perpendicular Magnetic Anisotropy by Oxygen Octahedral Rotations in ( La 1 – x Sr x MnO 3 ) / ( SrIrO 3 ) Superlattices

Here, perpendicular magnetic anisotropy (PMA) plays a critical role in the development of spintronics, thereby demanding new strategies to control PMA. Here we demonstrate a conceptually new type of interface induced PMA that is controlled by oxygen octahedral rotation. In superlattices comprised of La 1–x Sr x MnO 3 and SrIrO 3 , we find that all superlattices (0 ≤ x ≤ 1) exhibit ferromagnetism despite the fact that La 1–x Sr x MnO 3 is antiferromagnetic for x > 0.5. PMA as high as 4 × 10 6 erg/cm 3 is observed by increasing x and attributed to a decrease of oxygen octahedral rotation at interfaces. We also demonstrate that oxygen octahedral deformation cannot explain the trend in PMA. These results reveal a new degree of freedom to control PMA, enabling discovery of emergent magnetic textures and topological phenomena.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic Excitations across the Metal-Insulator Transition in the Pyrochlore Iridate Eu 2 Ir 2 O 7 [Evolution of Magnetic Excitations across the Metal-Insulator Transition in the Pyrochlore Iridate Eu 2 Ir 2 O 7 ]

Here, we report a resonant inelastic x-ray scattering study of the magnetic excitation spectrum in a highly insulating Eu 2 Ir 2 O 7 single crystal that exhibits a metal-insulator transition at T MI = 111(7) K. A propagating magnon mode with a 20 meV bandwidth and a 28 meV magnon gap is found in the excitation spectrum at 7 K, which is expected in the all-in-all-out magnetically ordered state. This magnetic excitation exhibits substantial softening as the temperature is raised towards T MI and turns into a highly damped excitation in the paramagnetic phase. Remarkably, the softening occurs throughout the whole Brillouin zone including the zone boundary. This observation is inconsistent with the magnon renormalization expected in a local moment system and indicates that the strength of the electron correlation in Eu 2 Ir 2 O 7 is only moderate, so that electron itinerancy should be taken into account in describing its magnetism.

74 ATOMIC AND MOLECULAR PHYSICS↗

Real-space investigation of short-range magnetic correlations in fluoride pyrochlores NaCaCo 2 F 7 and NaSrCo 2 F 7 with magnetic pair distribution function analysis

Here, we present time-of-flight neutron total scattering and polarized neutron scattering measurements of the magnetically frustrated compounds NaCaCo 2 F 7 and NaSrCo 2 F 7 , which belong to a class of recently discovered pyrochlore compounds based on transition metals and fluorine. The magnetic pair distribution function (mPDF) technique is used to analyze and model the total scattering data in real space. We find that a previously-proposed model of short-range XY-like correlations with a length scale of 10-15 Å, combined with nearest-neighbor collinear antiferromagnetic correlations, accurately describes the mPDF data at low temperature, confirming the magnetic ground state in these materials. This model is further verified by the polarized neutron scattering data. From an analysis of the temperature dependence of the mPDF and polarized neutron scattering data, we find that short-range correlations persist on the nearest-neighbor length scale up to 200 K, approximately two orders of magnitude higher than the spin freezing temperatures of these compounds. These results highlight the opportunity presented by these new pyrochlore compounds to study the effects of geometric frustration at relatively high temperatures, while also advancing the mPDF technique and providing a novel opportunity to investigate a genuinely short-range-ordered magnetic ground state directly in real space.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Designs and Prospects of Bi-2212 Canted-Cosine-Theta Magnets to Increase the Magnetic Field of Accelerator Dipoles Beyond 15 T

The critical current density of Bi-2212 round wires has seen significant improvement over the past two years. We present the magnetic design and stress analysis of two Bi-2212 dipoles based on Canted-Cosine-Theta (CCT) technology using the state-of-the-art wires. The first design, based on a 19-strand Rutherford cable of θ0.8mm strands, is a two-layer dipole with a bore diameter of 40 mm and an outer diameter of 98.4 mm; it generates 5.4 T when operating in stand-alone configuration and 18.9 T in 15 T background field. The second design, based on a 13-strand Rutherford cable of θ0.8mm strands, is also a two-layer dipole with a bore diameter of 40 mm and an outer diameter of 81 mm; it generates 4.0 T when operating in stand-alone configuration and 17.8 T in 15 T background field. Normal stresses on the conductor in these magnets do not exceed 35 MPa when working under background field.Moreover, we propose a novel approach for increasing the efficiency of CCT magnets using keystoned Rutherford cable while removing the midplane ribs. with this method, it is possible to increase the efficiency of small radius CCT coils by 20%. We conclude that Bi-2212 can be used to increase the limit of accelerator magnet dipole fields beyond 15 T while managing stresses in the coils to acceptable levels.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnetic Measurements of Fermilab Rapid-Cycling Booster Gradient Magnets

Fermilab is upgrading its Booster synchrotron to increase ramp rate and intensity. This is part of the Proton Improvement Plan (PIP-II) that will allow the Main Injector to achieve proton beam power of 1.2 MW within the next few years. This upgrade includes running the 55-year-old Booster magnets at 20 Hz instead of the usual 15 Hz, and construction of some shorter and wider aperture versions of these combined-function gradient magnets. Magnetic measurements were performed to characterize the present 15 Hz AC performance, and then again with 20 Hz ramp cycle to ensure performance and compatibility in this new operating regime. A 3 m-long curved flat-coil was developed for these measurements using Printed Circuit Board (PCB) technology. The probe also has a separate 0.5 m-long body-field probe, allowing integral, body, and end fields to be measured across 100 mm of the magnet aperture. The sampling rate for these measurements during the AC cycle was 200 kHz, and field resolution was better than 0.01%. Details of the probe, measurements, and results are presented.

DiMarco, J. [Fermilab] (ORCID:0000000228400036)↗

A pyroxene-based quantum magnet with multiple magnetization plateaus

Pyroxenes (AMX 2 O 6 ) consisting of infinite one-dimensional edge-sharing MO 6 chains and bridging XO 4 tetrahedra are fertile ground for finding quantum materials. Thus, here, we have studied calcium cobalt germanate (CaCoGe 2 O 6 ) and calcium cobalt silicate (CaCoSi 2 O 6 ) crystals in depth. Heat capacity data show that the spins in both compounds are dominantly Ising-like, even after being manipulated by high magnetic fields. On cooling below the Néel temperatures, a sharp field–induced transition in magnetization is observed for CaCoGe 2 O 6 , while multiple magnetization plateaus beneath the full saturation moment are spotted for CaCoSi 2 O 6 . Our analysis shows that these contrasting behaviors potentially arise from the different electron configurations of germanium and silicon, in which the 3d orbitals are filled in the former but empty in the latter, enabling electron hopping. Thus, silicate tetrahedra can aid the interchain superexchange pathway between cobalt(II) ion centers, while germanate ones tend to block it during magnetization.

Science & Technology - Other Topics↗

Quasi-static and dynamic magnetic tension forces in arched, line-tied magnetic flux ropes

Solar eruptions are often driven by magnetohydrodynamic instabilities such as the torus and kink instabilities that act on line-tied magnetic flux ropes. Recent laboratory experiments designed to study these eruptive instabilities have demonstrated the key role of both dynamic (Myers et al 2015 Nature 528, 526) and quasi-static (Myers et al 2016 Phys. Plasmas, in press) magnetic tension forces in contributing to the equilibrium and stability of line-tied magnetic flux ropes. In this paper, we synthesize these laboratory results and explore the relationship between the dynamic and quasi-static tension forces. While the quasi-static tension force is found to contribute to the flux rope equilibrium in a number of regimes, the dynamic tension force is substantial mostly in the so-called failed torus regime where magnetic self-organization events prevent the flux rope from erupting.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Enhanced Energy Density in Permanent Magnets using Controlled High Magnetic Field during Processing

This ORNL Manufacturing Demonstraction Facility (MDF) technical collaboration focused on the use of high magnetic field processing (>2Tesla) using energy efficient large bore superconducting magnet technology and high frequency electromagnetics to improve magnet performance and reduce the energy budget associated with Alnico thermal processing. Alnico, alloys containing Al, Ni, Co and Fe, represent a class of functional nanostructured alloys, and show the greatest potential for supplementing or replacing commercial Nd-based rare-earth alloy magnets.

36 MATERIALS SCIENCE↗

Microscopic subsurface characterization of layered magnetic materials using magnetic resonance force microscopy

This project resulted in the following accomplishments: 1) The invention of scanned probe ferromagnetic resonance microscopy. Upon implementation and refinement this approach was used to measure static and dynamic magnetic resonance properties of ferromagnets with an unprecedented combination of spectral and spatial resolution. 2) Demonstration and study of spin pumping in a pristine ferromagnet across a boundary defined entirely by a magnetic field gradient, and so free of materials discontinuities. 3) First demonstrated highly efficient dynamic spin injection from Y 3 Fe 5 O 12 (YIG) into NiO, an antiferromagnetic (AF) insulator and robust spin propagation in AF NiO over distances up to 100-nm thickness; both spin injection and spin transport are mediated by the AF spin correlations. 4) Demonstration of exceptionally high efficiency conversion of spin current to charge current achieved in spin pumping from the dynamic magnetization of a ferromagnetic insulator into a variety of adjacent metal films. 5) Seminal study of the nature of spin-orbit coupling in d-electron metals that revealed the dominant sensitivity of the d-orbital moment to the d-electron count and revealing the important roles of both d-electron configuration and atomic number in the physics of the spin Hall effect. 6) Demonstration of observation of FMR by means of optically-detected NV diamond relaxometry that provided a highly sensitive, spatially resolved FMR detection method and revealed spin pumping across 100-nm length scales by means of dipolar coupling. 7) Using magnetic field localization, developed for FMR imaging, demonstrated a novel approach to discretizing spin wave modes to improve the characteristics of auto-oscillators driven by pure spin currents produced by the spin Hall effect. 8) We demonstrated large spin pumping signals from propagating high wavevector spinwaves in thin film YIG find that the spin pumping efficiency was insensitive to wavevector thus emphasizing the promise of thin YIG films for spinwave-based spintronics by allowing for predictable down-scaling of device dimensions and enabling a broad range of operational frequencies.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗