Summary of ALSEP Test Loop Solvent Irradiation Testing
Separating the minor actinide elements (americium and curium) from the fission product lanthanides is an important step in closing the nuclear fuel cycle. Isolating the minor actinides will allow transmuting them to short lived or stable isotopes in fast reactors, thereby reducing the long-term hazard associated with these elements. The Actinide Lanthanide Separation Process (ALSEP) is being developed by the DOE-NE Material Recovery and Waste Form Development Campaign to accomplish this separation with a single process. To develop a fundamental understanding of the solvent degradation mechanisms for the ALSEP Process, testing was performed in the INL Radiolysis/Hydrolysis Test Loop for the extraction section of the ALSEP flowsheet. This work culminated in the completion of the level two milestone (M2FT-16IN030102021) "Complete ALSEP test loop solvent irradiation test.” This report summarizes the testing performed and the impact of radiation on the ALSEP Process performance as a function of dose.