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At least 613 records · Page 34

Modeling of fission and activation products in molten salt reactors and their potential impact on the radionuclide monitoring stations of the International Monitoring System

Molten Salt Reactors (MSRs) are one of six Generation IV reactor designs currently under development around the world. Because of the unique operating conditions of MSRs, which include molten fuel and the continuous removal of gaseous fission products during operation, work was performed to analyze the potential impact of emissions on the International Monitoring System (IMS) of the Comprehensive Nuclear-Test-Ban Treaty (CTBT). Simulations were performed to predict the production of IMS-relevant radionuclides in four MSR designs operating under two scenarios – (1) a sealed reactor with releases only during operational shutdown and (2) continuous reprocessing or sparging of the fuel salt. From these production estimates the radioxenon and radioiodine signatures were extracted and compared to three current reactor designs (PWR, BWR, RBMK). In the cases where continuous reprocessing of the fuel salt occurred both the radioxenon and radioiodine signatures are nearly indistinguishable from a nuclear explosion. Estimates were also made of the potential emission rate of radioxenon for three reactor designs and it was found that MSRs have the potential to emit radioxenon isotopes at a rate of 1015 – 8×1016 Bq/d for 133Xe if no abatement is used. An assessment was also made of activation products using a candidate fuel salt (FLiBe) mixed with corrosion products for the Thorium Molten Salt Reactor (TMSR-LF1)

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Health Physics Research Reactor Criticality Accident Alarm System Benchmark Overview

From the countless critical experiments performed in the world during the past century, high-quality integral benchmarks experiments have been collected and gathered into the International Handbook of Evaluated Criticality Safety Benchmark Experiments (ICSBEP Handbook), managed by the International Criticality Safety Benchmark Evaluation Project (ICSBEP) Working Group. This information preservation and dissemination effort is crucial for reactor licensing as well as criticality and radiation transport modeling validation. This summary reports on the status of a tentative benchmark addition to the ICSBEP Handbook. The proposed benchmark arises from legacy operation data of the Oak Ridge National Laboratory (ORNL) Health Physics Research Reactor (HPRR). The HPRR was a small, unmoderated, unshielded fast burst reactor that was used for research in health physics and radiobiology as well as teaching and training. As part of a comprehensive investigation of the available HPRR operation data and characteristics, different possibilities for use of the valuable results were studied. A critical experiment benchmark evaluation was performed, analyzing data coming from sub-critical and critical operation of the HPRR during operator training, steady-state irradiation of samples and before critical bursts. The results of the evaluation do not satisfy for the ICSBEP standards as the benchmark relative standard uncertainty is of about 4% for k eff , and the relative difference between sample calculations and expected k eff results is of about 1.5%. Due to those unsatisfactory results, it was decided not to pursue critical experiments evaluation of the HPRR presently and to focus instead on shielding type data for the creation of a criticality accident alarm system (CAAS) and shielding category benchmark, which is currently very scarce in the ICSBEP handbook—especially concerning critical, pulsed assembly, or reactor operation data. Several dosimetry and shielding experiments from HPRR burst operation were evaluated, with different benchmark metrics as sulfur fluence, Element 57 dose, or neutron fluence at different distances and under different shield materials conditions. An evaluation focusing on the Element 57 neutron dose as a benchmark metric was submitted to the ICSBEP Technical Review Group (TRG) meeting in October 2021, and the inclusion of the evaluation in the ICSBEP Handbook was deferred. The main change proposed by the international experiment evaluation experts is to use the neutron fluence measured by Bonner spheres as a benchmark metric. This represents a quantity closer to that actually measured by the experimentalists of the HPRR compared to the Element 57 dose, which adds another step of data transformation, thus potentially adding uncertainty to the benchmark. The evaluation has been updated and will be submitted to the 2022 ICSBEP TRG meeting for inclusion in the 2023 edition of the ICSBEP Handbook. The evaluation is performed using the KENO and MAVRIC combination from the SCALE 6.2.4 code suite which was previously used in similar CAAS benchmarks to allow for the use of variance reduction techniques.

61 RADIATION PROTECTION AND DOSIMETRY↗

High-temperature stability and thermal expansion behavior of equi-atomic refractory multi-principal element alloys based on MoNbTi system for Gen IV reactor applications

The present study investigates the thermal stability and thermal expansion behavior of seven equi-atomic refractory multi-principal element alloys (MPEAs) based on the MoNbTi ternary system composed of low neutron absorption cross section elements. Through an integrated approach utilizing in-situ high-temperature X-ray diffraction (HT-XRD) in conjunction with differential scanning calorimetry (DSC), dilatometry and ageing heat treatment, the thermal stability of the MPEAs was comprehensively analyzed. In-situ HT-XRD experiment confirmed the stability of the room temperature phases up to 1000 °C with no peaks observed corresponding to additional phases in the HT-XRD patterns at 500, 800 and 1100 °C. DSC thermograms showed the absence of peaks up to 1000 °C, while peaks and valleys corresponding to exothermic and endothermic events were observed above 1000 °C. Coefficient of thermal expansion (CTE) derived from second order polynomial fitting of linear thermal expansion data from the dilatometry experiment showed linear increment up to 1000 °C for all the alloys except those containing Zr. The Cr containing alloys exhibited notably higher CTE values, particularly the Al containing alloy exhibited the highest value. Ageing heat treatment at 800 and 1000 °C for 96 h and subsequent microstructural analysis revealed significant precipitation of secondary phases in MoNbTiZr, MoNbTiZrV and MoNbTiCrAl. In conclusion, a substantial increase in hardness was observed in MoNbTiZr and MoNbTiCrAl due to secondary phase precipitation, while the other alloys maintained hardness values comparable to their as-cast and homogenized states.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Reassessing Double-Ended Guillotine Break Requirements: Evidence-Based Analysis of Regulatory Assumptions After Five Decades of Nuclear Operation

After five decades of nuclear power operation encompassing more than 20,000 reactor-years across 35 countries and 647 reactors, zero double-ended guillotine breaks (DEGBs) have been documented in commercial reactor coolant systems—despite DEGB being the fundamental design-basis assumption driving Emergency Core Cooling System (ECCS) sizing, structural protection requirements, and containment design specifications. This report examines the basis for DEGB requirements in nuclear power plant design. The DEGB postulate assumes the instantaneous, complete circumferential severance of the largest diameter pipes in reactor coolant systems, driving major design requirements under 10 Code of Federal Regulations 50.46, General Design Criterion 4 and containment design specifications. The United States (4,880 reactor-years) and France (2,505 reactor-years) contribute the largest operational datasets. Probabilistic assessments estimate direct DEGB occurrence probabilities with extremely low event frequencies, far below the 10-5/reactor-year thresholds typically used to define non-credible events in nuclear-safety analyses; i.e., events with probability this low fall into beyond-design-basis events. Current material-science knowledge demonstrates that the ductile steel materials used in nuclear piping systems exhibit stable crack-growth behavior fundamentally incompatible with instantaneous severance. International regulatory experience, particularly Germany’s comprehensive break-preclusion implementation, and successful leak-before-break (LBB) applications in almost all of U.S. pressurized water reactor units validate that alternatives can maintain safety performance while reducing economic burden. Current DEGB protection systems impose estimated lifetime costs of hundreds of millions of dollars per unit, over the life of a plant across the nuclear industry (including ongoing costs), representing substantial resource allocation toward scenarios with extremely low probability. Although this report acknowledges uncertainties regarding long-term aging effects, potential synergistic degradation mechanisms, and site-specific seismic considerations that warrant continued evaluation as regulatory policy evolves, there remains no documented evidence that a DEGB has occurred as a consequence of the conditions or mechanisms described in this report. This report acknowledges the Nuclear Regulatory Commission’s (NRC’s) recent efforts—outlined in the draft Interim Staff Guidance (ISG) NRC-DSS-ISG-2025-XX (“Treatment of Certain Loss-of-Coolant Accident Locations as Beyond-Design-Basis Accidents Draft Interim Staff Guidance”)—to reduce overly conservative requirements for large-break loss of coolant accidents through technical justifications and exemptions. However, extensive operating experience and validated methodologies—such as LBB and in-service inspection programs—demonstrate that the probability of a DEGB in reactor coolant-loop piping is extremely low, even under seismic conditions. The authors and reviewers of this report recommend that DEGB be removed as a design-basis event through formal rulemaking, rather than case-by-case exemptions, to better reflect credible failure modes, align with current data, and align with modern, risk-informed safety analysis.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

Report on Year-3 of Water NSTF Matrix Testing: Two-Phase Parametric Test Series

The Natural convection Shutdown heat removal Test Facility (NSTF) is large scale test facility constructed at Argonne National Laboratory to generate NQA-1 qualified validation data for passive decay heat removal systems in advanced reactor concepts. With support from the Department of Energy (DOE) offices of Advanced Reactor Technologies (ART) and Advanced Reactors Regulatory Development (RD), this facility reflects key features of a ½ scale, water-based, Reactor Cavity Cooling System (RCCS) and is intended to study the behavior, bound performance, and ultimately guide design decisions for passive decay heat removal systems. Since the facility also retains all aspects common to a fundamental boiling water thermosiphon, the generated experimental data sets are well poised to advance the understanding of fundamental natural circulation boiling and two-phase flow phenomena.

22 GENERAL STUDIES OF NUCLEAR REACTORS↗

Modeling of fission and activation products in molten salt reactors and their potential impact on the radionuclide monitoring stations of the International Monitoring System

Molten Salt Reactors (MSRs) are one of six Generation IV reactor designs currently under development around the world. Because of the unique operating conditions of MSRs, which include molten fuel and the continuous removal of gaseous fission products during operation, work was performed to analyze the potential impact of emissions on the International Monitoring System (IMS) of the Comprehensive Nuclear-Test-Ban Treaty (CTBT). Simulations were performed to predict the production of IMS-relevant radionuclides in four MSR designs operating under two scenarios: (1) a sealed reactor with releases only during operational shutdown, and (2) continuous reprocessing or sparging of the fuel salt. From these production estimates the radioxenon and radioiodine signatures were extracted and compared to three current reactor designs (Pressurized Water Reactor (PWR), BWR, RBMK). In cases where continuous reprocessing of the fuel salt occurred, both the radioxenon and radioiodine signatures were nearly indistinguishable from a nuclear explosion. Estimates were also made of the potential emission rate of radioxenon for three reactor designs and it was found that MSRs have the potential to emit radioxenon isotopes at a rate of 10^15-8×10^16 Bq/d for 133Xe if no abatement is used. An assessment was made of activation products using a candidate fuel salt (FLiBe) mixed with corrosion products for the Thorium Molten Salt Reactor (TMSR-LF1).

Johnson, Christine M.↗

The Physical and Engineering Limits of Coupled In situ TEM Experiments

Almost all future energy systems (advanced nuclear reactors, fusion energy system, concentrating solar-thermal power (CSP), and wind technologies) are limited by degradation of key material systems exposed to multiple environmental stressors. The degradation during exposure to high temperatures, radiation, mechanical loading, and chemical attack is often dictated by mechanisms active at the microstructural level. The nature of these mechanisms and the associated variations between sequential and concurrent interplay can be explored if the transmission electron microscope (TEM) is utilized as a toolbox for exploration [1]. One such tool developed at Sandia National Laboratories to couple several of these environments is the In situ Ion Irradiation TEM (I3TEM) [2]. Several studies over the last decade utilizing this tool have shown that the scientific intuition developed over decades of sequential experiments is not always a good indicator of concurrent mechanisms or failure routes. This presentation will highlight the recent and planned additions into the I3TEM facility of a Waviks gas injection system and Raman system, respectively, as can be seen in Fig. 1, permitting environmental degradation from gas species leaked into the pole piece region during quantitative mechanical loading (indentation, monotonic loading, high temperature creep, irradiation induced creep, and high-cycle fatigue); multi-beam ion irradiation (energies ranging from 1 keV to 48 MeV and species from H to Au); laser exposure (20 W and 1064 nm), or various combinations thereof that are already possible [3]. This addition permits the facility to explore both sequential or concurrently the four axes of stressors: thermal, mechanical, radiation, and chemical. This information can be directly coupled to modeling, expediting the refinement and validation of both atomistic and mesoscale models.

degradation↗

FY25 Report on Water NSTF Testing: Parametric and Accident Testing with Lower Tank Inlet

The Natural Convection Shutdown Heat Removal Test Facility (NSTF) at Argonne National Laboratory has continued to generate empirical validation data on the performance of water-based reactor cavity cooling system (RCCS) for seven years. This data is actively being used to support the development of passive decay heat removal systems for advanced reactors. Distinguishing this facility are 1) the large, ½ scale of the facility and 2) its governance under an NQA-1 qualified program for producing data of the highest pedigree for advanced reactor designers and regulators. In addition to the experimental activities discussed in this report, a computational modeling program continues to support the experimental program and further accuracy and understanding of the computational models. Together, the experimental and computational work create a mutually beneficial relationship integral to the overall program objective of advancing the understanding of the RCCS technology.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Systems definition space based power conversion systems: Executive summary

Potential space-located systems for the generation of electrical power for use on earth were investigated. These systems were of three basic types: (1) systems producing electrical power from solar energy; (2) systems producing electrical power from nuclear reactors; (3) systems for augmenting ground-based solar power plants by orbital sunlight reflectors. Configurations implementing these concepts were developed through an optimization process intended to yield the lowest cost for each. A complete program was developed for each concept, identifying required production rates, quantities of launches, required facilities, etc. Each program was costed in order to provide the electric power cost appropriate to each concept.

Source record↗

The NASA CSTI high capacity power project

The SP-100 Space Nuclear Power Program was established in 1983 by DOD, DOE, and NASA as a joint program to develop technology for military and civil applications. Starting in 1986, NASA has funded a technology program to maintain the momentum of promising aerospace technology advancement started during Phase 1 of SP-100 and to strengthen, in key areas, the chances for successful development and growth capability of space nuclear reactor power systems for a wide range of future space applications. The elements of the Civilian Space Technology Initiative (CSTI) High Capacity Power Project include Systems Analysis, Stirling Power Conversion, Thermoelectric Power Conversion, Thermal Management, Power Management, Systems Diagnostics, Environmental Interactions, and Material/Structural Development. Technology advancement in all elements is required to provide the growth capability, high reliability and 7 to 10 year lifetime demanded for future space nuclear power systems. The overall project will develop and demonstrate the technology base required to provide a wide range of modular power systems compatible with the SP-100 reactor which facilitates operation during lunar and planetary day/night cycles as well as allowing spacecraft operation at any attitude or distance from the sun. Significant accomplishments in all of the project elements will be presented, along with revised goals and project timelines recently developed.

Winter, J.↗

Power-Conversion Concept Designed for the Jupiter Icy Moons Orbiter

The Jupiter Icy Moons Orbiter (JIMO) is a bold new mission being developed by NASA's Office of Space Science under Project Prometheus. JIMO is examining the potential of nuclear electric propulsion (NEP) technology to efficiently deliver scientific payloads to three of Jupiter's moons: Callisto, Ganymede, and Europa. A critical element of the NEP spacecraft is the space reactor power system (SRPS), consisting of the nuclear reactor, power conversion, heat rejection, and power management and distribution (PMAD).

Mason, Lee S.↗

Assessment of nuclear data needs for advanced reactor demonstrations: application to the molten chloride reactor experiment (MCRE)

A number of advanced reactor concepts are planned for near-term demonstrations including micro-reactors, larger demonstrations and space nuclear systems. These reactor concepts are based on a wide variety of reactor technologies, including sodium, gas, and salt cooling. An overlooked area in the development and ultimate startup of these reactors is addressing nuclear data needs that allow confident prediction of the criticality, safety requirements, and operation of the reactors. In this paper we try to address the problem of assessing nuclear data needs and possible remedies to reduce the existing uncertainties for advanced nuclear reactors. A methodology for defining these needs is described. The case of the Molten Chloride Reactor Experiment (MCRE) has been considered and the related investigation highlights the specific needs for reducing uncertainty on the {sup 235}U capture and {sup 35}Cl (n,p) reactions. Relatively inexpensive integral experiments are indicated as possible solutions for significantly reducing the current associated uncertainties. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Adaptive Control for Load-Following of Boiling Water Reactors Part I: Linear Systems and Fully-Observable Dynamics

Automation control is a key strategy to improve the economic competitiveness of nuclear power plants. Not only does it help reduce operational costs, but it also extends the value proposition of these plants to nontraditional markets, including unattended operations in remote villages and space. However, the dynamics of the operating environments of nuclear reactors are subject to changes over time, and there are no widely adopted methods to ensure that the automation strategy will remain effective over the extended durations required for these applications. Adaptive control is a discipline that offers the possibility to accommodate such changes online. However, it relies on mathematical assumptions that must be respected to ensure robustness and reliability. In this work, we derive an adaptive control formulation for linear systems in which all states are observable and apply it to an instance of load-follow operation for Boiling Water Reactors. We assumed uncertainty in two factors: the temperature coefficient and the control rod worth, both of which are affected over time by the evolution of the nuclear reactor core environment. With an arbitrary penalty factor of 5, we found that the mean absolute and integral time absolute errors can be reduced by more than 90%, underscoring the strength of adaptive control. To extend the application to more challenges, different uncertainties and load-follow trajectories, as well as new formulations that include non-linearity and partial observability, are currently being developed.

22 - GENERAL STUDIES OF NUCLEAR REACTORS↗

SPC-70734 Rev 1 MARVEL Primary Coolant System (PCS) Fill and Eutectic NaK Procurement

This specification contains the requirements for the filling the Microreactor Applications Research Validation and Evaluation (MARVEL) reactor Primary Coolant System (PCS) with eutectic sodium-potassium (NaK). The subcontractor will design and fabricate a NaK filling system (referred to herein as the PCS Fill System), the requisite volume of high purity NaK, and perform filling operations in conjunction with the Contractor Operations. The MARVEL reactor system will be operated by the Contractor, and the PCS fill system will be operated by Subcontractor personnel.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Methods and systems for rebalancing electrolytes for a redox flow battery system

A rebalancing reactor for a redox flow battery system may include a first side through which hydrogen gas is flowed, a second side through which electrolyte from the redox flow battery system is flowed, and a porous layer separating and fluidly coupled to the first side and the second side, wherein, the hydrogen gas and the electrolyte are fluidly contacted at a surface of the porous layer, and a pressure drop across the second side is less than a pressure drop across the porous layer. In this way, rebalancing of electrolyte charges in a redox flow battery system may be performed with increased efficiency and cost effectiveness as compared to conventional rebalancing reactors.

Evans, Craig E.↗

Design and Assessments of Liquid Metal Systems for a Fusion Power Reactor

This three-year research program at UCLA builds on the Fusion Engineering System Study (FESS) and has the major goal of identifying and accessing the most critical MHD/Mass & Heat Transfer phenomena associated with LM MHD flows in fusion breeding/cooling applications. The computed results and their analyses provide a strong basis to overcome present design limitations and will eventually lead to feasible, more effective solutions for LM systems of a fusion power reactor, such as breeding blankets and LM plasma facing components (PFCs). The project focuses on three research thrusts: Identification and characterization of the most important generic issues common to LM breeders (hereinafter called “Blanket”: ~47% of the resources); Design, implementation and assessments of two LM breeding-blanket concepts, DCLL and HCLL, for particular fusion devices, such as the US Fusion Nuclear Science Facility (FNSF) or the Fusion Pilot Plant (FPP) (hereinafter called “System Studies”: ~40% of the resources); Design and analysis of LM (Li) divertor concepts for FNSF or FPP, including scoping and detailed 2D and 3D computations (hereinafter called “LM PFC”: ~13% of the resources).

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗