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At least 631 records · Page 35

Radiative Heating Profiles over Ascension Island during the 2016 and 2017 Biomass Burning Seasons

Marine boundary layer clouds, including the transition from stratocumulus to cumulus, are poorly represented in numerical weather prediction and general circulation models. In many cases, the complex physical relationships between cloud morphology and the environmental conditions in which marine boundary layer clouds exist are not well understood. Such uncertainties arise in the presence of biomass burning carbonaceous aerosol, as is the case over the southeast Atlantic Ocean, where it is likely that the absorbing and heating properties of these aerosols modify the microphysical composition and macrophysical arrangement of marine stratocumulus and trade cumulus. The deployment of the Atmospheric Radiation Measurement Mobile Facility #1 (AMF1) in support of LASIC (Layered Atlantic Smoke Interactions with Clouds) provided a unique opportunity to observe thermodynamic, cloud and aerosol properties during two consecutive biomass burning seasons from July through October of 2016 and 2017 over Ascension Island (7.96 S, 14.35 W). These observations in conjunction with radiation transfer modeling were used to assess the impact of biomass burning carbonaceous aerosol plumes as they passed over the site.Thermodynamic profiles were generated using a combination of radiosonde data and thermodynamic profilers to provide high temporal resolution profiles of quantities that are important for cloud development, such as CAPE and CIN. Coincident Ka-band radar and lidar profiles were used to characterize the cloud and sub-cloud structure. The resulting thermodynamic and cloud profiles are used as input forcing for the Rapid Radiative Transfer Model (RRTM) to compute radiative heating profiles over the observation site. Idealized experiments using RRTM, with and without aerosols present, are used to assess the impacts of the absorbing aerosol on the heating rate profiles.

Cumulus↗

The winter central Arctic surface energy budget: A model evaluation using observations from the MOSAiC campaign

This study evaluates the simulation of wintertime (15 October, 2019, to 15 March, 2020) statistics of the central Arctic near-surface atmosphere and surface energy budget observed during the MOSAiC campaign with short-term forecasts from 7 state-of-the-art operational and experimental forecast systems. Five of these systems are fully coupled ocean-sea ice-atmosphere models. Forecast systems need to simultaneously simulate the impact of radiative effects, turbulence, and precipitation processes on the surface energy budget and near-surface atmospheric conditions in order to produce useful forecasts of the Arctic system. This study focuses on processes unique to the Arctic, such as, the representation of liquid-bearing clouds at cold temperatures and the representation of a persistent stable boundary layer. It is found that contemporary models still struggle to maintain liquid water in clouds at cold temperatures. Given the simple balance between net longwave radiation, sensible heat flux, and conductive ground flux in the wintertime Arctic surface energy balance, a bias in one of these components manifests as a compensating bias in other terms. This study highlights the different manifestations of model bias and the potential implications on other terms. Three general types of challenges are found within the models evaluated: representing the radiative impact of clouds, representing the interaction of atmospheric heat fluxes with sub-surface fluxes (i.e., snow and ice properties), and representing the relationship between stability and turbulent heat fluxes.

54 ENVIRONMENTAL SCIENCES↗

How Well are Recent Climate Variability Signals Resolved by Satellite Radiative Flux Estimates?

One notable aspect of Earth s climate is that although the planet appears to be very close to radiative balance at top-of-atmosphere (TOA), the atmosphere itself and underlying surface are not. Profound exchanges of energy between the atmosphere and oceans, land and cryosphere occur over a range of time scales. Recent evidence from broadband satellite measurements suggests that even these TOA fluxes contain some detectable variations. Our ability to measure and reconstruct radiative fluxes at the surface and at the top of atmosphere is improving rapidly. Understanding the character of radiative flux estimates and relating them to variations in other energy fluxes and climate state variables is key to improving our understanding of climate. In this work we will evaluate several recently released estimates of radiative fluxes, focusing primarily on surface estimates. The International Satellite Cloud Climatology Project FD radiative flux profiles are available from rnid-1983 to near present and have been constructed by driving the radiative transfer physics from the Goddard Institute for Space Studies (GISS) global model with ISCCP clouds and HlRS operational soundings profiles. Full and clear sky SW and LW fluxes are produced. A similar product from the NASA/GEWEX Surface Radiation Budget Project using different radiative flux codes and thermodynamics from the NASA/Goddard Earth Observing System assimilation model makes a similar calculation of surface fluxes. However this data set currently extends only through 1995. Several estimates of downward LW flux at the surface inferred from microwave data are also examined. Since these products have been evaluated with Baseline Surface Radiation Network data over land we focus over ocean regions and use the DOE/NOAA/NASA Shipboard Ocean Atmospheric Radiation (SOAR) surface flux measurements to characterize performance of these data sets under both clear and cloudy conditions. Some aspects of performance are stratified according to SST and vertical motion regimes. Comparisons to the TRMM/CERES SRB data in 1998 are also interpreted. These radiative fluxes are then analyzed to determine how surface (and TOA) radiative exchanges respond to interannual signals of ENS0 warm and cold events. Our analysis includes regional changes as well as integrated signals over land, ocean and various latitude bands. Changes in water vapor and cloud forcing signatures are prominent on interannual time scales. Prominent signals are also found in the SW fluxes for the Pinatubo volcanic event. These systematic changes in fluxes are related to changes in large-scale circulations and energy transport in the atmosphere and ocean. Some estimates of signal-to-noise and reliability are discussed to place our results in context.

Robertson, Franklin R.↗

Can Biomass Burning Aerosol Induced Surface Cooling Be Amplified Through Sea Surface Temperature‐Cloud Feedback Over the Southeast Atlantic?

Biomass burning (BB) aerosols exert a strong surface cooling effect over the southeast Atlantic (SEA) via aerosol-radiation and aerosol-cloud interactions. The reduction of the sea surface temperature (SST) can trigger the SST-low cloud feedback. Whether this feedback can amplify the surface cooling effect is examined. The modeling results from the Community Earth System Model version 2 (CESM2) demonstrate that counterintuitively the cloud radiative effect (CRE) caused by the BB aerosols is weaker if SST-low cloud feedback is considered compared to fixed-SST simulation (-2.99 W m -2 vs. -4.79 W m -2 ). This is caused by (a) stronger sea breeze due to larger sea-land temperature contrast causing less smoke transport over SEA and (b) less moisture supply from surface due to colder SST. Changes in SST also lead to counterclockwise rotation of ocean circulation anomalies. Consequently, the excess heat transport from the equator reverses the direction of SST-cloud feedback in this region.

0305↗

Cloud/climate sensitivity experiments

A study of the relationships between large-scale cloud fields and large scale circulation patterns is presented. The basic tool is a multi-level numerical model comprising conservation equations for temperature, water vapor and cloud water and appropriate parameterizations for evaporation, condensation, precipitation and radiative feedbacks. Incorporating an equation for cloud water in a large-scale model is somewhat novel and allows the formation and advection of clouds to be treated explicitly. The model is run on a two-dimensional, vertical-horizontal grid with constant winds. It is shown that cloud cover increases with decreased eddy vertical velocity, decreased horizontal advection, decreased atmospheric temperature, increased surface temperature, and decreased precipitation efficiency. The cloud field is found to be well correlated with the relative humidity field except at the highest levels. When radiative feedbacks are incorporated and the temperature increased by increasing CO2 content, cloud amounts decrease at upper-levels or equivalently cloud top height falls. This reduces the temperature response, especially at upper levels, compared with an experiment in which cloud cover is fixed.

Roads, J. O.↗

Radiative Transfer Through Clouds and Its Applications in Support of the Ice, Cloud, and Land Elevation Satellite-2 (ICESat-2) Mission

The Greenland and Antarctic ice sheets, which contain enough ice to raise sea level by about 7 and 60 m, respectively, are losing mass at an increasing rate. To acquire continuous information of the cryosphere, after the Ice, Cloud, and land Elevation Satellite (ICESat) (2003-2010), NASA is actively planning for the ICESat-2 mission. Both ICESat and ICESat-2 are space-borne lidar altimetry systems. The systems measure the time of flight of the arriving photons that are reflected by the surface to deduce the elevation of the underlying terrain. As one of NASA's top priority missions, ICESat-2 is scheduled to launch in 2016. One of the major science goals of ICESat-2 is to quantify the ice sheet mass balance to determine its contributions to the sea level change and its impacts on ocean circulation (Abdalati et al. 2010). Compared to ICESat, which operates at 40 Hz and records the reflected laser energy as a waveform, the significantly improved ICESat-2 lidar employs a 532 nm micro-pulse photon counting system that operates at a high frequency of 10kHz with single photon detectability (Yang et al. 2012). To achieve its science goals, ICESat-2 requires the ability of detecting the elevation change with an accuracy of 0.2 cm/year over the entire ice sheet. Since every photon emitted by the lidar system will travel through the atmosphere, clouds can certainly affect the flight time of the arriving photons. Forward scattering by cloud particles increases the photon path length, thus resulting in biases in ice sheet elevation measurements known as atmospheric path delay (Duta et al. 2001, Yang et al. 2010, 2011). To ensure the accuracy of ICESat-2 surface elevation measurements, it is critical to understand how clouds would affect the travel time of arriving photons. In this talk, we will first present a framework that simulates the behavior of a space-borne 532 mn micro-pulse photon counting lidar in cloudy and clear atmospheres. To investigate the process of laser propagation through clouds, a 3-D Monte Carlo radiative transfer model is used to simulate the photon path distribution and the Poisson distribution is adopted for the number of photon returns. Since the photon counting system only registers the time of the first arriving photon within the detector "dead time", the retrieved average surface elevation tends to bias towards higher values. This is known as the first photon bias. With the scenarios simulated here, the first photon bias for clear sky is about 6.5 cm. Clouds affect surface altimetry in two ways: (1) cloud attenuation lowers the average number of arriving photons and hence reduces the first photon bias; (2) cloud forward scattering increases the photon path length and makes the surface appear further away from the satellite. Compared to clear sky, the average surface elevation detected by the photon counting system for cloudy sky with optical depth 1.0 is 4.0 to 6.0 cm lower for the simulations conducted. The effect of surface roughness on the accuracy of elevation retrievals will also discussed.

Yang, Yuekui↗

Microphysics in the Multi-Scale Modeling Systems with Unified Physics

In recent years, exponentially increasing computer power has extended Cloud Resolving Model (CRM) integrations from hours to months, the number of computational grid points from less than a thousand to close to ten million. Three-dimensional models are now more prevalent. Much attention is devoted to precipitating cloud systems where the crucial 1-km scales are resolved in horizontal domains as large as 10,000 km in two-dimensions, and 1,000 x 1,000 km2 in three-dimensions. Cloud resolving models now provide statistical information useful for developing more realistic physically based parameterizations for climate models and numerical weather prediction models. It is also expected that NWP and mesoscale model can be run in grid size similar to cloud resolving model through nesting technique. Recently, a multi-scale modeling system with unified physics was developed at NASA Goddard. It consists of (l) a cloud-resolving model (Goddard Cumulus Ensemble model, GCE model), (2) a regional scale model (a NASA unified weather research and forecast, WRF), (3) a coupled CRM and global model (Goddard Multi-scale Modeling Framework, MMF), and (4) a land modeling system. The same microphysical processes, long and short wave radiative transfer and land processes and the explicit cloud-radiation, and cloud-surface interactive processes are applied in this multi-scale modeling system. This modeling system has been coupled with a multi-satellite simulator to use NASA high-resolution satellite data to identify the strengths and weaknesses of cloud and precipitation processes simulated by the model. In this talk, the microphysics developments of the multi-scale modeling system will be presented. In particular, the results from using multi-scale modeling system to study the heavy precipitation processes will be presented.

Tao, Wei-Kuo↗

An Improved Algorithm for Estimating Surface Shortwave Radiation: Preliminary Evaluation With MODIS Products

Cloud parameters, as key inputs in radiative transfer algorithms, have a critical impact on surface shortwave radiation (SSR) computation. By introducing a parameterization of cloud transmittance and reflectance, based on radiative transfer simulations, this study improves the accuracy of an existing physically based model which severely underestimates SSR under thick cloud conditions. The cloud parameterization adopts the single-layer cloud model and simulates cloud transmittances and reflectances by varying cloud optical thickness, cloud particle size, and solar zenith angle. The revised model is applied to estimate instantaneous SSR using Moderate-resolution Imaging Spectroradiometer (MODIS) atmospheric and land products. The retrieved SSR is evaluated against observation data from 41 Baseline Surface Radiation Network (BSRN) stations and is also compared with the MODIS official SSR product. The root mean square error (RMSE) of the estimated instantaneous radiation is approximately 52 and 98 W m -2 under clear-sky and all-sky conditions, respectively. The accuracy of the improved parameterization is higher than that of the original model, and there is no obvious underestimation of SSR in the case of high cloud optical thickness. Therefore, the new algorithm improves the accuracy of SSR estimates in the presence of thick clouds. Retrievals with the improved model also achieve higher accuracy than the MODIS official SSR product (MCD18A1). To conclude, the reliable performance of the scheme at most BSRN stations illustrates that the improved model can be used to map SSR on a global scale.

42 ENGINEERING↗

The Diurnal Cycle in TOGA-COARE: Regional Scale Model Simulations

The diurnal variation of precipitation processes over the tropics is a well-known phenomenon and has been studied using surface rainfall data, radar reflectivity data, and satellite-derived cloudiness and precipitation. Recently, Sui (1997) analyzed observations from TOGA COARE in the tropical western Pacific ocean to study the relevant mechanisms producing diurnal variation of precipitation. They found that the diurnal SST cycle is important for afternoon showers in the undisturbed periods and diurnal radiative processes for nocturnal rainfall. Takayabu (1996) found a quasi-2-day cycle in precipitation during TOGA COARE and they suggested that inertia-gravity waves may be associated with this 2-day cycle. Chen and Houze (1997), however, suggested that the quasi-2-day oscillation is mainly a function of the time required by the lower-tropospheric moisture field to recover from the drying caused by deep convection. In this study, the Penn State/NCAR Mesoscale Model (MM5) with improved physics (i.e., cloud microphysics, radiation, land-soil-vegetation-surface processes, and TOGA COARE flux scheme) and a multiple level nesting technique will be used to simulate two TOGA COARE convective espisodes, one convectively suppressed phase (mid to late January 1993) and one convectively active phase (mid to late December 1992). We will examine precipitation processes over the open ocean and over land by comparing MM5 simulated rainfall and out-going longwave radiation. By examining the OLR and precipitation, we can determine if there is a temporal lag between the maximum precipitation and the coldest upwelling longwave radiation (the time-lag between stratiform-cirrus and convective towers). The boundary layer response by (or recovery from) precipitation processes will also be shown by examining the PBL thermodynamic structure and the sensible and latent heat fluxes. A preliminary MM5 simulation showed a clear diurnal variation in rainfall over both land and open ocean for the convectively active phase. The results also indicated that a quasi-2-day cycle in precipitation was simulated only over part of the ocean.

Tao, W.-K.↗

Laboratory Studies of Cloud Particle Formation, Mixing State, and Physiochemical and Optical Properties of Carbonaceous Aerosols

Aerosol particles affect climate through direct and indirect interactions. In direct interactions, non-absorbing particles such as sulfate aerosols, backscatter solar radiation to space, leading to atmospheric cooling. By contrast, particles containing absorbing material such as refractory black carbon (rBC) produced during incomplete fuel combustion and to some extent also brown carbon components of biomass burning organic aerosol (BBOA) and secondary organic aerosol (SOA), absorb incoming solar radiation leading to atmospheric warming. Indirect effects include the ability of aerosol particles to alter the formation and properties of liquid water clouds (acting as cloud condensation nuclei or CCN) and ice clouds (acting as ice nuclei or IN), thereby affecting cloud albedo, coverage and lifetimes. The largest uncertainty in the modeling of climate impacts due to radiative forcing is caused by inadequate representation of aerosol-cloud interactions. The total radiative forcing on climate due to aerosol particles may be as large as that of the greenhouse gases, but predominantly opposite in sign (in the direction of cooling) and much more uncertain. All the direct and indirect radiative forcing effects may be influenced by the chemical composition of the particles.

54 ENVIRONMENTAL SCIENCES↗

Sensitivity Study for Forecasting Variables of WRF-Solar Using a Tangent Linear Approach

Integrating solar generation in recent years has highlighted the need for improved accuracy in predicting solar power. Confidence in solar power forecasting can be achieved by designing an ensemble that provides reliable probabilistic information for solar radiation with reduced uncertainty and error. Ideally, ensemble members are created through the optimized perturbation of the initial conditions in numerical weather prediction (NWP) models. Tangent linear models are capable of efficiently investigating the sensitivity of solar radiation to model input parameters because they do not require individual perturbation of each variable. This sensitivity study using tangent linear models provide us the capability to identify the right variables to perturb in an ensemble prediction system. In this study, we developed tangent linear models for WRF-Solar modules that directly impact the computation of solar radiation and the simulation of cloud formation and dissipation including the Fast All-sky Model for Solar Applications (FARMS), the Noah land surface model (LSM), the Thompson microphysics, the Mello-Yamada-Nakanishi-Niino (MYNN) boundary layer parameterization, and the Deng scheme for a shallow-convection parameterization. A sensitivity analysis was conducted under various scenarios based on satellite observations and model simulations from the National Solar Radiation Data Base (NSRDB) and WRF-Solar, respectively. Critical forecasting variables that are highly sensitive to the forecasting of global horizontal irradiance (GHI), direct normal irradiance (DNI), cloud mixing ratio, cloud tendency, cloud fraction, and sensible and latent heat fluxes were determined using the relevant WRF-Solar module. This study will be used as a guidance on future research leading to high-quality probabilistic solar forecasting. In this presentation, we discuss the validation of tangent linear approach for WRF-Solar modules and illustrate how the sensitivity results are valuable in the improvement of probabilistic solar prediction.

24 POWER TRANSMISSION AND DISTRIBUTION↗

X-ray emission from active galactic nuclei

It is often held that the X-ray emission from active galactic nuclei (AGN) arises from a region close to the central energy source. Thus X-ray observations may provide the best constraints on the central engine. In particular, the shape of the X-ray continuum gives information about the mechanism for photon generation, X-ray time variability data can constrain the size and mass of the continuum source, and X-ray occultation data give constraints on the relative sizes of the continuum source and the intervening absorbing material (often assumed to be the broad line clouds). In addition, since a fair fraction of the total energy of an AGN is emitted at X-ray wavelengths, direct measurement of the amount and spectral form of this radiation is important for modeling of the optically emitting clouds.

Mushotzky, R.↗

A Surface Radiation Balance Data Set from Siple Dome in West Antarctica for Atmospheric and Climate Model Evaluation

A field campaign at Siple Dome in West Antarctica during the austral summer 2019-2020 offers an opportunity to evaluate climate model performance, particularly cloud microphysical simulation. Over Antarctic ice sheets and ice shelves, clouds are a major regulator of the surface energy balance, and in the warm season their presence occasionally induces surface melt that can gradually weaken an ice shelf structure. This dataset from Siple Dome, obtained using transportable and solar-poweredequipment, includes surface energy balance measurements, meteorology and cloud remote sensing. To demonstrate how these data can be used to evaluate model performance, comparisons are made with meteorological reanalysis known to give generally good performance over Antarctica (ERA5). Surface albedo measurements show expected variability with observed cloud amount, and can be used to evaluate a model's snowpack parameterization. One case study discussed involves a squall with northerly winds, during which ERA5 fails to produce cloud cover throughout one of the days. A second case study illustrates how shortwave spectroradiometer measurements that encompass the 1.6-micron atmospheric window reveal cloud phase transitions associated with cloud lifecycle. Here, continuously precipitating mixed-phase clouds become mainly liquid water clouds from local morning through the afternoon, not reproduced by ERA5. We challenge researchers to run their various regional or global models in a manner that has the large-scale meteorology follow the conditions of this field campaign, compare cloud and radiation simulations with this Siple Dome dataset, and potentially investigate why cloud microphysical simulations or other model components might produce discrepancies with these observations.

cloud remote sensing↗

TPSAS-NF1676L-18074-DND

Motivations - Radiative Transfer (RT) model is a component in satellite remote sensing (Observation System Simulation Experiment, sensor performance end-to-end simulations or sensitivity studies, and retrieval and data assimilations); - Line-by-line RT model is too slow, over a million RT needed to cover infrared spectral region; - Traditional Channel-based RT models deal with one channel at a time. Modern sensors have thousands of channels and 0.1-1 million spectra per day, only 4-10% of data are used in satellite data assimilations (too slow for climate OSSE). It is essential to have a RT model: - Accurate and fast - Works in all spectral regions - Includes as accurate physics as possible - Takes advantage of spectral correlations - Can handle cloud and aerosols PCRTM (Principal Component-based Radiative Transfer model) was developed to satisfy the need listed above.

Xu Liu↗

Positive low cloud and dust feedbacks amplify tropical North Atlantic Multidecadal Oscillation

Abstract The Atlantic Multidecadal Oscillation (AMO) is characterized by a horseshoe pattern of sea surface temperature (SST) anomalies and has a wide range of climatic impacts. While the tropical arm of AMO is responsible for many of these impacts, it is either too weak or completely absent in many climate model simulations. Here we show, using both observational and model evidence, that the radiative effect of positive low cloud and dust feedbacks is strong enough to generate the tropical arm of AMO, with the low cloud feedback more dominant. The feedbacks can be understood in a consistent dynamical framework: weakened tropical trade wind speed in response to a warm middle latitude SST anomaly reduces dust loading and low cloud fraction over the tropical Atlantic, which warms the tropical North Atlantic SST. Together they contribute to the appearance of the tropical arm of AMO. Most current climate models miss both the critical wind speed response and two positive feedbacks though realistic simulations of them may be essential for many climatic studies related to the AMO.

58 GEOSCIENCES↗

Evaluation of WRF-Solar Cloud Forecast Using the NSRDB: Preprint

Cloud forecast is a crucial component in predicting solar irradiance from numerical weather prediction (NWP) models. Assessing cloud properties from the NWP models requires significant work due to the need for high-quality data, spatial analysis covering model extent, and detailed analysis of model performance for different types of clouds. This study presents an evaluation of the WRF-Solar cloud forecast using the National Solar Radiation Database (NSRDB). We propose an evaluation framework applied to a single model prediction as well as ensemble-based forecasts. Various cloud detection metrics are calculated when comparing with the satellite-derived dataset. The mismatched clouds from the WRF-Solar model are quantified using nine cloud types classified by cloud top height and cloud optical depth. The results based on the WRF-Solar forecasts covering the entire U.S. for the full year of 2018 shows mismatched cloud frequency in the range of 8% - 46% for thick and high-level (deep convective) to thin and low-level (cumulus) clouds.

cloud mask forecast↗

Outer satellite atmospheres: Their extended nature and planetary interactions

Highly developed numerical models are applied to interpret extended-atmosphere data for the sodium cloud of Io and the hydrogen torus of Titan. Solar radiation pressure was identified and verified by model calculations as the mechanism to explain two different east-west asymmetries observed in the sodium cloud. Analysis of sodium line profile data, suggesting that a Jupiter magnetospheric wind may be responsible for high speed sodium atoms emitted from Io, and preliminary modeling of the interaction of the Io plasma torus and Io's sodium cloud are also reported. Models presented for Titan's hydrogen torus are consistent both with the recent Pioneer 11 measurements and earlier Earth-orbiting observations by the Copernicus satellite. Progress is reported on developing models for extended gas and dust atmospheres of comets.

Smyth, W. H.↗

Dynamics, thermodynamics, radiation, and cloudiness associated with cumulus-topped marine boundary layers

The overall goal of this project was to improve the understanding of marine boundary clouds by using data collected at the Atmospheric Radiation Measurement (ARM) sites, so that they can be better represented in global climate models (GCMs). Marine boundary clouds are observed regularly over the tropical and subtropical oceans. They are an important element of the Earth’s climate system because they have substantial impact on the radiation budget together with the boundary layer moisture, and energy transports. These clouds also have an impact on large-scale precipitation features like the Inter Tropical Convergence Zone (ITCZ). Because these clouds occur at temporal and spatial scales much smaller than those relevant to GCMs, their effects and the associated processes need to be parameterized in GCM simulations aimed at predicting future climate and energy needs. Specifically, this project’s objectives were to (1) characterize the surface turbulent fluxes, boundary layer thermodynamics, radiation field, and cloudiness associated with cumulus-topped marine boundary layers; (2) explore the similarities and differences in cloudiness and boundary layer conditions observed in the tropical and trade-wind regions; and (3) understand similarities and differences by using a simple bulk boundary layer model. In addition to working toward achieving the project’s three objectives, we also worked on understanding the role played by different forcing mechanisms in maintaining turbulence within cloud-topped boundary layers We focused our research on stratocumulus clouds during the first phase of the project, and cumulus clouds during the rest of the project. Below is a brief description of manuscripts published in peer-reviewed journals that describe results from our analyses.

54 ENVIRONMENTAL SCIENCES↗