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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 631 records · Page 35

DOE/NNSA Nuclear Criticality Safety Program – Brief Overview [Slides]

This presentation discusses nuclear data measurements and evaluation work for the NCSP. The objective of the NCSP is to provide measured and evaluated thermal, resonance, unresolved resonance, and fast region cross section data to address the priority NCSP nuclear data needs. It also discusses its vision which is to address multiple Nuclear Data 5- and 10-year goals and attributes identified in the NCSP. The intended final product is for rigorous ENDF/B evaluations to be produced from cross section measurements and analyses. It also discusses NCSP integral experiments and differential experiments in addition to NCSP support of SCALE in the future.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

SFCOMPO Database of Spent Nuclear Fuel Assay Data – the Next Frontier

SFCOMPO is the world’s largest database for measured spent nuclear fuel assay data. An international effort coordinated by the Nuclear Energy Agency (NEA) resulted in a significant expansion of the database and its release online in 2017 as a downloadable application. The SFCOMPO Technical Review Group (TRG) was recently formed under the direction of NEA’s Nuclear Science Committee/Working Party on Nuclear Criticality Safety and was mandated to maintain and further coordinate the development of SFCOMPO. This TRG is currently focused on (1) critical evaluation of the experimental assay data by independent experts and (2) development of benchmarks and benchmark models that can be applied to validate burnup codes. This will improve the quality and documentation of the experimental datasets and enable their use by the international community to support code validation for design and safety analysis of spent nuclear fuel transportation, storage, and repository applications. It follows the precedent and draws on the experience gained from similar NEA efforts in the International Reactor Physics Experiment Evaluation Project and the International Criticality Safety Benchmark Experiment Project. Ongoing SFCOMPO evaluations have served as a test bed to develop templates for documenting evaluations, develop review guidance, improve approaches for a global uncertainty analysis, and devise a strategy focused on providing practical information of highest value to the user community. The current effort, status, and associated challenges are discussed.

Ilas, Germina↗

Analysis of a Bulk 237 Np Oxide Sample for Trace Actinides

A neptunium oxide sample was dissolved and trace actinide constituents were measured by isotope dilution ICP-MS (for 239–244 Pu, 233–238 U, 237 Np, 241–243 Am) and alpha spectrometry ( 238 Pu, 242 Cm, 244 Cm). This material contained significant quantities of transuranic elements, notably americium and curium. The isotopic composition of the material will continue to evolve over time due to radioactive decay; the measurements reported here include all isotopes decay corrected to a reference date of 1/1/2022. These factors may be considerations in criticality studies of the related 237 Np sphere.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Uncertainty-informed selection of CMIP6 Earth System Model subsets for use in multisectoral and impact models

Earth system models (ESMs) and general circulation models (GCMs) are heavily used to provide inputs to sectoral impact and multisector dynamic models, which include representations of energy, water, land, economics, and their interactions. Therefore, representing the full range of model uncertainty, scenario uncertainty, and interannual variability that ensembles of these models capture is critical to the exploration of the future co-evolution of the integrated human–Earth system. The pre-eminent source of these ensembles has been the Coupled Model Intercomparison Project (CMIP). With more modeling centers participating in each new CMIP phase, the size of the model archive is rapidly increasing, which can be intractable for impact modelers to effectively utilize due to computational constraints and the challenges of analyzing large datasets. In this work, we present a method to select a subset of the latest phase, CMIP6, featuring models for use as inputs to a sectoral impact or multisector dynamics models, while prioritizing preservation of the range of model uncertainty, scenario uncertainty, and interannual variability in the full CMIP6 ensemble results. This method is intended to help impact modelers select climate information from the CMIP archive efficiently for use in downstream models that require global coverage of climate information. This is particularly critical for large-ensemble experiments of multisector dynamic models that may be varying additional features beyond climate inputs in a factorial design, thus putting constraints on the number of climate simulations that can be used. We focus on temperature and precipitation outputs of CMIP6 models, as these are two of the most used variables among impact models, and many other key input variables for impacts are at least correlated with one or both of temperature and precipitation (e.g., relative humidity). Besides preserving the multi-model ensemble variance characteristics, we prioritize selecting CMIP6 models in the subset that preserve the very likely distribution of equilibrium climate sensitivity values as assessed by the latest Intergovernmental Panel on Climate Change (IPCC) report. This approach could be applied to other output variables of climate models and, possibly when combined with emulators, offers a flexible framework for designing more efficient experiments on human-relevant climate impacts. It can also provide greater insight into the properties of existing CMIP6 models.

Snyder, Abigail C.↗

Nuclear Criticality Safety Program @ ORNL [Slides]

This presentation provides an overview of the Nuclear Criticality Safety Program (NCSP) and its activities at Oak Ridge National Lab, including the program's history, mission and vision, accomplishments, challenges, initiatives, and tasks, as well as information regarding ORNL's NCSP budget.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Probing the electronic properties of the electrified silicon/water interface by combining simulations and experiments.

Silicon (Si) is broadly used in electrochemical and photoelectrochemical devices, where the capacitive and Faradaic reactions at the Si/water interfaces are critical for signal transduction or noise generation. However, probing the electrified Si/water interface at the microscopic level remains a challenging task. Here we focus on hydrogenated Si surfaces in contact with water, relevant to transient electronics and photoelectrochemical modulation of biological cells and tissues. We show that by carrying out first principles molecular dynamics simulations of the Si(100)/water interface in the presence of an electric field we can realistically correlate the computed flat-band potential and tunneling current images at the interface with experimentally measured capacitive and Faradaic currents. Specifically, we validate our simulations in the presence of bias by performing pulsed chronoamperometry measurements on Si wafers in solution. Consistent with prior experiments, our measurements and simulations indicate the presence of voltage-dependent capacitive currents at the interface. We also find that Faradaic currents are weakly dependent on the applied bias, which we relate to surface defects present in newly prepared samples.

Ye, Zifan↗

Reactor physics benchmark experiments at the JSI TRIGA MARK II reactor - Current status and future outlook

Full text of publication follows. With the development of new high-fidelity computational methods, improvement of nuclear data, and multiphysics modelling, there is an increased need for benchmark experiments to experimentally validate the models, methods and input data. Many of the nuclear facilities designed to perform reactor physics benchmark experiments have been shut down. Therefore, research reactors offer a great opportunity for benchmark experiments, if they are well designed and performed with great care and accuracy. In this presentation we provide an overview of the past and ongoing activities related to benchmark experiments at the Jozef Stefan Institute TRIGA Mark II research reactor. The following experiments have been performed: criticality with fresh fuel, {sup 197}Au(n,γ) and {sup 27}Al(n,α) reaction rates in irradiation channels, absolute and relative {sup 197}Au(n,γ), {sup 235}U(n,f) and {sup 238}U(n,f) reaction rates in the core, burnup, kinetic parameters, control rod worth, isothermal reactivity coefficient, self-shielding, slow and fast (pulse) transients, nuclear heating, delayed and prompt gamma ray production, temperature profiles for multi-physics. Since the existing fleet of research reactors is ageing very rapidly and new experiments are needed, new research reactors should be designed and built to meet the needs of future advanced reactors, education and training, and other technologies in the coming years. We will review planned activities at the JSI TRIGA reactors and plans for the new research reactor in Slovenia. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Neutronics analysis of Full Size Plate–1 Experiment using MC21

Qualification and testing of Low Enriched Uranium fuel is desired so that it can be used in research reactors instead of High Enriched Uranium. The Full Size Plate - 1 (FSP-1) experiment involves irradiating a low enriched metallic fuel in the Advanced Test Reactor to assist in this general qualification. Prior to irradiation, an in-depth neutronics analysis is needed to ensure the safety requirements of the Advanced Test Reactor are met. To accomplish this, the MC21 software was used to analyze the FSP-1 experiment, which will allow a test run to be performed with this new fuel in the Advanced Test Reactor Critical facility. By verifying and validating the results of the MC21 software with comparisons to other codes and the preliminary irradiation in the Advanced Test Reactor Critical facility, the FSP-1 experiment will be ready to irradiate using the Advanced Test Reactor. This work is concerned with the neutronics analysis of the FSP-1 experiment using the MC21 software.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Jemima Plate Characterization

The HEU Jemima plates have been utilized in numerous International Criticality Safety Benchmark Evaluation Project (ICSBEP) evaluations. ICSBEP evaluations are a vital com ponent of nuclear data validation for applications across the nuclear community. In the past, different combinations of mass, caliper measurements, and drawing dimensions have been used to define the HEU Jemima plates in ICSBEP evaluations. Some of these combinations result in large density ranges (17 g/cm 3 to 19 g/cm 3 ) or unrealistic densities (greater than 19 g/cm 3 ). Additionally, oxidation of the plates has led to questioning the flatness of each plate, which can add additional gaps in experiment configurations. This work proposes a standardized method of defining the commonly used HEU Jemima plates across different experiments.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Studies on the scintillation light detection in the ProtoDUNE Dual Phase liquid-argon TPC and its capability for the supernova trigger in DUNE

The Deep Underground Neutrino Experiment (DUNE) is a long-baseline neutrino oscillation experiment that aims at addressing key questions in neutrino physics in the next decades. Its scientific program includes the detection of the neutrino flux from a core-collapse supernova. The DUNE far detector will have four 17-kt mass liquid-argon (LAr) time-projection chamber (TPC) modules. ProtoDUNE Dual Phase (DP), a dual-phase LAr TPC with 300 t of active mass and 6 m of drift distance, was operated with cosmic muons in 2019-2020 as part of an R&D program at the CERN Neutrino Platform to demonstrate the feasibility of the technology at such a large scale. In a LAr TPC, the photon detection system (PDS) provides fun- damental timing information and trigger capabilities. The PDS of ProtoDUNE-DP, which consisted of 36 photomultiplier tubes (PMTs), counted on a dedicated light calibration system (LCS) to monitor the PMT response. In this dissertation, the characterization and validation of the ProtoDUNE-DP PDS and LCS components before their installation will be reviewed, highlighting the results of general interest for experiments that use liquid noble gasses as target medium. The results from the stable performance of both systems in the detector during 15 months will be presented next as well as the studies on the scintillation light detection in ProtoDUNE-DP, where the collection of light produced in LAr at 7 m from the photosensors has been achieved for the first time. It is worth pointing out that the excellent LAr purity and the large size of the detector have enabled to develop a unique data-driven investigation on aspects that are critical for LAr- based experiments but that are not completely understood. The analyses cover the characterization of the low-energy background detected by the PDS, the quantification of the electric field impact on the light yield, the evaluation of the Rayleigh scattering affecting the light propagation, and the analysis of the PMT detection efficiency. The effect of the VUV reflectivity of the detector materials will be also discussed. In addition, the estimation of the cosmic muon flux crossing the TPC and the study of the observed light yield by the PDS will be reported. Finally, the results from the simulation-based study of the supernova burst trigger capability with the PDS of a 12.1-kt active mass dual-phase LAr TPC as the one proposed for DUNE will be summarized. Several configurations of reflective foils installed in the TPC to enhance the light collection will be compared

Gallego-Ros, Ana↗

Update on Benchmark Analysis of Component Critical Configurations of KRUSTY

Kilowatt Reactor Using Stirling Technology (KRUSTY) is prototype designed as a proof of concept for NASA’s Kilo power program, which was funded in order to create a small reactor for various space applications such as providing power for a colony on Mars or the moon and eventually as a possible option for powering rockets on deep space missions. Before the final prototype design was tested in March 2018, the component critical configuration, which had less external equipment than the prototype design, was created in November 2017. Both of these designs had less external equipment than the final version will have. This component critical con figuration was used to determine the worth of the beryllium oxide (BeO) reflector and of the boron carbide (B4C) control rod as well as creating necessary benchmark configurations.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

MTA Secondary Beamline Production and Optics Optimization

A new secondary beamline was recently installed in the MeV Test Area (MTA) with the objective of enhancing mu+/mu- production by factors of 3/8 by using a tungsten target versus the conventional graphite production target using the 400 MeV Fermilab proton Linac beam. Ultra-low energy muon beams can support world-class physics experiments for fundamental muon measurements, sensitive searches for symmetry violation, and precision tests of theory. Extensive production studies have confirmed higher muon yield from heavy targets (tungsten vs carbon), but also, surprisingly, showed significant differences in production fluence and energy spectrum between modern hadronic models (GENIEhad) and between GEANT and MCNP. Studies are also underway towards a high-efficiency source of muonium by stopping the mu+ beam in superfluid helium. Muon fluxes can be measured at MTA including using higher-Z and novel target geometries to test hadronic and production models which are critical to understanding ongoing experiments (Mu2e) and will significantly impact the planning of future HEP experiments and planning PIP II facilities. The MTA beamline will additionally support a broad user muon test beam for future experiments and R&D.

Ahmed, Shiza↗

Thermodynamic signatures of an antiferromagnetic quantum critical point inside a superconducting dome

Recent experiments in unconventional superconductors, and in particular iron-based materials, have reported evidence of an antiferromagnetic quantum critical point (AFM-QCP) emerging inside the superconducting dome of the phase diagram. Fluctuations associated with such an AFM-QCP are expected to promote unusual temperature dependencies of thermodynamic quantities. Here, we compute the T dependence of the specific heat C(T) deep inside a fully gapped s +– superconducting state as the AFM-QCP is approached. We find that at the AFM-QCP, the specific heat C(T) vanishes quadratically with temperature, as opposed to the typical exponential suppression seen in fully gapped BCS superconductors. This robust result is due to a nonanalytic contribution to the free energy arising from the general form of the bosonic (AFM) propagator in the SC state. Away from the AFM-QCP, as temperature is lowered, C(T) shows a crossover from a T2 behavior to an exponential behavior, with the crossover temperature scale set by the value of the superconducting gap and the distance to the QCP. As a result, we argue that these features in the specific heat can be used to unambiguously determine the existence of AFM-QCPs inside the superconducting domes of iron-based and other fully gapped unconventional superconductors.

36 MATERIALS SCIENCE↗

Hydrokinetic Turbines in Yawed Conditions: Toward Synergistic Fluvial Installations

Laboratory experiments were performed in critical mobility conditions to study the effects of an in-stream horizontal axis turbine in yawed conditions. The misalignment between the rotor axis and the incoming flow velocity is observed to alter the near and far wake of the turbine, as well as the scour and deposition patterns in the proximity of the monopile support tower. Various hydraulic conditions may lead to such misalignment, e.g., as a result of complex fluvial bathymetries distorting the flow or as a strategy to steer the wake away from downstream units and maximize energy production in a turbine array. The research first investigates the simplest case of a single turbine deployed along the channel centerline and oriented at different yaw angles to study the wake deflection and the turbine performance. A second set of experiments is performed moving the turbine relatively close to a nonerodible lateral wall to explore a potential passive yaw control strategy devoted to protect the banks from erosion by steering the wake toward the channel center and favor deposition along the bank.

42 ENGINEERING↗

Development and Validation of a Two-Phase Thermal-Hydraulic CFD Code NEK-2P

A project is underway to develop, verify and validate an advanced two-phase flow modeling capability for the highly-scalable, high-performance Computational Fluid Dynamics (CFD) code NEK5000. The goal of this work is to verify and validate the two-phase version of the NEK5000 code, named NEK-2P, to simulate the two-phase flow and heat transfer phenomena that occur in a Boiling Water Reactor (BWR) fuel bundle under various operating conditions. The NEK-2P two-phase flow models follow the approach used for the Extended Boiling Framework (EBF) previously developed at Argonne but include more fundamental physical models of boiling phenomena and advanced numerical algorithms for improved computational accuracy, robustness, and computational speed. The development of the NEK-2P two-phase solver and the implementation of the Extended Boiling Framework two-phase models were initially supported by Argonne National Laboratory (Argonne) through a Laboratory Directed Research and Development (LDRD) project during FY2014-2016. The development and validation of the two-phase models through analyses of selected two-phase boiling flow experiments was supported by the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program in FY2017-2020. This report focuses on verification and validation of the water-steam boiling model NEK-2P Two-Phase, CFD code. The NEK-2P was validated with Nuclear Power Engineering Corporation (NUPEC) Pressurized Water Reactor (PWR) Sub-channel and Bundle Test (PSBT) void distribution benchmark. Three different simulations were performed and analyzed for various operating conditions such as wall-heat flux and sub-cooled inlet temperatures. Reasonably good agreement with measured data was obtained in predicting the measured void distributions. Simulations were performed for Virginia Tech. (VT) 3x3 rod bundle geometry with and without spacers. The preliminary results were presented for Simplified Spacer Grid (SSG). In addition, the implementation of interface reconstruction model was tested with one of the Becker benchmark Critical Heat Flux (CHF) experiments.

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

Nuclear Data Sensitivity/Uncertainty Studies of Tantalum-Reflected Systems

Tantalum (Ta) is a refractory metal with high melting point and high corrosion resistance. This makes it useful as a mold material for plutonium casting operations. Unfortunately, there are few criticality benchmarks with high nuclear data sensitivities. Given that, it is desirable to design new experiments to provide additional validation data for nuclear criticality safety, which is the objective of the Thales project. Multiple application models were used to represent process conditions (either normal conditions or credible upset conditions) both at Los Alamos National Laboratory (LANL) and Savannah River Site (SRS). A total of 40 application models were obtained. Given this, it was useful to down-select the number of needed application models. This work documents the down-selection based on several nuclear data sensitivity/uncertainty metrics. In addition to showing the result of the specific down-selection used for the Thales project, this work discusses potential ways to represent a large number of application models with a smaller number of proposed experiment designs.

42 ENGINEERING↗

Rossi-alpha Uncertainty Quantification by Analytic, Bootstrap, and Sample Methods to Inform Fitting Best Practices

The prompt neutron period (the negative reciprocal of the prompt neutron decay constant) can be estimated using the Rossi-alpha technique that is predicated on fitting Rossi alpha histograms and of interest in nuclear criticality safety and nonproliferation. The histograms are traditionally fit with a one-exponential model; however, recent work has proposed a two-exponential model to account for reflector induced phenomenon. Until recently, the uncertainty quantification for either model was inadequate (inaccurate and demanded large measurement times). Measurement uncertainty quantification by sample and analytic methods was developed and validated in Ref. The purpose of this transaction is to (i) validate a new bootstrap method by comparing bin-by-bin error bar estimates and (ii) demonstrate how to choose bin widths and reset times to optimize precision and accuracy.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗