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At least 631 records · Page 35

Broadband titanium nitride disordered metasurface absorbers

We experimentally demonstrate titanium nitride (TiN) broadband metasurface perfect absorbers by conformally coating plasmonic TiN films onto disordered anodic aluminum oxide (AAO) nanotemplates. The disordered metasurface absorbers exhibit polarization-insensitive and weak angle-dependent perfect absorption over the entire visible and near-infrared spectral regions (300 < λ < 2500 nm). We show from experimental results and numerical simulations that the light scattering induced by the strong disorder of the AAO nanopores and the strong absorption of the TiN deposited on their sidewall are of critical importance for achieving broadband perfect absorption. The TiN disordered metasurface perfect absorbers are superior to many other types of broadband perfect absorbers previously reported and are more suitable for practical applications especially in harsh environments. The device concept for broadband perfect absorption based on plasmonic metal-nitride film coated disordered dielectric media could potentially be extended to significantly enhance the efficiency of solar energy harvesting and the performance of hot-carrier based optoelectronics.

Chang, Chun-Chieh (ORCID:0000000337282454)↗

Investigating controls on sea ice algal production using E3SMv1.1-BGC

We present the analysis of global sympagic primary production (PP) from 300 years of pre-industrial and historical simulations of the E3SMv1.1-BGC model. The model includes a novel, eight-element sea ice biogeochemical component, MPAS-Seaice zbgc, which is resolved in three spatial dimensions and uses a vertical transport scheme based on internal brine dynamics. Modeled ice algal chlorophyll-a concentrations and column-integrated values are broadly consistent with observations, though chl-a profile fractions indicate that upper ice communities of the Southern Ocean are underestimated. Simulations of polar integrated sea ice PP support the lower bound in published estimates for both polar regions with mean Arctic values of 7.5 and 15.5 TgC/a in the Southern Ocean. However, comparisons of the polar climate state with observations, using a maximal bound for ice algal growth rates, suggest that the Arctic lower bound is a significant underestimation driven by biases in ocean surface nitrate, and that correction of these biases supports as much as 60.7 TgC/a of net Arctic PP. Simulated Southern Ocean sympagic PP is predominantly light-limited, and regional patterns, particularly in the coastal high production band, are found to be negatively correlated with snow thickness.

54 ENVIRONMENTAL SCIENCES↗

Partial Wave Analysis of Meson Resonances That Decay K*K¯ Using Data from the GlueX Experiment

The GlueX experiment housed in Hall D of the Thomas Jefferson National Laboratory was created to map the light meson spectrum in order to contribute to the Standard Model of particle physics by strengthening our understanding of the strong interaction. GlueX is a medium-energy photoproduction experiment that utilizes a linearly polarized photon beam to create hadronic forms of matter.

Cole, Sebastian↗

Broadband fibre-pigtailed acousto-optic frequency shifter

A two-crystal fibre-pigtailed acousto-optic frequency shifter has been developed and investigated. An optimal configuration of acousto-optic cells is chosen. A two-crystal acousto-optic frequency shifter of 785-nm laser radiation in the range from 156 to 196 MHz, with single-mode polarisation maintaining fibres at the input and output, is described. Some recommendations are given how to improve the shifter transmission coefficient and increase the frequency shift range. (acousto-optic modulation of light)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Radiation by a laser-driven flying-focus electron wave packet

An exact solution of the Dirac equation in the presence of an arbitrary electromagnetic plane wave is found, which corresponds to a focused electron wave packet, with the focus of the wave packet moving at the speed of light in the opposite direction of the average momentum of the electron wave packet (unless the plane wave is so intense to reflect the electron). The photon spectrum emitted by such an electron wave packet in the presence of a linearly polarized plane wave is studied both analytically and numerically. The spectrum is also compared with the one emitted by a single-momentum, plane-wave electron in the case of the electron being initially counterpropagating (on average for the flying-focus case) with the plane wave and within the locally constant field approximation. It is found that if the electron flying-focus wave packet is focused beyond a Compton wavelength, the angular distribution of the emitted radiation along the magnetic field of the electromagnetic plane wave is broader than for an electron with definite momentum. Corresponding the maximum value of the photon yield on the transverse plane is smaller in the flying-focus electron case. This could represent an experimental signature of a laser-driven flying-focus electron wave packet.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Comparison of spontaneous emission in trapped-ion multiqubit gates at high magnetic fields

Penning traps have been used for performing quantum simulations and sensing with hundreds of ions and provide a promising route toward scaling up trapped ion quantum platforms because of the ability to trap and control hundreds or thousands of ions in two- and three-dimensional crystals. In both Penning traps and the more common RF Paul traps, lasers are often used to drive multi-qubit entangling operations. A leading source of decoherence in these operations is off resonant spontaneous emission. While many trapped ion quantum computers or simulators utilize clock qubits, other systems, especially those with high magnetic fields such as Penning traps, rely on Zeeman qubits, which require a more complex calculation of this decoherence. We therefore examine theoretically the impacts of spontaneous emission on quantum gates performed with trapped-ion ground state Zeeman qubits in a high magnetic field. In particular, we consider two types of gates—light-shift ($\hat{σ}^z_i$ $\hat{σ}^z_j$) gates and Mølmer-Sørensen ($\hat{σ}^x_i$ $\hat{σ}^x_j$) gates—obtained with laser beams directed approximately perpendicular to the magnetic field (the quantization axis) and compare the decoherence errors in each. Within each gate type, we also compare different operating points with regards to the detunings, polarizations, and required intensity of the laser beams used to drive the gates. Here, we show that both gates can have similar performance at their optimal operating conditions at high magnetic fields and examine the experimental feasibility of various operating points. By examining the magnetic field dependence of each gate, we demonstrate that, when the P state fine structure splitting is large compared to the Zeeman splittings, the theoretical performance of the Mølmer-Sørensen gate is significantly better than that of the light-shift gate. Additionally, for the light-shift gate, we make an approximate comparison between the fidelities that can be achieved at high fields with the fidelities of state-of-the-art two-qubit trapped ion quantum gates. We show that, with regards to spontaneous emission, the achievable fidelity of the current NIST configuration is about an order of magnitude below that of the best low-field gates, but we also discuss several alternative configurations with potential error rates that are comparable with those for state-of-the art trapped ion gates.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Observation of Polarization-Dependent Changes in Higher-Order Mode Responses as a Function of Transverse Beam Position in Tesla-Type Cavities at FAST

Higher-order modes (HOMs) in superconducting rf cavities present problems for an electron bunch traversing the cavity in the form of long-range wakefields from previous bunches. These may dilute the emittance of the macropulse average, especially with low emittance beams at facilities such as the European X-ray Free-electron Laser (XFEL) and the upgraded Linac Coherent Light Source (LCLS-II). Here we present observations of HOMs driven by the beam at the Fermilab Accelerator Science and Technology (FAST) facility. The FAST facility features two independent TESLA-type cavities (CC1 and CC2) after a photocathode rf gun followed by an 8-cavity cryomodule. The HOM signals were acquired from cavities using bandpass filters of 1.75 ± 0.15 GHz, 2.5 ± 0.2 GHz, and 3.25 ± 0.2 GHz and recorded using an 8-GHz, 20 GSa/s oscilloscope. The frequency resolution obtained is sufficient to separate polarization components of many of the HOMs. These HOM signals were captured from CC1 and cavities 1 and 8 of the cryomodule for various initial trajectories through the cavities, and we observe correlations between trajectory, HOM signals, and which polarization component of a mode is affected.

Thurman-Keup, Randy Michael↗

The CLAS12 High Threshold Cherenkov Counter

The High Threshold Cherenkov Counter (HTCC) is one of the detector systems of the CLAS12 spectrometer, and is used to generate a fast trigger signal in electron scattering experiments in the polar angle range from 5°to 35°. The HTCC is installed in front of the drift chambers and introduces a minimal amount of additional material within the acceptance. The HTCC is one unit whose core component is a multifocal mirror that consists of 60 lightweight ellipsoidal mirrors. It is important that the HTCC provides efficient coverage of the CLAS12 forward acceptance with no gaps. In order to achieve this, each sector of the CLAS12 Forward Detector is covered by 2 identical half-sector mirrors that focus Cherenkov light on 8 phototubes. The HTCC has a total of 48 channels with Electron Tubes 9823QKB photomultipliers that have a 5-in quartz face plate to detect Cherenkov light. The system provides rejection of charged -mesons with momenta below 4.8 GeV for the reliable identification of scattered electrons. In this paper the details of the design, construction, calibration, and performance results of the HTCC are presented

Sharabian, Y. G.↗

The CLAS12 Central Time-of-Flight system

The Central Time-of-Flight system for the large-acceptance CLAS12 spectrometer in Hall B at the Thomas Jefferson National Accelerator Facility is described. The system consists of a hermetic barrel of 48 scintillation counters at a radius of 25 cm from the beamline. The wedge-shaped counters are 3.4 cm wide, 3.0 cm thick, and 90 cm long, and span a range of polar angles relative to the center of the nominal target location from roughly 35° to 125°. The counters reside in the 5-T field of the CLAS12 superconducting solenoid. The bars are read out via bent light guides 1 m long on the upstream end of the counters and 1.6 m long on the downstream end. The phototubes are shielded by a multi-layer dynamical magnetic shield system to reduce the local fringe fields in the range from 400 G to 1000 G down to the level of 0.2 G at the location of the photocathodes. The average effective time resolution of the counters is 80 ps.

47 OTHER INSTRUMENTATION↗

Active Plasmonics and Active Chiral Plasmonics through Orientation-Dependent Multipolar Interactions

While most active plasmonic efforts focus on responsive metamaterials to modulate optical response, we present a simple alternative based on applied orientation control that can likely be implemented for many passive plasmonic materials. Passive plasmonic motifs are simpler to prepare but cannot be altered postfabrication. Here, we show that such systems can be easily manipulated through substrate orientation control to generate both active plasmonic and active chiral plasmonic responses. Using gold nanocrescents as our model platform, we demonstrate tuning of optical extinction from -21% to +36% at oblique incidence relative to normal incidence. Variation of substrate orientation in relation to incident polarization is also demonstrated to controllably switch chiroptical handedness (e.g., Δg = ± 0.55). These active plasmonic responses arise from the multipolar character of resonant modes. In particular, we correlate magnetoelectric and dipole–quadrupole polarizabilities with different light-matter orientation-dependence in both near- and far-field localized surface plasmon activity. Additionally, the attribution of far-field optical response to higher-order multipoles highlights the sensitivity offered by these orientation-dependent characterization techniques to probe the influence of localized electromagnetic field gradients on a plasmonic response. The sensitivity afforded by orientation-dependent optical characterization is further observed by the manifestation in both plasmon and chiral plasmon responses of unpredicted structural nanocrescent variance (e.g., left- and right-tip asymmetry) not physically resolved through topographical imaging.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Spatially co-registered wide-field nonlinear optical imaging of living and complex biosystems in a total internal reflection geometry

Nonlinear optical microscopy that leverages an objective based total internal reflection (TIR) excitation scheme is an attractive means for rapid, wide-field imaging with enhanced surface sensitivity. Through select combinations of distinct modalities, one can, in principle, access complementary chemical and structural information for various chemical species near interfaces. Here, we report a successful implementation of such a wide-field nonlinear optical microscope system, which combines coherent anti-Stokes Raman scattering (CARS), two-photon fluorescence (TPF), second harmonic generation (SHG), and sum frequency generation (SFG) modalities on the same platform. The intense optical fields needed to drive these high order nonlinear optical processes are achieved through the use of femtosecond pulsed light in combination with the intrinsic field confinement induced by TIR over a large field of view. The performance of our multimodal microscope was first assessed through the experimental determination of its chemical fidelity, intensity and polarization dependences, and spatial resolution using a set of well-defined model systems. Subsequently, its unique capabilities were validated through imaging complex biological systems, including Hydrangea quercifolia pollen grains and Pantoea sp. YR343 bacterial cells. Specifically, the spatial distribution of different molecular groups in the former was visualized via vibrational contrast mechanisms of CARS, whereas co-registered TPF imaging allowed the identification of spatially localized intrinsic fluorophores. We further demonstrate the feasibility of our microscope for wide-field CARS imaging on live cells through independent characterization of cell viability using spatially co-registered TPF imaging. Overall, this approach to TIR enabled wide-field imaging is expected to provide new insights into bacterial strains and their interactions with other species in the rhizosphere in a time-resolved and chemically selective manner.

47 OTHER INSTRUMENTATION↗

Zero curvature is a necessary and sufficient condition for a spin-orbital decomposition

There has been an extended debate regarding the existence of a spin-orbital decomposition of the angular momentum of photons and other massless particles. It was recently shown that there are both geometric and topological obstructions preventing any such decomposition. Here we show that any geometric connection on a particle’s state space induces a splitting of the angular momentum into two operators. These operators are well-defined angular momentum operators if and only if the connection has zero curvature. Massive particles have two canonical curved connections corresponding to boosts and rotations, respectively. Furthermore, these can be uniquely combined to produce a flat connection, and this gives a novel derivation of the Newton-Wigner position operator and the corresponding spin and orbital angular momenta for relativistic massive particles. When the mass is taken to zero, transverse boosts and rotations degenerate, leaving only a single connection for massless particles. This connection produces a commonly proposed splitting of the massless angular momentum into two operators. However, the connection is not flat, explaining why these operators do not satisfy the angular momentum commutation relations and are thus not true spin and orbital angular momentum operators.

Angular momentum↗

Self-interacting neutrinos, the Hubble parameter tension, and the cosmic microwave background

Here, we perform a comprehensive study of cosmological constraints on nonstandard neutrino self-interactions using cosmic microwave background and baryon acoustic oscillation data. We consider different scenarios for neutrino self-interactions distinguished by the fraction of neutrino states allowed to participate in self-interactions and how the relativistic energy density, N eff , is allowed to vary. Specifically, we study cases in which all neutrino states self-interact and N eff varies; two species free-stream, which we show alleviates tension with laboratory constraints, while the energy in the additional interacting states varies; and a variable fraction of neutrinos self-interact with either the total N eff fixed to the Standard Model value or allowed to vary. In no case do we find compelling evidence for new neutrino interactions or nonstandard values of N eff . In several cases, we find additional modes with neutrino decoupling occurring at lower redshifts z dec ~ 10 3–4 . We do a careful analysis to examine whether new neutrino self-interactions solve or alleviate the so-called H 0 tension and find that, when all Planck 2018 CMB temperature and polarization data are included, none of these examples eases the tension more than allowing a variable N eff comprised of free-streaming particles. Although we focus on neutrino interactions, these constraints are applicable to any light relic particle.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Cosmic-ray Antinuclei as Messengers of New Physics: Status and Outlook for the New Decade

The precise measurement of cosmic-ray antinuclei serves as an important means for identifying the nature of dark matter and other new astrophysical phenomena, and could be used with other cosmic-ray species to understand cosmic-ray production and propagation in the Galaxy. For instance, low-energy antideuterons would provide a "smoking gun" signature of dark matter annihilation or decay, essentially free of astrophysical background. Studies in recent years have emphasized that models for cosmic-ray antideuterons must be considered together with the abundant cosmic antiprotons and any potential observation of antihelium. Therefore, a second dedicated Antideuteron Workshop was organized at UCLA in March 2019, bringing together a community of theorists and experimentalists to review the status of current observations of cosmic-ray antinuclei, the theoretical work towards understanding these signatures, and the potential of upcoming measurements to illuminate ongoing controversies. This review aims to synthesize this recent work and present implications for the upcoming decade of antinuclei observations and searches. This includes discussion of a possible dark matter signature in the AMS-02 antiproton spectrum, the most recent limits from BESS Polar-II on the cosmic antideuteron flux, and reports of candidate antihelium events by AMS-02; recent collider and cosmic-ray measurements relevant for antinuclei production models; the state of cosmic-ray transport models in light of AMS-02 and Voyager data; and the prospects for upcoming experiments, such as GAPS. This provides a roadmap for progress on cosmic antinuclei signatures of dark matter in the coming years.

79 ASTRONOMY AND ASTROPHYSICS↗

Evaluation of Bifacial Modules and PV Technologies with Combined-Accelerated Stress Testing

In view of the increasing interest and market share of bifacial cells and modules, suitable substrates such as glass and transparent backsheets along with ethylene vinyl acetate (EVA) and polyolefin elastomer (POE) encapsulants were examined in combined-accelerated stress testing (C-AST) to evaluate and compare degradation modes. Testing with both monofacial and bifacial cells, we found glass-glass modules with monofacial cells led to greater grid finger breakage than those with polymeric backsheets. This is attributed to previous x-ray topography work showing higher stress in cells in glass-glass modules than glass backsheet modules. Consistent with the objectives of C-AST, which stresses modules at levels corresponding to the limits seen in the natural environment, we observed the UV-fluorescence signatures of modules tested in C-AST (considering the degradation associated with developing chromophores, moisture penetration and photobleaching effects) to be like those in fielded modules, more so than other chamber stress testing implemented for comparison. Finally, among multiple cell degradation modes that we observed such as light-induced degradation (LID), we differentiated susceptibility to potential-induced degradation (PID) on the back of the bifacial Passivated Emitter Back Cells (PERC) in C-AST. Confirming with ex-situ tests, we found polarization-type PID most prevalent in glass/glass modules with EVA as would be anticipated considering the greater leakage current through such module encapsulation. Unlike PID tests performed in the dark, which can lead to false positive PID test results, field-representative illumination is experienced by the modules on the front and back side while -1200 V system voltage is applied in C-AST, supporting the conclusion that this module type would be susceptible to PID in the field.

bifacial modules↗

Quenched lattice fluctuations in optically driven SrTiO3

Abstract Crystal lattice fluctuations, which are known to influence phase transitions of quantum materials in equilibrium, are also expected to determine the dynamics of light-induced phase changes. However, they have only rarely been explored in these dynamical settings. Here we study the time evolution of lattice fluctuations in the quantum paraelectric SrTiO 3 , in which mid-infrared drives have been shown to induce a metastable ferroelectric state. Crucial in these physics is the competition between polar instabilities and antiferrodistortive rotations, which in equilibrium frustrate the formation of long-range ferroelectricity. We make use of high-intensity mid-infrared optical pulses to resonantly drive the Ti–O-stretching mode at 17 THz, and we measure the resulting change in lattice fluctuations using time-resolved X-ray diffuse scattering at a free-electron laser. After a prompt increase, we observe a long-lived quench in R-point antiferrodistortive lattice fluctuations. Their enhancement and reduction are theoretically explained by considering the fourth-order nonlinear phononic interactions to the driven optical phonon and third-order coupling to lattice strain, respectively. These observations provide a number of testable hypotheses for the physics of light-induced ferroelectricity.

36 MATERIALS SCIENCE↗

A case study of high-temperature polyetherimide film capacitor fabrication

Capacitors, as the basic building block of power electronics and electrical systems, are the major constraint of the increasingly integrated power systems that require new capable polymer dielectric films operating at higher temperatures >125 °C. Despite tremendous research efforts on the lab scale, there remains a considerable barrier and knowledge basis for converting polymeric films to functioning capacitors desired in actual applications. Here, the authors tackled the polyetherimide (PEI) film scale up issues and developed various engineering processes for film de-wrinkling, optimal metallization, static elimination, and capacitor fabrication improvement. The authors discovered various fabrication challenges such as the electrostatic charge, metallization scheme, winding tension, and end electrode disconnects. To fabricate a high yield of PEI capacitor bobbins, it is necessary to utilize static eliminators (radioactive ionizers), moderately thick aluminum metallization (15–30 Ω/sq), and winding tension (60–100 g). It is also effective to evaluate capacitance, dielectric loss, equivalent series resistance, and thermal cycling stability of capacitors. This work sheds some light on converting PEI films and other polymeric films to capacitors on a scale up fabrication effort. The practical learning from film handling to capacitor fabrication in this work provided the necessary knowledge for manufacturing high-temperature polar film capacitors.

36 MATERIALS SCIENCE↗

Integrating collapsible plasmonic gaps on near-field probes for polarization-resolved mapping of plasmon-enhanced emission in 2D material

Scanning near-field optical microscopy (SNOM) is an important technique used to study the optical properties of material systems at the nanoscale. In previous work, we reported on the use of nanoimprinting to improve the reproducibility and throughput of near-field probes including complicated optical antenna structures such as the ‘campanile’ probe. However, precise control over the plasmonic gap size, which determines the near-field enhancement and spatial resolution, remains a challenge. Here, we present a novel approach to fabricating a sub-20 nm plasmonic gap in a near-field plasmonic probe through the controlled collapse of imprinted nanostructures using atomic layer deposition (ALD) coatings to define the gap width. The resulting ultranarrow gap at the apex of the probe provides a strong polarization-sensitive near-field optical response, which results in an enhancement of the optical transmission in a broad wavelength range from 620 to 820 nm, enabling tip-enhanced photoluminescence (TEPL) mapping of 2-dimensional (2D) materials. We demonstrate the potential of this near-field probe by mapping a 2D exciton coupled to a linearly polarized plasmonic resonance with below 30 nm spatial resolution. This work proposes a novel approach for integrating a plasmonic antenna at the apex of the near-field probe, paving the way for the fundamental study of light-matter interactions at the nanoscale.

Zhou, Junze (ORCID:000000020682767X)↗