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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 631 records · Page 35

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DOE OSTI2023

Window obscuration sensors for mobile gas and chemical imaging cameras

An infrared (IR) imaging system for determining a concentration of a target species in an object is disclosed. The imaging system can include an optical system including a focal plane array (FPA) unit behind an optical window. The optical system can have components defining at least two optical channels thereof, said at least two optical channels being spatially and spectrally different from one another. Each of the at least two optical channels can be positioned to transfer IR radiation incident on the optical system towards the optical FPA. The system can include a processing unit containing a processor that can be configured to acquire multispectral optical data representing said target species from the IR radiation received at the optical FPA. One or more of the optical channels may be used in detecting objects on or near the optical window, to avoid false detections of said target species.

Mallery, Ryan↗

DOE OSTI2024

Window obscuration sensors for mobile gas and chemical imaging cameras

Mallery, Ryan↗

DOE OSTI2024

Window obscuration sensors for mobile gas and chemical imaging cameras

Mallery, Ryan↗

DOE OSTI2022

Characterization, Chemistry, and Particle Size Distribution of Fallout Particles Isolated from Filter Samples

Nuclear particulate fallout is the radioactive byproduct of a nuclear event formed by the mixture of proximate environmental materials with vaporized bomb debris. The debris can be transported into the atmosphere during cloud rise, raining out locally and globally constituting a radiation hazard. Questions remain on how entrainment of environmental material in the fireball affects fallout formation processes and radionuclide incorporation during cooling.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

DOE OSTI2022

Long-term 3D MHD simulations of black hole accretion discs formed in neutron star mergers

ABSTRACT We examine the long-term evolution of accretion tori around black hole (BH) remnants of compact object mergers involving at least one neutron star, to better understand their contribution to kilonovae and the synthesis of r-process elements. To this end, we modify the unsplit magnetohydrodynamic (MHD) solver in flash 4.5 to work in non-uniform three-dimensional spherical coordinates, enabling more efficient coverage of a large dynamic range in length scales while exploiting symmetries in the system. This modified code is used to perform BH accretion disc simulations that vary the initial magnetic field geometry and disc compactness, utilizing a physical equation of state, a neutrino leakage scheme for emission and absorption, and modelling the BH’s gravity with a pseudo-Newtonian potential. Simulations run for long enough to achieve a radiatively inefficient state in the disc. We find robust mass ejection with both poloidal and toroidal initial field geometries, and suppressed outflow at high disc compactness. With the included physics, we obtain bimodal velocity distributions that trace back to mass ejection by magnetic stresses at early times, and to thermal processes in the radiatively inefficient state at late times. The electron fraction distribution of the disc outflow is broad in all models, and the ejecta geometry follows a characteristic hourglass shape. We test the effect of removing neutrino absorption or nuclear recombination with axisymmetric models, finding ${\sim} 50{{\ \rm per\ cent}}$ less mass ejection and more neutron-rich composition without neutrino absorption, and a subdominant contribution from nuclear recombination. Tests of the MHD and neutrino leakage implementations are included.

Fahlman, Steven (ORCID:0000000348759940)↗

DOE OSTI2024

Coherent gluon radiation: beyond leading-log accuracy

Abstract Results are presented for the medium-induced, soft coherent radiation spectrum for all 2 → 2 partonic channels in QCD, at leading-order inα s but beyond leading logarithmic accuracy. The general formula is valid in the full kinematic range of the underlying process, and reduces to previous results in special cases. The soft gluon radiation spectrum is expressed in terms of thecolor density matrixspecific to each channel, quantifying the entanglement between the color components of the 2 → 2 production amplitude. Beyond the leading logarithm, the spectrum depends explicitly on the off-diagonal elements of this matrix, owing to the soft gluon’s ability to probe the internal color structure of the parton pair.

Physics↗

DOE OSTI2023

Modeling Hydrodynamic Instabilities, Shocks, and Radiation Waves in High Energy Density Experiments [Dissertation]

This thesis presents the computational design, modeling, and analysis of three experiments in high-energy density physics (HEDP), all of them concerning fundamental radiation flows. The first experiment is a laboratory astrophysics experiment to investigate the role of the Kelvin-Helmholtz instability (KHI) in the process of galactic filaments supplying gas to galactic halos. The achieved goal was to provide a first study in which the role of the instability is maximal and predict behavior in future iterations of an experiment accessing a more radiative regime where the role of the instability is stifled. This experiment would help answer how certain galaxies are able to grow so rapidly and produce many stars as the KHI limits this process. The second experiment, COAX, is a radiation flow experiment with a novel spectroscopy diagnostic configuration, designed to spatially measure the temperature of a radiation wave as it travels down a doped foam. A key result of this work was the development of a synthetic spectroscopy application and application of modern spectroscopy comparison techniques to provide our first temperature reconstructions from the experimental data. This experimental platform serves as the launching ground for a number of new experiments that vary the basic premise and thus is foundational to our ongoing research. The final experiment is a full integration of modeling, design, and theoretical development for the Radishock experiment. This experimental platform studies the head-on collision of a radiation wave with a counter-propagating shock, and like COAX, uses spectroscopy to diagnose and detect the interaction. My research analyzes the successful shots, indicating aspects of successful detections and suggests improvements to future iterations of the design.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2021

Vertical variation of turbulent entrainment mixing processes in marine stratocumulus clouds using high-resolution digital holography

Marine stratocumulus clouds contribute signi?cantly to the Earth’s radiation budget due to their extensive coverage and high albedo. Yet, subgrid variability in cloud properties such as aerosol concentration, droplet number and precipitation rates lead to considerable errors in global climate models. While these clouds usually have small vertical ex-tent, turbulent entrainment-mixing and precipitation can generate signi?cant variations in droplet number, size and relative dispersion with altitude. In this paper, we analyze turbulent entrainment-mixing processes and the variability in cloud microphysical properties as a function of height within a warm marine stratocumulus cloud layer over the Eastern North Atlantic. We use high resolution airborne holographic measurements and compare them with local turbulence measurements. We ?nd that entrainment-mixing is primarily inhomogeneous near cloud top leading to larger droplet sizes and homogeneous near cloud base leading to smaller droplet sizes. Further analysis of Damk¨ohler number measurements are able to explain the mixing mechanisms at di?erent cloud heights, reinforcing the importance of turbulent mixing and microphysical time scales in deter-mining cloud microphysics.

Desai, Neel↗

DOE OSTI2026

Chloride modification of vacuum-assisted blade-coated perovskite solar cells and mini-modules in ambient environment

Scalable deposition of perovskite thin films under ambient conditions remains a key challenge for the commercialization of perovskite photovoltaics, primarily due to the difficulty of controlling crystallization kinetics and suppressing non-radiative recombination during film formation. In this work, we present an effective strategy to modulate crystallization kinetics and non-radiative recombination in vacuum-quenched blade-coated perovskite films processed in air using chloride-based additives. By systematically comparing PbCl 2 and 3-chloropropylamine hydrochloride (Cl-PACl), we elucidate how different chloride incorporation pathways influence crystallization behavior and optoelectronic properties. In situ transmission and in situ photoluminescence measurements reveal that PbCl 2 acts as a transient additive that slows intermediate/perovskite phase formation while suppressing non-radiative recombination, leading to improved film quality. In contrast, Cl-PACl introduces additional trap states that deteriorate optoelectronic performance. As a result, PbCl 2 -modified perovskite solar cells achieve a champion power conversion efficiency (PCE) of 24.2% and remarkable operational stability, retaining over 90% of their initial performance after 800 hours of continuous illumination. Furthermore, we successfully scaled the process, fabricating a perovskite mini-module that delivered a champion efficiency of 18.0%. This study underscores the critical importance of coupling vacuum-assisted blade coating with transient additive engineering for achieving high-performance, stable, and scalable perovskite photovoltaics processed in ambient air.

14 SOLAR ENERGY↗

DOE OSTI2020

Self-compression of laser pulses in a discrete medium

Using the discrete nonlinear Schrödinger equation, we study the laser radiation self-action dynamics in a nanostructured waveguide system. It is shown that for a laser pulse energy exceeding the critical value, the nonlinear evolution of the wave field markedly differs from the corresponding process in a continuous medium. While the pulse propagates in a discrete medium, its length decreases to values comparable to the scale of the structure and the velocity decreases to zero. The system parameters are determined at which the wave field after the laser pulse termination begins to propagate in the opposite direction in a compressed form. The process of slowing down and stopping the pulse is accompanied by strong radiation losses, so that about a third of the energy of the initial field distribution remains in the final compressed state. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2026

Technoeconomic Analysis of a Novel Microwave Process to Produce Ethylene from Methane

Ethylene is a critical feedstock in industrial processes, serving as a raw material in the petrochemical industry to produce plastics and commodity chemicals. Conventional ethylene production routes are energy-intensive and contribute substantially to the carbon footprint of chemical manufacturing. In this study, an industrial-scale novel microwave process was simulated using ASPEN Plus to assess its economic viability. Technoeconomic analysis confirmed the economic competitiveness of the novel microwave process, with a levelized cost of ethylene of USD 0.51/kg compared to USD 0.56/kg for the conventional base case. Key economic drivers of the process were identified, and sensitivity analyses were conducted to evaluate their impact on project economics. Furthermore, 87.7% of the total utility consumption in the novel microwave process is electricity, highlighting its potential to contribute to the electrification of the chemical industry. The findings of this study confirm the economic feasibility of both industrial-scale microwave reactors and modular plant configurations for the production of ethylene from methane, offering a promising alternative to conventional processes.

electromagnetic radiation↗

DOE OSTI2023

Natural attenuation of uranium in a fluvial Wetland: Importance of hydrology and speciation

A nuclear fuel fabrication facility released 43,500 kg of uranium into a riparian wetland located on the Savannah River Site between 1955 and 1988. Studies were undertaken to evaluate hydrological and geochemical processes influencing uranium accumulation in the wetland. Gamma-radiation-mapping surveys were conducted by systematically walking over the contaminated wetland with backpacks equipped with global positioning systems and NaI gamma detectors. Based on maps compiled from >700,000 gamma spectra and eight sediment uranium depth profiles, it was determined that 94% of the released uranium remained in the wetland. The uranium in the wetland is concentrated in five multi-hectare areas along the stream, accounting for ~11% of the land area adjacent to the stream. While land type (upland or wetland) and topography provided a reasonable first approximation of where much of the uranium was deposited, hydrological watershed modeling revealed that the stream velocity was especially slow through many of the hot spots. Here, using autoradiography combined with SEM/EDX measurements of contaminated sediments, surprisingly few hot particles were detected. Instead, uranium was evenly distributed throughout the sampled sediment, suggesting that dissolved uranium had bound to sediment particles that became suspended and later deposited in low energy (low flow velocity) portions of the stream. EXAFS suggested that U atoms were present as individual ions in disordered complexes within the sediment. Furthermore, linear combination analyses suggested that the predominant component of the U(VI) was adsorbed to sediment minerals (~70%) and a minor component (~30%) was associated with organic matter phases. Furthermore, these studies show that wetlands can be extraordinarily effective at binding and retaining uranium, thereby providing a natural barrier to the transport of uranium out of a watershed. However, significant anthropogenic or climatic changes to wetlands, such as those associated with flooding, forest fires, or land use, may disrupt the complex hydrological and biogeochemical balance necessary to maintain long-term immobilization of uranium.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

DOE OSTI2022

Comparison of Energetic Electron Fluxes Measured by GPS and THEMIS Spacecraft in the Inner Magnetosphere

Key elements of space weather models are energetic electron fluxes in the inner magnetosphere and the outer radiation belt. Flux depletion is driven by various loss processes: scattering into atmosphere, magnetopause shadowing. Flux enhancement is driven by various acceleration processes: local wave-particle interactions, radial transport, plasma sheet injections. Many of these processes operate on ~ hour timescales. Such mesoscale flux variations are not well traced by equatorial spacecraft with much longer orbits. Energetic electron detectors onboard the Global Positioning System (GPS) constellation provide a unique opportunity for probing such ~ hour-scale flux variations. Measurements from up to 23 identically instrumented GPS satellites cover a wide energy and L-shell range with a subhour time resolution. However, their orbits are inclined and thus all measurements at L-shell >4.3 are off-equatorial. Here, in this report, we present a comparison of equatorial THEMIS and nonequatorial GPS measurements of omnidirectional ≤600 keV electron fluxes. Such a comparison allows us to derive coefficients for using off-equatorial GPS fluxes to infer the equatorial values. These coefficients depend on particle energy and L-shell. We demonstrate a new data set derived from GPS measurements and discuss how it can be used to investigate mesoscale dynamics of energetic electron fluxes in the inner magnetosphere.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2023

Modelling populations of kilonovae

Abstract The 2017 detection of a kilonova coincident with gravitational-wave emission has identified neutron star mergers as the major source of the heaviest elements and dramatically constrained alternative theories of gravity. Observing a population of such sources has the potential to transform cosmology, nuclear physics, and astrophysics. However, with only one confident multi-messenger detection currently available, modelling the diversity of signals expected from such a population requires improved theoretical understanding. In particular, models that are quick to evaluate and are calibrated with more detailed multi-physics simulations are needed to design observational strategies for kilonovae detection and to obtain rapid-response interpretations of new observations. We use grey-opacity models to construct populations of kilonovae, spanning ejecta parameters predicted by numerical simulations. Our modelling focuses on wavelengths relevant for upcoming optical surveys, such as the Rubin Observatory Legacy Survey of Space and Time (LSST). In these simulations, we implement heating rates that are based on nuclear reaction network calculations. We create a Gaussian-process emulator for kilonova grey opacities, calibrated with detailed radiative transfer simulations. Using recent fits to numerical relativity simulations, we predict how the ejecta parameters from binary neutron star (BNS) mergers shape the population of kilonovae, accounting for the viewing-angle dependence. Our simulated population of BNS mergers produce peak i-band absolute magnitudes of −20 ≤ Mi ≤ −11. A comparison with detailed radiative transfer calculations indicates that further improvements are needed to accurately reproduce spectral shapes over the full light curve evolution.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Phase-contrast 3D tomography of HeLa cells grown in PLLA polymer electrospun scaffolds using synchrotron X-rays

Advanced imaging is useful for understanding the three-dimensional (3D) growth of cells. X-ray tomography serves as a powerful noninvasive, nondestructive technique that can fulfill these purposes by providing information about cell growth within 3D platforms. There are a limited number of studies taking advantage of synchrotron X-rays, which provides a large field of view and suitable resolution to image cells within specific biomaterials. In this study, X-ray synchrotron radiation microtomography at Diamond Light Source and advanced image processing were used to investigate cellular infiltration of HeLa cells within poly L-lactide (PLLA) scaffolds. This study demonstrates that synchrotron X-rays using phase contrast is a useful method to understand the 3D growth of cells in PLLA electrospun scaffolds. Two different fiber diameter (2 and 4 µm) scaffolds with different pore sizes, grown over 2, 5 and 8 days in vitro , were examined for infiltration and cell connectivity. After performing visualization by segmentation of the cells from the fibers, the results clearly show deeper cell growth and higher cellular interconnectivity in the 4 µm fiber diameter scaffold. Finally, this indicates the potential for using such 3D technology to study cell–scaffold interactions for future medical use.

3D culture↗

DOE OSTI2023

JuliaOceanWaves

SAND2023-05107O JuliaOceanWaves is a collection of packages and functions for modeling wave energy converters. The open-source software is designed to be used by the wave energy community to model new concepts, perform design optimization, and more. Capabilities include: • A representation of ocean wave spectra and input/output (e.g. read from National Oceanic and Atmospheric Administration buoys) and post-processing functionalities; • A solver for the linear potential flow radiation and diffraction equations for wave forcing on floating structures. • Solving the floating body linear dynamics in the frequency domain. Future additions to the software will include solving non-linear floating body dynamics in the time-domain through time-marching Ordinary Differential Equation solvers and the pseudo-spectral optimization method. Sandia National Laboratories is a multimission laboratory managed and operated by National Technology & Engineering Solutions of Sandia, LLC, a wholly owned subsidiary of Honeywell International Inc., for the U.S. Department of Energy’s National Nuclear Security Administration under contract DE-NA0003525.

Michelen Strofer, Carlos↗

DOE OSTI2020

ARM Mobile Facility Leaving Alaska for U.S. Southeast

The Atmospheric Radiation Measurement (ARM) user facility will soon begin the process of moving its third mobile facility (AMF3) from Alaska to the Southeastern United States. A workshop in August 2018 identified the Southeast as a priority region of interest for further study by ARM. The Southeast is a region with abundant atmospheric convection, yet the land surface, boundary layer, vegetation, and aerosol properties are markedly different from those seen at ARM’s fixed observatory in Oklahoma, allowing opportunities to explore new research questions. To maximize the scientific value of the new site, DOE’s Biological and Environmental Research program selected a site science team that will help guide the move of AMF3. Brookhaven National Laboratory (BNL) in New York will lead the AMF3 relocation effort. Supported by ARM and DOE’s Atmospheric System Research (ASR), the multi-institutional team is responsible for developing a science plan and initial research project for the Southeastern U.S. deployment.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

MANIPULATE-2020: An Interface Tool for Nuclear Data Processing

This report provides basic background data on the Manipulate-2020 code. This code is used for processing and "manipulation" of nuclear data in support of radiation metrology applications. The code is made available on the open GitHub repository and is available to the general nuclear data community.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗