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At least 631 records · Page 35

The 50-MHz meteor radar observation at Syowa Station, Antarctica

The 50-MHz Doppler radar installed at Syowa Station (69 deg 00'S, 39 deg 35'E), Antarctica, in 1982 can detect continuously a meteor echo if an operator assigns the meteor mode operation to the radar. The radar has two narrow antenna beams (4 deg in the horizontal plane), one toward geomagnetic south and the other toward approximately geographic south, with a crossing angle of about 33 deg. The minicomputer annexed to the radar controls the transmission and reception of a 50-MHz wave. If the receiver detects a meteor echo, the flag signal is sent to the computer. Then the computer begins to determine the echo range with a time resolution of 1 micro s and to sample every 200 microns/s for 1 s the Doppler signal and echo intensity at the particular range (R). The line-of-sight velocity (V sub D) of the echo trail is calculated from the output from the Doppler signal detection circuit having an offset frequency by using the so-called zero-crossing method. The echo amplitude decay time calculated by a least-mean square method is used to obtain the ambipolar diffusion coefficient (D) and then to calculate the echo height (H). About 120 day observations were made during 1982-1983. Some early results are presented. magnetic tapes together with V sub D, D, H and R for later analysis in Japan. About 120 day observation were made during 1982-1983. Some early results are presented.

Tanaka, T.↗

The Complete Spectral Catalog of Bright BATSE Gamma-Ray Bursts

We present a systematic spectral analysis of 350 bright Gamma-Ray Bursts (GRBs) observed by the Burst and Transient Source Experiment (BATSE; approx. 30 keV - 2 MeV; including 17 short GRBs) with high energy and time resolution. Our sample was selected from the complete set of 2704 BATSE GRBs based on their energy fluence or peak photon flux values to assure good statistics. To obtain well-constrained, model-unbiased spectral parameters, a set of various photon models is used to fit each spectrum, and internal characteristics of each model are also investigated. A thorough analysis has been performed on 342 time-integrated and 8459 time-resolved burst spectra, and the effects of integration times in determining the spectral parameters are explored. The analysis results presented here provide the most detailed perspective of spectral aspects of the GRB prompt emission to date. Using the results, we study correlations among spectral parameters and spectral evolutions. The results of all spectral fits are available electronically in FITS format, from the High-Energy Astrophysics Science Archive Research Center (HEASARC).

Kaneko, Yuki↗

Observations of Turbulence in a Kelvin-Helmholtz Event on 8 September 2015 by the Magnetospheric Multiscale Mission

Spatial and high-time-resolution properties of the velocities, magnetic field, and 3-D electric field within plasma turbulence are examined observationally using data from the Magnetospheric Multiscale mission. Observations from a Kelvin-Helmholtz instability (KHI) on the Earth's magnetopause are examined, which both provides a series of repeatable intervals to analyze, giving better statistics, and provides a first look at the properties of turbulence in the KHI. For the first time direct observations of both the high-frequency ion and electron velocity spectra are examined, showing differing ion and electron behavior at kinetic scales. Temporal spectra exhibit power law behavior with changes in slope near the ion gyrofrequency and lower hybrid frequency. The work provides the first observational evidence for turbulent intermittency and anisotropy consistent with quasi two-dimensional turbulence in association with the KHI. The behavior of kinetic-scale intermittency is found to have differences from previous studies of solar wind turbulence, leading to novel insights on the turbulent dynamics in the KHI.

Stawarz, J. E.↗

Collaborative Research Proposal: Time Resolved Optical Emissions Spectroscopy and Laser Induced Fluorescence Spectroscopy of Nanosecond Pulsed Discharges in a Gas-Liquid Water Film Reactor

Electrical discharge plasma formed in contact with liquid water is of interest for a wide range of applications in chemical, biomedical, agricultural, electrical, and materials science and engineering. Such plasma reactors are of very timely importance since they also have significant disinfection capability by inactivating bacteria, viruses and other pathogens. Many types of plasma sources including those driven by AC, DC, RF, microwave, and pulsed electrical power supplies coupled to a wide range of different electrode configurations and reactor designs have been developed and explored which contact the plasma with liquid water. Recent roadmaps have recommended that further work is needed to develop our understanding of the fundamental chemical and physical process which occur at the interface of non-thermal plasma with liquid water solutions in order to advance this large diversity of applications which ultimately depend upon efficient production of key reactive chemical species. There is a wide range of interacting factors that affect the chemical reactions that occur in the plasma, in the liquid phase, and at the interface. These factors ultimately govern the key reactive chemical species formed and used in the various applications and they include a) the reactor design and input parameters, b) the discharge and transport processes, c) the plasma properties, and d) the resulting chemical reactions. For pulsed discharges, the power supply design and output parameters control the applied voltage, frequency, rise time, and width (duration) of the applied pulses. The reactor design involves specification of the gas-liquid contacting methods, electrode gap distance, reactor volume and shape, and gas and liquid flow rates achievable. The gas and liquid compositions as well as the liquid properties such as pH and conductivity are also of key importance in determination of the resulting chemical reactions. In addition, the important plasma properties include plasma gas temperature, electron density, electron energy (distribution), and size of the plasma channels which are all affected by the discharge and transport properties. Many studies have focused on specific aspects of these various processes. Of particular important and relevance to the proposed work is the utilization of nanosecond pulses to generate plasma in gas-liquid systems, liquid bubbles, underwater, and in gases. Recent advances in nanosecond pulses provide significant advantages in utilization with liquid water. For example, fast rise time and short pulses are less sensitive to water conductivity, such short pulses may provide advantages in fast temporal quenching of the plasma, and fundamental analysis of pulse properties, including pulse shape and width, may be facilitated by investigation of single filamentary fast pulses. Many studies have also dealt with the role of the gas composition on formation of reactive oxygen species (ROS) (i.e., hydroxyl radicals – ·OH, hydrogen peroxide – H 2 O 2 , various atomic oxygen species, ozone-O 3 , hydroperoxyl radicals HO 2 ·) and reactive nitrogen species (RNS) (i.e., nitrogen oxides – NO, NO 2 , N 2 O - collectively termed NO X , nitrite-NO 2 - , nitrate-NO 3 - , peroxynitrite-ONOO - ). The hydroxyl radical is the critical species in many chemical oxidation reactions for chemical degradation of toxic compounds in water and gases and for synthesis of some compounds. The mixture of various nitrogen oxide species is important for many biochemical and biological processes involved in biomedical and agricultural applications including disinfection and fertilizer production. The present proposal focuses on determination of the effects of time resolved electron density and hydroxyl radicals on plasma chemical reactions through collaboration with the Princeton Collaborative Low Temperature Plasma Research Facility (PCRF) at the Princeton Plasma Physics Laboratory (PPPL). In order to further investigate the role of the plasma generated electrons and hydroxyl radicals on the overall formation of the key species including hydrogen peroxide, hydroxyl radicals, and nitrogen oxides, the proposed work, thus seeks to determine high resolution time resolved electron density by optical emissions spectroscopy and time resolved hydroxyl radicals using laser induced fluorescence in the nanosecond discharge reactor. The combination of data on electron density and hydroxyl radical concentration will be utilized in the present work to more fully characterize the chemical reaction processes in this system and to advance the design, development, and operation of such chemical reactors for a wide range of applications.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Magnetospheric impulse response for many levels of geomagnetic activity

The temporal relationship between the solar wind and magnetospheric activity has been studied using 34 intervals of high time resolution IMP 8 solar wind data and the corresponding AL auroral activity index. The median values of the AL index for each interval were utilized to rank the intervals according to geomagnetic activity level. The linear prediction filtering technique was then applied to model magnetospheric response as measured by the AL index to the solar wind input function VB(s). The linear prediction filtering routine produces a filter of time-lagged response coefficients which estimates the most general linear relationship between the chosen input and output parameters of the magnetospheric system. It is found that the filters are composed of two response pulses speaking at time lags of 20 and 60 min. The amplitude of the 60-min pulse is the larger for moderate activity levels, while the 20-min pulse is the larger for strong activity levels. A possible interpretation is that the 20-min pulse represents magnetospheric activity driven directly by solar wind coupling and that the 60-min pulse represents magnetospheric activity driven by the release of energy previously stored in the magnetotail. If this interpretation is correct, the linear filtering results suggest that both the driven and the unloading models of magnetospheric response are important facets of a more comprehensive response model.

Bargatze, L. F.↗

Ground Calibration of the Silicon Drift Detectors for NICER

The Neutron star Interior Composition ExploreR (NICER) is set to be deployed on the International Space Station (ISS) in early 2017. It will use an array of 56 Silicon Drift Detectors (SDDs) to detect soft X-rays (0.2 - 12 keV) with 100 nanosecond timing resolution. Here we describe the e ort to calibrate the detectors in the lab primarily using a Modulated X-ray Source (MXS). The MXS that was customized for NICER provides more than a dozen emission lines spread over the instrument bandwidth, providing calibration measurements for detector gain and spectral resolution. In addition, the fluorescence source in the MXS was pulsed at high frequency to enable measurement of the delay due to charge collection in the silicon and signal processing in the detector electronics. A second chamber, designed to illuminate detectors with either 55Fe, an optical LED, or neither, provided additional calibration of detector response, optical blocking, and effectiveness of background rejection techniques. The overall ground calibration achieved total operating time that was generally in the range of 500-1500 hours for each of the 56 detectors.

Silicon Drift Detectors↗

Femtosecond two-photon-resonant parametric four-wave mixing detection of atomic hydrogen

Here, we demonstrate an ultrafast parametric four-wave mixing method for the collisional-quenching-free detection of atomic hydrogen. Two photons of 243 nm light resonantly excite the n = 1 to n = 2 transition of atomic hydrogen, and a third probe photon scatters from the electronic coherence to generate the parametric emission of a degenerate signal photon. Laser-induced photofragmentation fluorescence from water, also excited with the same 243 nm pulses, is used as a convenient method to visualize beam overlap in space and time. The femtosecond time resolution enables the suppression of unwanted nonresonant contributions to the signal and separation from resonant mixing in water molecules because of the significantly different coherence lifetimes. A folded BOXCARS phase-matching configuration yields a spatially isolated, laser-like, signal beam, amenable to measurements in highly luminous backgrounds. Measurements in an H 2 /CH 4 /air flame demonstrate quantitative agreement with simulated H-atom concentration profiles. A coherence decay time constant of 42 ps is recorded in the atmospheric pressure flame.

Kliewer, Christopher Jesse [Sandia National Labora↗

Diurnal Variations of Stratospheric Ozone Measured by Ground-Based Microwave Remote Sensing at the Mauna Loa NDACC Site: Measurement Validation and GEOSCCM Model Comparison

There is presently renewed interest in diurnal variations of stratospheric and mesospheric ozone for the purpose of supporting homogenization of records of various ozone measurements that are limited by the technique employed to being made at certain times of day. We have made such measurements for 19 years using a passive microwave remote sensing technique at the Mauna Loa Observatory (MLO) in Hawaii, which is a primary station in the Network for Detection of Atmospheric Composition Change (NDACC). We have recently reprocessed these data with hourly time resolution to study diurnal variations. We inspected differences between pairs of the ozone spectra (e.g., day and night) from which the ozone profiles are derived to determine the extent to which they may be contaminated by diurnally varying systematic instrumental or measurement effects. These are small, and we have reduced them further by selecting data that meet certain criteria that we established. We have calculated differences between profiles measured at different times: morning-night, afternoon-night, and morning-afternoon and have intercompared these with like profiles derived from the Aura Microwave Limb Sounder (Aura-MLS), the Upper Atmosphere Research Satellite Microwave Limb Sounder (UARS-MLS),t he Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES), and Solar Backscatter Ultraviolet version 2 (SBUV2) measurements. Differences between averages of coincident profiles are typically less than 1.5 percent of typical nighttime values over most of the covered altitude range with some exceptions. We calculated averages of ozone values for each hour from the Mauna Loa microwave data, and normalized these to the average for the first hour after midnight for comparison with corresponding values calculated with the Goddard Earth Observing System Chemistry Climate Model (GEOSCCM). We found that the measurements and model output mostly agree to better than 1.5 percent of the midnight value, with one noteworthy exception: The measured morning-night values are significantly (2-3 percent) higher than the modeled ones from 3.2 to 1.8 hPa (approximately 39-43 km), and there is evidence that the measured values are increasing compared to the modeled values before sunrise in this region.

GEOSCCM model comparison↗

All-optical single-shot complete electric field measurement of extreme ultraviolet free electron laser pulses

Recent advances in ultrafast extreme ultraviolet (EUV) and x-ray light sources provide direct access to fundamental time and length scales for biology, chemistry, and materials physics. However, such light pulses are challenging to measure due to the need for femtosecond time resolution at difficult-to-detect wavelengths. Also, single-shot measurements are needed because severe pulse-to-pulse fluctuations are common. Here we demonstrate single-shot, complete field measurements by applying a novel version of frequency resolved optical gating. An EUV free electron laser beam creates a transient grating containing the pulse’s electric field information, which is read out with a 400 nm probe pulse. By varying the time delay between two copies of the EUV pump, rather than between the pump and the probe, we separate the needed coherent wave mixing from the slow incoherent response. Because this approach uses photoionization, it should be applicable from the vacuum ultraviolet to hard x rays.

36 MATERIALS SCIENCE↗

Pioneer 9 and Pioneer 10 observations of the solar wind associated with the August 1972 events

Observations are presented of the changes in the solar wind proton parameters at 0.8 and 2.2 AU as a result of the solar flares in August 1972. These observations were obtained by the NASA Ames Research Center solar wind plasma analyzer experiments on Pioneer 9 and Pioneer 10. High time resolution measurements are presented of the solar wind proton speed associated with the arrival of the interplanetary shocks at Pioneer 9 and Pioneer 10. For these events, differential ion energy per unit charge spectra are shown which indicate the changes in the solar wind ion distribution function associated with the arrival of each of the interplanetary shocks. Four fast shocks are identified at Pioneer 9, and it is found that previously the time of arrival of the first interplanetary shock at Pioneer 9 was not correctly identified. Two fast shocks and one reverse shock are identified at Pioneer 10.

Intriligator, D. S.↗

Observational evidence of continual heating in X-ray emitting coronal loops

A 90 s time resolution study of the soft X-ray emission from three active region loops shows the emission to be constant to about two percent over the half hour period of observation. Soft X-ray observations in two wavebands are used to deduce the temperature and density of these loops. The data unambiguously demonstrate that energy is supplied to each loop during the observations. If heating is due to discrete events, the time interval between events is shown to be less than 10 min, which is short relative to the radiative cooling time of the loops.

Gerassimenko, M.↗

Observations of Pc 1-2 waves in the outer magnetosphere

High time resolution measurements made inside the magnetopause from L = 7 to L = 14 by the flux gate magnetometer aboard the Ogo 5 satellite, which demonstrate that the Pc 1-2 magnetic field oscillations are present in the outer magnetosphere, are examined. The solar wind dynamic pressure and the magnetospheric cold plasma were enhanced, and the IMF had a southward component 2 hours before the events, but there was no significant correlation between the time of the events and either storm recovery phase or substorm onset. The magnetic field perturbations in each event were transverse to the ambient field with amplitudes from 2 to 8 gamma, and most of the transverse perturbations showed left-handed polarization. Excursions into the magnetosheath during two events revealed a disturbed magnetic field with significant power in frequencies of minimum 0.1 Hz, and although the magnetosheath was a source of free energy for waves at Pc 1-2 frequencies, the data within the magnetosphere suggest that the observed pulsations were ion cyclotron waves generated at the geomagnetic equator at large radial distances.

Kaye, S. M.↗

Simultaneous measurements of velocity and pressure fields in subsonic and supersonic flows through image-intensified detection of laser-induced fluorescence

An optical technique is presented for combined, spatially resolved measurements of two-dimensional velocity and pressure fields in compressible flows. The single-mode frequency of an argon laser is fixed in the wing of an absorption line of iodine molecules, seeded in an underexpanded round jet of nitrogen gas. The emitted fluorescence, being proportional to the amount of absorbed radiation and hence the absorption line-shape function, is detected with an intensified 100 x 100 photodiode array camera. A single-microchannel-plate image intensifier is fiber-optically coupled to the array in order to improve time resolution and SNR. Three components of the velocity vector in a cross-sectional plane are sequentially probed with four laser sheets from three different directions. By shifting the laser frequency in one of the sheets with a piezo-tuned intra-cavity etalon, the slope of the absorption line can be measured in situ in order to provide the required scaling factor for the velocity measurement. With its short measurement times of less than 250 ms, this method is well suited for blow-down wind tunnel experiments.

Hiller, B.↗

The Spectral Evolution of Solar Flare Hard X-Ray Emission Observed with BATSE

We present a more detailed characterization of spectral evolution in solar flare hard X-ray emission than has been previously described. Our characterization is consistent with some earlier results but utilizes higher time resolution data and reveals nuances in spectral evolution that have never been reported. We employ an underutilized data set, the Burst and Transient Source Experiment (BATSE) solar flare catalog, for our investigation and different methodology than previous studies. Our findings support the conclusion that properties of the particle Abstract: acceleration mechanism in flares, such as the acceleration rate or efficiency, are indeed important to understanding spectral evolution. On the other hand, time-of-flight models, which assume accelerator properties to be negligible, cannot explain the observed detailed spectral evolution, and correlations that we would expect to exist between spectral evolution patterns and parameters derived from time-of-flight model inversions are not supported by the data. In this fashion, we establish an observational context in which to interpret future High Energy Solar Spectroscopic Imager (HESSI) observations and delineate some constraints for theoretical models of particle acceleration.

Newton, Elizabeth K.↗

Resolving length-scale-dependent transient disorder through an ultrafast phase transition

Abstract Material functionality can be strongly determined by structure extending only over nanoscale distances. The pair distribution function presents an opportunity for structural studies beyond idealized crystal models and to investigate structure over varying length scales. Applying this method with ultrafast time resolution has the potential to similarly disrupt the study of structural dynamics and phase transitions. Here we demonstrate such a measurement of CuIr 2 S 4 optically pumped from its low-temperature Ir-dimerized phase. Dimers are optically suppressed without spatial correlation, generating a structure whose level of disorder strongly depends on the length scale. The redevelopment of structural ordering over tens of picoseconds is directly tracked over both space and time as a transient state is approached. This measurement demonstrates the crucial role of local structure and disorder in non-equilibrium processes as well as the feasibility of accessing this information with state-of-the-art XFEL facilities.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Solar flare hard and soft x ray relationship determined from SMM HXRBS and BCS data

The exact nature of the solar flare process is still somewhat a mystery. A key element to understanding flares if the relationship between the hard x rays emitted by the most energetic portions of the flare and the soft x rays from other areas and times. This relationship was studied by comparing hard x ray light curved from the Hard X-Ray Burst Spectrometer (HXRBS) with the soft x ray light curve and its derivation from the Bent Crystal Spectrometer (BCS) which is part of the X-Ray Polychrometer (XRP), these instruments being on the Solar Maximum Mission spacecraft (SMM). Data sample was taken from flares observed with the above instruments during 1980, the peak of the previous maximum of solar activity. Flares were chosen based on complete coverage of the event by several instruments. The HXRBS data covers the x ray spectrum from about 25 keV to about 440 keV in 15 spectral channels, while the BCS data used covers a region of the Spectrum around 3 angstroms including emission from the Ca XIX ion. Both sets of data were summed over their spectral ranges and plotted against time at a maximum time resolution of around 3 seconds. The most popular theory of flares holds that a beam of electrons produces the hard x rays by bremsstrahlung while the soft x rays are the thermal response to this energy deposition. The question is whether the rate of change of soft x ray emission might reflect the variability of the electron beam and hence the variability of the hard x rays. To address this, we took the time derivative of the soft x ray light curve and compared it to the hard flares, 12 of them showed very closed agreement between the soft x ray derivative and the hard x ray light curve. The other five did not show this behavior but were similar to each other in general soft x ray behavior. Efforts to determine basic differences between the two kinds of flares continue. In addition the behavior of soft x ray temperature of flares was examined.

Toot, G. David↗

Ultrafast all-optical coherence of molecular electron spins in room-temperature water solution

The tunability and spatial precision of paramagnetic molecules makes them attractive for quantum sensing. However, usual microwave-based detection methods have poor temporal and spatial resolution, and optical methods compatible with room-temperature solutions have remained elusive. In this study, we utilized pump-probe polarization spectroscopy to initialize and track electron spin coherence in a molecule. Designed to efficiently couple spins to light, aqueous potassium hexachloroiridate(IV) enabled detection of few-picosecond free-induction decay at room temperature and micromolar concentrations. Viscosity was found to strongly vary decoherence lifetimes. This approach has improved the experimental time resolution by up to five orders of magnitude, making it possible to observe molecular electron spin coherence in a system that only exhibits coherence below 25 kelvin with traditional techniques.

74 ATOMIC AND MOLECULAR PHYSICS↗

Rapid measurement of RH-dependent aerosol hygroscopic growth using a humidity-controlled fast integrated mobility spectrometer (HFIMS)

Abstract. The ability of aerosol particles to uptake water (hygroscopic growth) is an important determinant of aerosol optical properties and radiative effects. Aerosol hygroscopic growth is traditionally measured by humidified tandem differential mobility analyzers (HTDMA), in which size-selected dry particles are exposed to elevated relative humidity (RH), and the size distribution of humidified particles is subsequently measured using a scanning mobility particle sizer. As a scanning mobility particle sizer can measure only one particle size at a time, HTDMA measurements are time consuming, and ambient measurements are often limited to a single RH level. Pinterich et al. (2017b) showed that fast measurements of aerosol hygroscopic growth are possible using a humidity-controlled fast integrated mobility spectrometer (HFIMS). In HFIMS, the size distribution of humidified particles is rapidly captured by a water-based fast integrated mobility spectrometer (WFIMS), leading to a factor of ∼10 increase in measurement time resolution. In this study we present a prototype HFIMS that extends fast hygroscopic growth measurements to a wide range of atmospherically relevant RH values, allowing for more comprehensive characterizations of aerosol hygroscopic growth. A dual-channel humidifier consisting of two humidity conditioners in parallel is employed such that aerosol RH can be quickly stepped among different RH levels by sampling from alternating conditioners. The measurement sequence is also optimized to minimize the transition time between different particle sizes. The HFIMS is capable of measuring aerosol hygroscopic growth of six particle diameters under five RH levels ranging from 20 % to 85 % (30 separate measurements) every 25 min. The performance of this HFIMS is characterized and validated using laboratory-generated ammonium sulfate aerosol standards. Measurements of ambient aerosols are shown to demonstrate the capability of HFIMS to capture the rapid evolution of aerosol hygroscopic growth and its dependence on both size and RH.

54 ENVIRONMENTAL SCIENCES↗