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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 631 records · Page 35
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Phase diagram of infinite layer praseodymium nickelate Pr 1– x Sr x NiO 2 thin films

In this paper, we report the phase diagram of infinite layer Pr 1-x Sr x NiO 2 thin films synthesized via topotactic reduction from the perovskite precursor phase using CaH 2 . Based on the electrical transport properties, we find a doping-dependent superconducting dome extending between x = 0.12 and 0.28, with a maximum superconducting transition temperature T c of 14 K at x = 0.18, bounded by weakly insulating behavior on both sides. In contrast to the narrower dome observed in Nd 1–x Sr x NiO 2 , a local T c suppression near x = 0.2 was not observed for the Pr 1-x Sr x NiO 2 system. Normal state Hall effect measurements indicate mixed carrier contributions of both electrons and holes, and show a sign change in the Hall coefficient as functions of temperature and x, quite similar to that in Nd 1-x Sr x NiO 2 . Also similar is the observation of a minimum in the normal state resistivity associated with the superconducting compositions. These findings indicate an infinite layer nickelate phase diagram that is relatively insensitive to the rare-earth element, but suggest that disorder arising from the variations of the ionic radii on the rare-earth site affects the superconducting dome.

36 MATERIALS SCIENCE↗
NASA NTRS1981

Observations of large scale steady magnetic fields in the nightside Venus ionosphere and near wake

Based on an analysis of a large sample of Pioneer Venus Orbiter magnetometer data, characteristics of the magnetic fields near nightside periapsis are discussed. The observations generally indicate a weak average field of less than 10 gammas between 200 km and the periapsis altitude of 150 km, except when (1) the local solar wind dynamic pressure is high or (2) the spacecraft is in a 70 deg wide solar zenith angle range, which includes the midnight meridian and is centered west of it at 1 hr local time. The presence of radial field of alternating sign at low altitudes and in the nightside ionosphere suggests that the antiparallel magnetotail fields can terminate very close to the planet.

Luhmann, J. G.↗
NASA NTRS1995

Four large-scale field-aligned current systmes in the dayside high-latitude region

A system of four current sheets of large-scale field-aligned currents (FACs) was discovered in the data set of simultaneous Viking and Defense Meteorological Satellire Program-F7 (DMSP-F7) crossing of the dayside high-latitude region. This paper reports four examples of this system that were observed in the prenoon sector. The flow polarities of FACs are upward, downward, upward, and downward, from equatorward to poleward. The lowest-latitude upward current is flowing mostly in the central plasma sheet (CPS) precipitation region, often overlapping with the boundary plasma sheet (BPS) at its poleward edge, andis interpreted as a region 2 current. The pair of downward and upward FACs in the middle of te structure are collocated with structured electron precipitation. The precipitation of high-energy (greater than 1 keV) electrons is more intense in the lower-latitude downward current sheet. The highest-latitude downward flowing current sheet is located in a weak, low-energy particle precipitation region, suggesting that this current is flowing on open field lines. Simulaneous observations in the postnoon local time sector reveal the standard three-sheet structure of FACs, sometimes described as region 2, region 1, and mantle (referred to the midday region O) currents. A high correlation was found between the occurrence of the four FAC sheet structure and negative interplanetary magnetic field (IMF) B(sub Y). We discuss the FAC structurein terms of three types of convection cells: the merging, viscous, andlobe cells. During strongly negative IMF B(sub Y), two convection reversals exist in the prenoon sector; one is inside the viscous cell, and the other is between the viscous cell and the lobe cell. This structure of convection flow is supported by the Viking electric field and auroral UV image data. Based on the convection pattern, the four FAC sheet structure is interpreted as the latitude overlap of midday and morning FAC systems. We suggest that the for-current sheet structure is common in a certain prenoon localtime sector during strongly negative IMF B(sub Y).

Ohtani, S.↗
NASA NTRS1995

Energization of Ions in near-Earth current sheet disruptions

In this study we examine observations made by AMPTE/CCE of energetic ion bursts during seven substorm periods when the satellite was located near the neutral sheet, and CCE observed the disruption cross-tail current in situ. We compare ion observations to analytic calculations of particle acceleration. We find that the acceleration region size, which we assume to be essentially the current disruption region, to be on the order of 1 R(sub E). Events exhibiting weak acceleration had either relatively small acceleration regions (apparently associated with pseudobreakup activity on the ground) or relatively small changes in the local magnetic field (suggesting that the magnitude of the local current disruption region was limited). These results add additional support for the view that the particle bursts observed during turbulent current sheet disruptions are due to inductive acceleration of ions.

Taktakishvili, A.↗
NASA NTRS2013

A Measurement of the Millimeter Emission and the Sunyaev-zel'dovich Effect Associated with Low-frequency Radio Sources

We present a statistical analysis of the millimeter-wavelength properties of 1.4 GHz-selected sources and a detection of the Sunyaev-Zel'dovich Effect associated with the halos that host them. The Atacama Cosmology Telescope (ACT) has conducted a survey at 148 GHz, 218 GHz and 277 GHz along the celestial equator. Using samples of radio sources selected at 1.4 GHz from the Faint Images of the Radio Sky at Twenty-Centimeters (FIRST) Survey and the National Radio Astronomy Observatory Very Large Array Sky Survey (NVSS), we measure the stacked 148, 218 and 277 GHz flux densities for sources with 1.4 GHz flux densities ranging from 5 to 200 mJy. At these flux densities, the radio source population is dominated by active galactic nuclei (AGN), with both steep and at spectrum populations, which have combined radio-to-millimeter spectral indices ranging from 0.5 to 0.95, reecting the prevalence of steep spectrum sources at high flux densities and the presence of at spectrum sources at lower flux densities. The thermal Sunyaev-Zelapos;dovich (SZ) eect associated with the halos that host the AGN is detected at the 5 level through its spectral signature. When we compare the SZ eect with weak lensing measurements of radio galaxies, we find that the relation between the two is consistent with that measured by Planck for local bright galaxies. We present a detection of the SZ eect in some of the lowest mass halos (average M(sub 200) approx. equals 10(exp 13) solar M h(sup-1) (sub 70) ) studied to date. This detection is particularly important in the context of galaxy evolution models, as it confirms that galaxies with radio AGN also typically support hot gaseous halos. With Herschel* observations, we show that the SZ detection is not significantly contaminated by dusty galaxies or by dust associated with the AGN or galaxies hosting the AGN. We show that 5 mJy < S(sub 1:4) < 200 mJy radio sources contribute l(l +1)C(sub l)/(2 pi ) = 0:37+/- 0:03 micro K(exp 2) to the angular power spectrum at l = 3000 at 148 GHz, after accounting for the SZ effect associated with their host halos.

galaxies↗
NASA NTRS1995

Linear Wave Motion from Concentrated Harmonic Sources in Blasius Flow

The motion of individual linear instability waves in shear flows is well described by existing theoretical and numerical methods. However, naturally occuring sources produce coherent wave motions with broadband spanwise wavenumber and frequency spectra, and the different spectral components interact both linearly and nonlinearily. This paper describes a series of calculations for the parameters of three different experiments using locally parallel linear stability theory (LST), the Parabolized Stability Equations (PSE), and Direct Numerical Simulation (DNS). The calculations illustrate the strengths and weaknesses of the different methods, the extent to which the methods agree or disagree, and, finally the extent to which agreement with the measurements can be attained, given that the experiments also have their own difficulties.

linear↗
DOE OSTI2026

Diabatization with Electrostatic Embedding for Studying Photophysics in Organic Molecular Crystals

Highly emissive organic molecular crystals find applications in several areas, such as organic electronics, solar cells, and sensors. Understanding the excited-state mechanisms underlying these applications is essential for optimizing and controlling them effectively. Exciton models coupled with nonadiabatic dynamics, particularly quantum dynamics, provide crucial insights into photochemical and photophysical processes in molecular crystals. Nevertheless, there remains a lack of general tools and automated workflows to facilitate such simulations. In this paper, we present a computational strategy to investigate the photoactivated dynamics of organic molecular crystals, bridging methodologies traditionally used for molecular systems and materials science, with a particular focus on the interplay between local excitations and charge transfer (CT) processes. We have implemented an interface between the fromage and Overdia programs, enabling the construction of vibronic Hamiltonians for molecular crystals within an excited-state ONIOM(QM:QM′) framework, incorporating long-range electrostatics through a RESP-based Ewald summation. Fragment-based diabatization provides a route to quantum dynamics simulations in weak-to-intermediate coupling regimes. The method was applied to the photophysics of dibenzo[g,p]chrysene (DBC) crystals using time-dependent DFT. The fromage/ Overdia interface was employed to compute the couplings of local excitations and CT states for 18 unique DBC dimers in the crystal and to quantify the influence of electrostatic embedding, which was found to be modest (10−20%). Simulations on π-stacked dimers reproduced the small red shift observed experimentally from solution to crystal, attributed to electronic interactions among fixed monomers rather than crystal electrostatics. Quantum dynamics simulations revealed ultrafast population transfer from bright local excitations to CT states. This approach establishes a robust framework linking molecular and solid-state excited-state dynamics, with potential applications for studying excitations, defects, and impurities in molecular crystals.

Crystals↗
NASA NTRS1998

Reverse Energy Cascade in Turbulent Weakly Ionized Plasmas

For systems far from equilibrium, the neglect of a role for viscous effects in turbulence may be generally inappropriate when the relaxation time for the molecular process approaches the local flow time (Orou et al. (1996)). Furthermore, for stationary collisional plasmas, the conventional Reynolds number is irrelevant under circumstances where the standard features of turbulence in ordinary gases are observed in the plasma (Johnson et al. (1987)). The current theoretical understanding of these turbulent phenomenon is particularly inadequate for turbulence associated with ionizing shock waves; generally speaking, thermodynamic, acoustic and pressure fluctuations are all seen as amplified across the shock wave followed by a dramatic decay (relaminarization) usually attributed to a lack of importance of viscosity in the turbulent regions. This decay would be accelerated when the flow speed is also reduced due to the importance usually given to the conventional Reynolds number (which is directly proportional to velocity) as a quality of turbulence index. However, evidence supporting this consensus is lacking. By contrast, recent evidence of vanishing triple correlations form De Silva et al. (1996) provides strong support for early theoretical speculation of inherently molecular effects in macroscopic turbulence in Tsuge (1974). This specifically suggests that the role of compressive effects ordinarily associated with the shock wave could be significantly muted by the existence of a strongly turbulent local environment. There is also more recent theoretical speculation (Frisch et al. (1984)) of an inherently and previously unsuspected non-dissipative nature to turbulence, with energy conservation being nurtured by reverse energy cascades in the turbulent fluctuation spectra. Furthermore, the role which might be played by fluctuations on quantum mechanical phenomena and variations in molecular parameters is completely unknown, especially of the sort which might be found in optical spectra. A determination of the role which changing turbulent parameters might play on optical signatures behind a reflected shock wave should therefore provide a useful tool for the evolution of theoretical models for turbulence.

Williams, Kyron↗
DOE OSTI2016

Soft x-ray ptychography studies of nanoscale magnetic and structural correlations in thin SmCo 5 films

High spatial resolution magnetic x-ray spectromicroscopy at x-ray photon energies near the cobalt L 3 resonance was applied to probe an amorphous 50 nm thin SmCo 5 film prepared by off-axis pulsed laser deposition onto an x-ray transparent 200 nm thin Si 3 N 4 membrane. Alternating gradient magnetometry shows a strong in-plane anisotropy and an only weak perpendicular magnetic anisotropy, which is confirmed by magnetic transmission soft x-ray microscopy images showing over a field of view of 10 μm a primarily stripe-like domain pattern but with local labyrinth-like domains. Soft x-ray ptychography in amplitude and phase contrast was used to identify and characterize local magnetic and structural features over a field of view of 1 μm with a spatial resolution of about 10 nm. There, the magnetic labyrinth domain patterns are accompanied by nanoscale structural inclusions that are primarily located in close proximity to the magnetic domain walls. In conclusion, our analysis suggests that these inclusions are nanocrystalline Sm 2 Co 17 phases with nominally in-plane magnetic anisotropy.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
NASA NTRS1999

Directional Solidification of a Binary Alloy into a Cellular Convective Flow: Localized Morphologies

A steady, two dimensional cellular convection modifies the morphological instability of a binary alloy that undergoes directional solidification. When the convection wavelength is far longer than that of the morphological cells, the behavior of the moving front is described by a slow, spatial-temporal dynamics obtained through a multiple-scale analysis. The resulting system has a "parametric-excitation" structure in space, with complex parameters characterizing the interactions between flow, solute diffusion, and rejection. The convection stabilizes two dimensional disturbances oriented with the flow, but destabilizes three dimensional disturbances in general. When the flow is weak, the morphological instability behaves incommensurably to the flow wavelength, but becomes quantized and forced to fit into the flow-box as the flow gets stronger. At large flow magnitudes the instability is localized, confined in narrow envelopes with cells traveling with the flow. In this case the solutions are discrete eigenstates in an unbounded space. Their stability boundary and asymptotics are obtained by the WKB analysis.

Chen, Y.- J.↗
DOE OSTI2018

On Multiple Hall-Like Electron Currents and Tripolar Guide Magnetic Field Perturbations During Kelvin-Helmholtz Waves

Two magnetopause current sheet crossings with tripolar guide magnetic field signatures were reported by multiple Magnetosphere Multiscale (MMS) spacecraft during Kelvin-Helmholtz wave activity. The two out-of-plane magnetic field depressions of the tripolar guide magnetic field are largely supported by the observed in-plane electron currents, which are reminiscent of two clockwise Hall current loop systems. A comparison with a three-dimensional kinetic simulation of Kelvin-Helmholtz waves and vortex-induced reconnection indicates that MMS likely encountered the two Hall magnetic field depressions on either side of a magnetic reconnection X-line. Moreover, MMS observed an out-of-plane current reversal and a corresponding in-plane magnetic field rotation at the center of one of the current sheets, suggesting the presence of two adjacent flux ropes. The region inside one of the ion-scale flux ropes was characterized by an observed decrease of the total magnetic field, a strong axial current, and significant enhancements of electron density and parallel electron temperature. The flux rope boundary was characterized by currents opposite this axial current, strong in-plane and converging electric fields, parallel electric fields, and weak electron-frame Joule dissipation. These return current region observations may reflect a need to support the axial current rather than representing local reconnection signatures in the absence of any exhausts.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

Future Projections of EURO‐CORDEX Raw and Bias‐Corrected Daily Maximum Wind Speeds Over Scandinavia

Twenty historical and future Coordinated Regional Climate Downscaling Experiment ensemble for Europe simulations are bias corrected to investigate the future changes in the daily maximum wind speed over Scandinavia. We use quantile mapping to adjust the wind for the historical period (1985–2014) and quantile delta mapping for two future periods (2041–2070, 2071–2100, RCP8.5) with the 3-km spatial resolution NORA3 hindcast as the reference data set. Decomposing the variance, we find that most of the inter-model spread in the bias and the response to climate change is due to the regional climate model over land and mainly to the general climate model over sea. On average, the mean daily maximum wind speed is projected to increase everywhere except along the western coast of Norway and Denmark. In summer, we see an opposite sign over Sweden and Finland. The Norwegian Sea experiences weaker mean and high wind whereas the Baltic Sea experiences a strengthening. Bias correction influences the amplitude of the response, not the response pattern. Wind speed distributions can have different shapes in the future, with, for example, a flattening of the distribution off the coast of Norway with more frequent weak and very strong winds. Apart from a few locations in Norway, we find an increase in the number of days in the local highest historical wind category. Overall, summer exhibits opposite signals compared to the three other seasons. At country scale, the sign of the change in the mean and 98th percentile varies greatly depending on the region and among the simulations, especially for Norway.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2016

A charge inverter for III-nitride light-emitting diodes

In this work, we propose a charge inverter that substantially increases the hole injection efficiency for InGaN/GaN light-emitting diodes (LEDs). The charge inverter consists of a metal/electrode, an insulator, and a semiconductor, making an Electrode-Insulator-Semiconductor (EIS) structure, which is formed by depositing an extremely thin SiO{sub 2} insulator layer on the p{sup +}-GaN surface of a LED structure before growing the p-electrode. When the LED is forward-biased, a weak inversion layer can be obtained at the interface between the p{sup +}-GaN and SiO{sub 2} insulator. The weak inversion region can shorten the carrier tunnel distance. Meanwhile, the smaller dielectric constant of the thin SiO{sub 2} layer increases the local electric field within the tunnel region, and this is effective in promoting the hole transport from the p-electrode into the p{sup +}-GaN layer. Due to the improved hole injection, the external quantum efficiency is increased by 20% at 20 mA for the 350 × 350 μm{sup 2} LED chip. Thus, the proposed EIS holds great promise for high efficiency LEDs.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Asymmetric and endogenous magnetic reconnection processes in quasi-collisionless plasmas

We define an endogenous magnetic reconnection process as the one having a driving factor that lies within the region where a drastic change in magnetic field topology occurs. A process of this kind is shown to take place when an electron temperature gradient is present in a plasma column and when, referring to quasi-collisionless regimes, the evolving electron temperature fluctuations are anisotropic. A two-fluid theory, for weakly collisional plasma regimes and confinement configurations which have sheared magnetic fields, is formulated, and two classes of reconnecting modes are identified. The localized class of modes is characterized by a transverse reconnecting magnetic field $\tilde{B}_x$ of odd parity, as a function of the radial variable (across the reconnection layer). The width of this remains significant even when large macroscopic distances, such as those of interest to space and astrophysics, are considered. The relevant reconnection can be referred to as antisymmetric. In fact, the (additional and realistic) presence of a finite current density gradient leads to finding modes with mixed $\tilde{B}_x$ parity which are no longer localized within the reconnection layer. Then, the resulting magnetic islands are not symmetric. In view of the fact that there are plasmas in the Universe with considerable electron thermal energy contents, the features of the novel reconnecting modes can be relied upon in order to produce generation of magnetic fields or conversion of magnetic energy into particle energy (through a sequence of mode-particle resonances).

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2024

First-principles investigation of near-field energy transfer between localized quantum emitters in solids

We present a predictive and general approach to investigate near-field energy transfer processes between localized defects in semiconductors, which couples first-principles electronic structure calculations and a nonrelativistic quantum electrodynamics description of photons in the weak-coupling regime. The approach is general and can be readily applied to investigate broad classes of defects in solids. We apply our approach to investigate an exemplar point defect in an oxide, the F center in MgO, and we show that the energy transfer from a magnetic source, e.g., a rare-earth impurity, to the vacancy can lead to spin nonconserving long-lived excitations that are dominant processes in the near field, at distances relevant to the design of photonic devices and ultrahigh dense memories. We also define a descriptor for coherent energy transfer to predict geometrical configurations of emitters to enable long-lived excitations, that are useful to design optical memories in semiconductor and insulators. Published by the American Physical Society 2024

Chattaraj, Swarnabha (ORCID:0000000329333581)↗
DOE OSTI2024

Wind-driven emissions of coarse-mode particles in an urban environment

Abstract. Quantifying surface–atmosphere exchange rates of particles is important for understanding the role of suspended particulate matter in radiative transfer, clouds, precipitation, and climate change. Emissions of coarse-mode particles with a diameter greater than 0.5 µm provide giant cloud condensation nuclei and ice nuclei. These emissions are critical for understanding the evolution of cloud microphysical properties yet remain poorly understood. Here we introduce a new method that uses lidar retrievals of the elastic backscatter and Doppler velocity to obtain surface number emissions of particles with a diameter greater than 0.53 µm. The technique is applied to study particle number fluxes over a 2-month period from 1 June to 10 August 2022 during the TRACER campaign at an urban site near Houston, TX, USA. We found that all the observed fluxes were positive (upwards), indicating particle emission from the surface. The fluxes followed a diurnal pattern and peaked near noon local time. Flux intensity varied through the 2 months with multi-day periods of strong fluxes and multi-day periods of weak fluxes. Emission particle number fluxes peaked near ∼ 100 cm−2 s−1. The daily averaged emission fluxes correlated with friction velocity and were anticorrelated with surface relative humidity. The emission flux can be parameterized as F= 3000 u*4, where u* is the friction velocity in m s−1 and the emission flux F is in cm−2 s−1. The u* dependence is consistent with emission from wind-driven erosion. Estimated values for the mass flux are in the lower range of literature values from non-urban sites. These results demonstrate that urban environments may play an important role in supplying coarse-mode particles to the boundary layer. We anticipate that quantification of these emissions will help constrain aerosol–cloud interaction models that use prognostic aerosol schemes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2017

The synaptonemal complex has liquid crystalline properties and spatially regulates meiotic recombination factors

The synaptonemal complex (SC) is a polymer that spans ~100 nm between paired homologous chromosomes during meiosis. Its striated, periodic appearance in electron micrographs led to the idea that transverse filaments within this structure ‘crosslink’ the axes of homologous chromosomes, stabilizing their pairing. SC proteins can also form polycomplexes, three-dimensional lattices that recapitulate the periodic structure of SCs but do not associate with chromosomes. Here we provide evidence that SCs and polycomplexes contain mobile subunits and that their assembly is promoted by weak hydrophobic interactions, indicative of a liquid crystalline phase. We further show that in the absence of recombination intermediates, polycomplexes recapitulate the dynamic localization of pro-crossover factors during meiotic progression, revealing how the SC might act as a conduit to regulate chromosome-wide crossover distribution. Properties unique to liquid crystals likely enable long-range signal transduction along meiotic chromosomes and underlie the rapid evolution of SC proteins.

59 BASIC BIOLOGICAL SCIENCES↗
NASA NTRS1989

Transpiration cooling in hypersonic flight

A preliminary numerical study of transpiration cooling applied to a hypersonic configuration is presented. Air transpiration is applied to the NASA all-body configuration flying at an altitude of 30500 m with a Mach number of 10.3. It was found that the amount of heat disposal by convection is determined primarily by the local geometry of the aircraft for moderate rates of transpiration. This property implies that different areas of the aircraft where transpiration occurs interact weakly with each other. A methodology for quick assessments of the transpiration requirements for a given flight configuration is presented.

Tavella, Domingo↗